arXiv subjects

D. Schweitzer

Publications and source records attributed to D. Schweitzer.

18 recordsLinked to original sources

arXiv2024

Orders of Magnitude Improved Cyclotron-Mode Cooling for Non-Destructive Spin Quantum Transition Spectroscopy with Single Trapped Antiprotons

We demonstrate efficient sub-thermal cooling of the modified cyclotron mode of a single trapped antiproton and reach particle temperatures $T_+=E_+/k_\text{B}$ below $200\,$mK in preparation times shorter than $500\,$s. This corresponds to the fastest resistive single-particle cyclotron cooling to sub-thermal temperatures ever demonstrated. By cooling trapped particles to such low energies, we demonstrate the detection of antiproton spin transitions with an error-rate $<0.000025$, more than three orders of magnitude better than in previous best experiments. This method will have enormous impact on multi-Penning-trap experiments that measure magnetic moments with single nuclear spins for tests of matter/antimatter symmetry, high-precision mass-spectrometry, and measurements of electron $g$-factors bound to highly-charged ions that test quantum electrodynamics.

physics.atom-ph↗

arXiv2023

Image-current mediated sympathetic laser cooling of a single proton in a Penning trap down to 170 mK axial temperature

We demonstrate a new temperature record for image-current mediated sympathetic cooling of a single proton in a cryogenic Penning trap by laser-cooled $^9$Be$^+$. An axial mode temperature of 170 mK is reached, which is a 15-fold improvement compared to the previous best value. Our cooling technique is applicable to any charged particle, so that the measurements presented here constitute a milestone towards the next generation of high-precision Penning-trap measurements with exotic particles.

physics.atom-ph↗

arXiv2023

Ultra thin polymer foil cryogenic window for antiproton deceleration and storage

We present the design and characterisation of a cryogenic window based on an ultra-thin aluminised PET foil at T < 10K, which can withstand a pressure difference larger than 1bar at a leak rate < $1\times 10^{-9}$ mbar$\cdot$ l/s. Its thickness of approximately 1.7 $μ$m makes it transparent to various types of particles over a broad energy range. To optimise the transfer of 100keV antiprotons through the window, we tested the degrading properties of different aluminium coated PET foils of thicknesses between 900nm and 2160nm, concluding that 1760nm foil decelerates antiprotons to an average energy of 5 keV. We have also explicitly studied the permeation as a function of coating thickness and temperature, and have performed extensive thermal and mechanical endurance and stress tests. Our final design integrated into the experiment has an effective open surface consisting of 7 holes with 1 mm diameter and will transmit up to 2.5% of the injected 100keV antiproton beam delivered by the AD/ELENA-facility of CERN.

physics.ins-det↗

arXiv2020

A stringent upper limit on the direct 3$α$ decay of the Hoyle State in $^{12}$C

We investigate an implication of the most recent observation of a second $J^π= 2^+$ state in $^{12}$C, which was measured using the $^{12}$C($γ$,$α$)$^8$Be$_{\textrm{(g.s.)}}$ reaction. In addition to the dissociation of $^{12}$C to an $α$-particle and $^8$Be in its ground state, a small fraction of events (2%) were identified as direct decays and decays to excited states in $^8$Be. This allowed a limit on the direct 3$α$ partial decay width to be determined as $Γ_{3α} < 32(4)$ keV. Since this 2$^+$ state is predicted by all theoretical models to be a collective excitation of the Hoyle state, the 3$α$ partial width of the Hoyle state is calculable from the ratio of 3$α$ decay penetrabilities of the Hoyle and 2$^+$ states. This was calculated using the semi-classical WKB approach and we deduce a stringent upper limit for the direct decay branching ratio of the Hoyle state of ${Γ_{3α} \over Γ} < 5.7 \times 10^{-6}$, over an order of magnitude lower than previously reported. This result places the direct measurement of this rare decay mode beyond current experimental capabilities.

nucl-ex↗

arXiv2018

Time Projection Chamber (TPC) Detectors for Nuclear Astrophysics Studies With Gamma Beams

