arXiv subjects

D. W. Savin

Publications and source records attributed to D. W. Savin.

At least 37 records · Page 2Linked to original sources

arXiv2011

Storage-ring measurement of the hyperfine-induced 2s 2p 3P0 -> 2s2 1S0 transition rate in beryllium-like sulfur

The hyperfine induced 2s 2p 3P0 -> 2s2 1S0 transition rate in Be-like sulfur was measured by monitoring the decay of isotopically pure beams of 32-S12+ and 33-S12+ ions in a heavy-ion storage ring. Within the 4% experimental uncertainty the experimental value of 0.096(4)/s agrees with the most recent theoretical results of Cheng et al. [Phys. Rev. A 77, 052504 (2008)] and Andersson et al. [Phys. Rev. A 79, 032501 (2009)]. Repeated experiments with different magnetic fields in the storage-ring bending magnets demonstrate that artificial quenching of the 2s 2p 3P0 state by these magnetic fields is negligible.

physics.atom-ph↗

arXiv2011

Associative Detachment of H$^{-$ + H $\rightarrow$ H$_{2}$ + e$^{-}$

Using a merged beams apparatus we have measured the associative detachment (AD) reaction of ${\rm H}^- + {\rm H} \to {\rm H}_2 + e^-$ for relative collision energies up to \textit{E}$_{\rm{r}} \leq 4.83$ eV. These data extend above the 1 eV limit of our earlier results. We have also updated our previous theoretical work to account for AD via the repulsive $^2Σ^+_{\rm g}$ H$_2^-$ potential energy surface and for the effects at $E_{\rm r} \ge 0.76$ eV on the experimental results due to the formation of H$_2$ resonances lying above the ${\rm H} + {\rm H}$ separated atoms limit. Merging both experimental data sets, our results are in good agreement with our new theoretical calculations and confirm the prediction that this reaction essentially turns off for $E_{\rm r} \gtrsim 2$ eV. Similar behavior has been predicted for the formation of protonium from collisions of antiprotons and hydrogen atoms.

physics.atom-ph↗

arXiv2011

Storage Ring Cross Section Measurements for Electron Impact Ionization of Fe^11+ Forming Fe^12+ and Fe^13+

We report ionization cross section measurements for electron impact single ionization (EISI) of Fe^11+$ forming Fe^12+ and electron impact double ionization (EIDI) of Fe^11+ forming Fe^13+. The measurements cover the center-of-mass energy range from approximately 230 eV to 2300 eV. The experiment was performed using the heavy ion storage ring TSR located at the Max-Planck-Institut fur Kernphysik in Heidelberg, Germany. The storage ring approach allows nearly all metastable levels to relax to the ground state before data collection begins. We find that the cross section for single ionization is 30% smaller than was previously measured in a single pass experiment using an ion beam with an unknown metastable fraction. We also find some significant differences between our experimental cross section for single ionization and recent distorted wave (DW) calculations. The DW Maxwellian EISI rate coefficient for Fe^11+ forming Fe^12+ may be underestimated by as much as 25% at temperatures for which Fe^11+ is abundant in collisional ionization equilibrium. This is likely due to the absence of 3s excitation-autoionization (EA) in the calculations. However, a precise measurement of the cross section due to this EA channel was not possible because this process is not distinguishable experimentally from electron impact excitation of an n=3 electron to levels of n > 44 followed by field ionization in the charge state analyzer after the interaction region. Our experimental results also indicate that the double ionization cross section is dominated by the indirect process in which direct single ionization of an inner shell 2l electron is followed by autoionization resulting in a net double ionization.

astro-ph.IM↗

arXiv2011

Dielectronic recombination of xenonlike tungsten ions

Dielectronic recombination (DR) of xenonlike W20+ forming W19+ has been studied experimentally at a heavy-ion storage-ring. A merged-beams method has been employed for obtaining absolute rate coefficients for electron-ion recombination in the collision energy range 0-140 eV. The measured rate coefficient is dominated by strong DR resonances even at the lowest experimental energies. At plasma temperatures where the fractional abundance of W20+ is expected to peak in a fusion plasma, the experimentally derived plasma recombination rate coefficient is over a factor of 4 larger than the theoretically-calculated rate coefficient which is currently used in fusion plasma modeling. The largest part of this discrepancy stems most probably from the neglect in the theoretical calculations of DR associated with fine-structure excitations of the W20+([Kr] 4d10 4f8) ion core.

