arXiv subjects

D. V. Efremov

Publications and source records attributed to D. V. Efremov.

At least 55 records · Page 3Linked to original sources

arXiv2016

Ba2YIrO6: A cubic double perovskite material with Ir5+ ions

Materials with a 5d4 electronic configuration are generally considered to have a nonmagnetic ground state (J=0). Interestingly, Sr2YIrO6 (Ir5+ having 5d4 electronic configuration) was recently reported to exhibit long-range magnetic order at low temperature and the distorted IrO6 octahedra were discussed to cause the magnetism in this material. Hence, a comparison of structurally distorted Sr2YIrO6 with cubic Ba2YIrO6 may shed light on the source of magnetism in such Ir5+ materials with 5d4 configuration. Besides, Ir5+ materials having 5d4 are also interesting in the context of recently predicted excitonic types of magnetism. Here we report a single-crystal-based analysis of the structural, magnetic, and thermodynamic properties of Ba2YIrO6. We observe that in Ba2YIrO6 for temperatures down to 0.4 K, long-range magnetic order is absent but at the same time correlated magnetic moments are present. We show that these moments are absent in fully relativistic ab initio band-structure calculations; hence, their origin is presently unclear.

cond-mat.str-el↗

arXiv2014

Orbital-driven nematicity in FeSe

A very fundamental and unconventional characteristic of superconductivity in iron-based materials is that it occurs in the vicinity of {\it two} other instabilities. Apart from a tendency towards magnetic order, these Fe-based systems have a propensity for nematic ordering: a lowering of the rotational symmetry while time-reversal invariance is preserved. Setting the stage for superconductivity, it is heavily debated whether the nematic symmetry breaking is driven by lattice, orbital or spin degrees of freedom. Here we report a very clear splitting of NMR resonance lines in FeSe at $T_{nem}$ = 91K, far above superconducting $T_c$ of 9.3 K. The splitting occurs for magnetic fields perpendicular to the Fe-planes and has the temperature dependence of a Landau-type order-parameter. Spin-lattice relaxation rates are not affected at $T_{nem}$, which unequivocally establishes orbital degrees of freedom as driving the nematic order. We demonstrate that superconductivity competes with the emerging nematicity.

cond-mat.supr-con↗

arXiv2014

Unexpected impact of magnetic disorder on multiband superconductivity

We analyze how the magnetic disorder affects the properties of the two-band $s_\pm$ and $s_{++}$ models, which are subject of hot discussions regarding iron-based superconductors and other multiband systems like MgB$_2$. We show that there are several cases when the transition temperature $T_c$ is not fully suppressed by magnetic impurities in contrast to the Abrikosov-Gor'kov theory, but a saturation of $T_c$ takes place in the regime of strong disorder. These cases are: (1) the purely interband impurity scattering, (2) the unitary scattering limit. We show that in the former case the $s_\pm$ gap is preserved, while the $s_{++}$ state transforms into the $s_\pm$ state with increasing magnetic disorder. For the case (2), the gap structure remains intact.

cond-mat.supr-con↗

arXiv2014

Superconducting properties of K$_{1-x}$Na$_x$Fe$_2$As$_2$ under pressure

The effect of hydrostatic pressure and partial Na substitution on the normal-state properties and the superconducting transition temperature ($T_c$) of K$_{1-x}$Na$_x$Fe$_2$As$_2$ single crystals were investigated. It was found that a partial Na substitution leads to a deviation from the standard $T^2$ Fermi-liquid behavior in the temperature dependence of the normal-state resistivity. It was demonstrated that non-Fermi liquid like behavior of the resistivity for K$_{1-x}$Na$_{x}$Fe$_2$As$_2$ and some KFe$_2$As$_2$ samples can be explained by disorder effect in the multiband system with rather different quasiparticle effective masses. Concerning the superconducting state our data support the presence of a shallow minimum around 2 GPa in the pressure dependence of $T_c$ for stoichiometric KFe$_2$As$_2$. The analysis of $T_c$ in the K$_{1-x}$Na$_{x}$Fe$_2$As$_2$ at pressures below 1.5 GPa showed, that the reduction of $T_c$ with Na substitution follows the Abrikosov-Gor'kov law with the critical temperature $T_{c0}$ of the clean system (without pair-breaking) which linearly depends on the pressure. Our observations, also, suggest that $T_c$ of K$_{1-x}$Na$_x$Fe$_2$As$_2$ is nearly independent of the lattice compression produced by the Na substitution. Further, we theoretically analyzed the behavior of the band structure under pressure within the generalized gradient approximation (GGA). A qualitative agreement between the calculated and the recently in de Haas-van Alphen experiments [T. Terashima et al., Phys.Rev.B89, 134520(2014)] measured pressure dependencies of the Fermi-surface cross-sections has been found. These calculations, also, indicate that the observed minimum around 2~GPa in the pressure dependence of $T_c$ may occur without a change of the pairing symmetry.

