arXiv subjects

D. Nagae

Publications and source records attributed to D. Nagae.

15 recordsLinked to original sources

arXiv2025

Investigation of Direct Nuclear Reactions in a Storage Ring Using In-Ring Detection

\textbf{Background:} Experiments involving nuclear reactions in a storage ring offer exceptional possibilities for precise measurements in inverse kinematics. These experiments provide excellent angular and energy resolution by particle spectroscopy, in addition to high luminosities. However, the extremely low-pressure environment maintained in the storage rings poses significant difficulties for experiments employing detectors or any outgassing material in the ring. \textbf{Purpose:} To investigate nuclear reactions in inverse kinematics using the storage-ring technique. The reactions were induced by scattering of a ${}^{20}\mathrm{Ne}$ beam off a hydrogen target at an energy of 50~MeV/u. \textbf{Method:} A beam of fully stripped ${}^{20}$Ne ions was injected into the ESR storage ring at an energy of 50 MeV/u. The beam interacted with an internal hydrogen gas-jet target. An ultra-high vacuum compatible detector setup was installed around the gas jet inside the ring to measure the recoiling particles generated by nuclear reactions. \textbf{Results:} Multiple reaction channels were observed during the experiment. In particular, we present the results from studies on elastic and inelastic scattering, as well as the neutron transfer reaction ${}^{20}\mathrm{Ne}(p,d){}^{19}\mathrm{Ne}^*$. The experimental data were compared to calculations that took into account the most significant excited states, using a coupled-reaction channel approach. A very good agreement with the experimental data was achieved. \textbf{Conclusions:} The present results are the first demonstration of the investigation transfer reactions using detectors directly installed in the ring. This provides an important proof-of-principle for prospective studies with far-from-stability radioactive beams in the future.

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arXiv2024

Isochronous mass spectrometry at the RIKEN Rare-RI Ring facility

A dedicated isochronous storage ring, named the Rare-RI Ring, was constructed at the RI Beam Factory of RIKEN, aiming at precision mass measurements of nuclei located in uncharted territories of the nuclear chart. The Rare-RI Ring employs the isochronous mass spectrometry technique with the goal to achieve a relative mass precision of $10^{-6}$ within a measurement time of less than 1 ms. The performance of the facility was demonstrated through mass measurements of neutron-rich nuclei with well-known masses. Velocity or magnetic rigidity is measured for every particle prior to its injection into the ring, wherein its revolution time is accurately determined. The latter quantity is used to determine the mass of the particle, while the former one is needed for non-isochronicity corrections. Mass precisions on the order of $10^{-5}$ were achieved in the first commissioning, which demonstrates that Rare-RI Ring is a powerful tool for mass spectrometry of short-lived nuclei.

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arXiv2022

First application of mass measurement with the Rare-RI Ring reveals the solar r-process abundance trend at A=122 and A=123

The Rare-RI Ring (R3) is a recently commissioned cyclotron-like storage ring mass spectrometer dedicated to mass measurements of exotic nuclei far from stability at Radioactive Isotope Beam Factory (RIBF) in RIKEN. The first application of mass measurement using the R3 mass spectrometer at RIBF is reported. Rare isotopes produced at RIBF, $^{127}$Sn, $^{126}$In, $^{125}$Cd, $^{124}$Ag, $^{123}$Pd, were injected in R3. Masses of $^{126}$In, $^{125}$Cd, and $^{123}$Pd were measured whereby the mass uncertainty of $^{123}$Pd was improved. This is the first reported measurement with a new storage ring mass spectrometery technique realized at a heavy-ion cyclotron and employing individual injection of the pre-identified rare nuclei. The latter is essential for the future mass measurements of the rarest isotopes produced at RIBF. The impact of the new $^{123}$Pd result on the solar $r$-process abundances in a neutron star merger event is investigated by performing reaction network calculations of 20 trajectories with varying electron fraction $Y_e$. It is found that the neutron capture cross section on $^{123}$Pd increases by a factor of 2.2 and $β$-delayed neutron emission probability, $P_\mathrm{1n}$, of $^{123}$Rh increases by 14\%. The neutron capture cross section on $^{122}$Pd decreases by a factor of 2.6 leading to pileup of material at $A=122$, thus reproducing the trend of the solar $r$-process abundances. The trend of the two-neutron separation energies (S$_\mathrm{2n}$) was investigated for the Pd isotopic chain. The new mass measurement with improved uncertainty excludes large changes of the S$_\mathrm{2n}$ value at $N=77$. Such large increase of the S$_\mathrm{2n}$ values before $N=82$ was proposed as an alternative to the quenching of the $N=82$ shell gap to reproduce $r$-process abundances in the mass region of $A=112-124$.