physics.atom-ph↗

arXiv2010

Properties of a Polar Coronal Hole During the Solar Minimum in 2007

We report measurements of a polar coronal hole during the recent solar minimum using the Extreme Ultraviolet Imaging Spectrometer on Hinode. Five observations are analyzed that span the polar coronal hole from the central meridian to the boundary with the quiet Sun corona. We study the observations above the solar limb in the height range of 1.03 - 1.20 solar radii. The electron temperature Te and emission measure EM are found using the Geometric mean Emission Measure (GEM) method. The EM derived from the elements Fe, Si, S, and Al are compared in order to measure relative coronal-to-photospheric abundance enhancement factors. We also studied the ion temperature Ti and the non-thermal velocity Vnt using the line profiles. All these measurements are compared to polar coronal hole observations from the previous (1996-1997) solar minimum and to model predictions for relative abundances. There are many similarities in the physical properties of the polar coronal holes between the two minima at these low heights. We find that Te, electron density Ne, and Ti are comparable in both minima. Te shows a comparable gradient with height. Both minima show a decreasing Ti with increasing charge-to-mass ratio q/M. A previously observed upturn of Ti for ions above q/M > 0.25 was not found here. We also compared relative coronal-to-photospheric elemental abundance enhancement factors for a number of elements. These ratios were about 1 for both the low first ionization potential (FIP) elements Si and Al and the marginally high FIP element S relative to the low FIP element Fe, as is expected based on earlier observations and models for a polar coronal hole. These results are consistent with no FIP effect in a polar coronal hole.

astro-ph.SR↗

arXiv2009

Deriving the Coronal Hole Electron Temperature: Electron Density Dependent Ionization/Recombination Considerations

Comparison of appropriate theoretical derived line ratios with observational data can yield estimates of a plasma's physical parameters, such as electron density or temperature. The usual practice in the calculation of the line ratio is the assumption of excitation by electrons/protons followed by radiative decay. Furthermore, it is normal to use the so-called coronal approximation, i.e. one only considers ionization and recombination to and from the ground state. A more accurate treatment is to include the ionization/recombination to and from meta-stable levels. Here, we apply this to two lines from adjacent ionization stages; Mg IX 368A and Mg X 625A, which has been shown to be a very useful temperature diagnostic. At densities typical of coronal hole conditions, the difference between the electron temperature derived assuming the zero density limit compared with the electron density dependent ionization/recombination is small. This however is not the case for flares where the electron density is orders of magnitude larger. The derived temperature for the coronal hole at solar maximum is around 1.04 MK compared to just below 0.82 MK at solar minimum.

astro-ph.SR↗

arXiv2009

Electron-ion Recombination of Fe X forming Fe IX and of Fe XI forming Fe X: Laboratory Measurements and Theoretical Calculations

We have measured electron-ion recombination for Fe$^{9+}$ forming Fe$^{8+}$ and for Fe$^{10+}$ forming Fe$^{9+}$ using merged beams at the TSR heavy-ion storage-ring in Heidelberg. The measured merged beams recombination rate coefficients (MBRRC) for relative energies from 0 to 75 eV are presented, covering all dielectronic recombination (DR) resonances associated with 3s->3p and 3p->3d core transitions in the spectroscopic species Fe X and Fe XI, respectively. We compare our experimental results to multi-configuration Breit-Pauli (MCBP) calculations and find significant differences. From the measured MBRRC we have extracted the DR contributions and transform them into plasma recombination rate coefficients (PRRC) for astrophysical plasmas with temperatures from 10^2 to 10^7 K. This spans across the regimes where each ion forms in photoionized or in collisionally ionized plasmas. For both temperature regimes the experimental uncertainties are 25% at a 90% confidence level. The formerly recommended DR data severely underestimated the rate coefficient at temperatures relevant for photoionized gas. At the temperatures relevant for photoionized gas, we find agreement between our experimental results and MCBP theory. At the higher temperatures relevant for collisionally ionized gas, the MCBP calculations yield a Fe XI DR rate coefficent which is significantly larger than the experimentally derived one. We present parameterized fits to our experimentally derived DR PRRC.

