arXiv subjects

D. R. Grempel

Publications and source records attributed to D. R. Grempel.

At least 19 recordsLinked to original sources

arXiv2007

Disorder effects in the quantum Heisenberg model: An Extended Dynamical mean-field theory analysis

We investigate a quantum Heisenberg model with both antiferromagnetic and disordered nearest-neighbor couplings. We use an extended dynamical mean-field approach, which reduces the lattice problem to a self-consistent local impurity problem that we solve by using a quantum Monte Carlo algorithm. We consider both two- and three-dimensional antiferromagnetic spin fluctuations and systematically analyze the effect of disorder. We find that in three dimensions for any small amount of disorder a spin-glass phase is realized. In two dimensions, while clean systems display the properties of a highly correlated spin-liquid (where the local spin susceptibility has a non-integer power-low frequency and/or temperature dependence), in the present case this behavior is more elusive unless disorder is very small. This is because the spin-glass transition temperature leaves only an intermediate temperature regime where the system can display the spin-liquid behavior, which turns out to be more apparent in the static than in the dynamical susceptibility.

cond-mat.dis-nn↗

arXiv2006

Electron-Phonon Correlation Effects in Molecular Transistors

The interplay of electron-electron and electron-phonon interactions is studied analytically in the Kondo regime. A Holstein electron-phonon coupling is shown to produce a weakening of the gate voltage dependence of the Kondo temperature and may explain the observed anomalies in some of these devices. A molecular center-of-mass mode opens a new channel for charge and spin fluctuations and in the antiadabatic limit the latter are described by an asymmetric two-channel Kondo model. Below the Kondo temperature the system develops a dynamical Jahn-Teller distortion and a low energy peak emerges in the phonon spectral density that could be observed in Raman microscopy experiments.

cond-mat.str-el↗

arXiv2006

Universal Distribution of Kondo Temperatures in Dirty Metals

Kondo screening of diluted magnetic impurities in a disordered host is studied analytically and numerically in one, two and three dimensions. It is shown that in the T_K \to 0 limit the distribution of Kondo temperatures has a universal form, P(T_K) \sim T_K^{-α} that holds in the insulating phase and persists in the metallic phase close to the metal insulator transition. Moreover, the exponent αdepends only on the dimensionality. The most important consequence of this result is that the T-dependence of thermodynamic properties is smooth across the metal-insulator transition in three dimensional systems.

cond-mat.str-el↗

arXiv2005

Magnetic Quantum Phase Transitions in Kondo Lattices

The identification of magnetic quantum critical points in heavy fermion metals has provided an ideal setting for experimentally studying quantum criticality. Motivated by these experiments, considerable theoretical efforts have recently been devoted to reexamine the interplay between Kondo screening and magnetic interactions in Kondo lattice systems. A local quantum critical picture has emerged, in which magnetic interactions suppress Kondo screening precisely at the magnetic quantum critical point (QCP). The Fermi surface undergoes a large reconstruction across the QCP and the coherence scale of the Kondo lattice vanishes at the QCP. The dynamical spin susceptibility exhibits $ω/T$ scaling and non-trivial exponents describe the temperature and frequency dependence of various physical quantities. These properties are to be contrasted with the conventional spin-density-wave (SDW) picture, in which the Kondo screening is not suppressed at the QCP and the Fermi surface evolves smoothly across the phase transition. In this article we discuss recent microscopic studies of Kondo lattices within an extended dynamical mean field theory (EDMFT). We summarize the earlier work based on an analytical $ε$-expansion renormalization group method, and expand on the more recent numerical results. We also discuss the issues that have been raised concerning the magnetic phase diagram. We show that the zero-temperature magnetic transition is second order when double counting of the RKKY interactions is avoided in EDMFT.

cond-mat.str-el↗

arXiv2005

Magnetoconductance through a vibrating molecule in the Kondo regime

The effect of a magnetic field on the equilibrium spectral and transport properties of a single-molecule junction is studied using the numerical renormalization group method. The molecule is described by the Anderson-Holstein model in which a single vibrational mode is coupled to the electron density. The effect of an applied magnetic field on the conductance in the Kondo regime is qualitatively different in the weak and strong electron-phonon coupling regimes. In the former case, the Kondo resonance is split and the conductance is strongly suppressed by a magnetic field $g mu_B B \gtrsim k_BT_K$, with $T_K$ the Kondo temperature. In the strong electron-phonon coupling regime a charge analog of the Kondo effect develops. In this case the Kondo resonance is not split by the field and the conductance in the Kondo regime is enhanced in a broad range of values of $B$.

