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D. Michelle Bailey

Publications and source records attributed to D. Michelle Bailey.

3 recordsLinked to original sources

Bridging Theory and Experiment in Virtually Imaged Phased Array (VIPA) Spectrometers

Virtually imaged phased array (VIPA) spectrometers provide high resolution and fast acquisition in a compact design, but their performance is sensitive to fabrication tolerances, component dimensions, and alignment. Here, leveraging numerical simulations validated by experimental data, we present a framework to identify the parameters that limit VIPA spectrometer resolution. This framework is applied to the construction of a new mid-infrared VIPA spectrometer, tested at wavelengths near $λ$ = 4.6 $μ$m with both continuous-wave and frequency-comb laser sources, with a resolving power predicted by analytical expressions to be as high as $RP$ = 830 000 (corresponding to a resolution of $δν$ = 78 MHz). Validated numerical simulations, however, provided a more realistic estimate that captures limits set by all the optical components. By minimizing aberrations and optimizing alignment, a resolving power of $RP$ = 440 000 ($δν$ = 150 MHz) was experimentally achieved, corresponding to 80 % of the value predicted by numerical simulation of the entire spectrometer. The results bridge the gap between analytical expressions and experimental results for compact, high-resolution VIPA spectrometers to enable more efficient fabrication and advanced design across critical areas like space optics, line-by-line pulse shaping, and broadband spectral sensors.

physics.optics↗

Precision Spectroscopy of Nitrous Oxide Isotopocules with a Cross-Dispersed Spectrometer and Mid-Infrared Frequency Comb

As a potent greenhouse gas and ozone depleting agent, nitrous oxide (N$_2$O) plays a critical role in the global climate. Effective mitigation relies on understanding global sources and sinks which can be supported through isotopic analysis. We present a cross-dispersed spectrometer, coupled with a mid-infrared frequency comb, capable of simultaneously monitoring all singly substituted, stable isotopic variants of N$_2$O. Rigorous evaluation of the instrument lineshape function and data treatment are discussed. Laboratory characterization of the spectrometer demonstrates sub-GHz spectral resolution and an average precision of $7.4\times10^{-6}$ for fractional isotopic abundance retrievals in 1 s.

physics.ins-det↗

Doppler-Free Two-Photon Cavity Ring-Down Spectroscopy of a Nitrous Oxide (N$_2$O) Vibrational Overtone Transition

We report Doppler-free two-photon absorption of N$_2$O at $λ$ = 4.53 $μ$m, measured by cavity ring-down spectroscopy. High power was achieved by optical self-locking of a quantum cascade laser to a linear resonator of finesse $F$ = 22730, and accurate laser detuning over a 400 MHz range was measured relative to an optical frequency comb. At a sample pressure of p = 0.13 kPa, we report a large two-photon cross-section of $σ_{13}^{(2)}$ = 8.0 $\times$ 10$^{-41}$ cm$^4$ s molecule$^{-1}$ for the $Q$(18) rovibrational transition at a resonant frequency of $ν_0$ = 66179400.8 MHz.

physics.chem-ph↗