astro-ph.GA↗

arXiv2008

Molecular cloud chemistry and the importance of dielectronic recombination

Dielectronic recombination (DR) of singly charged ions is a reaction pathway that is commonly neglected in chemical models of molecular clouds. In this study we include state-of-the-art DR data for He$^+$, C$^+$, N$^+$, O$^+$, Na$^+$, and Mg$^+$ in chemical models used to simulate dense molecular clouds, protostars, and diffuse molecular clouds. We also update the radiative recombination (RR) rate coefficients for H$^+$, He$^+$, C$^+$, N$^+$, O$^+$, Na$^+$, and Mg$^+$ to the current state-of-the-art values. The new RR data has little effect on the models. However, the inclusion of DR results in significant differences in gas-grain models of dense, cold molecular clouds for the evolution of a number of surface and gas-phase species. We find differences of a factor of 2 in the abundance for 74 of the 655 species at times of $10^4$--$10^6$ years in this model when we include DR. Of these 74 species, 16 have at least a factor of 10 difference in abundance. We find the largest differences for species formed on the surface of dust grains. These differences are due primarily to the addition of C$^+$ DR, which increases the neutral C abundance, thereby enhancing the accretion of C onto dust. These results may be important for the warm-up phase of molecular clouds when surface species are desorbed into the gas phase. We also note that no reliable state-of-the-art RR or DR data exist for Si$^+$, P$^+$, S$^+$, Cl$^+$, and Fe$^+$. Modern calculations for these ions are needed to better constrain molecular cloud models.

astro-ph↗

arXiv2008

A new approach to analyzing solar coronal spectra and updated collisional ionization equilibrium calculations. II. Additional ionization rate coefficients

We have reanalyzed SUMER observations of a parcel of coronal gas using new collisional ionization equilibrium (CIE) calculations. These improved CIE fractional abundances were calculated using state-of-the-art electron-ion recombination data for K-shell, L-shell, Na-like, and Mg-like ions of all elements from H through Zn and, additionally, Al- through Ar-like ions of Fe. They also incorporate the latest recommended electron impact ionization data for all ions of H through Zn. Improved CIE calculations based on these recombination and ionization data are presented here. We have also developed a new systematic method for determining the average emission measure ($EM$) and electron temperature ($T_e$) of an isothermal plasma. With our new CIE data and our new approach for determining average $EM$ and $T_e$, we have reanalyzed SUMER observations of the solar corona. We have compared our results with those of previous studies and found some significant differences for the derived $EM$ and $T_e$. We have also calculated the enhancement of coronal elemental abundances compared to their photospheric abundances, using the SUMER observations themselves to determine the abundance enhancement factor for each of the emitting elements. Our observationally derived first ionization potential (FIP) factors are in reasonable agreement with the theoretical model of Laming (2008).

astro-ph↗

arXiv2008

Is H3+ cooling ever important in primordial gas?

Studies of the formation of metal-free Population III stars usually focus primarily on the role played by H2 cooling, on account of its large chemical abundance relative to other possible molecular or ionic coolants. However, while H2 is generally the most important coolant at low gas densities, it is not an effective coolant at high gas densities, owing to the low critical density at which it reaches local thermodynamic equilibrium (LTE) and to the large opacities that develop in its emission lines. It is therefore possible that emission from other chemical species may play an important role in cooling high density primordial gas. A particularly interesting candidate is the H3+ molecular ion. This ion has an LTE cooling rate that is roughly a billion times larger than that of H2, and unlike other primordial molecular ions such as H2+ or HeH+, it is not easily removed from the gas by collisions with H or H2. It is already known to be an important coolant in at least one astrophysical context -- the upper atmospheres of gas giants -- but its role in the cooling of primordial gas has received little previous study. In this paper, we investigate the potential importance of H3+ cooling in primordial gas using a newly-developed H3+ cooling function and the most detailed model of primordial chemistry published to date. We show that although H3+ is, in most circumstances, the third most important coolant in dense primordial gas (after H2 and HD), it is nevertheless unimportant, as it contributes no more than a few percent of the total cooling. We also show that in gas irradiated by a sufficiently strong flux of cosmic rays or X-rays, H3+ can become the dominant coolant in the gas, although the size of the flux required renders this scenario unlikely to occur.

astro-ph↗

arXiv2007

Electron-ion recombination of Si IV forming Si III: Storage-ring measurement and multiconfiguration Dirac-Fock calculations

The electron-ion recombination rate coefficient for Si IV forming Si III was measured at the heavy-ion storage-ring TSR. The experimental electron-ion collision energy range of 0-186 eV encompassed the 2p(6) nl n'l' dielectronic recombination (DR) resonances associated with 3s to nl core excitations, 2s 2p(6) 3s nl n'l' resonances associated with 2s to nl (n=3,4) core excitations, and 2p(5) 3s nl n'l' resonances associated with 2p to nl (n=3,...,infinity) core excitations. The experimental DR results are compared with theoretical calculations using the multiconfiguration Dirac-Fock (MCDF) method for DR via the 3s to 3p n'l' and 3s to 3d n'l' (both n'=3,...,6) and 2p(5) 3s 3l n'l' (n'=3,4) capture channels. Finally, the experimental and theoretical plasma DR rate coefficients for Si IV forming Si III are derived and compared with previously available results.

