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Dan M. Stamper-Kurn

Publications and source records attributed to Dan M. Stamper-Kurn.

At least 19 recordsLinked to original sources

Narrow-line magneto-optical trap of titanium atoms

We realize narrow-linewidth magneto-optical traps of $^{46}$Ti, $^{48}$Ti and $^{50}$Ti atoms based on a 1040 nm-wavelength transition, cooling atoms to a minimum temperature in one dimension of $T_z=990(20)$ nK and a three-dimensional temperature of $T_\mathrm{3D}=1.28(7)$ $μ$K. Atoms are pre-cooled in a broad-line magneto-optical trap and then transferred with about 25% efficiency to the narrow-line trap. We operate the narrow-line trap in two stages over 85 ms. First, a single cooling beam, blue-detuned from the narrow-linewidth atomic resonance, optically pumps and traps the atoms on a two-dimensional surface where the Zeeman shift from the applied spherical quadrupole magnetic field brings the light nearly to resonance. Second, four additional beams, counter-propagating in the transverse directions, cool and compress the atoms in all dimensions. The high magnetic moment of the laser cooling state makes the dynamics of the narrow-line titanium trap similar to those of other magnetic atoms. We measure the lifetime of the excited state of the transition to be $τ=8.2(9)$ $μ$s, indicating a transition linewidth of $γ/2π=20(2)$ kHz, and also measure isotope shifts on the narrow-line transition. We use Stern-Gerlach separation on the ultracold Ti gas to measure the $m_J$-distribution in the narrow-line magneto-optical trap, finding over 98% of the atoms in the stretched spin state.

physics.atom-ph↗

Rapid Cavity-Based Mid-Circuit Measurement and Feedforward in a Neutral Atom Array

Measuring part of a quantum system in the midst of its evolution and acting on the result in real time is essential for numerous quantum information protocols. Neutral-atom arrays are a leading platform for quantum information processing, but their mid-circuit measurement-and-feedforward cycle times have remained slow, typically exceeding 1 ms. Here we demonstrate fast mid-circuit measurement and real-time feedforward in an array of atomic qubits coupled to a high-finesse optical cavity. Local light shifts tune individual data qubits out of resonance with the cavity, shielding their coherence, while a near-resonant probe drives a selected qubit whose emission is collected with Purcell enhancement. Mid-circuit measurements of four qubits with sub percent infidelity reduce the coherence of a fifth unmeasured data qubit by less than 2%. We implement real-time feedforward to correct measurement-induced phase shifts and to realize an adaptive circuit for optimal quantum state discrimination and conditional state preparation. Our approach reduces the measurement-and-feedforward cycle time to below 100 $μ$s and establishes optical cavities as a route to fast control of neutral-atom quantum systems.

quant-ph↗

Interband Berry connection measurement in the optical honeycomb lattice

The geometry of Bloch bands affects many physical properties of crystalline solids and other spatially periodic systems. Direct experimental determination of such geometry is an active area of research. In this work, we focus on the fundamental connection between optical excitations and the relative geometry of pairs of Bloch bands, as characterized by the interband Berry connection. We simulate the response of electrons in solids to optical excitation by the response of ultracold fermionic atoms in optical lattices to periodic modulation of the lattice position. The strength of resonant excitation between bands, measured at each quasimomentum and for various lattice-shaking polarizations, directly maps out the interband Berry connection. We apply this method to the optical honeycomb lattice, driving excitations between the ground $n=1$ band and the excited $n'=\{2,3,4\}$ bands. We observe transparency lines of quasimomenta at which the response to excitation of specific polarization is zero. Further, the interband Berry connection between bands 1 and 3 shows irreducible Dirac strings connecting the $K$ and $K'$ points in the Brillouin zone, lines along which the interband Berry connection abruptly changes orientation. Our work establishes optical response as a powerful tool for characterizing geometrical and topological properties of band structure.

cond-mat.quant-gas↗

$\mathrm{^{130}Te_2}$ spectroscopic reference for neutral Ti lines at 391 nm and 498 nm

We report on the use of ditellurium ($\mathrm{^{130}Te_2}$) as a frequency reference for laser locking at 391 nm and 498 nm optical wavelengths, which are of interest in titanium (Ti) laser-cooling experiments. In the ultraviolet region near the optical wavelength of 391 nm, 36 previously unobserved transitions were found using laser absorption spectroscopy in a 256 GHz range. Based on the established molecular structure of $\mathrm{^{130}Te_2}$, we attribute these lines to the $\mathrm{0_u^+\rightarrow 0_g^+}$ subsystem of the $\mathrm{^3Σ_u^-\rightarrow\ ^3Σ_g^-}$ transition with possible vibrational transitions of $ν=(28,27,26,25,24)\rightarrow 0$ and $(27,26)\rightarrow 1$. We measure the frequencies of these lines, and also of lines near 498 nm wavelength, and subsequently stabilize lasers at wavelengths of 391 nm (and 498 nm) to $\sim$60 MHz ($\sim$50 MHz) wide resonances in $\mathrm{^{130}Te_2}$, near the optical-pumping (laser-cooling) transitions in $\mathrm{^{48}Ti}$. We observe robust laser frequency locks, with Allan deviations of $4.9\times 10^{-10}$ ($3.6\times 10^{-11}$) at 10 s of averaging time for the 391 nm (498 nm) wavelength lasers.

