arXiv subjects

D. Sanvitto

Publications and source records attributed to D. Sanvitto.

At least 37 records · Page 2Linked to original sources

arXiv2018

Tunable out-of-plane excitons in 2D single crystal perovskites

Hybrid organic-inorganic perovskites have emerged as very promising materials for photonic applications, thanks to the great synthetic versatility that allows to tune their optical properties. In the two-dimensional (2D) crystalline form, these materials behave as multiple quantum-well heterostructures with stable excitonic resonances up to room temperature. In this work strong light-matter coupling in 2D perovskite single-crystal flakes is observed, and the polarization-dependent exciton-polariton response is used to disclose new excitonic features. For the first time, an out-of-plane component of the excitons is observed, unexpected for such 2D systems and completely absent in other layered materials, such as transition-metal dichalcogenides. By comparing different hybrid perovskites with the same inorganic layer but different organic interlayers, it is shown how the nature of the organic ligands controllably affects the out-of-plane exciton-photon coupling. Such vertical dipole coupling is particularly sought in those systems, e.g. plasmonic nanocavities, in which the direction of the field is usually orthogonal to the material sheet. Organic interlayers are shown to affect also the strong birefringence associated to the layered structure, which is exploited in this work to completely rotate the linear polarization degree in only few microns of propagation, akin to what happens in metamaterials.

cond-mat.mes-hall↗

arXiv2018

Superluminal X-waves in a polariton quantum fluid

In this work we experimentally demonstrate for the first time spontaneous generation of two-dimensional exciton-polariton X-waves. X-waves belong to the family of localized packets, which are capable of sustaining their shape with no spreading even in the linear regime. This allows to keep the packet shape and size for very low densities and very long times compared, for instance, to soliton waves, which always necessitate a nonlinearity to compensate the diffusion. Here we exploit the polariton nonlinearity and unique structured dispersion, comprising both positive- and negative-mass curvatures, to trigger an asymmetric four wave mixing in the momentum space. This ultimately enables self-formation of a spatial X-wave front. By means of ultrafast imaging experiments we observe the early reshaping of the initial Gaussian packet into the X-pulse and its propagation even for vanishing small densities. This allows us to outline the crucial effects and parameters driving the phenomena and to tune the degree of peak superluminal propagation, which we found to be in a good agreement with numerical simulations.

cond-mat.other↗

arXiv2016

The colored Hanbury Brown--Twiss effect

The Hanbury Brown--Twiss effect is one of the celebrated phenomenologies of modern physics that accommodates equally well classical (interferences of waves) and quantum (correlations between indistinguishable particles) interpretations. The effect was discovered in the late thirties with a basic observation of Hanbury Brown that radio-pulses from two distinct antennas generate signals on the oscilloscope that wiggle similarly to the naked eye. When Hanbury Brown and his mathematician colleague Twiss took the obvious step to propose bringing the effect in the optical range, they met with considerable opposition as single-photon interferences were deemed impossible. The Hanbury Brown--Twiss effect is nowadays universally accepted and, being so fundamental, embodies many subtleties of our understanding of the wave/particle dual nature of light. Thanks to a novel experimental technique, we report here a generalized version of the Hanbury Brown--Twiss effect to include the frequency of the detected light, or, from the particle point of view, the energy of the detected photons. In addition to the known tendencies of indistinguishable photons to arrive together on the detector, we find that photons of different colors present the opposite characteristic of avoiding each others. We postulate that fermions can be similarly brought to exhibit positive (boson-like) correlations by frequency filtering.

quant-ph↗

arXiv2016

Spontaneous rotating vortex rings in a parametrically driven polariton fluid

We present the theoretical prediction of spontaneous rotating vortex rings in a parametrically driven quantum fluid of polaritons -- coherent superpositions of coupled quantum well excitons and microcavity photons. These rings arise not only in the absence of any rotating drive, but also in the absence of a trapping potential, in a model known to map quantitatively to experiments. We begin by proposing a novel parametric pumping scheme for polaritons, with circular symmetry and radial currents, and characterize the resulting nonequilibrium condensate. We show that the system is unstable to spontaneous breaking of circular symmetry via a modulational instability, following which a vortex ring with large net angular momentum emerges, rotating in one of two topologically distinct states. Such rings are robust and carry distinctive experimental signatures, and so they could find applications in the new generation of polaritonic devices.

