arXiv subjects

D. Zhu

Publications and source records attributed to D. Zhu.

At least 37 records · Page 2Linked to original sources

arXiv2020

Single-shot X-ray Absorption Spectroscopy at X-ray Free Electron Lasers

X-ray Absorption Spectroscopy (XAS) is a widely used X-ray diagnostic method. While synchrotrons have large communities of XAS users, its use on X-Ray Free Electron Lasers (XFEL) facilities has been rather limited. At a first glance, the relatively narrow bandwidth and the highly fluctuating spectral structure of XFEL sources seem to prevent high-quality XAS measurements without accumulating over many shots. Here, we demonstrate for the first time the collection of single-shot XAS spectra on an XFEL, with error bars of only a few percent, over tens of eV. We show how this technique can be extended over wider spectral ranges towards Extended X-ray Absorption Fine Structure (EXAFS) measurements, by concatenating a few tens of single-shot measurements. Such results open indisputable perspectives for future femtosecond time resolved XAS studies, especially for transient processes that can be initiated at low repetition rate.

physics.ins-det↗

arXiv2020

Generation of Thermofield Double States and Critical Ground States with a Quantum Computer

Finite-temperature phases of many-body quantum systems are fundamental to phenomena ranging from condensed-matter physics to cosmology, yet they are generally difficult to simulate. Using an ion trap quantum computer and protocols motivated by the Quantum Approximate Optimization Algorithm (QAOA), we generate nontrivial thermal quantum states of the transverse-field Ising model (TFIM) by preparing thermofield double states at a variety of temperatures. We also prepare the critical state of the TFIM at zero temperature using quantum-classical hybrid optimization. The entanglement structure of thermofield double and critical states plays a key role in the study of black holes, and our work simulates such nontrivial structures on a quantum computer. Moreover, we find that the variational quantum circuits exhibit noise thresholds above which the lowest depth QAOA circuits provide the best results.

quant-ph↗

arXiv2019

Training of Quantum Circuits on a Hybrid Quantum Computer

Generative modeling is a flavor of machine learning with applications ranging from computer vision to chemical design. It is expected to be one of the techniques most suited to take advantage of the additional resources provided by near-term quantum computers. We implement a data-driven quantum circuit training algorithm on the canonical Bars-and-Stripes data set using a quantum-classical hybrid machine. The training proceeds by running parameterized circuits on a trapped ion quantum computer, and feeding the results to a classical optimizer. We apply two separate strategies, Particle Swarm and Bayesian optimization to this task. We show that the convergence of the quantum circuit to the target distribution depends critically on both the quantum hardware and classical optimization strategy. Our study represents the first successful training of a high-dimensional universal quantum circuit, and highlights the promise and challenges associated with hybrid learning schemes.

quant-ph↗

arXiv2019

Demonstration of microwave multiplexed readout of DC biased superconducting nanowire detectors

Superconducting nanowires are widely used as sensitive single photon detectors with wide spectral coverage and high timing resolution. We describe a demonstration of an array of DC biased superconducting nanowire single photon detectors read out with a microwave multiplexing circuit. In this design, each individual nanowire is part of a resonant LC circuit where the inductance is dominated by the kinetic inductance of the nanowire. The circuit also contains two parallel plate capacitors, one of them is in parallel with the inductor and the other is coupled to a microwave transmission line which carries the signals to a cryogenic low noise amplifier. All of the nanowires are connected via resistors to a single DC bias line that enables the nanowires to be current biased close to their critical current. When a photon hits a nanowire it creates a normal hot spot which produces a voltage pulse across the LC circuit. This pulse rings down at the resonant frequency of the LC circuit over a time period that is fixed by the quality factor. We present measurements of an array of these devices and an evaluation of their performance in terms of frequency and time response.

physics.ins-det↗

arXiv2019

Determining the depairing current in superconducting nanowire single-photon detectors

We estimate the depairing current of superconducting nanowire single photon detectors (SNSPDs) by studying the dependence of the nanowires kinetic inductance on their bias current. The kinetic inductance is determined by measuring the resonance frequency of resonator style nanowire coplanar waveguides both in transmission and reflection configurations. Bias current dependent shifts in the measured resonant frequency correspond to the change in the kinetic inductance, which can be compared with theoretical predictions. We demonstrate that the fast relaxation model described in the literature accurately matches our experimental data and provides a valuable tool for direct determination of the depairing current. Accurate and direct measurement of the depairing current is critical for nanowire quality analysis, as well as modeling efforts aimed at understanding the detection mechanism in SNSPDs.

