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Damien Vandembroucq

Publications and source records attributed to Damien Vandembroucq.

At least 19 recordsLinked to original sources

Activation and Avalanche Length Scales in the Finite-Temperature Creep of an Elastic Interface

We investigate the creep dynamics of a driven elastic line at finite temperature, well below the depinning threshold. We show that creep is governed by two distinct length scales. The first, $\ell_{\mathrm{opt}}$, corresponds to the optimal activated rearrangements that control the dynamics' bottleneck and remains essentially temperature-independent. The second, $\ell_{\mathrm{av}}$, characterizes the spatial extent of thermally activated avalanches and grows as temperature decreases. By combining structural and dynamical observables, we show that $\ell_{\mathrm{av}}$ governs both the crossover in the structure factor and the growth of the four-point dynamical susceptibility, while the relaxation time remains controlled by activation over large barriers associated with $\ell_{\mathrm{opt}}$. We find that the avalanche scale follows $\ell_{\mathrm{av}}(T)\sim T^{-ν_{\mathrm{dep}}}$, thereby selecting a unique scenario among competing theoretical predictions. These results establish a unified picture of finite-temperature creep in which activation controls temporal scales while depinning criticality governs spatial correlations.

cond-mat.stat-mech

Self-organization, Memory and Learning: From Driven Disordered Systems to Living Matter

Disordered systems subject to a fluctuating environment can self-organize into a complex history-dependent response, retaining a memory of the driving. In sheared amorphous solids, self-organization is established by the emergence of a persistent system of mechanical instabilities that can repeatedly be triggered by the driving, leading to a state of high mechanical reversibility. As a result of self-organization, the response of the system becomes correlated with the dynamics of its environment, which can be viewed as a sensing mechanism of the system's environment. Such phenomena emerge across a wide variety of soft matter systems, suggesting that they are generic and hence may depend very little on the underlying specifics. We review self-organization in driven amorphous solids, concluding with a discussion of what self-organization in driven disordered systems can teach us about how simple organisms sense and adapt to their changing environments.

cond-mat.soft

Memory behavior of a randomly driven model glass

We investigate by atomistic simulations the memory behavior a model glass subjected to random driving protocols. The training consists of a random walk of forward and/or backward shearing sequences bounded by a maximal shear strain of absolute value γT . We show that such a stochastic training protocol is able to record the training amplitude. Different read-out protocols are also tested and are shown to be able to retrieve the training amplitude. We then emphasize the ten- sorial character of the memory encoded in the glass sample and then characterize the anisotropic mechanical behavior of the trained samples.

cond-mat.soft

Self-organization and memory in an disordered solid subject to random loading

We consider self-organization and memory formation in a mesoscopic model of an amorphous solid subject to a random shear strain protocol confined to a strain range $\pm \varepsilon_{\rm max}$. We develop proper read-out protocols to show that the response of the driven system retains a memory of the strain range, which can be subsequently retrieved. Our findings generalize previous results obtained upon oscillatory driving and suggest that self-organization and memory formation of disordered materials can emerge under more general conditions, such as a disordered system interacting with its fluctuating environment. The self-organization results in a correlation between the dynamics of the system and its environment. We conclude by discussing our results within the context of environmental sensing, highlighting their generalizability to adaptation strategies of simple organisms under changing conditions.

cond-mat.soft

Self-organization and memory in a cyclically driven elasto-plastic model of an amorphous solid

The mechanical behavior of disordered materials such as dense suspensions, glasses or granular materials depends on their thermal and mechanical past. Here we report the memory behavior of a quenched mesoscopic elasto-plastic (QMEP) model. After prior oscillatory training, a simple read-out protocol gives access to both the training protocol's amplitude and the last shear direction. The memory of direction emerges from the development of a mechanical polarization during training. The analysis of sample-to-sample fluctuations gives direct access to the irreversibility transition. Despite the quadrupolar nature of the elastic interactions in amorphous solids, a behavior close to Return Point Memory (RPM) is observed. The quasi RPM property is used to build a simple Preisach-like model of directional memory.

