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Daan B. Boltje

Publications and source records attributed to Daan B. Boltje.

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Direct Observation of Channelised Supercurrents in a Kagome Superconductor

Superconductors are many-body quantum states in which current flows without dissipation. Theory predicts that supercurrents follow a relatively simple spatial pattern in both conventional and unconventional superconductors. Recent studies into the AV3Sb5 (A = Cs, K, Rb) family of Kagome superconductors indicate that CsV3Sb5 has unconventional transport properties that cannot be accounted for with these simple theories, including reports of intrinsic Josephson junctions, higher order Cooper pairing and the zero field diode effect. Attempts to interpret these findings have focused on the interplay of superconductivity with the unconventional charge density wave (CDW) order in these materials, with which superconductivity competes. A current roadblock to understanding how these kagome superconductors give rise to their intriguing properties is the lack of spatially resolved information about transport. Here we show, using a recently developed superconducting quantum interference device (SQUID) microscope, that flakes of CsV3Sb5-xSnx host a network of narrow supercurrent channels. These supercurrent channels emerge at the critical temperature and remain stable for all temperatures and currents. Their non-linear behaviour is consistent with a network of Josephson junctions linked by narrow supercurrent filaments, which naturally leads to the observed transport anomalies. Intriguingly, these observations are much weaker in undoped samples, which suggests links to the physics of charge density waves, disorder, and electronic correlations, all of which are greatly influenced by the doping strength. These results establish new frontiers for the local investigation of charge transport and competing orders in strongly correlated electron systems, and shine a new light on the anomalous transport properties of the AV3Sb5 kagome superconductors.

cond-mat.supr-con

Tapping-mode SQUID-on-tip Microscopy with Proximity Josephson Junctions

Studying nanoscale dynamics is essential for understanding quantum materials and advancing quantum chip manufacturing. Still, it remains a major challenge to measure non-equilibrium properties such as current and dissipation, and their relation to structure. Scanning nanoprobes utilizing superconducting quantum interference devices (SQUIDs) are uniquely suited here, due to their unparalleled magnetic and thermal sensitivity. Here, we introduce tapping-mode SQUID-on-tip, which combines atomic force microscopy (AFM) with nanoSQUID sensing. Our probes minimize nanoSQUID-sample distance, provide in-plane magnetic sensitivity, and operate without lasers. Frequency multiplexing enables simultaneous imaging of currents, magnetism, dissipation and topography. The large voltage output of our proximity-junction nanoSQUIDs allows us to resolve nanoscale currents as small as 100 nA using a simple four-probe electronic readout without cryogenic amplification. By capturing local magnetic, thermal, and electronic response without external radiation, our technique offers a powerful non-invasive route to study dynamic phenomena in exotic materials and delicate quantum circuits.

cond-mat.mes-hall

Striped nanoscale phase separation at the metal-insulator transition of heteroepitaxial nickelates

Nucleation processes of mixed-phase states are an intrinsic characteristic of first-order phase transitions, typically related to local symmetry breaking. Direct observation of emerging mixed-phase regions in materials showing a first-order metal-insulator transition (MIT) offers unique opportunities to uncover their driving mechanism. Using photoemission electron microscopy, we image the nanoscale formation and growth of insulating domains across the temperature-driven MIT in NdNiO3 epitaxial thin films. Heteroepitaxy is found to strongly determine the nanoscale nature of the phase transition, inducing preferential formation of striped domains along the terraces of atomically flat stepped surfaces. We show that the distribution of transition temperatures is an intrinsic local property, set by surface morphology and stable across multiple temperature cycles. Our data provides new insights into the MIT of heteroepitaxial nickelates and points to a rich, nanoscale phenomenology in this strongly correlated material.

cond-mat.str-el