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Dajun Wang

Publications and source records attributed to Dajun Wang.

35 records · Page 2Linked to original sources

Dipolar Collisions of Ultracold Ground-state Bosonic Molecules

The dipolar collision between ultracold polar molecules is an important topic both by its own right from the fundamental point of view and for the successful exploration of many-body physics with strong and long-range dipolar interactions. Here, we report the investigation of collisions between ultracold ground-state sodium-rubidium molecules in electric fields with induced electric dipole moments as large as 0.7$\;$D. We observe a step-wise enhancement of losses due to the coupling between different partial waves induced by the increasingly stronger anisotropic dipolar interactions. Varying the temperature of our sample, we find good agreement with theoretical loss rates assuming complex formation as the main loss process. Our results shed new light on the understanding of complex molecular collisions in the presence of strong dipolar interactions and also demonstrate the versatility of modifying molecular interactions with electric fields.

cond-mat.quant-gas↗

Longitudinal Safety Analysis For Heterogeneous Platoon Of Automated And Human Vehicles

With the recent advancement in environmental sensing, vehicle control and vehicle-infrastructure cooperation technologies, more and more autonomous driving companies start to put their intelligent cars into road test. But in the near future, we will face a heterogeneous traffic with both intelligent connected vehicles and human vehicles. In this paper, we investigated the impacts of four collision avoidance algorithms under different intelligent connected vehicles market penetration rate. A customized simulation platform is built, in which a platoon can be initiated with many key parameters. For every short time interval, the dynamics of vehicles are updated and input in a kinematics model. If a collision occurs, the energy loss is calculated to represent the crash severity. Four collision avoidance algorithms are chosen and compared in terms of the crash rate and severity at different market penetration rate and different locations of the platoon. The results generate interesting debates on the issues of heterogeneous platoon safety.

eess.SY↗

Collisions of ultracold ^{23}Na^{87}Rb molecules with controlled chemical reactivities

The collision of molecules at ultracold temperatures is of great importance for understanding the chemical interactions at the quantum regime. While much theoretical work has been devoted to this, experimental data are only available sparsely mainly due to the difficulty in producing ground-state molecules at ultracold temperatures. We report here the creation of optically trapped samples of ground-state bosonic sodium-rubidium molecules with precisely controlled internal states and, enabled by this, a detailed study on the inelastic loss with and without the NaRb + NaRb $\rightarrow$ Na$_2$ + Rb$_2$ chemical reaction. Contrary to intuitive expectations, we observed very similar loss and heating, regardless of the chemical reactivities. In addition, as evidenced by the reducing loss rate constants with increasing temperatures, we found that these collisions are already outside the Wigner region even though the sample temperatures are sub-microkelvin. Our measurement agrees semi-quantitatively with models based on long-range interactions, but calls for a deeper understanding on the short-range physics for a more complete interpretation.

cond-mat.quant-gas↗

High-resolution Internal State Control of Ultracold $^{23}$Na$^{87}$Rb Molecules

We report the full control over the internal states of ultracold $^{23}$Na$^{87}$Rb molecules, including vibrational, rotational and hyperfine degrees of freedom. Starting from a sample of weakly bound Feshbach molecules, we realize the creation of molecules in single hyperfine levels of both the rovibrational ground and excited states with a high-efficiency and high-resolution stimulated Raman adiabatic passage. Starting from the rovibrational and hyperfine ground state, we demonstrate rotational and hyperfine control with one- and two-photon microwave spectroscopy. This achievement of fully controlling the molecular internal states paves the way to study state dependent molecular collisions and state controlled chemical reactions.

cond-mat.quant-gas↗

Unfolding multi-particle quantum correlations hidden in decoherence

Quantum coherence is a fundamental characteristic to distinguish quantum systems from their classical counterparts. Though quantum coherence persists in isolated non-interacting systems, interactions inevitably lead to decoherence, which is in general believed to cause the lost of quantum correlations. Here, we show that, accompanying to the single-particle decoherence, interactions build up quantum correlations on the two-, three-, and multi-particle levels. Using the quantitative solutions of the quantum dynamics of a condensate occupying two modes, such as two bands of an optical lattice, we find out that such dynamically emergent multi-particle correlations not only reveal how interactions control the quantum coherence of a many-body system in a highly intriguing means, but also evince the rise of exotic fragmented condensates, which are difficult to access at the ground state. We further develop a generic interferometry that can be used in experiments to measure high order correlation functions directly.

cond-mat.quant-gas↗

High Resolution Molecular Spectroscopy for Producing Ultracold Absolute Ground-State $^{23}$Na$^{87}$Rb Molecules

