arXiv subjects

D. Rugar

Publications and source records attributed to D. Rugar.

16 recordsLinked to original sources

arXiv2021

Merged-Element Transmons: Design and Qubit Performance

We have demonstrated a novel type of superconducting transmon qubit in which a Josephson junction has been engineered to act as its own parallel shunt capacitor. This merged-element transmon (MET) potentially offers a smaller footprint and simpler fabrication than conventional transmons. Because it concentrates the electromagnetic energy inside the junction, it reduces relative electric field participation from other interfaces. By combining micrometer-scale Al/AlOx/Al junctions with long oxidations and novel processing, we have produced functional devices with $E_{J}$/$E_{C}$ in the low transmon regime ($E_{J}$/$E_{C}$ $\lesssim$30). Cryogenic I-V measurements show sharp dI/dV structure with low sub-gap conduction. Qubit spectroscopy of tunable versions show a small number of avoided level crossings, suggesting the presence of two-level systems (TLS). We have observed mean T1 times typically in the range of 10-90 microseconds, with some annealed devices exhibiting T1 > 100 microseconds over several hours. The results suggest that energy relaxation in conventional, small-junction transmons is not limited by junction loss.

quant-ph↗

arXiv2015

Decoherence of near-surface nitrogen-vacancy centers due to electric field noise

We show that electric field noise from surface charge fluctuations can be a significant source of spin decoherence for near-surface nitrogen-vacancy (NV) centers in diamond. This conclusion is based on the increase in spin coherence observed when the diamond surface is covered with high-dielectric-constant liquids, such as glycerol. Double resonance experiments show that improved coherence occurs even though the coupling to nearby electron spins is unchanged when the liquid is applied. Multipulse spin echo experiments reveal the effect of glycerol on the spectrum of NV frequency noise.

cond-mat.mes-hall↗

arXiv2015

Multipulse Double-Quantum Magnetometry With Near-Surface Nitrogen Vacancy Centers

We discuss multipulse magnetometry that exploits all three magnetic sublevels of the S=1 nitrogen-vacancy center in diamond to achieve enhanced magnetic field sensitivity. Based on dual frequency microwave pulsing, the scheme works in arbitrary magnetic bias fields and is twice as sensitive to ac magnetic fields as conventional two-level magnetometry. We derive the spin evolution operator for dual frequency microwave excitation and show its effectiveness for double-quantum state swaps. Using multipulse sequences of up to 128 pulses under optimized conditions, we show enhancement of the SNR by up to a factor of 2 in detecting NMR statistical signals, with a 4 times enhancement theoretically possible.

cond-mat.mes-hall↗

arXiv2015

Spurious harmonic response of multipulse quantum sensing sequences

Multipulse sequences based on Carr-Purcell decoupling are frequently used for narrow-band signal detection in single spin magnetometry. We have analyzed the behavior of multipulse sensing sequences under real-world conditions, including finite pulse durations and the presence of detunings. We find that these non-idealities introduce harmonics to the filter function, allowing additional frequencies to pass the filter. In particular, we find that the XY family of sequences can generate signals at the 2fac, 4fac and 8fac harmonics and their odd subharmonics, where fac is the ac signal frequency. Consideration of the harmonic response is especially important for diamond-based nuclear spin sensing where the NMR frequency is used to identify the nuclear spin species, as it leads to ambiguities when several isotopes are present.

quant-ph↗

arXiv2014

Proton magnetic resonance imaging with a nitrogen-vacancy spin sensor

Nuclear magnetic resonance (NMR) imaging with nanometer resolution requires new detection techniques with sensitivity well beyond the capability of conventional inductive detection. Here, we demonstrate two dimensional imaging of $^1$H NMR from an organic test sample using a single nitrogen-vacancy center in diamond as the sensor. The NV center detects the oscillating magnetic field from precessing protons in the sample as the sample is scanned past the NV center. A spatial resolution of 12 nm is shown, limited primarily by the scan accuracy. With further development, NV-detected magnetic resonance imaging could lead to a new tool for three-dimensional imaging of complex nanostructures, including biomolecules.