physics.atom-ph↗

Astigmatism-free 3D Optical Tweezer Control for Rapid Atom Rearrangement

Reconfigurable neutral-atom arrays are a promising platform for quantum computing, quantum simulation, and quantum metrology, but atom transport using frequency-chirped acousto-optic deflectors (AODs) is limited by chirp-induced acoustic lensing and trajectory distortion. We address these limitations using a three-dimensional acousto-optic deflector lens (3D-AODL), a design predicted to reduce long-range transport times by more than a factor of two. We further introduce fading-Shepard waveforms that circumvent finite AOD bandwidth, enabling sustained axial displacement. We demonstrate unrestricted three-dimensional optical-tweezer motion over a 200 $μ$m $\times$ 200 $μ$m $\times$ 136 $μ$m volume with velocities exceeding 4.2 m/s. Arbitrary three-dimensional control of optical-tweezer trajectories enables rapid atom rearrangement and dynamical engineering of optical potentials in tweezer arrays and optical lattices. This capability advances quantum control and atom manipulation in neutral-atom quantum processors by enabling faster rearrangement, higher clock rates, and scalable sorting in complex geometries.

physics.optics↗

Higher symmetry breaking and non-reciprocity in a driven-dissipative Dicke model

Higher symmetries in interacting many-body systems often give rise to new phases and unexpected dynamical behavior. Here, we theoretically investigate a variant of the Dicke model with higher-order discrete symmetry, resulting from complex-valued coupling coefficients between quantum emitters and a bosonic mode. We propose a driven-dissipative realization of this model focusing on optomechanical response of a driven atom tweezer array comprised of $n$ sub-ensembles and placed within an optical cavity, with the phase of the driving field advancing stepwise between sub-ensembles. Examining stationary points and their dynamical stability, we identify a phase diagram for $n\geq 3$ with three distinctive features: a $\mathbb{Z}_n$ ($\mathbb{Z}_{2n}$) symmetry-breaking superradiant phase for even (odd) $n$, a normal unbroken-symmetry phase that is dynamically unstable due to non-reciprocal forces between emitters, and a first-order phase transition separating these phases. This $n$-phase Dicke model may be equivalently realized in a variety of optomechanical or opto-magnonic settings, where it can serve as a testbed for studying high-order symmetry breaking and non-reciprocal interactions in open systems.

quant-ph↗

Hyperfine spectroscopy and laser cooling of the fermionic isotopes $^{47}$Ti and $^{49}$Ti

We report on magneto-optical trapping of the two fermionic isotopes of atomic titanium, $^{47}$Ti and $^{49}$Ti. Unlike the even mass-number isotopes, which were recently laser cooled, $^{47}$Ti and $^{49}$Ti have nonzero nuclear spins and, consequently, their atomic levels are split by hyperfine structure. Combining and comparing theoretical calculations and atomic beam-spectroscopy measurements, we determine the hyperfine structures and isotope shifts of the $\mathrm{3d^24s^2}$ $\mathrm{a^3F_4\rightarrow 3d^2(^3P)4s4p(^3P^o)}$ $\mathrm{y^5D_4^o}$ optical-pumping transition at optical wavelength 391nm and the $\mathrm{3d^3(^4F)4s}$ $\mathrm{a^5F_5\rightarrow 3d^3(^4F)4p}$ $\mathrm{y^5G_6^o}$ laser-cooling transition at wavelength 498nm. With this information, we produce magneto-optical traps of both $^{47}$Ti and $^{49}$Ti by applying two additional tones of light to repump atoms to the maximum-spin states on the laser-cooling transition. Directly loading from the atomic flux of a titanium sublimation pump, we produce $^{47}$Ti and $^{49}$Ti traps with 731(190) and 1142(240) atoms, and with lifetimes of 330(15)ms and 310(8)ms, respectively.

physics.atom-ph↗

Autler-Townes spectroscopy of a Rydberg ladder

Ladder-type two-photon excitation of an atom from a ground state $|g\rangle$, to an intermediate excited state $|e\rangle$, and, finally, to a Rydberg state $|r\rangle$, has a variety of uses from quantum information to sensing. A common scheme for detecting this transition optically is through electromagnetically induced transparency (EIT). However, in inverted wavelength schemes, where the ground-to-excited transition wavelength is shorter than the excited-to-Rydberg transition wavelength, the strength of the EIT feature on the lower-leg beam is strongly reduced in a Doppler-broadened medium. Here, we report on an alternative two-photon spectroscopic feature, which we term the two-photon Autler-Townes resonance, observed on the upper-leg beam. Compared to the EIT signal, this feature's superior signal-to-noise ratio allows one to resolve Rydberg resonances with principal quantum number as high as $n=80$. We also show that such a feature can be utilized to generate an error signal for stabilizing the frequency of the upper-leg beam.