cond-mat.quant-gas↗

arXiv2015

Polariton superfluids reveal quantum hydrodynamic solitons

A quantum fluid passing an obstacle behaves differently from a classical one. When the flow is slow enough, the quantum gas enters a superfluid regime and neither whirlpools nor waves form around the obstacle. For higher flow velocities, it has been predicted that the perturbation induced by the defect gives rise to the turbulent emission of quantised vortices and to the nucleation of solitons. Using an interacting Bose gas of exciton-polaritons in a semiconductor microcavity, we report the transition from superfluidity to the hydrodynamic formation of oblique dark solitons and vortex streets in the wake of a potential barrier. The direct observation of these topological excitations provides key information on the mechanisms of superflow and shows the potential of polariton condensates for quantum turbulence studies.

cond-mat.quant-gas↗

arXiv2015

Vortex and half-vortex dynamics in a spinor quantum fluid of interacting polaritons

Spinorial or multi-component Bose-Einstein condensates may sustain fractional quanta of circulation, vorticant topological excitations with half integer windings of phase and polarization. Matter-light quantum fluids, such as microcavity polaritons, represent a unique test bed for realising strongly interacting and out-of-equilibrium condensates. The direct access to the phase of their wavefunction enables us to pursue the quest of whether half vortices ---rather than full integer vortices--- are the fundamental topological excitations of a spinor polariton fluid. Here, we are able to directly generate by resonant pulsed excitations, a polariton fluid carrying either the half or full vortex states as initial condition, and to follow their coherent evolution using ultrafast holography. Surprisingly we observe a rich phenomenology that shows a stable evolution of a phase singularity in a single component as well as in the full vortex state, spiraling, splitting and branching of the initial cores under different regimes and the proliferation of many vortex anti-vortex pairs in self generated circular ripples. This allows us to devise the interplay of nonlinearity and sample disorder in shaping the fluid and driving the phase singularities dynamics

cond-mat.quant-gas↗

arXiv2015

Exciting polaritons with quantum light

We discuss the excitation of polaritons---strongly-coupled states of light and matter---by quantum light, instead of the usual laser or thermal excitation. As one illustration of the new horizons thus opened, we introduce Mollow spectroscopy, a theoretical concept for a spectroscopic technique that consists in scanning the output of resonance fluorescence onto an optical target, from which weak nonlinearities can be read with high precision even in strongly dissipative environments.

cond-mat.mes-hall↗

arXiv2015

Real-space collapse of a polariton condensate

Polaritons in microcavities are versatile quasi-2D bosonic particles with a high degree of coherence and strong nonlinearities, thanks to their hybrid light-matter character. In their condensed form, they display striking quantum hydrodynamic features analogous to atomic Bose-Einstein condensates, such as long-range order coherence, superfluidity and quantized vorticity. Their variegated dispersive and dissipative properties, however, set significant differences from their atomic counterpart. In this work, we report the unique phenomenology that is observed when a pulse of light impacts the polariton vacuum: the condensate that is instantaneously formed does not splash in real space but instead coheres into an enigmatic structure, featuring concentric rings and, most notably, a sharp and bright peak at the center. Using a state-of-the-art ultrafast imaging with 50 fs time steps, we are able to track the dynamics of the polariton mean-field wavefunction in both real and reciprocal space. The observation of the real-space collapse of the condensate into an extremely localized---resolution limited---peak is at odd with the repulsive interactions of polaritons and their positive effective mass. An unconventional mechanism is therefore at play to account for our observations. Our modeling suggests that self-trapping due to a local heating of the crystal lattice---that can be described as a collective polaron formed by a polariton condensate---could be involved. These observations hint at the fascinating fluid dynamics of polaritons in conditions of extreme intensities and ultrafast times.