cond-mat.supr-con↗

arXiv2019

Multiple Fourier Component Analysis of X-ray Second Harmonic Generation in Diamond

The unprecedented brilliance of X-ray free-electron lasers (XFELs) [1, 2] has enabled first studies of nonlinear interactions in the hard X-ray range. In particular, X-ray-optical mixing [3], X-ray second harmonic generation (XSHG) [4] and nonlinear Compton scattering (NLCS) [5] have been recently observed for the first time using XFELs. The former two experiments as well as X-ray parametric downconversion (XPDC)[6, 7] are well explained by nonlinearities in the impulse approximation[8], where electrons in a solid target are assumed to be quasi free for X-ray interactions far from atomic resonances. However, the energy of the photons generated in NLCS at intensities reaching up to 4 x 1020 W/cm2 exhibit an anomalous red-shift that is in violation with the free-electron model. Here we investigate the underlying physics of X-ray nonlinear interactions at intensities on order of 1016 W/cm2. Specifically, we perform a systematic study of XSHG in diamond. While one phase-matching geometry has been measured in Shwartz et al.[4], we extend these studies to multiple Fourier components and with significantly higher statistics, which allows us to determine the second order nonlinear structure factor. We measure the efficiency, angular dependence, and contributions from different source terms of the process. We find good agreement of our measurements with the quasi-free electron model.

physics.optics↗

arXiv2019

Jitter Characterization of a Dual-Readout SNSPD

To better understand the origins of the timing resolution, also known as jitter, of superconducting nanowire single-photon detectors (SNSPDs), we have performed timing characterizations of a niobium nitride SNSPD with a dual-ended readout. By simultaneously measuring both readout pulses along with an optical timing reference signal, we are able to quantify each independent contribution to the total measured jitter. In particular, we are able to determine values for the jitter due to the stochastic nature of hotspot formation and the jitter due to the variation of the photon detection location along the length of the nanowire. We compare the results of this analysis for measurements at temperatures of 1.5 K and 4.5 K.

physics.ins-det↗

arXiv2018

Parallel Entangling Operations on a Universal Ion Trap Quantum Computer

The circuit model of a quantum computer consists of sequences of gate operations between quantum bits (qubits), drawn from a universal family of discrete operations. The ability to execute parallel entangling quantum gates offers clear efficiency gains in numerous quantum circuits as well as for entire algorithms such as Shor's factoring algorithm and quantum simulations. In cases such as full adders and multiple-control Toffoli gates, parallelism can provide an exponential improvement in overall execution time. More importantly, quantum gate parallelism is essential for the practical fault-tolerant error correction of qubits that suffer from idle errors. The implementation of parallel quantum gates is complicated by potential crosstalk, especially between qubits fully connected by a common-mode bus, such as in Coulomb-coupled trapped atomic ions or cavity-coupled superconducting transmons. Here, we present the first experimental results for parallel 2-qubit entangling gates in an array of fully-connected trapped ion qubits. We demonstrate an application of this capability by performing a 1-bit full addition operation on a quantum computer using a depth-4 quantum circuit. These results exploit the power of highly connected qubit systems through classical control techniques, and provide an advance toward speeding up quantum circuits and achieving fault tolerance with trapped ion quantum computers.

quant-ph↗

arXiv2018

Coherent order parameter dynamics in SmTe$_3$

We present a combined ultrafast optical pump-probe and ultrafast x-ray diffraction measurement of the CDW dynamics in SmTe$_3$ at 300 K. The ultrafast x-ray diffraction measurements, taken at the Linac Coherent Light Source reveal a $\sim 1.55$ THz mode that becomes overdamped with increasing fluence. We identify this oscillation with the lattice component of the amplitude mode. Furthermore, these data allow for a more clear identification of the frequencies present in the optical pump-probe data. In both, reflectivity and diffraction, we observe a crossover of the response from linear (for small displacements) to quadratic in the amplitude of the order parameter displacement. Finally, a time-dependent Ginzburg-Landau model captures the essential features of the experimental observations.

