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Dakun Wu

Publications and source records attributed to Dakun Wu.

6 recordsLinked to original sources

Electron-beam Writing of Spectrally Uniform Green Single-photon Emitters in Hexagonal Boron Nitride

Scalable quantum photonic technologies require single-photon emitters whose positions and emission energies can be engineered simultaneously. Hexagonal boron nitride (hBN) is an attractive room-temperature host, but deterministic creation of spectrally reproducible emitters remains challenging. Here, we use a standard scanning electron microscope as a direct-writing tool to activate bright green single-photon emitters in hBN at predefined sites, without ion implantation or post-fabrication thermal annealing. The written emitters exhibit reproducible zero-phonon-line emission centered near 536 nm, room-temperature antibunching with g(2)(0) as low as 0.08, high brightness, strong linear polarization, and stable emission. Thickness-dependent activation, stacking experiments, cathodoluminescence spectroscopy, and first-principles calculations support a carbon-related defect complex as the most plausible origin of the emission. As a proof of nanophotonic compatibility, we further activate emitters in a nanoparticle-on-mirror plasmonic nanocavity and observe photoluminescence enhancement accompanied by shortened emission lifetimes. These results establish electron-beam direct writing as a practical route to site-selective, spectrally uniform green quantum emitters in hBN, offering a promising basis for integrated room-temperature quantum photonic architectures.

physics.optics

Delivery of nanosecond laser pulses by multimode anti-resonant hollow core fiber at 1 um wavelength

In this paper we explore the application of low-loss multimode anti-resonant hollow-core fiber (MM-AR-HCF) in the delivery of nanosecond laser pulses at 1 um wavelength. MM-AR-HCF of large core offers a rich content of low-loss higher-order modes which plays a key role in the efficient coupling and transmission of high-power laser of degraded beam quality. In the experiment, laser pulses of an average pulse energy of 21.8 mJ with 14.6 ns pulse width (corresponding a peak power of 1.49 MW) are transmitted through MM-AR-HCF of 9.8 m length without damaging. Up to 94 % coupling efficiency is achieved where the incident laser beam suffers a degraded beam quality with and of 2.18 and 1.99 respectively. Laser-induced damage threshold (LIDT) of MM-AR-HCF measures 22.6 mJ for 94 % coupling efficiency, which is 7 times higher than that for multimode silica optical fiber with a core diameter of 200 um.

physics.optics

Broadband Dispersive-Wave Emission Coupled with Two-Stage Soliton Self-Compression in Gas-Filled Anti-Resonant Hollow-Core Fibers

We studied the underlying mechanism of broadband dispersive-wave emission within a resonance band of gas-filled anti-resonant hollow-core fiber. Both theoretical and experimental results unveiled that the high-order soliton, launched into the hollow-core fiber, experienced two stages of pulse compression, resulting in a multi-peak structure of the dispersive-wave spectrum. Over the first-stage pulse compression, a sharp increase of the pulse peak power triggered the first time of dispersion-wave emission, and simultaneously caused ionization of the noble gas filled in the fiber core. Strong soliton-plasma interactions led to blue shifting of the pump pulse, and the blue-shifted pulse experienced a decreasing dispersion value in the fiber waveguide, resulting in an increase of its soliton order. Then, the second-stage pulse compression due to the high-order soliton effect triggered the second time of dispersive-wave emission at a phase-matched frequency slightly lower than that in the first stage. Multi-peak spectra of the output dispersive-waves and their formation dynamics were clearly observed in our experiments, which can be understood using a delicate coupling mechanism among three nonlinear effects including high-order-soliton compression, soliton-plasma interaction and phase-matched dispersive-wave emission. The output broadband dispersive-wave could be potentially compressed to sub-30 fs duration using precise chirp-compensation technique.

physics.optics

Measurements of microjoule-level, few-femtosecond ultraviolet dispersive-wave pulses generated in gas-filled hollow capillary fibers

High-energy ultraviolet pulse generation in gas-filled hollow capillary fibers (HCFs) through dispersive-wave-emission process, has attracted considerable attentions in recent several years due to its great application potentials in ultraviolet spectroscopy and photochemistry. While the ability of this technique to deliver high-energy, ultrafast ultraviolet pulses is widely recognized, few-fs duration of μJ-level dispersive-wave (DW) pulses has, however, escaped direct measurements. In this letter, we demonstrate that using several chirped mirrors, few-fs ultraviolet DW pulses can be obtained in atmosphere environment without the use of vacuum chambers. The pulse temporal profiles, measured using a self-diffraction frequency-resolved optical gating set-up, exhibit full-width-half-maximum pulse widths of 9.6 fs at 384 nm and 9.4 fs at 430 nm, close to the Fourier-transform limits. Moreover, theoretical and experimental studies reveal the strong influences of driving pulse energy and HCF length on temporal width and shape of the measured DW pulses. The ultraviolet pulses obtained in atmosphere environment with μJ-level pulse energy, few-fs pulse width and broadband wavelength tunability are ready to be used in many applications.

physics.optics

Photoionization-induced broadband dispersive wave generated in an Ar-filled hollow-core photonic crystal fiber

The resonance band in hollow-core photonic crystal fiber (HC-PCF), while leading to high-loss region in the fiber transmission spectrum, has been successfully used for generating phase-matched dispersive wave (DW). Here, we report that the spectral width of the resonance-induced DW can be largely broadened due to plasma-driven blueshifting soliton. In the experiment, we observed that in a short length of Ar-filled single-ring HC-PCF the soliton self-compression and photoionization effects caused a strong spectral blueshift of the pump pulse, changing the phase-matching condition of the DW emission process. Therefore, broadening of DW spectrum to the longer-wavelength side was obtained with several spectral peaks, which correspond to the generation of DW at different positions along the fiber. In the simulation, we used super-Gauss windows with different central wavelengths to filter out these DW spectral peaks, and studied the time-domain characteristics of these peaks respectively using Fourier transform method. The simulation results verified that these multiple-peaks on the DW spectrum have different delays in the time domain, agreeing well with our theoretical prediction. Remarkably, we found that the whole time-domain DW trace can be compressed to ~29 fs using proper chirp compensation. The experimental and numerical results reported here provide some insight into the resonance-induced DW generation process in gas-filled HC-PCFs, they could also pave the way to ultrafast pulse generation using DW-emission mechanism.

physics.optics

Photoionization-assisted, high-efficiency emission of dispersive wave in gas-filled hollow-core photonic crystal fibers

We demonstrate that the phase-matched dispersive wave (DW) emission within the resonance band of a 25-cm-long gas-filled hollow-core photonic crystal fiber (HC-PCF) can be strongly enhanced by the photoionization effect of the pump pulse. In the experiments we observe that as the pulse energy increases, the pump pulse gradually shifts to shorter wavelengths due to soliton-plasma interactions. When the central wavelength of the blueshifting soliton is close to the resonance band of the HC-PCF, high-efficiency energy transfer from the pump light to the DW in the visible region can be obtained. During this DW emission process, we also observe that the spectral center of the DW gradually shifts to longer wavelengths leading to a slightly-increased DW bandwidth, which can be well explained as the consequence of phase-matched coupling between the pump pulse and the DW. In particular, at an input pulse energy of 6 uJ, the spectral ratio of the DW at the fiber output is measured to be as high as ~53% together with a conversion efficiency of ~19%. These experimental results, explained by numerical simulations, pave the way to high-brightness light sources based on high-efficiency frequency-upconversion processes in gas-filled HC-PCFs.

physics.optics