physics.atom-ph↗

arXiv2007

Dielectronic Recombination of Fe XV forming Fe XIV: Laboratory Measurements and Theoretical Calculations

We have measured resonance strengths and energies for dielectronic recombination (DR) of Mg-like Fe XV forming Al-like Fe XIV via N=3 -> N' = 3 core excitations in the electron-ion collision energy range 0-45 eV. All measurements were carried out using the heavy-ion Test Storage Ring at the Max Planck Institute for Nuclear Physics in Heidelberg, Germany. We have also carried out new multiconfiguration Breit-Pauli (MCBP) calculations using the AUTOSTRUCTURE code. For electron-ion collision energies < 25 eV we find poor agreement between our experimental and theoretical resonance energies and strengths. From 25 to 42 eV we find good agreement between the two for resonance energies. But in this energy range the theoretical resonance strengths are ~ 31% larger than the experimental results. This is larger than our estimated total experimental uncertainty in this energy range of +/- 26% (at a 90% confidence level). Above 42 eV the difference in the shape between the calculated and measured 3s3p(^1P_1)nl DR series limit we attribute partly to the nl dependence of the detection probabilities of high Rydberg states in the experiment. We have used our measurements, supplemented by our AUTOSTRUCTURE calculations, to produce a Maxwellian-averaged 3 -> 3 DR rate coefficient for Fe XV forming Fe XIV. The resulting rate coefficient is estimated to be accurate to better than +/- 29% (at a 90% confidence level) for k_BT_e > 1 eV. At temperatures of k_BT_e ~ 2.5-15 eV, where Fe XV is predicted to form in photoionized plasmas, significant discrepancies are found between our experimentally-derived rate coefficient and previously published theoretical results. Our new MCBP plasma rate coefficient is 19-28% smaller than our experimental results over this temperature range.

astro-ph↗

arXiv2006

Collisional Ionization Equilibrium for Optically Thin Plasmas. I. Updated Recombination Rate Coefficients for Bare though Sodium-like Ions

Reliably interpreting spectra from electron-ionized cosmic plasmas requires accurate ionization balance calculations for the plasma in question. However, much of the atomic data needed for these calculations have not been generated using modern theoretical methods and are often highly suspect. This translates directly into the reliability of the collisional ionization equilibrium (CIE) calculations. We make use of state-of-the-art calculations of dielectronic recombination (DR) rate coefficients for the hydrogenic through Na-like ions of all elements from He up to and including Zn. We also make use of state-of-the-art radiative recombination (RR) rate coefficient calculations for the bare through Na-like ions of all elements from H through to Zn. Here we present improved CIE calculations for temperatures from $10^4$ to $10^9$ K using our data and the recommended electron impact ionization data of \citet{Mazz98a} for elements up to and including Ni and Mazzotta (private communication) for Cu and Zn. DR and RR data for ionization stages that have not been updated are also taken from these two additional sources. We compare our calculated fractional ionic abundances using these data with those presented by Mazzotta et al. for all elements from H to Ni. The differences in peak fractional abundance are up to 60%. We also compare with the fractional ionic abundances for Mg, Si, S, Ar, Ca, Fe, and Ni derived from the modern DR calculations of \citet{Gu03a,Gu04a} for the H-like through Na-like ions, and the RR calculations of \citet{Gu03b} for the bare through F-like ions. These results are in better agreement with our work, with differences in peak fractional abundance of less than 10%.

astro-ph↗

arXiv2006

Electron-ion recombination measurements motivated by AGN X-ray absorption features: Fe XIV forming Fe XIII

Recent spectroscopic models of active galactic nuclei (AGN) have indicated that the recommended electron-ion recombination rate coefficients for iron ions with partially filled M-shells are incorrect in the temperature range where these ions form in photoionized plasmas. We have investigated this experimentally for Fe XIV forming Fe XIII. The recombination rate coefficient was measured employing the electron-ion merged beams method at the Heidelberg heavy-ion storage-ring TSR. The measured energy range of 0-260 eV encompassed all dielectronic recombination (DR) 1s2 2s2 2p6 3l 3l' 3l'' nl''' resonances associated with the 3p1/2 -> 3p3/2, 3s -> 3p, 3p -> 3d and 3s -> 3d core excitations within the M-shell of the Fe XIV 1s2 2s2 2p6 3s2 3p parent ion. This range also includes the 1s2 2s2 2p6 3l 3l' 4l'' nl''' resonances associated with 3s -> 4l'' and 3p -> 4l'' core excitations. We find that in the temperature range 2--14 eV, where Fe XIV is expected to form in a photoionized plasma, the Fe XIV recombination rate coefficient is orders of magnitude larger than previously calculated values.