cond-mat.mtrl-sci↗

arXiv2018

Disentangling charge and structural contributions during coherent atomic motions studied by ultrafast resonant x-ray diffraction

We report on the ultrafast dynamics of charge order and structural response during the photoinduced suppression of charge and orbital order in a mixed-valence manganite. Employing femtosecond time-resolved resonant x-ray diffraction below and at the Mn K absorption edge, we present a method to disentangle the transient charge order and structural dynamics in thin films of Pr0.5Ca0.5MnO3. Based on the static resonant scattering spectra, we extract the dispersion correction of charge ordered Mn3+ and Mn4+ ions, allowing us to separate the transient contributions of purely charge order from structural contributions to the scattering amplitude after optical excitation. Our finding of a coherent structural mode at around 2.3 THz, which primarily modulates the lattice, but does not strongly affect the charge order, confirms the picture of the charge order being the driving force of the combined charge, orbital and structural transition.

cond-mat.str-el↗

arXiv2018

Coincident onset of charge density wave order at a quantum critical point in underdoped YBCO

The recently demonstrated x-ray scattering approach using a free electron laser with a high field pulsed magnet has opened new opportunities to explore the charge density wave (CDW) order in cuprate high temperature superconductors. Using this approach, we substantially degrade the superconductivity with magnetic fields up to 33 T to investigate the onset of CDW order in YBa$_2$Cu$_3$O$_x$ at low temperatures near a putative quantum critical point (QCP) at $p_1\sim $ 0.08 holes per Cu. We find no CDW can be detected in a sample with a doping concentration less than $p_1$. Our results indicate that the onset of the CDW ground state lies inside the zero-field superconducting dome, and broken translational symmetry is associated with the putative QCP at $p_1$

cond-mat.supr-con↗

arXiv2018

Demonstrating sub-3 ps temporal resolution in a superconducting nanowire single-photon detector

Improving the temporal resolution of single photon detectors has an impact on many applications, such as increased data rates and transmission distances for both classical and quantum optical communication systems, higher spatial resolution in laser ranging and observation of shorter-lived fluorophores in biomedical imaging. In recent years, superconducting nanowire single-photon detectors (SNSPDs) have emerged as the highest efficiency time-resolving single-photon counting detectors available in the near infrared. As the detection mechanism in SNSPDs occurs on picosecond time scales, SNSPDs have been demonstrated with exquisite temporal resolution below 15 ps. We reduce this value to 2.7$\pm$0.2 ps at 400 nm and 4.6$\pm$0.2 ps at 1550 nm, using a specialized niobium nitride (NbN) SNSPD. The observed photon-energy dependence of the temporal resolution and detection latency suggests that intrinsic effects make a significant contribution.

physics.ins-det↗

arXiv2017

Diffraction based Hanbury Brown and Twiss interferometry performed at a hard x-ray free-electron laser

We demonstrate experimentally Hanbury Brown and Twiss (HBT) interferometry at a hard X-ray Free Electron Laser (XFEL) on a sample diffraction patterns. This is different from the traditional approach when HBT interferometry requires direct beam measurements in absence of the sample. HBT analysis was carried out on the Bragg peaks from the colloidal crystals measured at Linac Coherent Light Source (LCLS). We observed high degree (80%) spatial coherence of the full beam and the pulse duration of the monochromatized beam on the order of 11 fs that is significantly shorter than expected from the electron bunch measurements.

physics.optics↗

arXiv2017

Direct Experimental Observation of the Gas Filamentation Effect using a Two-bunch X-ray FEL Beam

We report the experimental observation of the filamentation effect in gas devices designed for X-ray Free-electron Lasers. The measurements were carried out at the Linac Coherent Light Source on the X-ray Correlation Spectroscopy (XCS) instrument using a Two-bunch FEL beam at 6.5 keV with 122.5 ns separation passing through an Argon gas cell. The relative intensities of the two pulses of the Two-bunch beam were measured, after and before the gas cell, from the X-ray scattering off thin targets by using fast diodes with sufficient temporal resolution. It was found that the after-to-before ratio of the intensities of the second pulse was consistently higher than that of the first pulse, revealing lower effective attenuation of the gas cell due to the heating and subsequent gas density reduction in the beam path by the first pulse. This measurement is important in guiding the design and/or mitigating the adverse effect in gas devices for high repetition-rate FELs such as the LCLS-II and the European XFEL or other future high repetition-rate upgrade to existing FEL facilities