cond-mat.str-el↗

arXiv2004

Many Body Effects on the Transport Properties of Single-Molecule Devices

The conductance through a molecular device including electron-electron and electron-phonon interactions is calculated using the Numerical Renormalization Group method. At low temperatures and weak electron-phonon coupling the properties of the conductance can be explained in terms of the standard Kondo model with renormalized parameters. At large electron-phonon coupling a charge analog of the Kondo effect takes place that can be mapped into an anisotropic Kondo model. In this regime the molecule is strongly polarized by a gate voltage which leads to rectification in the current-voltage characteristics of the molecular junction.

cond-mat.str-el↗

arXiv2004

Quantum transport through a deformable molecular transistor

The linear transport properties of a model molecular transistor with electron-electron and electron-phonon interactions were investigated analytically and numerically. The model takes into account phonon modulation of the electronic energy levels and of the tunnelling barrier between the molecule and the electrodes. When both effects are present they lead to asymmetries in the dependence of the conductance on gate voltage. The Kondo effect is observed in the presence of electron-phonon interactions. There are important qualitative differences between the cases of weak and strong coupling. In the first case the standard Kondo effect driven by spin fluctuations occurs. In the second case, it is driven by charge fluctuations. The Fermi-liquid relation between the spectral density of the molecule and its charge is altered by electron-phonon interactions. Remarkably, the relation between the zero-temperature conductance and the charge remains unchanged. Therefore, there is perfect transmission in all regimes whenever the average number of electrons in the molecule is an odd integer.

cond-mat.mes-hall↗

arXiv2004

Strongly correlated regimes in a double quantum-dot device

The transport properties of a double quantum-dot device with one of the dots coupled to perfect conductors are analyzed using the numerical renormalization group technique and slave-boson mean-field theory. The coupling between the dots strongly influences the transport through the system leading to a non-monotonic dependence of the conductance as a function of the temperature and the magnetic field. For small inter-dot coupling and parameters such that both dots are in the Kondo regime, there is a two-stage screening of the dot's magnetic moments that is reflected in the conductance. In an intermediate temperature regime Kondo correlations develop on one of the dots and the conductance is enhanced. At low temperatures the Kondo effect takes place on the second dot leading to a singlet ground state in which the conductance is strongly suppressed.

cond-mat.mes-hall↗

arXiv2004

Heterogeneous dynamics of the three dimensional Coulomb glass out of equilibrium

The non-equilibrium relaxational properties of a three dimensional Coulomb glass model are investigated by kinetic Monte Carlo simulations. Our results suggest a transition from stationary to non-stationary dynamics at the equilibrium glass transition temperature of the system. Below the transition the dynamic correlation functions loose time translation invariance and electron diffusion is anomalous. Two groups of carriers can be identified at each time scale, electrons whose motion is diffusive within a selected time window and electrons that during the same time interval remain confined in small regions in space. During the relaxation that follows a temperature quench an exchange of electrons between these two groups takes place and the non-equilibrium excess of diffusive electrons initially present decreases logarithmically with time as the system relaxes. This bimodal dynamical heterogeneity persists at higher temperatures when time translation invariance is restored and electron diffusion is normal. The occupancy of the two dynamical modes is then stationary and its temperature dependence reflects a crossover between a low-temperature regime with a high concentration of electrons forming fluctuating dipoles and a high-temperature regime in which the concentration of diffusive electrons is high.

cond-mat.dis-nn↗

arXiv2004

Off-equilibrium dynamics of the two-dimensional Coulomb glass

The dynamics of the 2D Coulomb glass model is investigated by kinetic Monte Carlo simulation. An exponential divergence of the relaxation time signals a zero-temperature freezing transition. At low temperatures the dynamics of the system is glassy. The local charge correlations and the response to perturbations of the local potential show aging. The dynamics of formation of the Coulomb gap is slow and the density of states at the Fermi level decays in time as a power law. The relevance of these findings for recent transport experiments in Anderson-insulating films is pointed out.

cond-mat.dis-nn↗

arXiv2003

Effects of dissipation on disordered quantum spin models

We study the effects of the coupling to an Ohmic quantum reservoir on the static and dynamical properties of a family of disordered SU(2) spin models in a transverse magnetic field using a method of direct spin summation. The tendency to form a glassy phase increases with the strength of the coupling of the system to the environment. We study the influence of the environment on the features of the phase diagram of the various models as well as the stability of the possible phases.

cond-mat.dis-nn↗

arXiv2003

Continuous quantum phase transition in a Kondo lattice model

We study the magnetic quantum phase transition in an anisotropic Kondo lattice model. The dynamical competition between the RKKY and Kondo interactions is treated using an extended dynamic mean field theory (EDMFT) appropriate for both the antiferromagnetic and paramagnetic phases. A quantum Monte Carlo approach is used, which is able to reach very low temperatures, of the order of 1% of the bare Kondo scale. We find that the finite-temperature magnetic transition, which occurs for sufficiently large RKKY interactions, is first order. The extrapolated zero-temperature magnetic transition, on the other hand, is continuous and locally critical.