We report a detailed molecular spectroscopy study on the lowest excited electronic states of $^{23}\rm{Na}^{87}\rm{Rb}$ for producing ultracold $^{23}\rm{Na}^{87}\rm{Rb}$ molecules in the electronic, rovibrational and hyperfine ground state. Starting from weakly-bound Feshbach molecules, a series of vibrational levels of the $A^{1}Σ^{+}-b^{3}Π$ coupled excited states were investigated. After resolving, modeling and interpreting the hyperfine structure of several lines, we successfully identified a long-lived level resulting from the accidental hyperfine coupling between the $0^+$ and $0^-$ components of the $b^3Π$ state, satisfying all the requirements for the population transfer toward the lowest rovibrational level of the X$^1Σ^+$ state. Using two-photon spectroscopy, its binding energy was measured to be 4977.308(3) cm$^{-1}$, the most precise value to date. We calibrated all the transition strengths carefully and also demonstrated Raman transfer of Feshbach molecules to the absolute ground state.

cond-mat.quant-gas↗

Creation of an ultracold gas of ground-state $^{23}\rm{Na}^{87}\rm{Rb}$ molecules

We report the successful production of an ultracold sample of absolute ground-state $^{23}$Na$^{87}$Rb molecules. Starting from weakly-bound Feshbach molecules formed via magneto-association, the lowest rovibrational and hyperfine level of the electronic ground state is populated following a high efficiency and high resolution two-photon Raman process. The high purity absolute ground-state samples have up to 8000 molecules and densities of over $10^{11}$ cm$^{-3}$. By measuring the Stark shifts induced by external electric fields, we determined the permanent electric dipole moment of the absolute ground-state $^{23}$Na$^{87}$Rb and demonstrated the capability of inducing an effective dipole moment over one Debye. Bimolecular reaction between ground-state $^{23}$Na$^{87}$Rb molecules is endothermic, but we still observed a rather fast decay of the molecular sample. Our results pave the way toward investigation of ultracold molecular collisions in a fully controlled manner, and possibly to quantum gases of ultracold bosonic molecules with strong dipolar interactions.

cond-mat.quant-gas↗

Magnetic field induced dynamical instabilities in an anti-ferromagnetic spin-1 Bose-Einstein condensate

We theoretically investigate four types of dynamical instability, in particular the periodic and oscillatory type $I_O$, in an anti-ferromagnetic spin-1 Bose-Einstein condensate in a nonzero magnetic field, by employing the coupled-mode theory and numerical method. This is in sharp contrast to the dynamical stability of the same system in zero field. Remarkably, a pattern transition from a periodic dynamical instability $I_O$ to a uniform one $III_O$ occurs at a critical magnetic field. All the four types of dynamical instability and the pattern transition are ready to be detected in $^{23}$Na condensates within the availability of the current experimental techniques.

cond-mat.quant-gas↗

Long-range states of the NaRb molecule near the Na($3^2S_{1/2}$)+Rb($5^2P_{3/2}$) asymptote

We report a high-resolution spectroscopic investigation of the long-range states of the $^{23}$Na$^{87}$Rb molecule near its Na($3^2S_{1/2}$)+Rb($5^2P_{3/2}$) asymptote. This study was performed with weakly bound ultracold molecules produced via magneto-association with an inter-species Feshbach resonance. We observed several regular vibrational series, which are assigned to the 5 attractive long-range states correlated with this asymptote. The vibrational levels of two of these states have sharp but complex structures due to hyperfine and Zeeman interactions. For the other states, we observed significant linewidth broadenings due to strong predissociation caused by spin-orbit couplings with states correlated to the lower Na($3^2S_{1/2}$)+Rb($5^2P_{1/2}$) asymptote. The long-range $C_6$ van der Waals coefficients extracted from our spectrum are in good agreement with theoretical values.

physics.atom-ph↗

A double species $^{23}$Na and $^{87}$Rb Bose-Einstein condensate with tunable miscibility via an interspecies Feshbach resonance

We have realized a dual-species Bose-Einstein condensate (BEC) of $^{23}$Na and $^{87}$Rb atoms and observed their immiscibility. Because of the favorable background intra- and inter-species scattering lengths, stable condensates can be obtained via efficient evaporative cooling and sympathetic cooling without the need for fine tuning of the interactions. Our system thus provides a clean platform for studying inter-species interactions driven effects in superfluid mixtures. With a Feshbach resonance, we have successfully created double BECs with largely tunable inter-species interactions and studied the miscible-immiscible phase transition.

cond-mat.quant-gas↗

Coherent spin mixing dynamics in thermal $^{87}$Rb spin-1 and spin-2 gases

We study the non-equilibrium coherent spin mixing dynamics in ferromagnetic spin-1 and antiferromagnetic spin-2 thermal gases of ultracold $^{87}$Rb atoms. Long lasting spin population oscillations with magnetic field dependent resonances are observed in both cases. Our observations are well reproduced by Boltzmann equations of the Wigner distribution function. Compared to the equation of motion of spinor Bose-Einstein condensates, the only difference here is a factor of two increase in the spin-dependent interaction, which is confirmed directly in the spin-2 case by measuring the relation between the oscillation amplitude and the sample's density.

