arXiv subjects
Publications and source records attributed to D. Qian.
The first normal emission experiment result on bcc Ni ultrathin film is presented in comparison with the one on fcc Ni. Its agreement with band structure calculation, by supplementing our former results on the magnetic properties of bcc Ni, verifies from the electronic viewpoint the successful epitaxy of this metastable phase of Ni which doesn't exist in nature.
Recently discovered class of cobaltate superconductors (Na0.3CoO2.nH2O) is a novel realization of interacting quantum electron systems in a triangular network with low-energy degrees of freedom. We employ angle-resolved photoemission spectroscopy to uncover the nature of microscopic electron motion in the parent superconductors for the first time. Results reveal a large hole-like Fermi surface (consistent with Luttinger theorem) generated by the crossing of super-heavy quasiparticles. The measured quasiparticle parameters collectively suggest a two orders of magnitude departure from the conventional Bardeen-Cooper-Schrieffer electron dynamics paradigm and unveils cobaltates as a rather hidden class of relatively high temperature superconductors.
Electron behavior in doped Mott systems continues to be a major unsolved problem in quantum many-electron physics. A central issue in understanding the universal Mott behavior in a variety of complex systems is to understand the nature of their electron-hole pair excitation modes. Using high resolution resonant inelastic x-ray scattering (RIXS) we resolve the momentum dependence of electron-hole pair excitations in two major classes of doped copper oxides which reveals a Mott pseudogap over the full Brillouin zone and over the entire phase diagram. The pair bandwidth and zone-boundary pair velocity renormalize on either sides of the phase diagram at very different rates indicating strong particle-hole doping asymmetries observed for the first time.
We present an angle-resolved photoemission study of Na0.7CoO2, the host cobaltate of the NaxCoO2.yH2O series. Our results show a large hexagonal-like hole-type Fermi surface, an extremely narrow strongly renormalized quasiparticle band and a small Fermi velocity. Along the Gamma to M high symmetry line, the quasiparticle band crosses the Fermi level from M toward Gamma consistent with a negative sign of effective single-particle hopping (t ): t is estimated to be about 8 meV which is on the order of exchange coupling J in this system. This suggests that t ~ J ~ 10 meV is an important energy scale in the system. Quasiparticles are well defined only in the T-linear resistivity regime. Small single particle hopping and unconventional quasiparticle dynamics may have implications for understanding the unusual behavior of this new class of compounds.