astro-ph↗

arXiv2003

Assessment of the Fluorescence and Auger Data Base used in Plasma Modeling

We have investigated the accuracy of the 1s-vacancy fluorescence data base of Kaastra & Mewe (1993, A&AS, 97, 443) resulting from the initial atomic physics calculations and the subsequent scaling along isoelectronic sequences. In particular, we have focused on the relatively simple Be-like and F-like 1s-vacancy sequences. We find that the earlier atomic physics calculations for the oscillator strengths and autoionization rates of singly-charged B II and Ne II are in sufficient agreement with our present calculations. However, the substantial charge dependence of these quantities along each isoelectronic sequence, the incorrect configuration averaging used for B II, and the neglect of spin-orbit effects (which become important at high-Z) all cast doubt on the reliability of the Kaastra & Mewe data for application to plasma modeling.

astro-ph↗

arXiv2003

Recombination rate coefficients for astrophysical applications from storage-ring experiments

The basic approach for measuring electron-ion recombination rate coefficients in merged-beams electron-ion collision experiments at heavy-ion storage rings is outlined. As an example experimental results for the low temperature recombination of C IV ions are compared with the recommended theoretical rate coefficient by Mazzotta et al. The latter deviates by factors of up to 5 from the experimental one.

astro-ph↗

arXiv2001

Dielectronic Recombination (via N=2 --> N'=2 Core Excitations) and Radiative Recombination of Fe XX: Laboratory Measurements and Theoretical Calculations

We have measured the resonance strengths and energies for dielectronic recombination (DR) of Fe XX forming Fe XIX via N=2 --> N'=2 (Delta_N=0) core excitations. We have also calculated the DR resonance strengths and energies using AUTOSTRUCTURE, HULLAC, MCDF, and R-matrix methods, four different state-of-the-art theoretical techniques. On average the theoretical resonance strengths agree to within <~10% with experiment. However, the 1 sigma standard deviation for the ratios of the theoretical-to-experimental resonance strengths is >~30% which is significantly larger than the estimated relative experimental uncertainty of <~10%. This suggests that similar errors exist in the calculated level populations and line emission spectrum of the recombined ion. We confirm that theoretical methods based on inverse-photoionization calculations (e.g., undamped R-matrix methods) will severely overestimate the strength of the DR process unless they include the effects of radiation damping. We also find that the coupling between the DR and radiative recombination (RR) channels is small. We have used our experimental and theoretical results to produce Maxwellian-averaged rate coefficients for Delta_N=0 DR of Fe XX. For kT>~1 eV, which includes the predicted formation temperatures for Fe XX in an optically thin, low-density photoionized plasma with cosmic abundances, our experimental and theoretical results are in good agreement. We have also used our R-matrix results, topped off using AUTOSTRUCTURE for RR into J>=25 levels, to calculate the rate coefficient for RR of Fe XX. Our RR results are in good agreement with previously published calculations.

astro-ph↗

arXiv1999

Experimentally Derived Dielectronic Recombination Rate Coefficients for Heliumlike C V and Hydrogenic O VIII

Using published measurements of dielectronic recombination (DR) resonance strengths and energies for C V to C IV and O VIII to O VII, we have calculated the DR rate coefficient for these ions. Our derived rates are in good agreement with multiconfiguration, intermediate-coupling and multiconfiguration, fully-relativistic calculations as well as with most LS coupling calculations. Our results are not in agreement with the recommended DR rates commonly used for modeling cosmic plasmas. We have used theoretical radiative recombination (RR) rates in conjunction with our derived DR rates to produce a total recombination rate for comparison with unified RR+DR calculations in LS coupling. Our results are not in agreement with undamped, unified calculations for C V but are in reasonable agreement with damped, unified calculations for O VIII. For C V, the Burgess general formula (GF) yields a rate which is in very poor agreement with our derived rate. The Burgess & Tworkowski modification of the GF yields a rate which is also in poor agreement. The Merts et al. modification of the GF yields a rate which is in fair agreement. For O VIII the GF yields a rate which is in fair agreement with our derived rate. The Burgess & Tworkowski modification of the GF yields a rate which is in good agreement. And the Merts et al. modification yields a rate which is in very poor agreement. These results suggest that for DN=1 DR it is not possible to know a priori which formula will yield a rate closer to the true DR rate. We describe the technique used to obtain DR rate coefficients from laboratory measurements of DR resonance strengths and energies. For use in plasma modeling, we also present easy-to-use fitting formulae for the experimentally derived DR rates.

astro-ph↗