cond-mat.soft

Anomalous softness in amorphous matter in the reversible plastic regime

We study an integer automaton elasto-plastic model of an amorphous solid subject to cyclic shear of amplitude $Γ$. We focus on the reversible plastic regime at intermediate $Γ_0<Γ<Γ_y$, where, after a transient, the system settles into a periodic limit cycle with hysteretic, dissipative plastic events which repeat after an integer number of cycles. We study the plastic strain rate, $\frac{dε}{dγ}$, (where $γ$ is the applied strain and $ε$ is the plastic strain) during the terminal limit cycles and show that it consists of a creeping regime at low $γ$ with very low $\frac{dε}{dγ}$ followed by a sharp transition at a characteristic strain, $γ_*$, and stress, $σ_*$, to a flowing regime with higher $\frac{dε}{dγ}$. We show that while increasing $Γ$ above $Γ_0$ results in lower terminal ground state energy, $U_{\text{min}}$, and a correspondingly narrower distribution of stresses, it, surprisingly, results in lower $γ_*$, and $σ_*$. The stress distribution, $P(σ)$, also becomes skewed for $Γ>Γ_0$. That is, the systems in the RPR are anomalously soft and mechanically polarized. We relate this to an emergent characteristic feature in the stress distribution, $P(σ)$, at a value, $σ_0$, which is independent of $Γ$ and show that $σ_0$ implies a relation between the $Γ$ dependence of $σ_*$, $γ_*$, and the amplitude of plastic strain, $ε_p$. We show that the onset of hysteresis is characterized by a power-law scaling, indicative of a second order transition with $ε_p\propto (Γ-Γ_0)^{1.2\pm0.1}$. We argue that $σ_0$ and, correspondingly, the onset of the RPR at $Γ=Γ_0$, is simply set by the so-called Eshelby-stress. Furthermore, we show that cycling at $Γ_0$ results in a maximally hardened state.

cond-mat.soft

Relevance of Shear Transformations in the Relaxation of Supercooled Liquids

While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this dramatic slowdown is key for understanding the glass transition. Here, we show by atomistic simulations that the heterogeneous dynamics of glass-forming liquids strongly correlate with the local residual plastic strengths along soft directions computed in the initial inherent structures. The correlation increases with decreasing temperature and is maximum in the vicinity of the relaxation time. For the lowest temperature investigated, this maximum is comparable with the best values from the literature dealing with the structure-property relationship. However, the nonlinear probe of the local shear resistance in soft directions provides here a real-space picture of relaxation processes. Our detection method of thermal rearrangements allows us to investigate the first passage time statistics and to study the scaling between the activation energy barriers and the residual plastic strengths. These results shed new light on the nature of relaxations of glassy systems by emphasizing the analogy between the thermal relaxations in viscous liquids and the plastic shear transformation in amorphous solids.

cond-mat.mtrl-sci

Coarse-graining amorphous plasticity: impact of rejuvenation and disorder

The coarse-graining of amorphous plasticity from the atomistic to the mesoscopic scale is studied in the framework of a simple scalar elasto-plastic model. Building on recent results obtained on the atomistic scale, we discuss the interest in a disordered landscape-informed threshold disorder to reproduce the physics of amorphous plasticity. We show that accounting for a rejuvenation scenario allows us to reproduce quasi-quantitatively the evolution of the mean local yield stress and the localization behavior. We emphasize the crucial role of two dimensionless parameters: the relative strength of the yield stress disorder with respect to the typical stress drops associated with a plastic rearrangement, and the age parameter characterizing the relative stability of the initial glass with respect to the rejuvenated glass that emerges upon shear deformation.

cond-mat.soft

Hollow-core fibers with reduced surface roughness and ultralow loss in the short-wavelength range