cond-mat.supr-con↗

arXiv2014

Single 20meV boson mode in KFe2As2 detected by point-contact spectroscopy

We report an experimental and theoretical investigation of the electron-boson interaction in KFe2As2 by point-contact (PC) spectroscopy, model, and ab-initio LDA-based calculations for the standard electron-phonon Eliashberg function. The PC spectrum viz. the second derivative of the I - V characteristic of representative PC exhibits a pronounced maximum at about 20meV and surprisingly a featureless behavior at lower and higher energies. We discuss phonon and non-phonon (excitonic) mechanisms for the origin of this peak. Analysis of the underlying source of this peak may be important for the understanding of serious puzzles of superconductivity in this type of compounds.

cond-mat.supr-con↗

arXiv2014

Superconducting specific heat jump $ΔC_{\rm el} \propto T_c^β\ (β\approx 2)$ for K$_{1-x}$Na$_x$Fe$_2$As$_2$

We present a systematic study of the electronic specific heat jump ($ΔC_{\rm el}$) at the superconducting transition temperature $T_c$ of K$_{1-x}$Na$_x$Fe$_2$As$_2$. Both $T_c$ and $ΔC_{\rm el}$ monotonously decrease with increasing $x$. The specific heat jump scales approximately with a power-law, $ΔC_{\rm el} \propto T_c^β$, with $β\approx 2$ determined by the impurity scattering rate, in contrast to most iron-pnictide superconductors, where the remarkable Bud'ko-Ni-Canfield (BNC) scaling $ΔC_{\rm el} \propto T^3$ has been found. Both the $T$ dependence of $C_{\rm el}(T)$ in the superconducting state and the nearly quadratic scaling of $ΔC_{\rm el}$ at $T_c$ are well described by the Eliashberg-theory for a two-band $d$-wave superconductor with weak pair-breaking due to nonmagnetic impurities. The disorder induced by the Na substitution significantly suppresses the small gaps leading to gapless states in the slightly disordered superconductor, which results in a large observed residual Sommerfeld coefficient in the superconducting state for $x > 0$.

cond-mat.supr-con↗

arXiv2013

Strain induced superconductivity in the parent compound BaFe2As2

The discovery of superconductivity (SC) with a transition temperature, Tc, up to 65K in single-layer FeSe (bulk Tc =8K) films grown on SrTiO3 substrates has attracted special attention to Fe-based thin films. The high Tc is a consequence of the combined effect of electron transfer from the oxygen-vacant substrate to the FeSe thin film and lattice tensile strain. Here we demonstrate the realization of SC in the parent compound BaFe2As2 (no bulk Tc) just by tensile lattice strain without charge doping. We investigate the interplay between strain and SC in epitaxial BaFe2As2 thin films on Fe-buffered MgAl2O4 single crystalline substrates. The strong interfacial bonding between Fe and the FeAs sublattice increases the Fe-Fe distance due to the lattice misfit which leads to a suppression of the antiferromagnetic spin density wave and induces SC with bulk-Tc ?10K. These results highlight the role of structural changes in controlling the phase diagram of Fe-based superconductors.

cond-mat.supr-con↗

arXiv2013

Evidence of d-wave Superconductivity in K_(1-x)Na_xFe_2As_2 (x = 0, 0.1) Single Crystals from Low-Temperature Specific Heat Measurements