cond-mat.mes-hall↗

arXiv2012

Detecting External Electron Spins Using Nitrogen-Vacancy Centers

Near-surface nitrogen-vacancy (NV) centers have been created in diamond through low energy implantation of 15N to sense electron spins that are external to the diamond. By performing double resonance experiments, we have verified the presence of g=2 spins on a diamond crystal that was subjected to various surface treatments, including coating with a polymer film containing the free radical 2,2-diphenyl-1-picrylhydrazyl (DPPH). Subsequent acid cleaning eliminated the spin signal without otherwise disrupting the NV center, providing strong evidence that the spins were at the surface. A clear correlation was observed between the size of the detected spin signal and the relaxation time T2 for the six NV centers studied. We have developed a model that takes into account the finite correlation time of the fluctuating magnetic fields generated by the external spins, and used it to infer the signal strength and correlation time of the magnetic fields from these spins. This model also highlights the sensitivity advantage of active manipulation of the longitudinal spin component via double resonance over passive detection schemes that measure the transverse component of spin.

cond-mat.mes-hall↗

arXiv2008

Force-detected nuclear double resonance between statistical spin polarizations

We demonstrate nuclear double resonance for nanometer-scale volumes of spins where random fluctuations rather than Boltzmann polarization dominate. When the Hartmann-Hahn condition is met in a cross-polarization experiment, flip-flops occur between two species of spins and their fluctuations become coupled. We use magnetic resonance force microscopy to measure this effect between 1H and 13C spins in 13C-enriched stearic acid. The development of a cross-polarization technique for statistical ensembles adds an important tool for generating chemical contrast in nanometer-scale magnetic resonance.

cond-mat.stat-mech↗

arXiv2008

Controlled Manipulation of Individual Vortices in a Superconductor

We report controlled local manipulation of single vortices by low temperature magnetic force microscope (MFM) in a thin film of superconducting Nb. We are able to position the vortices in arbitrary configurations and to measure the distribution of local depinning forces. This technique opens up new possibilities for the characterization and use of vortices in superconductors.

cond-mat.supr-con↗

arXiv2008

An off-board quantum point contact as a sensitive detector of cantilever motion

Recent advances in the fabrication of microelectromechanical systems (MEMS) and their evolution into nanoelectromechanical systems (NEMS) have allowed researchers to measure extremely small forces, masses, and displacements. In particular, researchers have developed position transducers with resolution approaching the uncertainty limit set by quantum mechanics. The achievement of such resolution has implications not only for the detection of quantum behavior in mechanical systems, but also for a variety of other precision experiments including the bounding of deviations from Newtonian gravity at short distances and the measurement of single spins. Here we demonstrate the use of a quantum point contact (QPC) as a sensitive displacement detector capable of sensing the low-temperature thermal motion of a nearby micromechanical cantilever. Advantages of this approach include versatility due to its off-board design, compatibility with nanoscale oscillators, and, with further development, the potential to achieve quantum limited displacement detection.

cond-mat.mes-hall↗

arXiv2007

Nuclear spin relaxation induced by a mechanical resonator

We report on measurements of the spin lifetime of nuclear spins strongly coupled to a micromechanical cantilever as used in magnetic resonance force microscopy. We find that the rotating-frame correlation time of the statistical nuclear polarization is set by the magneto-mechanical noise originating from the thermal motion of the cantilever. Evidence is based on the effect of three parameters: (1) the magnetic field gradient (the coupling strength), (2) the Rabi frequency of the spins (the transition energy), and (3) the temperature of the low-frequency mechanical modes. Experimental results are compared to relaxation rates calculated from the spectral density of the magneto-mechanical noise.

cond-mat.mes-hall↗

arXiv2007

The role of spin noise in the detection of nanoscale ensembles of nuclear spins

When probing nuclear spins in materials on the nanometer scale, random fluctuations of the spin polarization will exceed the mean Boltzmann polarization for sample volumes below about (100nm)^3. In this work, we use magnetic resonance force microscopy to observe nuclear spin fluctuations in real time. We show how reproducible measurements of the polarization variance can be obtained by controlling the spin correlation time and rapidly sampling a large number of independent spin configurations. A protocol to periodically randomize the spin ensemble is demonstrated, allowing significant improvement in the signal-to-noise ratio for nanometer-scale magnetic resonance imaging.

