D. Pavicevic | Searcharxiv

arXiv2025

Tunable narrowband THz generation in the organic crystal BNA

The generation of tunable narrowband pulses is increasingly being pursued in terahertz science, for example to study the nonlinear response of individual modes of solids and molecules. Here, we extend the chirp-and-delay method to achieve collinear phase-matched difference-frequency generation in the organic crystal N-benzyl-2-methyl-4-nitroaniline (BNA-S), which results in tunable narrowband terahertz pulses. In this configuration, the fundamental frequency of a Ti:sapphire amplifier is used - eliminating the need for optical parametric amplifiers typically required for THz generation in other organic crystals. Chirped-pulse excitation suppresses multiphoton absorption in BNA, improving stability and extending crystal lifetime. The source delivers THz transients tunable from 0.25 THz to 2.1 THz with adjustable spectral width.

physics.optics↗

arXiv2024

Squeezed Josephson plasmons in driven YBa$_2$Cu$_3$O$_{6+x}$

The physics of driven collective modes in quantum materials underpin a number of striking non-equilibrium functional responses, which include enhanced magnetism, ferroelectricity and superconductivity. However, the coherent coupling between multiple modes at once are difficult to capture by single-pump probe (one-dimensional) spectroscopy, and often remain poorly understood. One example is phonon-mediated amplification of Josephson plasmons in YBa$_2$Cu$_3$O$_{6+x}$, in which at least three normal modes of the solid are coherently mixed as a source of enhanced superconductivity. Here, we go beyond previous pump-probe experiments in this system and acquire two-dimensional frequency maps using pairs of mutually delayed, carrier envelope phase stable mid-infrared pump pulses, combined with measurements of the time-modulated second-order nonlinear optical susceptibility. We find that the driven zone-center phonons amplify coherent pairs of opposite-momentum Josephson plasma polaritons, generating a squeezed state of interlayer phase fluctuations. The squeezed state is a potentially important ingredient in the microscopic physics of photo-induced superconductivity in this and other materials.

cond-mat.supr-con↗