While optical fibers display excellent performances in the infrared, visible and ultraviolet ranges remain poorly addressed by them. Obtaining better fibers for the short-wavelength range has been restricted, in all fiber optics, by scattering processes. In hollow-core fibers, the scattering loss arises from the core roughness and represents the limiting factor in reducing their loss regardless of the fiber cladding confinement power. To attain fibers performing at short wavelengths, it is paramount developing means to minimize the height variations on the fiber microstructure boundaries. Here, we report on the reduction of the core surface roughness of hollow-core fibers by modifying their fabrication technique. In the novel process proposed herein, counter directional gas fluxes are applied within the fiber holes during fabrication to attain an increased shear rate on its microstructure. The effect of the process on the surface roughness has been quantified by optical profilometry and the results showed that the root-mean-square surface roughness has been reduced from 0.40 nm to 0.15 nm. The improvement in the fiber core surface quality entailed fibers with ultralow loss in the short-wavelength range. We report on fibers with record loss values as low as 50 dB/km at 290 nm, 9.7 dB/km at 369 nm, 5.0 dB/km at 480 nm, and 1.8 dB/km at 719 nm. The results reveal this new approach as a promising path for the development of hollow-core fibers guiding at short wavelengths with loss that can potentially be orders of magnitude lower than the ones achievable with their silica-core counterparts.

physics.optics

Mapping out the glassy landscape of a mesoscopic elastoplastic model

We develop a mesoscopic model to study the plastic behavior of an amorphous material under cyclic loading. The model is depinning-like and driven by a disordered thresholds dynamics which are coupled by long-range elastic interactions. We propose a simple protocol of "glass preparation" which allows us to mimic thermalisation at high temperature, as well as aging at vanishing temperature. Various levels of glass stabilities (from brittle to ductile) can be achieved by tuning the aging duration. The aged glasses are then immersed into a quenched disorder landscape and serve as initial configurations for various protocols of mechanical loading by shearing. The dependence of the plastic behavior upon monotonous loading is recovered. The behavior under cyclic loading is studied for different ages and system sizes. The size and age dependence of the irreversibility transition is discussed. A thorough characterization of the disorder-landscape is achieved through the analysis of the transition graphs, which describe the plastic deformation pathways under athermal quasi-static shear. In particular, the analysis of the stability ranges of the strongly connected components of the transition graphs reveals the emergence of a phase-separation like process associated with the aging of the glass. Increasing the age and hence stability of the initial glass, results in a gradual break-up of the landscape of dynamically accessible stable states into three distinct regions: one region centered around the initially prepared glass phase, and two additional regions, characterized by well-separated ranges of positive and negative plastic strains, each of which is accessible only from the initial glass phase by passing through the stress peak in the forward, respectively, backward shearing directions.

cond-mat.soft

Mechanical excitation and marginal triggering during avalanches in sheared amorphous solids

We study plastic strain during individual avalanches in overdamped particle-scale molecular dynamics (MD) and meso-scale elasto-plastic models (EPM) for amorphous solids sheared in the athermal quasi-static limit. We show that the spatial correlations in plastic activity exhibit a short lengthscale that grows as $t^{3/4}$ in MD and ballistically in EPM, and is generated by mechanical excitation of nearby sites not necessarily close to their stability thresholds, and a longer lengthscale that grows diffusively for both models and is associated with remote marginally stable sites. These similarities in spatial correlations explain why simple EPMs accurately capture the size distribution of avalanches observed in MD, though the temporal profiles and dynamical critical exponents are quite different.