cond-mat.str-el↗

arXiv2003

Locally critical point in an anisotropic Kondo lattice

We report the first numerical identification of a locally quantum critical point, at which the criticality of the local Kondo physics is embedded in that associated with a magnetic ordering. We are able to numerically access the quantum critical behavior by focusing on a Kondo-lattice model with Ising anisotropy. We also establish that the critical exponent for the q-dependent dynamical spin susceptibility is fractional and compares well with the experimental value for heavy fermions.

cond-mat.str-el↗

arXiv2003

A large-N analysis of the local quantum critical point and the spin-liquid phase

We study analytically the Kondo lattice model with an additional nearest-neighbor antiferromagnetic interaction in the framework of large-N theory. We find that there is a local quantum critical point between two phases, a normal Fermi-liquid and a spin-liquid in which the spins are decoupled from the conduction electrons. The local spin susceptibility displays a power-law divergence throughout the spin liquid phase. We check the reliability of the large-N results by solving by quantum Monte Carlo simulation the N=2 spin-liquid problem with no conduction electrons and find qualitative agreement. We show that the spin-liquid phase is unstable at low temperatures, suggestive of a first-order transition to an ordered phase.

cond-mat.str-el↗

arXiv2002

Heavy-fermion and spin-liquid behavior in a Kondo lattice with magnetic frustration

We study the competition between the Kondo effect and frustrating exchange interactions in a Kondo-lattice model within a large-${\cal N}$ dynamical mean-field theory. We find a T=0 phase transition between a heavy Fermi-liquid and a spin-liquid for a critical value of the exchange $J_c = T_{K}^0$, the single-impurity Kondo temperature. Close to the critical point, the Fermi liquid coherence scale $T^\star$ is strongly reduced and the effective mass strongly enhanced. The regime $T>T^\star$ is characterized by spin-liquid magnetic correlations and non-Fermi-liquid properties. It is suggested that magnetic frustration is a general mechanism which is essential to explain the large effective mass of some metallic compounds such as LiV$_2$O$_4$.

cond-mat.str-el↗

arXiv2000

The Quantum Spherical p-Spin-Glass Model

We study a quantum extension of the spherical $p$-spin-glass model using the imaginary-time replica formalism. We solve the model numerically and we discuss two analytical approximation schemes that capture most of the features of the solution. The phase diagram and the physical properties of the system are determined in two ways: by imposing the usual conditions of thermodynamic equilibrium and by using the condition of marginal stability. In both cases, the phase diagram consists of two qualitatively different regions. If the transition temperature is higher than a critical value $T^{\star}$, quantum effects are qualitatively irrelevant and the phase transition is {\it second} order, as in the classical case. However, when quantum fluctuations depress the transition temperature below $T^{\star}$, the transition becomes {\it first order}. The susceptibility is discontinuous and shows hysteresis across the first order line, a behavior reminiscent of that observed in the dipolar Ising spin-glass LiHo$_x$Y$_{1-x}$F$_4$ in an external transverse magnetic field. We discuss in detail the thermodynamics and the stationary dynamics of both states. The spectrum of magnetic excitations of the equilibrium spin-glass state is gaped, leading to an exponentially small specific heat at low temperatures. That of the marginally stable state is gapless and its specific heat varies linearly with temperature, as generally observed in glasses at low temperature. We show that the properties of the marginally stable state are closely related to those obtained in studies of the real-time dynamics of the system weakly coupled to a quantum thermal bath. Finally, we discuss a possible application of our results to the problem of polymers in random media.

cond-mat.dis-nn↗

arXiv2000

Non-Fermi-Liquid Scaling in Ce(Ru_{0.5}Rh_{0.5})_2Si_2

We study the temperature and field dependence of the magnetic and transport properties of the non-Fermi-liquid compound Ce(Ru_{1-x}Rh_x)_2Si_2 at x=0.5. For fields $\lesssim $0.1T the experimental results show signatures of the presence of Kondo-disorder, expected to be large at this concentration. For larger fields, however, magnetic and transport properties are controlled by the coupling of the conduction electrons to critical spin-fluctuations. The temperature dependence of the susceptibility as well as the scaling properties of the magnetoresistance are in very good agreement with the predictions of recent dynamical mean-field theories of Kondo alloys close to a spin-glass quantum critical point.

cond-mat.str-el↗

arXiv2000

Coherence scale of the Kondo lattice

It is shown that the large-N approach yields two energy scales for the Kondo lattice model. The single-impurity Kondo temperature, $T_K$, signals the onset of local singlet formation, while Fermi liquid coherence sets in only below a lower scale, $T^{\star}$. At low conduction electron density $n_c$ ("exhaustion" limit), the ratio $T^{\star}/T_K$ is much smaller than unity, and is shown to depend only on $n_c$ and not on the Kondo coupling. The physical meaning of these two scales is demonstrated by computing several quantities as a function of $n_c$ and temperature.

cond-mat.str-el↗