From the measurement and analysis of the specific heat of high-quality K_(1-x)Na_xFe_2As_2 single crystals we establish the presence of large T^2 contributions with coefficients alpha_sc ~ 30 mJ/mol K^3 at low-T for both x=0 and 0.1. Together with the observed square root field behavior of the specific heat in the superconducting state both findings evidence d-wave superconductivity on almost all Fermi surface sheets with an average gap amplitude of Delta_0 in the range of 0.4 - 0.8 meV. The derived Delta_0 and the observed T_c agree well with the values calculated within the Eliashberg theory, adopting a spin-fluctuation mediated pairing in the intermediate coupling regime.

cond-mat.supr-con↗

arXiv2012

Manifestation of impurity induced s_{+-} -> s_{++} transition: multiband model for dynamical response functions

We investigate effects of disorder on the density of states, the single particle response function and optical conductivity in multiband superconductors with s_{+-} symmetry of the order parameter, where s_{+-} -> s_{++} transition may take place. In the vicinity of the transition the superconductive gapless regime is realized. It manifests itself in anomalies in the above mentioned properties. As a result, intrinsically phase-insensitive experimental methods like ARPES, tunneling and terahertz spectroscopy may be used for revealing of information about the underlying order parameter symmetry.

cond-mat.supr-con↗

arXiv2011

Disorder induced transition between s_+- and s_++ states in two-band superconductors

We have reexamined the problem of disorder in two-band superconductors, and shown within the framework of the T-matrix approximation, that the suppression of T_c can be described by a single parameter depending on the intraband and interband impurity scattering rates. T_c is shown to be more robust against nonmagnetic impurities than would be predicted in the trivial extension of Abrikosov-Gor'kov theory. We find a disorder-induced transition from the s_{\pm} state to a gapless and then to a fully gapped s_{++} state, controlled by a single parameter -- the sign of the average coupling constant <λ> . We argue that this transition has strong implications for experiments.

cond-mat.supr-con↗

arXiv2011

Superconductivity in repulsive Fermi-systems at low density

In the large variety of models such as 3D and 2D Fermi-gas model with hard-core repulsion, 3D and 2D Hubbard model, and Shubin-Vonsovsky model we demonstrate the possibility of triplrt p-wave pairing at low electron density. We show that the critical temperature of the p-wave pairing can be strongly increased in a spin-polarized case or in a two-band situation already at low density and reach experimentally observable values of (1-5)K. We also discuss briefly d-wave pairing and high-Tc superconductivity with Tc~100K which arises in the t-J model in the range of parameters realistic for cuprates.

cond-mat.supr-con↗

arXiv2011

Triplet p-wave superconductivity in low-density extended Hubbard model with Coulomb repulsion

We analyze superconducting instabilities in 3D and 2D extended Hubbard model with Coulomb repulsion between electrons on neighboring sites in the limit of low electron density ($n_{el} \rightarrow 0$) on simple cubic (square) lattice. We show that in a realistic strong-coupling case $U\gg V\gg W$ ($U$ and $V$ are the onsite and the intersite Coulomb repulsions, $W$ the bandwidth) the main SC instability corresponds to the p-wave pairing and in the leading order is correctly described by the equations obtained earlier in the absence of the intersite Coulomb interaction V=0.

cond-mat.supr-con↗

arXiv2011

BCS - BEC crossover and quantum hydrodynamics in p-wave superfluids with a symmetry of the A1 - phase

We solve the Leggett equations for the BCS - BEC crossover in the three dimension resonance p-wave superfluid with the symmetry of the A1 - phase. We calculate the sound velocity, the normal density, and the specific heat for the BCS-domain (μ> 0), BEC-domain (μ< 0), and close to important point μ= 0 in 100% polarized case. We find the indications of quantum phase - transition close to the point μ(T = 0) = 0. Deep in the BCS and BEC-domains the crossover ideas of Leggett and Nozieres, Schmitt-Rink work pretty well. We discuss the spectrum of orbital waves, the paradox of intrinsic angular momentum and complicated problem of chiral anomaly in the BCS A1 - phase at T = 0. We present two different approaches to a chiral anomaly: one based on supersymmetric hydrodynamics, another one on the formal analogy with the Dirac equation in quantum electrodynamics. We evaluate the damping of nodal fermions due to different decay processes in superclean case at T = 0 and find that we are in a ballistic regime ωτ>> 1. We propose to use aerogel or nonmagnetic impurities to reach hydrodynamic regime ωτ<< 1 at T = 0. We discuss the concept of the spectral flow and exact cancellations between time-derivatives of anomalous and quasiparticle currents in the equation for the total linear momentum conservation. We propose to derive and solve the kinetic equation for the nodal quasiparticles both in the hydrodynamic and in the ballistic regimes to demonstrate this cancellation explicitly. We briefly discuss the role of the other residual interactions different from damping and invite experimentalists to measure the spectrum and damping of orbital waves in A-phase of 3He at low temperatures.