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arXiv2021

Charge-changing cross sections for $^{42\textrm{--}51}$Ca and effect of charged-particle evaporation induced by neutron removal reaction

Charge-changing cross sections $σ_\mathrm{CC}$ for $^{42\textrm{--}51}$Ca on a carbon target at around 280~MeV/nucleon have been measured. The measured $σ_\mathrm{CC}$ values differ significantly from the previously developed calculations based on the Glauber model. However, through introduction of the charged-particle evaporation effect induced by the neutron-removal reaction in addition to the Glauber-model calculation, experimental $σ_\mathrm{CC}$ values on $^{12}$C at around 300~MeV/nucleon for nuclides from C to Fe isotopes are all reproduced with approximately 1\% accuracy. This proposed model systematically reproduces $σ_\mathrm{CC}$ data without phenomenological corrections, and can also explain experimental $σ_\mathrm{CC}$ values obtained in other energy regions.

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arXiv2021

Alpha-decay-correlated mass measurement of 206,207Ra using an $α$-TOF detector equipped MRTOF-MS system

The atomic masses of the isotopes $^{206,207}$Ra have been measured via decay-correlated mass spectroscopy using a multi-reflection time-of-flight mass spectrograph equipped with an $α$-TOF detector. The Ra isotopes were produced as fusion-evaporation products in the $^{51}$V+$^{159}$Tb reaction system and delivered by the gas-filled recoil ion separator GARIS-II at RIKEN. The $α$-TOF detector provides for high-accuracy mass measurements by correlating time-of-flight signals with subsequent $α$-decay events. The masses of $^{206}$Ra and $^{207g,m}$Ra were directly measured using a multi-reflection time-of-flight mass spectrograph equipped with an $α$-TOF detector. A mass excess of ME = 3538(15) keV/c$^2$ and an excitation energy of E$_{\rm ex}$ = 552(42) keV were determined. The $α$-decay branching ratio of $^{207m}$Ra, b$α$ = 0.26(20), was directly determined from decay-correlated time-of-flight signals, and the reduced alpha width of $^{207m}$Ra was calculated to be $δ^2$ = 50+62-41 keV from the branching ratio. The spin-parity of $^{207m}$Ra was confirmed to be $J^π$ = 13/2$^-$ from decay correlated mass measurement results.

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arXiv2021

First high-precision direct determination of the atomic mass of a superheavy nuclide

We present the first direct measurement of the atomic mass of a superheavy nuclide. Atoms of $^{257}$Db ($Z$=105) were produced online at the RIKEN Nishina Center for Accelerator-Based Science using the fusion-evaporation reaction $^{208}$Pb($^{51}$V, 2n)$^{257}$Db. The gas-filled recoil ion separator GARIS-II was used to suppress both the unreacted primary beam and some transfer products, prior to delivering the energetic beam of $^{257}$Db ions to a helium gas-filled ion stopping cell wherein they were thermalized. Thermalized $^{257}$Db$^{3+}$ ions were then transferred to a multi-reflection time-of-flight mass spectrograph for mass analysis. An alpha particle detector embedded in the ion time-of-flight detector allowed disambiguation of the rare $^{257}$Db$^{3+}$ time-of-flight detection events from background by means of correlation with characteristic $α$-decays. The extreme sensitivity of this technique allowed a precision atomic mass determination from 11 events. The mass excess was determined to be $100\,063(231)_\textrm{stat}(132)_\textrm{sys}$~keV/c$^2$. Comparing to several mass models, we show the technique can be used to unambiguously determine the atomic number as $Z$=105 and should allow similar evaluations for heavier species in future work.

