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D. V. Guzatov

Publications and source records attributed to D. V. Guzatov.

8 recordsLinked to original sources

Density of states effects on emission and scattering of photons in plasmas

Plasma supports electromagnetic waves propagation for frequencies higher than plasma frequency but features dielectric permittivity less than 1. This property leads to photon density of states (DOS) lower than in vacuum and should result in subnatural spectral linewidths, sub-Planckian spectrum of thermal radiation, and sub-Rayleigh scattering as well as in lower inelastic photon scattering including Raman scattering. Lamb shift will be altered as well though the decisive contribution from high-energy modes in this case makes the photon DOS effect rather small since plasma DOS converges with the vacuum one in the limit of infinite frequencies. We emphasize the basic character of all these phenomena though absolute values of corrections in many real experiments may appear to be small as compared to other factors. We found that dissipative losses make possible DOS effects smaller though not vanishing and additionally bring about indefinite growth of DOS in the low-frequency limit.

physics.optics↗

Optical properties of a two-nanospheroid cluster: analytical approach

Optical properties of a plasmonic nano-antenna made of two metallic nanospheroids (prolate or oblate) are investigated analytically in quasistatic approximation. It is shown that in clusters of two nanospheroids, three types of plasmonic modes can be present. Two of them can be effectively excited by a plane electromagnetic wave, while the third one can be effectively excited only by a nanolocalized light source (an atom, a molecule, a quantum dot) placed in the gap between the nanoparticles. Analytical expressions for absorption and scattering cross-sections, enhancement of a local field, and radiative decay rate of a dipole source placed near such a nano-antenna are presented and analyzed.

physics.optics↗

Plasmon oscillations in ellipsoid nanoparticles: beyond dipole approximation

The plasmon oscillations of a metallic triaxial ellipsoid nanoparticle have been studied within the framework of the quasistatic approximation. A general method has been proposed for finding the analytical expressions describing the potential and frequencies of the plasmon oscillations of an arbitrary multipolarity order. The analytical expressions have been derived for an electric potential and plasmon oscillation frequencies of the first 24 modes. Other higher orders plasmon modes are investigated numerically.

physics.optics↗

Rationale for $10^{14}$ enhancement factor in single molecule Raman spectroscopy

We extend the Purcell's original idea [Phys. Rev. \textbf{69}, 682 (1946)] on modification of photon spontaneous \textit{emission} rate to modification of photon spontaneous \textit{scattering} rate. We find the interplay of local incident field enhancement and local density of photon states enhancement in close proximity to a silver nanoparticle may result in up to $10^{14}$-fold rise of Raman scattering cross-section. Thus single molecule Raman detection is found to be explained by consistent quantum electrodynamic description without any chemical mechanism involved. A model of the so-called "hot points" in surface enhanced spectroscopy has been elaborated as local areas with high Q-factor at incident and scattered (emitted) light frequencies. For verification of the model we consider further experiments including transient Raman experiments to clarify incident field enhancement and scanning near-field optical mapping of local density of photon states.

physics.optics↗

Plasmonic atoms and plasmonic molecules

The proposed paradigm of plasmonic atoms and plasmonic molecules allows one to describe and predict the strongly localized plasmonic oscillations in the clusters of nanoparticles and some other nanostructures in uniform way. Strongly localized plasmonic molecules near the contacting surfaces might become the fundamental elements (by analogy with Lego bricks) for a construction of fully integrated opto-electronic nanodevices of any complexity and scale of integration.

physics.optics↗

Strongly localized plasmon oscillations in a cluster of two metallic nanospheres and their influence on spontaneous emission of an atom

The plasmon oscillations in a cluster of two metallic nanospheres are studied theoretically. Particular attention is paid to the case of nearly touching spheres. Simple analytical expressions have been found for the spectra of plasmon oscillations of different symmetry in this case. A new type of the plasmon oscillations, which are strongly localized between the spheres, and which totally disappear at separation of the spheres, has been discovered. The found plasmon oscillations have a dramatic effect on optical properties of an atom localized between the spheres.

physics.optics↗

Radiative Decay Engineering by Triaxial Nanoellipsoids

Radiative decay rates of an atom placed near triaxial nanoellipsoid are investigated in long wavelength approximation. Analytical results are obtained in general case. It is shown that triaxial ellipsoid can be used for efficient control of decay rate of an atom, molecule or quantum dot. For example decay rate near silver ellipsoid can be enhanced by 5 orders of magnitude. It is also shown, that triaxial nanoellipsoid can be used for simultaneous efficient control of absorption and emission rates of fluorophores.

quant-ph↗