Gamma-Beams at the HIgS facility in the USA and anticipated at the ELI-NP facility, now constructed in Romania, present unique new opportunities to advance research in nuclear astrophysics; not the least of which is resolving open questions in oxygen formation during stellar helium burning via a precise measurement of the 12C(a,g) reaction. Time projection chamber (TPC) detectors operating with low pressure gas (as an active target) are ideally suited for such studies. We review the progress of the current research program and plans for the future at the HIγS facility with the optical readout TPC (O-TPC) and the development of an electronic readout TPC for the ELI-NP facility (ELITPC).

physics.ins-det↗

arXiv2016

Pressure-dependent optical investigations of $α$-(BEDT-TTF)$_2$I$_3$: tuning charge order and narrow gap towards a Dirac semimetal

Infrared optical investigations of $α$-(BEDT-TTF)$_2$I$_3$ have been performed in the spectral range from 80 to 8000~cm$^{-1}$ down to temperatures as low as 10~K by applying hydrostatic pressure. In the metallic state, $T > 135$~K, we observe a 50\% increase in the Drude contribution as well as the mid-infrared band due to the growing intermolecular orbital overlap with pressure up to 11~kbar. In the ordered state, $T<T_{\rm CO}$, we extract how the electronic charge per molecule varies with temperature and pressure: Transport and optical studies demonstrate that charge order and metal-insulator transition coincide and consistently yield a linear decrease of the transition temperature $T_{\rm CO}$ by $8-9$~K/kbar. The charge disproportionation $Δρ$ diminishes by $0.017~e$/kbar and the optical gap $Δ$ between the bands decreases with pressure by -47~cm$^{-1}$/kbar. In our high-pressure and low-temperature experiments, we do observe contributions from the massive charge carriers as well as from massless Dirac electrons to the low-frequency optical conductivity, however, without being able to disentangle them unambiguously.

cond-mat.str-el↗

arXiv2015

Ferroelectric properties of charge-ordered alpha-(BEDT-TTF)2I3

A detailed investigation of the out-of-plane electrical properties of charge-ordered alpha-(BEDT-TTF)2I3 provides clear evidence for ferroelectricity. Similar to multiferroic alpha-(BEDT-TTF)2Cu[N(CN)2]Cl, the polar order in this material is ascribed to the occurrence of bond- and site-centered charge order. Dielectric response typical for relaxor ferroelectricity is found deep in the charge-ordered state. We suggest an explanation in terms of the existence of polar and nonpolar stacks of the organic molecules in this material, preventing long-range ferroelectricity. The results are discussed in relation to the formation or absence of electronic polar order in related charge-transfer salts.

cond-mat.str-el↗

arXiv2012

Cooperative dynamics in charge-ordered state of alpha-(BEDT-TTF)2I3

Electric-field-dependent pulse measurements are reported in the charge-ordered state of alpha-(BEDT-TTF)2I3. At low electric fields up to about 50 V/cm only negligible deviations from Ohmic behavior can be identified with no threshold field. At larger electric fields and up to about 100 V/cm a reproducible negative differential resistance is observed with a significant change in shape of the measured resistivity in time. These changes critically depend whether constant voltage or constant current is applied to the single crystal. At high enough electric fields the resistance displays a dramatic drop down to metallic values and relaxes subsequently in a single-exponential manner to its low-field steady-state value. We argue that such an electric-field induced negative differential resistance and switching to transient states are fingerprints of cooperative domain-wall dynamics inherent to two-dimensional bond-charge density wave with ferroelectric-like nature.

cond-mat.str-el↗

arXiv2011

Electrodynamic Response of the Charge Ordering Phase: Dielectric and Optical Studies of alpha-(BEDT-TTF)2I3