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arXiv2020

Development and operation of an electrostatic time-of-flight detector for the Rare RI storage Ring

An electrostatic time-of-flight detector named E-MCP has been developed for quick diagnostics of circulating beam and timing measurement in mass spectrometry at the Rare-RI Ring in RIKEN. The E-MCP detector consists of a conversion foil, potential grids, and a microchannel plate. Secondary electrons are released from the surface of the foil when a heavy ion hits it. The electrons are accelerated and deflected by 90$^\circ$ toward the microchannel plate by electrostatic potentials. A thin carbon foil and a thin aluminum-coated mylar foil were used as conversion foils. We obtained time resolutions of 69(1) ps and 43(1) ps (standard deviation) for a $^{84}$Kr beam at an energy of 170 MeV/u when using the carbon and the aluminum-coated mylar foils, respectively. A detection efficiency of approximately 90% was obtained for both foils. The E-MCP detector equipped with the carbon foil was installed inside the Rare-RI Ring to confirm particle circulation within a demonstration experiment on mass measurements of nuclei around $^{78}$Ge produced by in-flight fission of uranium beam at the RI Beam Factory in RIKEN. Periodic time signals from circulating ions were clearly observed. Revolution times for $^{78}$Ge, $^{77}$Ga, and $^{76}$Zn were obtained. The results confirmed successful circulation of the short-lived nuclei inside the Rare-RI Ring.

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arXiv2019

Swelling of doubly magic $^{48}$Ca core in Ca isotopes beyond $N=28$

Interaction cross sections for $^{42\textrm{-}51}$Ca on a carbon target at 280 MeV/nucleon have been measured for the first time. The neutron number dependence of derived root-mean-square matter radii shows a significant increase beyond the neutron magic number $N=28$. Furthermore, this enhancement of matter radii is much larger than that of the previously measured charge radii, indicating a novel growth in neutron skin thickness. A simple examination based on the Fermi-type distribution, and the Mean-Field calculations point out that this anomalous enhancement of the nuclear size beyond $N=28$ results from an enlargement of the core by a sudden increase in the surface diffuseness of the neutron density distribution, which implies the swelling of the bare $^{48}$Ca core in Ca isotopes beyond $N=28$.

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arXiv2019

New Test of Modulated Electron Capture Decay of Hydrogen-Like $^{142}$Pm Ions: Precision Measurement of Purely Exponential Decay

An experiment addressing electron capture (EC) decay of hydrogen-like $^{142}$Pm$^{60+}$ ions has been conducted at the experimental storage ring (ESR) at GSI. The decay appears to be purely exponential and no modulations were observed. Decay times for about 9000 individual EC decays have been measured by applying the single-ion decay spectroscopy method. Both visually and automatically analysed data can be described by a single exponential decay with decay constants of 0.0126(7) s$^{-1}$ for automatic analysis and 0.0141(7) s$^{-1}$ for manual analysis. If a modulation superimposed on the exponential decay curve is assumed, the best fit gives a modulation amplitude of merely 0.019(15), which is compatible with zero and by 4.9 standard deviations smaller than in the original observation which had an amplitude of 0.23(4).

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arXiv2017

Evidence for Z=6 `magic number' in neutron-rich carbon isotopes

The nuclear shell structure, which originates in the nearly independent motion of nucleons in an average potential, provides an important guide for our understanding of nuclear structure and the underlying nuclear forces. Its most remarkable fingerprint is the existence of the so-called `magic numbers' of protons and neutrons associated with extra stability. Although the introduction of a phenomenological spin-orbit (SO) coupling force in 1949 helped explain the nuclear magic numbers, its origins are still open questions. Here, we present experimental evidence for the smallest SO-originated magic number (subshell closure) at the proton number 6 in 13-20C obtained from systematic analysis of point-proton distribution radii, electromagnetic transition rates and atomic masses of light nuclei. Performing ab initio calculations on 14,15C, we show that the observed proton distribution radii and subshell closure can be explained by the state-of-the-art nuclear theory with chiral nucleon-nucleon and three-nucleon forces, which are rooted in the quantum chromodynamics.

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arXiv2017

A new measurement of electron transverse polarization in polarized nuclear beta decay

The Mott polarimetry for T -Violation (MTV) experiment tests time-reversal symmetry in polarized nuclear beta decay by measuring an electron's transverse polarization as a form of angular asymmetry in Mott scattering using a thin metal foil. A Mott scattering analyzer system developed using a tracking detector to measure scattering angles offers better event selectivity than conventional counter experiments. In this paper, we describe a pilot experiment conducted at KEK-TRIAC using a prototype system with a polarized 8Li beam. The experiment confirmed the sound performance of our Mott analyzer system to measure T-violating triple correlation (R correlation), and therefore recommends its use in higher-precision experiments at the TRIUMF-ISAC.