physics.app-ph↗

arXiv2017

Photoinduced Enhancement of the Charge Density Wave Amplitude

Symmetry breaking and the emergence of order is one of the most fascinating phenomena in condensed matter physics. It leads to a plethora of intriguing ground states found in antiferromagnets, Mott insulators, superconductors, and density-wave systems. Exploiting states of matter far from equilibrium can provide even more striking routes to symmetry-lowered, ordered states. Here, we demonstrate for the case of elemental chromium that moderate ultrafast photo-excitation can transiently enhance the charge-density-wave (CDW) amplitude by up to 30% above its equilibrium value, while strong excitations lead to an oscillating, large-amplitude CDW state that persists above the equilibrium transition temperature. Both effects result from dynamic electron-phonon interactions, providing an efficient mechanism to selectively transform a broad excitation of the electronic order into a well defined, long-lived coherent lattice vibration. This mechanism may be exploited to transiently enhance order parameters in other systems with coupled degrees of freedom.

cond-mat.str-el↗

arXiv2016

Ultrafast terahertz-field-driven ionic response in ferroelectric BaTiO$_3$

The dynamical processes associated with electric field manipulation of the polarization in a ferroelectric remain largely unknown but fundamentally determine the speed and functionality of ferroelectric materials and devices. Here we apply sub-picosecond duration, single-cycle terahertz pulses as an ultrafast electric field bias to prototypical BaTiO$_3$ ferroelectric thin films with the atomic-scale response probed by femtosecond x-ray scattering techniques. We show that electric fields applied perpendicular to the ferroelectric polarization drive large amplitude displacements of the titanium atoms along the ferroelectric polarization axis, comparable to that of the built-in displacements associated with the intrinsic polarization and incoherent across unit cells. This effect is associated with a dynamic rotation of the ferroelectric polarization switching on and then off on picosecond timescales. These transient polarization modulations are followed by long-lived vibrational heating effects driven by resonant excitation of the ferroelectric soft mode, as reflected in changes in the c-axis tetragonality. The ultrafast structural characterization described here enables direct comparison with first-principles-based molecular dynamics simulations, with good agreement obtained.

cond-mat.mtrl-sci↗

arXiv2016

Ideal charge density wave order in the high-field state of superconducting YBCO

The existence of charge density wave (CDW) correlations in cuprate superconductors has now been established. However, the nature of the ground state order has remained uncertain because disorder and the presence of superconductivity typically limit the CDW correlation lengths to a dozen unit cells or less. Here we explore the CDW correlations in YBa2Cu3Ox (YBCO) ortho-II and ortho-VIII crystals, which belong to the cleanest available cuprate family, at magnetic fields in excess of the resistive upper critical field (Hc2) where the superconductivity is heavily suppressed. We find an incommensurate, unidirectional CDW with a well-defined onset at a critical field strength that is proportional to Hc2. It is related to but distinct from the short-range bidirectional CDW that exists at zero magnetic field. The unidirectional CDW possesses a long inplane correlation length as well as significant correlations between neighboring CuO2 planes, yielding a correlation volume that is at least 2 - 3 orders of magnitude larger than that of the zero-field CDW. This is by far the largest CDW correlation volume observed in any cuprate crystal and so is presumably representative of the high-field ground-state of an "ideal" disorder-free cuprate.

cond-mat.str-el↗

arXiv2016

Ultrafast THz Field Control of Electronic and Structural Interactions in Vanadium Dioxide

Vanadium dioxide, an archetypal correlated-electron material, undergoes an insulator-metal transition near room temperature that exhibits electron-correlation-driven and structurally-driven physics. Using ultrafast optical spectroscopy and x-ray scattering we show that these processes can be disentangled in the time domain. Specifically, following intense sub-picosecond electric-field excitation, a partial collapse of the insulating gap occurs within the first ps. Subsequently, this electronic reconfiguration initiates a change in lattice symmetry taking place on a slower timescale. We identify the kinetic energy increase of electrons tunneling in the strong electric field as the driving force, illustrating a novel method to control electronic interactions in correlated materials on an ultrafast timescale.

cond-mat.str-el↗