cond-mat.quant-gas↗

arXiv2015

On multicomponent polariton superfluidity in the optical parametric oscillator regime

Superfluidity, the ability of a liquid or gas to flow with zero viscosity, is one of the most remarkable implications of collective quantum coherence. In equilibrium systems like liquid 4He and ultracold atomic gases, superfluid behaviour conjugates diverse yet related phenomena, such as persistency of metastable flow in multiply connected geometries and the existence of a critical velocity for frictionless flow when hitting a static defect. The link between these different aspects of superfluid behaviour is far less clear in driven-dissipative systems displaying collective coherence, such as microcavity polaritons, which raises important questions about their concurrency. With a joint theoretical and experimental study, we show that the scenario is particularly rich for polaritons driven in a three-fluid collective coherent regime so-called optical parametric oscillator. On the one hand, the spontaneous macroscopic coherence following the phase locking of the signal and idler fluids has been shown to be responsible for their simultaneous quantized flow metastability. On the other hand, we show here that pump, signal and idler have distinct responses when hitting a static defect; while the signal displays hardly appreciable modulations, the ones appearing in pump and idler are determined by their mutual coupling due to nonlinear and parametric processes.

cond-mat.mes-hall↗

arXiv2014

Spanning the full Poincaré sphere with polariton Rabi oscillations

We propose theoretically and demonstrate experimentally a generation of light pulses whose polarization varies temporally to cover selected areas of the Poincaré sphere with tunable swirling speed and total duration (1 ps and 10 ps respectively in our implementation). The effect relies on the Rabi oscillations of two polarized fields in the strong coupling regime, excited by two counter-polarized and delayed pulses. The interferences of the oscillating fields result in the precession of the Stokes vector of the emitted light while polariton lifetime imbalance results in its drift from a circle on the sphere of controllable radius to a single point at long times. The positioning of the initial and final states allows to engineer the type of polarization spanning, including a full sweeping of the Poincaré sphere. The universality and simplicity of the scheme should allow for the deployment of time varying polarization fields at a technologically exploitable level.

cond-mat.quant-gas↗

arXiv2014

An acoustic black hole in a stationary hydrodynamic flow of microcavity polaritons

We report an experimental study of superfluid hydrodynamic effects in a one-dimensional polariton fluid flowing along a laterally patterned semiconductor microcavity and hitting a micron-sized engineered defect. At high excitation power, superfluid propagation effects are observed in the polariton dynamics, in particular, a sharp acoustic horizon is formed at the defect position, separating regions of sub- and super-sonic flow. Our experimental findings are quantitatively reproduced by theoretical calculations based on a generalized Gross-Pitaevskii equation. Promising perspectives to observe Hawking radiation via photon correlation measurements are illustrated.

cond-mat.mes-hall↗

arXiv2014

Ultrafast control of Rabi oscillations in a polariton condensate

We report the experimental observation and control of space and time-resolved light-matter Rabi oscillations in a microcavity. Our setup precision and the system coherence are so high that coherent control can be implemented with amplification or switching off of the oscillations and even erasing of the polariton density by optical pulses. The data is reproduced by a fundamental quantum optical model with excellent accuracy, providing new insights on the key components that rule the polariton dynamics.

cond-mat.quant-gas↗

arXiv2014

Comment on "Linear wave dynamics explains observations attributed to dark-solitons in a polariton quantum fluid"