cond-mat.soft

Origin of the Bauschinger Effect in Amorphous Solids

We study the structural origin of the Bauschinger effect by accessing numerically the local plastic thresholds in the steady state flow of a two-dimensional model glass under athermal quasistatic deformation. More specifically, we compute the local residual strength, $Δτ^{c}$, for arbitrary loading orientations and find that plastic deformation generically induces material polarization, i.e., a forward-backward asymmetry in the $Δτ^{c}$ distribution. In steady plastic flow, local packings are on average closer to forward (rather than backward) instabilities, due to the stress-induced bias of barriers. However, presumably due to mechanical noise, a significant fraction of zones lie close to reverse (backward) yielding, as the distribution of $Δτ^{c}$ for reverse shearing extends quasilinearly down to zero local residual strength. By constructing an elementary model of the early plastic response, we then show that unloading causes reverse plasticity of a growing amplitude, i.e., reverse softening, while it shifts away forward-yielding barriers. This result in an inversion of polarization in the low-$Δτ^{c}$ region and, consequently, in the Bauschinger effect. This scenario is quite generic, which explains the pervasiveness of the effect.

cond-mat.mtrl-sci

Rejuvenation and Shear-Banding in model amorphous solids

We measure the local yield stress, at the scale of small atomic regions, in a deeply quenched two-dimensional glass model undergoing shear banding in response to athermal quasistatic (AQS) deformation. We find that the occurrence of essentially a single plastic event suffices to bring the local yield stress distribution to a well-defined value for all strain orientations, thus essentially erasing the memory of the initial structure. It follows that in a well-relaxed sample, plastic events cause the abrupt (nucleation-like) emergence of a local softness contrast and thus precipitate the formation of a band, which, in its early stages, is measurably softer than the steady-state flow. Moreover, this postevent yield stress ensemble presents a mean value comparable to that of the inherent states of a supercooled liquid around the mode-coupling temperature $T_{\rm MCT}$. This, we argue, explains that the transition between brittle and ductile yielding in amorphous materials occurs around a comparable parent temperature. Our data also permit to capture quantitatively the contributions of pressure and density changes and demonstrate unambiguously that they are negligible compared with the changes of softness caused by structural rejuvenation.

cond-mat.mtrl-sci

Avalanches, thresholds, and diffusion in meso-scale amorphous plasticity

We present results on a meso-scale model for amorphous matter in athermal, quasi-static (a-AQS), steady state shear flow. In particular, we perform a careful analysis of the scaling with the lateral system size, $L$, of: i) statistics of individual relaxation events in terms of stress relaxation, $S$, and individual event mean-squared displacement, $M$, and the subsequent load increments, $Δγ$, required to initiate the next event; ii) static properties of the system encoded by $x=σ_y-σ$, the distance of local stress values from threshold; and iii) long-time correlations and the emergence of diffusive behavior. For the event statistics, we find that the distribution of $S$ is similar to, but distinct from, the distribution of $M$. We find a strong correlation between $S$ and $M$ for any particular event, with $S\sim M^{q}$ with $q\approx 0.65$. $q$ completely determines the scaling exponents for $P(M)$ given those for $P(S)$. For the distribution of local thresholds, we find $P(x)$ is analytic at $x=0$, and has a value $\left. P(x)\right|_{x=0}=p_0$ which scales with lateral system length as $p_0\sim L^{-0.6}$. Extreme value statistics arguments lead to a scaling relation between the exponents governing $P(x)$ and those governing $P(S)$. Finally, we study the long-time correlations via single-particle tracer statistics. The value of the diffusion coefficient is completely determined by $\langle Δγ\rangle$ and the scaling properties of $P(M)$ (in particular from $\langle M \rangle$) rather than directly from $P(S)$ as one might have naively guessed. Our results: i) further define the a-AQS universality class, ii) clarify the relation between avalanches of stress relaxation and diffusive behavior, iii) clarify the relation between local threshold distributions and event statistics.

cond-mat.soft

Chain level insights into tensile-compressive asymmetry in glassy and semicrystalline polymers

Using molecular dynamics simulations, we provide chain-level insights into the dissimilarities in rearrangements of polymers under uniaxial tensile and compressive deformation in glassy and semicrystalline samples of varying chain lengths. The organization of polymers under tension and compression is distinctively different. The chains align themselves along the tensile axis leading to a net global nematic ordering of their bonds and end-to-end vectors whereas under compression, the polymers arrange themselves in a plane perpendicular to the compressive axis resulting in emergence of an anti-nematic ordering of the bonds and the chain end-to-end vectors. Moreover, the degree of polymers unfolding is greater under tension and they deform less affinely when compared to chains under compression. The difference between the two responses strongly depends on the chain length and is the largest at intermediate chain lengths.