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arXiv2016

Charge-changing-cross-section measurements of $^{12-16}$C at around $45A$ MeV and development of a Glauber model for incident energies $10A-2100A$ MeV

We have measured for the first time the charge-changing cross sections ($σ_{\text{CC}}$) of $^{12-16}$C on a $^{12}$C target at energies below $100A$ MeV. To analyze these low-energy data, we have developed a finite-range Glauber model with a global parameter set within the optical-limit approximation which is applicable to reaction cross section ($σ_{\text{R}}$) and $σ_{\text{CC}}$ measurements at incident energies from 10$A$ to $2100A$ MeV. Adopting the proton-density distribution of $^{12}$C known from the electron-scattering data, as well as the bare total nucleon-nucleon cross sections, and the real-to-imaginary-part ratios of the forward proton-proton elastic scattering amplitude available in the literatures, we determine the energy-dependent slope parameter $β_{\rm pn}$ of the proton-neutron elastic differential cross section so as to reproduce the existing $σ_{\text{R}}$ and interaction-cross-section data for $^{12}$C+$^{12}$C over a wide range of incident energies. The Glauber model thus formulated is applied to calculate the $σ_{\text{\tiny R}}$'s of $^{12}$C on a $^9$Be and $^{27}$Al targets at various incident energies. Our calculations show excellent agreement with the experimental data. Applying our model to the $σ_{\text{\tiny R}}$ and $σ_{\text{\tiny CC}}$ for the "neutron-skin" $^{16}$C nucleus, we reconfirm the importance of measurements at incident energies below $100A$ MeV. The proton root-mean-square radii of $^{12-16}$C are extracted using the measured $σ_{\text{CC}}$'s and the existing $σ_{\text{R}}$ data. The results for $^{12-14}$C are consistent with the values from the electron scatterings, demonstrating the feasibility, usefulness of the $σ_{\text{CC}}$ measurement and the present Glauber model.

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arXiv2016

Development of a fast plastic scintillation detector with time resolution of less than 10 ps

Timing-pick up detectors with excellent timing resolutions are essential in many modern nuclear physics experiments. Aiming to develop a Time-Of-Flight system with precision down to about 10 ps, we have made a systematic study of the timing characteristic of TOF detectors, which consist of several combinations of plastic scintillators and photomultiplier tubes. With the conventional electronics, the best timing resolution of about 5.1 ps (σ) has been achieved for detectors with an area size of 3x1 cm2. It is found that for data digitalization a combination of TAC and ADC can achieve a better time resolution than currently available TDC. Simultaneously measurements of both time and pulse height are very valuable for correction of time-walk effect.

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arXiv2012

Nuclear structure of 30S and its implications for nucleosynthesis in classical novae

The uncertainty in the 29P(p,gamma)30S reaction rate over the temperature range of 0.1 - 1.3 GK was previously determined to span ~4 orders of magnitude due to the uncertain location of two previously unobserved 3+ and 2+ resonances in the 4.7 - 4.8 MeV excitation region in 30S. Therefore, the abundances of silicon isotopes synthesized in novae, which are relevant for the identification of presolar grains of putative nova origin, were uncertain by a factor of 3. To investigate the level structure of 30S above the proton threshold (4394.9(7) keV), a charged-particle spectroscopy and an in-beam gamma-ray spectroscopy experiments were performed. Differential cross sections of the 32S(p,t)30S reaction were measured at 34.5 MeV. Distorted wave Born approximation calculations were performed to constrain the spin-parity assignments of the observed levels. An energy level scheme was deduced from gamma-gamma coincidence measurements using the 28Si(3He,n-gamma)30S reaction. Spin-parity assignments based on measurements of gamma-ray angular distributions and gamma-gamma directional correlation from oriented nuclei were made for most of the observed levels of 30S. As a result, the resonance energies corresponding to the excited states in 4.5 MeV - 6 MeV region, including the two astrophysically important states predicted previously, are measured with significantly better precision than before. The uncertainty in the rate of the 29P(p,gamma)30S reaction is substantially reduced over the temperature range of interest. Finally, the influence of this rate on the abundance ratios of silicon isotopes synthesized in novae are obtained via 1D hydrodynamic nova simulations.

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arXiv2008

Ground-state electric quadrupole moment of 31Al

Ground-state electric quadrupole moment of 31Al (I =5/2+, T_1/2 = 644(25) ms) has been measured by means of the beta-NMR spectroscopy using a spin-polarized 31Al beam produced in the projectile fragmentation reaction. The obtained Q moment, |Q_exp(31Al)| = 112(32)emb, are in agreement with conventional shell model calculations within the sd valence space. Previous result on the magnetic moment also supports the validity of the sd model in this isotope, and thus it is concluded that 31Al is located outside of the island of inversion.

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