physics.atm-clus↗

Formation of Ultracold NaRb Feshbach Molecules

We report the creation of ultracold bosonic $^{23}$Na$^{87}$Rb Feshbach molecules via magneto-association. By ramping the magnetic field across an interspecies Feshbach resonance, at least 4000 molecules can be produced out of the near degenerate ultracold mixture. Fast loss due to inelastic atom-molecule collisions is observed, which limits the pure molecule number, after residual atoms removal, to 1700. The pure molecule sample can live for 21.8(8) ms in the optical trap, long enough for future molecular spectroscopy studies toward coherently transferring to the singlet ro-vibrational ground state, where these molecules are stable against chemical reaction and have a permanent electric dipole moment of 3.3 Debye. We have also measured the Feshbach molecule's binding energy near the Feshbach resonance by the oscillating magnetic field method and found these molecules have a large closed-channel fraction.

physics.atom-ph↗

Coherent heteronuclear spin dynamics in an ultracold spin-1 mixture

We report the observation of coherent heteronuclear spin dynamics driven by inter-species spin-spin interaction in an ultracold spinor mixture, which manifests as periodical and well correlated spin oscillations between two atomic species. In particular, we investigate the magnetic field dependence of the oscillations and find a resonance behavior which depends on {\em both} the linear and quadratic Zeeman effects and the spin-dependent interaction. We also demonstrate a unique knob for controlling the spin dynamics in the spinor mixture with species-dependent vector light shifts. Our finds are in agreement with theoretical simulations without any fitting parameters.

physics.atom-ph↗

Observation of Feshbach resonances between ultracold Na and Rb atoms

We have successfully prepared an optically trapped ultracold mixture of $^{23}$Na and $^{87}$Rb atoms and studied their interspecies Feshbach resonances. Using two different spin combinations, several s-wave and p-wave resonances are identified by observing a high inelastic loss and a temperature rising for both species near resonant magnetic field values. The two s-wave resonances observed below 500 G between atoms in the lowest energy level are possible candidates for Feshbach molecule association. Our results are well characterized by a coupled-channel model and are used refining the ground state interaction potentials between $^{23}$Na and $^{87}$Rb. This work opens up the prospect for preparing ultracold ensembles of ground-state bosonic NaRb molecules which are chemically stable and can provide strong dipolar interactions.

cond-mat.quant-gas↗

Production of a rubidium Bose-Einstein condensate in a hybrid trap with light induced atom desorption

We report on the production of a rubidium Bose-Einstein condensate in a simplified vacuum apparatus. Magneto-optical traps with large numbers and ultra-high vacuum for moderately long conservative trap lifetimes of 16 seconds are sequentially obtained with light induced rapid atomic vapor pressure modulation. Subsequent evaporative cooling is carried out in two stages in a hybrid magnetic quadrupole plus optical dipole trap. High evaporation efficiencies are observed in both stages and $^{87}$Rb BECs with more than 10$^5$ atoms can be reliably produced with total evaporation time of only 9.5 seconds.

cond-mat.quant-gas↗

Magneto-Optical Trap for Polar Molecules

We propose a method for laser cooling and trapping a substantial class of polar molecules, and in particular titanium (II) oxide (TiO). This method uses pulsed electric fields to nonadiabatically remix the ground-state magnetic sublevels of the molecule, allowing us to build a magneto-optical trap (MOT) based on a quasi-cycling $J'=J"-1$ transition. Monte-Carlo simulations of this electrostatically remixed MOT (ER-MOT) demonstrate the feasibility of cooling TiO to a temperature of 10 $\mathrmμK$ and trapping it with a radiation-pumping-limited lifetime on the order of 80 ms.

physics.atom-ph↗

Low-energy molecular collisions in a permanent magnetic trap

Cold, neutral hydroxyl radicals are Stark decelerated and confined within a magnetic trap consisting of two permanent ring magnets. The OH molecules are trapped in the ro-vibrational ground state at a density of $\sim10^{6}$ cm$^{-3}$ and temperature of 70 mK. Collisions between the trapped OH sample and supersonic beams of atomic He and molecular D$_{2}$ are observed and absolute collision cross sections measured. The He--OH and D$_{2}$--OH center-of-mass collision energies are tuned from 60 cm$^{-1}$ to 230 cm$^{-1}$ and 145 cm$^{-1}$ to 510 cm$^{-1}$, respectively, yielding evidence of reduced He--OH inelastic cross sections at energies below 84 cm$^{-1}$, the OH ground rotational level spacing.

physics.atom-ph↗