arXiv subjects

Daisy O'Mahoney

Publications and source records attributed to Daisy O'Mahoney.

5 recordsLinked to original sources

arXiv2026

Divergence between long- and short-wavelength magnon damping in spinel ferrites

The realization of practical, high-speed magnonic devices requires engineering magnetic materials with low dissipation over wide frequency ranges. While optical and microwave probes are used to infer the damping of low energy/long wavelength modes, the degree to which these $q\sim0$ properties translate into higher-energy, finite-momentum modes remains an important open question. Here, we utilize a combination of ferromagnetic resonance (FMR) and resonant inelastic x-ray scattering on spinel ferrites Li$_{0.5}$Al$_x$Fe$_{2.5-x}$O$_4$ to probe magnons in both the short- and long-wavelength limits. We observe that aluminum substitution both markedly reduces the magnon bandwidth and drastically shortens the high-$q$ magnon lifetimes, in sharp contrast to the ultralow magnon damping inferred from FMR. These findings demonstrate a disparity between how non-magnetic substituents impact magnon damping in the long- and short-wavelength limits, providing a new perspective for assessing candidate materials for magnonic devices.

cond-mat.mtrl-sci↗

arXiv2026

Two Strategies to Measure Spin-Orbit-Torque Efficiency Acting on the Insulating Magnet Li$_{0.5}$Al$_{0.7}$Fe$_{1.8}$O$_4$

For insulating magnets, widely-used electrically-based techniques to measure spin-orbit-torque efficiency can suffer from poor signal-to-noise ratios and unwanted artifacts, while optical measurements based on conventional magneto-optical Kerr effect (MOKE) imaging often lack sufficient sensitivity. Here we analyze two strategies for measuring the spin-torque efficiency acting on an insulating magnet, focusing on the torque from Pt acting on thin films of the low-damping magnet lithium aluminum ferrite (LAFO). First, lateral + longitudinal spin-torque ferromagnetic resonance (ST-FMR) allows separation of the spin-torque signal from artifacts due to spin-pumping and resonant heating. With this technique, we measure a spin-torque efficiency $ξ^\text{ST-FMR}_\text{DL}\sim\ 0.07$, comparable to but a bit less than for Pt acting on metallic ferromagnets. Second, we attempted optical measurements of spin-orbit-torque-induced magnetic deflection using Sagnac interferometry. We find that Sagnac interferometry provides sufficient sensitivity to measure signals from 14.4 nm LAFO thin films, but the inferred torque efficiency is much weaker than the result from lateral + longitudinal ST-FMR. We speculate that there may be another contribution to the Sagnac signal other than current-induced magnetic deflection, perhaps an out-of-plane component of itinerant electron spins. This becomes relevant for insulating magnets in which the magneto-optic coupling coefficient is very weak.

cond-mat.mes-hall↗

arXiv2026

Tuning perpendicular magnetic anisotropy in ultra-low damping Li$_{0.5}$Al$_{x}$Fe$_{(2.5-x)}$O$_4$ thin films for efficient spin-orbit torque switching

Ultra-thin magnetic insulator films that simultaneously exhibit ultra-low magnon damping, perpendicular magnetic anisotropy (PMA), and low spin-orbit torque (SOT) switching current densities are highly desirable, albeit challenging, for next-generation spintronic technologies that exploit spin waves to transport information without dissipative charge currents. Here, we demonstrate this combination of properties in ferrimagnetic spinel Li$_{0.5}$Al$_{x}$Fe$_{(2.5-x)}$O$_4$ (LAFO) thin films. Through this model system, we find that PMA can be tuned by epitaxial strain in the form of chemical composition and substrate choice and that low SOT switching current densities correlate with small but finite PMA. Ultra-low damping is stabilized primarily by having only Fe$^{3+}$ as magnetically active cations with secondary effects due to increased disorder from Al substitution distribution. SOT efficiency is governed by interface quality and independent of chemical composition. By varying the Al concentration, we systematically tune the saturation magnetization and magnetic anisotropy while maintaining ultra-low Gilbert damping parameters as low as $2\times10^{-4}$ and composition-independent damping-like SOT efficiencies. We identify an optimal composition LAFO x=0.7 (Li$_{0.5}$Al$_{0.7}$Fe$_{1.8}$O$_4$), which combines ultra-low damping, stable PMA with small anisotropy fields, and low critical current densities for SOT switching, establishing it as a promising material platform for energy-efficient spin-wave and spintronic devices.

cond-mat.mtrl-sci↗

arXiv2026

Nearly Isotropic Magnon Transport in Epitaxial Lithium Aluminum Ferrite Thin Films

Low-loss magnetic insulating thin films are promising for information transport via magnons, where isotropic in-plane magnon propagation is desirable. We report nonlocal measurements of electrically and thermally generated magnons in epitaxial (001) lithium aluminum ferrite Li$_{0.5}$Al$_{0.7}$Fe$_{1.8}$O$_4$ thin films with pronounced fourfold in-plane magnetic anisotropy. By measuring the inverse spin Hall signal as a function of the magnon diffusion distance, we deduce magnon diffusion lengths that are nearly identical along the [100] and [110] directions at 250~K. This isotropy is consistent with a nearly isotropic exchange stiffness. These results highlight spinel ferrites as viable platforms for isotropic magnon transport.

cond-mat.mtrl-sci↗

arXiv2023

Exploring the origins of perpendicular magnetic anisotropy in amorphous Tb-Co via changes in medium-range ordering

Amorphous thin films of Tb$_{17}$Co$_{83}$ (a-Tb-Co) grown by magnetron co-sputtering exhibit changes in magnetic anisotropy with varying growth and annealing temperatures. The magnetic anisotropy constant increases with increasing growth temperature, which is reduced or vanishes upon annealing at temperatures above the growth temperature. The proposed explanation for this growth-induced anisotropy in high orbital moment Tb-based transition metal alloys such as a-Tb-Co is an amorphous phase texturing with preferential in-plane and out-of-plane local bonding configurations for the rare-earth and transition metal atoms. Scanning nanodiffraction performed in a transmission electron microscope (TEM) is applied to a-Tb$_{17}$Co$_{83}$ films deposited over a range of temperatures to measure relative changes in medium-range ordering (MRO). These measurements reveal an increase in MRO with higher growth temperatures and a decrease in MRO with higher annealing temperatures. The trend in MRO indicates a relationship between the magnetic anisotropy and local atomic ordering. Tilting select films between 0$^{\circ}$ and 40$^{\circ}$ in the TEM measures variations in the local atomic structure a function of orientation within the films. The findings support claims that preferential ordering along the growth direction results from temperature-mediated adatom configurations during deposition, and that oriented MRO correlates with the larger anisotropy constants.

cond-mat.mtrl-sci↗