We report on the anisotropic response, the charge and lattice dynamics of normal and charge-ordered phases with horizontal stripes in single crystals of the organic conductor alpha-(BEDT-TTF)2I3 determined by dc resistivity, dielectric and optical spectroscopy. An overdamped Drude response and a small conductivity anisotropy observed in optics is consistent with a weakly temperature dependent dc conductivity and anisotropy at high temperatures. The splitting of the molecular vibrations nu27(Bu) evidences the abrupt onset of static charge order below TCO=136 K. The drop of optical conductivity measured within the ab plane of the crystal is characterized by an isotropic gap that opens of approximately 75 meV with several phonons becoming pronounced below. Conversely, the dc conductivity anisotropy rises steeply, attaining at 50 K a value 25 times larger than at high temperatures. The dielectric response within this plane reveals two broad relaxation modes of strength Deltaepsilon_LD ~= 5000 and Deltaepsilon_SD ~= 400, centered at 1 kHz < f_LD < 100 MHz and f_SD ~= 1 MHz. The anisotropy of the large-mode (LD) mean relaxation time closely follows the temperature behavior of the respective dc conductivity ratio. We argue that this phason-like excitation is best described as a long-wavelength excitation of a 2kF bond-charge density wave expected theoretically for layered quarter-filled electronic systems with horizontal stripes. Conversely, based on the theoretically expected ferroelectric-like nature of the charge-ordered phase, we associate the small-mode (SD) relaxation with the motion of domain-wall pairs, created at the interface between two types of domains, along the a and b axes. We also consider other possible theoretical interpretations and discuss their limitations.

cond-mat.str-el↗

arXiv2010

Collective Excitations in the Charge-Ordered Phase of alpha-(BEDT-TTF)2I3

The charge response of charge-ordered state in the organic conductor alpha-(BEDT-TTF)2I3 is characterized by dc resistivity, dielectric and optical spectroscopy in different crystallographic directions within the two-dimensional conduction layer. Two dielectric modes are detected. The large mode is related to the phason-like excitation of the 2kF bond-charge density wave which forms in the ab plane. The small dielectric mode is associated with the motion of domain-wall pairs along the a- and b-axes between two types of domains which are created due to inversion symmetry breaking.

cond-mat.str-el↗

arXiv2007

Anomalous Lattice Response at the Mott Transition in a Quasi-2D Organic Conductor

Discontinuous changes of the lattice parameters at the Mott metal-insulator transition are detected by high-resolution dilatometry on deuterated crystals of the layered organic conductor $κ$-(BEDT-TTF)$_{2}$Cu[N(CN)$_{2}$]Br. The uniaxial expansivities uncover a striking and unexpected anisotropy, notably a zero-effect along the in-plane c-axis along which the electronic interactions are relatively strong. A huge thermal expansion anomaly is observed near the end-point of the first-order transition line enabling to explore the critical behavior with very high sensitivity. The analysis yields critical fluctuations with an exponent $\tildeα \simeq$ 0.8 $\pm$ 0.15 at odds with the novel criticality recently proposed for these materials [Kagawa \textit{et al.}, Nature \textbf{436}, 534 (2005)]. Our data suggest an intricate role of the lattice degrees of freedom in the Mott transition for the present materials.

cond-mat.str-el↗

arXiv2007

Thermal Transient Multisource Simulation Using Cubic Spline Interpolation of Zth Functions

This paper presents a very straightforward method to compute the transient thermal response to arbitrary power dissipation profiles in electronic devices with multiple heat sources. Using cubic spline interpolation of simulated or measured unit power step response curves (Zth-functions), additional errors due to model reduction can be avoided. No effort has to be spent on the generation of compact models. The simple analytic form of the interpolating splines can be exploited to evaluate the convolution integral of the Zth-functions with arbitrary power profiles at low computational costs. An implementation of the algorithm in a spreadsheet program (EXCEL) is demonstrated. The results are in very good agreement with temperature profiles computed by transient Finite Element simulation but can be obtained in a fraction of the time.

cond-mat.mtrl-sci↗

arXiv2006

Determining ethylene group disorder levels in $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br

We present a detailed structural investigation of the organic superconductor $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br at temperatures $T$ from 9 to 300 K. Anomalies in the $T$ dependence of the lattice parameters are associated with a glass-like transition previously reported at $T_g$ = 77 K. From structure refinements at 9, 100 and 300 K, the orthorhombic crystalline symmetry, space group {\it Pnma}, is established at all temperatures. Further, we extract the $T$ dependence of the occupation factor of the eclipsed conformation of the terminal ethylene groups of the BEDT-TTF molecule. At 300 K, we find 67(2) %, with an increase to 97(3) % at 9 K. We conclude that the glass-like transition is not primarily caused by configurational freezing-out of the ethylene groups.