In a recent preprint (arXiv:1401.1128v1) Cilibrizzi and co-workers report experiments and simulations showing the scattering of polaritons against a localised obstacle in a semiconductor microcavity. The authors observe in the linear excitation regime the formation of density and phase patterns reminiscent of those expected in the non-linear regime from the nucleation of dark solitons. Based on this observation, they conclude that previous theoretical and experimental reports on dark solitons in a polariton system should be revised. Here we comment why the results from Cilibrizzi et al. take place in a very different regime than previous investigations on dark soliton nucleation and do not reproduce all the signatures of its rich nonlinear phenomenology. First of all, Cilibrizzi et al. consider a particular type of radial excitation that strongly determines the observed patterns, while in previous reports the excitation has a plane-wave profile. Most importantly, the nonlinear relation between phase jump, soliton width and fluid velocity, and the existence of a critical velocity with the time-dependent formation of vortex-antivortex pairs are absent in the linear regime. In previous reports about dark soliton and half-dark soliton nucleation in a polariton fluid, the distinctive dark soliton physics is supported both by theory (analytical and numerical) and experiments (both continuous wave and pulsed excitation).

physics.optics↗

arXiv2013

Effect of Interactions on Vortices in a Non-equilibrium Polariton Condensate

We demonstrate the creation of vortices in a macroscopically occupied polariton state formed in a semiconductor microcavity. A weak external laser beam carrying orbital angular momentum (OAM) is used to imprint a vortex on the condensate arising from the polariton optical parametric oscillator (OPO). The vortex core radius is found to decrease with increasing pump power, and is determined by polariton-polariton interactions. As a result of OAM conservation in the parametric scattering process, the excitation consists of a vortex in the signal and a corresponding anti-vortex in the idler of the OPO. The experimental results are in good agreement with a theoretical model of a vortex in the polariton OPO.

physics.optics↗

arXiv2013

Vortex stability and permanent flow in nonequilibrium polariton condensates

We study the effects of imprinting a single-quantized vortex on the steady state of a microcavity exciton-polariton condensate generated via parametric scattering. Interestingly we observe two distinct regimes: In the first case, at low polariton densities, the effect of the pulsed probe, containing the vortex state, is to generate a gain response in the condensate lasting for tens of picoseconds during which no dissipation of the circulating currents is detected. In the second regime, at higher densities, the gain lasts much less and the circulation is imprinted directly into the steady state, which acquires permanent rotation for as long as the vortex remains within the condensate. We use two different ways of measuring the circulation of the condensate and demonstrate that in both cases, polariton condensation in the parametric scattering regime can sustain permanent supercurrents.

cond-mat.mes-hall↗

arXiv2013

Motion of spin polariton bullets in semiconductor microcavities

The dynamics of optical switching in semiconductor microcavities in the strong coupling regime is studied using time- and spatially-resolved spectroscopy. The switching is triggered by polarised short pulses which create spin bullets of high polariton density. The spin packets travel with speeds of the order of 106 m/s due to the ballistic propagation and drift of exciton-polaritons from high to low density areas. The speed is controlled by the angle of incidence of the excitation beams, which changes the polariton group velocity.

cond-mat.mes-hall↗

arXiv2013

Control and ultrafast dynamics of a two-fluid polariton switch

We investigate the cross-interactions in a two-component polariton quantum fluid coherently driven by two independent pumping lasers tuned at different energies and momenta. We show that both the hysteresis cycles and the ON/OFF threshold of one polariton signal can be entirely controlled by a second polariton fluid. Furthermore, we study the ultrafast switching dynamics of a driven polariton state, demonstrating the ability to control the polariton population with an external laser pulse, in less than a few picoseconds.

cond-mat.mes-hall↗

arXiv2012

Propagation and amplification dynamics of 1D polariton condensates

The dynamics of propagating polariton condensates in one-dimensional microcavities is investigated through time resolved experiments. We find a strong increase in the condensate intensity when it travels through the non-resonantly excited area. This amplification is shown to come from bosonic stimulated relaxation of reservoir excitons into the polariton condensate, allowing for the repopulation of the condensate through non-resonant pumping. Thus, we experimentally demonstrate a polariton amplifier with a large band width, opening the way towards the transport of polaritons with high densities over macroscopic distances.

cond-mat.quant-gas↗