arXiv subjects

Dai-Sik Kim

Publications and source records attributed to Dai-Sik Kim.

6 recordsLinked to original sources

arXiv2026

Mechanical Activation of Terahertz Tunneling in Metallic Nanogaps

Metallic nanogaps concentrate terahertz (THz) fields into deep subwavelength volumes and support field-driven electron tunneling when the insulating barrier becomes sufficiently narrow. Here, we demonstrate mechanical control of tunneling-mediated nonlinear THz transmission in a flexible nanogap metasurface. The metasurface consists of Au/PMMA/Au nanogaps fabricated on a polyethylene terephthalate substrate, enabling continuous tuning of the gap geometry through macroscopic bending. In the flat state, the resonant transmission exhibits only a weak dependence on the incident THz field strength. Upon bending, increasing the incident field strength induces pronounced resonance suppression accompanied by saturation of the voltage developed across the nanogaps. This nonlinear response is consistent with the opening of a field-dependent tunneling conduction channel through the mechanically narrowed PMMA barriers. Simmons-model calculations illustrate the strong increase in tunneling current density and the associated dissipative gap response as the local gap width approaches the few-nanometer regime. These results establish mechanical deformation as a macroscopic means of controlling tunneling-mediated THz nonlinearities in flexible metasurfaces.

physics.optics↗

arXiv2025

Multimode Phonon-Polaritons in Lead-Halide Perovskites in the Ultrastrong Coupling Regime

Phonons play a central role in fundamental solid-state phenomena, including superconductivity, Raman scattering, and symmetry-breaking phases. Harnessing phonons to control these effects and enable quantum technologies is therefore of great interest. However, most existing phonon control strategies rely on external driving fields or anharmonic interactions, limiting their applicability. Here, we realize multimode ultrastrong light--matter coupling and theoretically show the modulation of phonon emission. This regime is realized by coupling two optical phonon modes in lead halide perovskites to a nanoslot array functioning as a single-mode cavity. The small mode volume of the nanoslots enables high coupling strengths in the phonon-polariton system. We show theoretically that the nanoslot resonator mediates an effective interaction between phonon modes, leading to superthermal phonon bunching in thermal equilibrium between distinct modes. Our findings are well described by a multimode Hopfield model. This work establishes a pathway for engineering phononic properties for light-harvesting and light-emitting technologies.

quant-ph↗

arXiv2023

Suppressed terahertz dynamics of water confined in nanometer gaps

Nanoconfined waters have been extensively studied within various systems, demonstrating low permittivity under static conditions; however, their dynamics have been largely unexplored due to the lack of a robust platform, particularly in the terahertz (THz) regime where hydrogen bond dynamics occur. We report the THz complex refractive index of nanoconfined water within metal gaps ranging in width from 2 to 20 nanometers, spanning mostly interfacial waters all the way to quasi-bulk waters. These loop nanogaps, encasing water molecules, sharply enhance light-matter interactions, enabling precise measurements of refractive index, both real and imaginary parts, of nanometer-thick layers of water. Under extreme confinement, the suppressed dynamics of the long-range correlation of hydrogen bond networks corresponding to the THz frequency regime result in a significant reduction in the terahertz permittivity of even 'non-interfacial' water. This platform provides valuable insights into the long-range collective dynamics of water molecules which is crucial to understanding water-mediated processes such as protein folding, lipid rafts, and molecular recognition.

physics.optics↗

arXiv2023

High-Efficiency Photodetector Based On CVD-Grown WS$_2$ Monolayer

Future generation technologies demand high efficiency photodetectors to enable sensing and switching devices for ultrafast communication and machine vision. This require direct-band gap materials with high photosensitivity, high detectivity and high quantum efficiency. Monolayered two- Dimensional (2D)-Semiconductors based photodetectors are the most promising materials for such applications, although experimental realization has been limited due to unavailability of high quality sample. In the current manuscript, we report about WS$_2$ based photodetector having sensitivity of 290 AW-1 upon 405 nm excitation and incident power density as low as 0.06 mW/cm$^2$. The fabricated device shows detectivity of 52*10^14 with external quantum efficiency of 89*10$^3$%. The observed superior photo-response parameters of CVD grown WS$_2$ based photodetector as compared to Si-detectors establishes it capability to replace the Si-photodetectors with monolayered ultrathin device having superior performance parameters.

physics.ins-det↗

arXiv2022

Photocurrent and photoacoustic detection of plasmonic behavior of CdSe quantum dots grown in Au nanogaps

In this work, the influence of Au plasmonics on photocurrent generation in the visible wavelength range in integrated thiol-linked CdSe quantum dot/Au nanogap structures is demonstrated. The plasmonic absorption is sensed utilizing photoacoustic (PA) detection technique. The laser diode is modulated to generate the PA excitation that oscillates the air-filled cell. When light absorption increases, an enhanced acoustic signal is captured by a microphone. The observed enhancement in the PA response is related to plasmonic absorption by the Au layers and the response is further enhanced by about 20% due to CdSe QDs. In our structure, the surface plasmon resonance (SPR) wavelength is approximately 500 nm. The SPR is utilized for generating photocurrents in CdSe quantum dots. Due to energy transfer from the dot to closely spaced Au surface through thiol links, a smooth transmission channel of electrons is established that forms a detectable photocurrent, which can be tuned by a bias voltage. These plasmonic nanogap structures can enable higher sensitivity in photovoltaics, photodetection and sensing.

cond-mat.mes-hall↗

arXiv2012

Terahertz nano antenna enabled early transition in VO2

We study terahertz transmission through nano-patterned vanadium dioxide thin film. It is found that the patterning allows the lowering of the apparent transition temperature. For the case of the smallest width nano antennas, the transition temperature is lower by as many as ten degrees relative to the bare film, so that the nano patterned hysteresis curves completely separate themselves from their bare film counterparts. This early transition comes from the one order of magnitude enhanced effective dielectric constants by nano antennas. This phenomenon opens up the possibility of transition temperature engineering.

physics.optics↗