cond-mat.mtrl-sci↗

arXiv2004

Resistivity studies under hydrostatic pressure on a low-resistance variant of the quasi-2D organic superconductor kappa-(BEDT-TTF)2Cu[N(CN)2]Br: quest for intrinsic scattering contributions

Resistivity measurements have been performed on a low (LR)- and high (HR)-resistance variant of the kappa-(BEDT-TTF)_2Cu[N(CN)_2]Br superconductor. While the HR sample was synthesized following the standard procedure, the LR crystal is a result of a somewhat modified synthesis route. According to their residual resistivities and residual resistivity ratios, the LR crystal is of distinctly superior quality. He-gas pressure was used to study the effect of hydrostatic pressure on the different transport regimes for both variants. The main results of these comparative investigations are (i) a significant part of the inelastic-scattering contribution, which causes the anomalous rho(T) maximum in standard HR crystals around 90 K, is sample dependent, i.e. extrinsic in nature, (ii) the abrupt change in rho(T) at T* approx. 40 K from a strongly temperature-dependent behavior at T > T* to an only weakly T-dependent rho(T) at T < T* is unaffected by this scattering contribution and thus marks an independent property, most likely a second-order phase transition, (iii) both variants reveal a rho(T) proportional to AT^2 dependence at low temperatures, i.e. for T_c < T < T_0, although with strongly sample-dependent coefficients A and upper bounds for the T^2 behavior measured by T_0. The latter result is inconsistent with the T^2 dependence originating from coherent Fermi-liquid excitations.

cond-mat.str-el↗

arXiv2002

Evidence of the superconducting energy gap in the optical spectra of $α_t$-(BEDT-TTF)$_{2}$I$_{3}$

The far-infrared in-plane reflectivity of the organic superconductor $α_t$-(BEDT-TTF)$_{2}$I$_{3}$ is measured down to frequencies of 10 cm$^{-1}$; the optical conductivity is obtained by a Kramers-Kronig procedure. In the superconducting state an energy gap opens at 25 cm$^{-1}$ which corresponds to $2Δ/k_BT_c = 4.4$ in agreement with moderate coupling. Even well below $T_c=8$ K a considerable absorption remains for $\hbarω<2Δ$. We discuss different posibilities to explain this behaviour.

cond-mat.supr-con↗

arXiv2002

Coherent vs incoherent interlayer transport in layered metals

The magnetic-field, temperature, and angular dependence of the interlayer magnetoresistance of two different quasi-two-dimensional (2D) organic superconductors is reported. For $κ$-(BEDT-TTF)$_2$I$_3$ we find a well-resolved peak in the angle-dependent magnetoresistance at $Θ= 90^\circ$ (field parallel to the layers). This clear-cut proof for the coherent nature of the interlayer transport is absent for $β$''-(BEDT-TTF)$_2$SF$_5$CH$_2$CF$_2$SO$_3$. This and the non-metallic behavior of the magnetoresistance suggest an incoherent quasiparticle motion for the latter 2D metal.

cond-mat.str-el↗

arXiv2001

Correlation gap in the optical spectra of the two-dimensional organic metal (BEDT-TTF)_4[Ni(dto)_2]

Optical reflection measurements within the highly conducting (a,b)-plane of the organic metal (BEDT-TTF)_4[Ni(dto)_2] reveal the gradual development of a sharp feature at around 200 cm as the temperature is reduced below 150 K. Below this frequency a narrow Drude-like response is observed which accounts for the metallic behavior. Since de Haas-von Alphen oscillations at low temperatures confirm band structure calculations of bands crossing the Fermi energy, we assign the observed behavior to a two-dimensional metallic state in the proximity of a correlation induced metal-insulator transition.

cond-mat↗

arXiv1999

kappa-(BEDT-TTF)_2Cu[N(CN)_2]Br: a Fully Gapped Strong-Coupling Superconductor

High-resolution specific-heat measurements of the organic superconductor kappa-(BEDT-TTF)_2Cu[N(CN)_2]Br in the superconducting (B = 0) and normal (B = 14 T) state show a clearly resolvable anomaly at Tc = 11.5 K and an electronic contribution, Ces, which can be reasonably well described by strong-coupling BCS theory. Most importantly, Ces vanishes exponentially in the superconducting state which gives evidence for a fully gapped order parameter.

cond-mat.supr-con↗