cond-mat.mes-hall↗

arXiv2007

Nuclear magnetic resonance force microscopy with a microwire rf source

We use a 1.0-um-wide patterned Cu wire with an integrated nanomagnetic tip to measure the statistical nuclear polarization of 19F in CaF2 by magnetic resonance force microscopy (MRFM). With less than 350 uW of dissipated power, we achieve rf magnetic fields over 4 mT at 115 MHz for a sample positioned within 100 nm of the "microwire" rf source. A 200-nm diameter FeCo tip integrated onto the wire produces field gradients greater than 10^5 T/m at the same position. The large rf fields from the broadband microwire enable long rotating-frame spin lifetimes of up to 15 s at 4 K.

cond-mat.other↗

arXiv2007

Nuclear Magnetic Resonance Imaging with 90 nm Resolution

Magnetic resonance imaging, based on the manipulation and detection of nuclear spins, is a powerful imaging technique that typically operates on the scale of millimeters to microns. Using magnetic resonance force microscopy, we have demonstrated that magnetic resonance imaging of nuclear spins can be extended to a spatial resolution better than 100 nm. The two-dimensional imaging of 19F nuclei was done on a patterned CaF2 test object, and was enabled by a detection sensitivity of roughly 1200 nuclear spins. To achieve this sensitivity, we developed high-moment magnetic tips that produced field gradients up to 1.4x10^6 T/m, and implemented a measurement protocol based on force-gradient detection of naturally occurring spin fluctuations. The resulting detection volume of less than 650 zl represents 60,000x smaller volume than previous NMR microscopy and demonstrates the feasibility of pushing magnetic resonance imaging into the nanoscale regime.

cond-mat.other↗

arXiv2007

Feedback cooling of a cantilever's fundamental mode below 5 mK

We cool the fundamental mechanical mode of an ultrasoft silicon cantilever from a base temperature of 2.2 K to 2.9 +/- 0.3 mK using active optomechanical feedback. The lowest observed mode temperature is consistent with limits determined by the properties of the cantilever and by the measurement noise. For high feedback gain, the driven cantilever motion is found to suppress or "squash" the optical interferometer intensity noise below the shot noise level.

cond-mat.other↗

arXiv2004

Electron spin detection in the frequency domain under the interrupted Oscillating Cantilever-driven Adiabatic Reversal (iOSCAR) Protocol

Magnetic Resonance Force Microscopy (MRFM) is an emergent technology for measuring spin-induced attonewton forces using a micromachined cantilever. In the interrupted Oscillating Cantilever-driven Adiabatic Reversal (iOSCAR) method, small ensembles of electron spins are manipulated by an external radio frequency (RF) magnetic field to produce small periodic deviations in the resonant frequency of the cantilever. These deviations can be detected by frequency demodulation, followed by conventional amplitude or energy detection. In this paper, we develop optimal detectors for several signal models that have been hypothesized for measurements induced by iOSCAR spin manipulation. We show that two simple variants of the energy detector--the filtered energy detector and a hybrid filtered energy/amplitude/energy detector--are approximately asymptotically optimal for the Discrete-Time (D-T) random telegraph signal model assuming White Gaussian Noise (WGN). For the D-T random walk signal model, the filtered energy detector performs close to the optimal Likelihood Ratio Test (LRT) when the transition probabilities are symmetric.

quant-ph↗

arXiv2003

Spin Relaxation Caused by Thermal Excitations of High Frequency Modes of Cantilever Vibrations

We consider the process of spin relaxation in the oscillating cantilever-driven adiabatic reversals technique in magnetic resonance force microscopy. We simulated the spin relaxation caused by thermal excitations of the high frequency cantilever modes in the region of the Rabi frequency of the spin sub-system. The minimum relaxation time obtained in our simulations is greater but of the same order of magnitude as one measured in recent experiments. We demonstrated that using a cantilever with nonuniform cross-sectional area may significantly increase spin relaxation time.

quant-ph↗