cond-mat.quant-gas↗

arXiv2009

Non-analytic spin susceptibility of a nested Fermi liquid: the case of Fe-based pnictides

We propose an explanation of the peculiar linear temperature dependence of the uniform spin susceptibility $χ(T)$ in ferropnictides. We argue that the linear in $T$ term appears due to non-analytic temperature dependence of $χ(T)$ in a two-dimensional Fermi liquid. We show that the prefactor of the $T$ term is expressed via the square of the spin-density-wave (SDW) amplitude connecting nested hole and electron pockets. Due to an incipient SDW instability, this amplitude is large, which, along with a small value of the Fermi energy, makes the $T$ dependence of $χ(T)$ strong. We demonstrate that this mechanism is in quantitative agreement with the experiment.

cond-mat.supr-con↗

arXiv2004

Orbital ordering in manganites in the band approach

We consider the orbital ordering in LaMnO3 and similar systems, proceeding from the band picture. We show that for the realistic magnetic structure of A-type there exists a complete nesting betweeen two e_g-bands. As a result there occurs an instability towards an excitonic insulator-like state -- an electron-hole pairing with the wave vector Q=(π,π), which opens a gap in the spectrum and makes the system insulating. In the resulting state there appeasr an orbital ordering -- orbital density wave (ODW), the type of which coincides with those existing in LaMnO3.

cond-mat.str-el↗

arXiv2004

Composite fermions and quartets in the Fermi-Bose mixture with attractive interaction between fermions and bosons

We consider a model of Fermi-Bose mixture with strong hard-core repulsion between particles of the same sort and attraction between particles of different sorts. In this case, besides the standard anomalous averages of the type $ $; $ $ and $ $, a pairing between fermion and boson of the type $bc$ is possible. This pairing corresponds to a creation of composite fermions in the system. At low temperatures and equal densities of fermions and bosons composite fermions are further paired in quartets. Our investigations are important for high-$T_c$ superconductors and in connection with recent observation of weakly bound dimers in magnetic traps at ultralow temperatures.

cond-mat.str-el↗

arXiv2004

Approximative treatment of 5f-systems with partial localization due to intra-atomic correlations

Increasing experimental and theoretical evidence points towards a dual nature of the 5$f$ electrons in actinide-based strongly correlated metallic compounds, with some 5$f$ electrons being localized and others delocalized. In a recent paper (PRB xxx, 2004), we suggested the interplay of intra-atomic correlations as described by Hund's rules and a weakly anisotropic hopping (hybridization) as a possible mechanism. The purpose of the present work is to provide a first step towards a microscopic description of partial localization in solids by analyzing how well various approximation schemes perform when applied to small clusters. It is found that many aspects of partial localization are described appropriately both by a variational wavefunction of Gutzwiller type and by a treatment which keeps only those interactions which are present in LDA+U calculations. In contrast, the energies and phase diagram calculated within the Hartree Fock approximation show little resemblence with the exact results. Enhancement of hopping anisotropy by Hund's rule correlations are found in all approximations.

cond-mat.str-el↗

arXiv2003

On a dual model for 5f electrons

We study the effect of intra-atomic correlations on anisotropies of hopping of 5f electrons. It is shown that they may considerably enhance these anisotropies to the extend that electrons in some of the 5f orbitals remain localized. This provide a microscopic basis for a previously made assumption that some of the 5f electrons must be partially localized when Fermi surfaces and effective masses of the component are calculated. Calculations are performed on two- and three-sites clusters. They include phase diagrams in the presence and absence of an external magnetic field as function of anisotropic hopping.

cond-mat↗