cond-mat.soft

Diffusion in mesoscopic lattice models of amorphous plasticity

We present results on tagged particle diffusion in a meso-scale lattice model for sheared amorphous material in athermal quasi-static conditions. We find a short time diffusive regime and a long time diffusive regime whose diffusion coefficients depend on system size in dramatically different ways. At short time, we find that the diffusion coefficient, $D$, scales roughly linearly with system length, $D\sim L^{1.05}$. This short time behavior is consistent with particle-based simulations. The long-time diffusion coefficient scales like $D\sim L^{1.6}$, close to previous studies which found $D\sim L^{1.5}$. Furthermore, we show that the near-field details of the interaction kernel do not affect the short time behavior, but qualitatively and dramatically affect the long time behavior, potentially causing a saturation of the mean-squared displacement at long times. Our finding of a $D\sim L^{1.05}$ short time scaling resolves a long standing puzzle about the disagreement between the diffusion coefficient measured in particle-based models and meso-scale lattice models of amorphous plasticity.

cond-mat.soft

Local yield stress statistics in model amorphous solids

We develop and extend a method presented in [S. Patinet, D. Vandembroucq, and M. L. Falk, Phys. Rev. Lett., 117, 045501 (2016)] to compute the local yield stresses at the atomic scale in model two-dimensional Lennard-Jones glasses produced via differing quench protocols. This technique allows us to sample the plastic rearrangements in a non-perturbative manner for different loading directions on a well-controlled length scale. Plastic activity upon shearing correlates strongly with the locations of low yield stresses in the quenched states. This correlation is higher in more structurally relaxed systems. The distribution of local yield stresses is also shown to strongly depend on the quench protocol: the more relaxed the glass, the higher the local plastic thresholds. Analysis of the magnitude of local plastic relaxations reveals that stress drops follow exponential distributions, justifying the hypothesis of an average characteristic amplitude often conjectured in mesoscopic or continuum models. The amplitude of the local plastic rearrangements increases on average with the yield stress, regardless of the system preparation. The local yield stress varies with the shear orientation tested and strongly correlates with the plastic rearrangement locations when the system is sheared correspondingly. It is thus argued that plastic rearrangements are the consequence of shear transformation zones encoded in the glass structure that possess weak slip planes along different orientations. Finally, we justify the length scale employed in this work and extract the yield threshold statistics as a function of the size of the probing zones. This method makes it possible to derive physically grounded models of plasticity for amorphous materials by directly revealing the relevant details of the shear transformation zones that mediate this process.

cond-mat.soft

Bending transition in the penetration of a flexible intruder in a 2D dense granular medium

We study the quasi-static penetration of a flexible beam in a two-dimensional dense granular medium lying on an horizontal plate. Rather than a buckling-like behavior we observe a transition between a regime of crack-like penetration in which the fiber only shows small fluctuations around a stable straight geometry and a bending regime in which the fiber fully bends and advances through series of loading/unloading steps. We show that the shape reconfiguration of the fiber is controlled by a single non dimensional parameter: L/Lc, the ratio of the length of the flexible beam L to Lc, a bending elasto-granular length scale that depends on the rigidity of the fiber and on the departure from the jamming packing fraction of the granular medium. We show moreover that the dynamics of the bending transition in the course of the penetration experiment is gradual and is accompanied by a symmetry breaking of the granular packing fraction in the vicinity of the fiber. Together with the progressive bending of the fiber, a cavity grows downstream of the fiber and the accumulation of grains upstream of the fiber leads to the development of a jammed cluster of grains. We discuss our experimental results in the framework of a simple model of bending-induced compaction and we show that the rate of the bending transition only depends on the control parameter L/Lc.

cond-mat.soft