quant-ph↗

Optomechanical self-organization in a mesoscopic atom array

Increasing the number of particles in a system often leads to qualitative changes in its properties, such as breaking of symmetries and the appearance of phase transitions. This renders a macroscopic system fundamentally different from its individual microscopic constituents. Lying between these extremes, mesoscopic systems exhibit microscopic fluctuations that influence behavior on longer length scales, leading to critical phenomena and dynamics. Therefore, tracing the properties of well-controlled mesoscopic systems can help bridge the gap between an exact description of few-body microscopic systems and the emergent description of many-body systems. Here, we explore mesoscopic signatures of an optomechanical self-organization phase transition using arrays of cold atoms inside an optical cavity. By precisely engineering atom-cavity interactions, we reveal how critical behavior depends on atom number, identify characteristic dynamical behaviors in the self-organized regime, and observe a finite optomechanical susceptibility at the critical point. These findings advance our understanding of particle-number- and time-resolved properties of phase transitions in mesoscopic systems.

quant-ph↗

Ground-state selection via many-body superradiant decay

For a single particle, relaxation into different ground states is governed by fixed branching ratios determined by the transition matrix element and the environment. Here, we show that in many-body open quantum systems the occupation probability of one ground state can be boosted well beyond what is dictated by single-particle branching ratios. Despite the competition, interactions suppress all but the dominant decay transition, leading to a 'winner takes all' dynamic where the system primarily settles into the dominant ground state. We prove that, in the presence of permutation symmetry, this problem is exactly solvable for any number of competing channels. Additionally, we develop an approximate model for the dynamics by mapping the evolution onto a fluid continuity equation, and analytically demonstrate that the dominant transition ratio converges to unity as a power law with increasing system size, for any branching ratios. This near-deterministic preparation of the dominant ground state has broad applicability. As an example, we discuss a protocol for molecular photoassociation where collective dynamics effectively acts as a catalyst, amplifying the yield in a specific final state. Our results open new avenues for many-body strategies in the preparation and control of quantum systems.

quant-ph↗

A Magneto-Optical Trap of Titanium Atoms

We realize laser cooling and trapping of titanium (Ti) atoms in a mangeto-optical trap (MOT). While Ti does not possess a transition suitable for laser cooling out of its $\mathrm{3d^24s^2}$ $\mathrm{a^3F}$ ground term, there is such a transition, at an optical wavelength of $λ=498\mathrm{nm}$, from the long-lived $\mathrm{3d^3(^4F)4s}$ $\mathrm{a^5F_5}$ metastable state to the $\mathrm{3d^3(^4F)4p}$ $\mathrm{y^5G^o_6}$ excited state. Without the addition of any repumping light, we observe MOTs of metastable $\mathrm{^{46}Ti}$, $\mathrm{^{48}Ti}$, and $\mathrm{^{50}Ti}$, the three stable nuclear-spin-zero bosonic isotopes of Ti. While MOTs can be observed when loaded directly from our Ti sublimation source, optical pumping of ground term atoms to the $\mathrm{a^5F_5}$ state increases the loading rate by a factor of 120, and the steady-state MOT atom number by a factor of 30. At steady state, the MOT of $\mathrm{^{48}Ti}$ holds up to $8.30(26)\times10^5$ atoms at a maximum density of $1.3(4)\times10^{11}\mathrm{cm}^{-3}$ and at a temperature of $90(15)\mathrm{μK}$. By measuring the decay of the MOT upon suddenly reducing the loading rate, we place upper bounds on the leakage branching ratio of the cooling transition $(\leq2.5\times 10^{-6})$ and the two-body loss coefficient $(\leq2\times10^{-10}\mathrm{cm}^3\mathrm{s}^{-1})$. Our approach to laser cooling Ti can be applied to other transition metals, enabling a significant expansion of the elements that can be laser cooled.

physics.atom-ph↗

State-insensitive wavelengths for light shifts and photon scattering from Zeeman states

Atoms are not two-level systems, and their rich internal structure often leads to complex phenomena in the presence of light. Here, we analyze off-resonant light scattering including the full hyperfine and magnetic structure. We find a set of frequency detunings where the induced atomic dipole is the same irrespective of the Zeeman state, and where two-photon transitions that alter the atomic state turn off. For alkali atoms and alkaline-earth ions, if the hyperfine splitting is dominated by the magnetic dipole moment contribution, these detunings approximately coincide. Therefore, at a given ``magical'' detuning, all Zeeman states in a hyperfine manifold behave almost identically, and can be traced out to good approximation. This feature prevents state decoherence due to light scattering, which impacts quantum optics experiments and quantum information applications.

quant-ph↗

Super-radiant and Sub-radiant Cavity Scattering by Atom Arrays

We realize collective enhancement and suppression of light scattered by an array of tweezer-trapped $^{87}$Rb atoms positioned within a strongly coupled Fabry-Pérot optical cavity. We illuminate the array with light directed transverse to the cavity axis, in the low saturation regime, and detect photons scattered into the cavity. For an array with integer-optical-wavelength spacing each atom scatters light into the cavity with nearly identical scattering amplitude, leading to an observed $N^2$ scaling of cavity photon number as the atom number increases stepwise from $N=1$ to $N=8$. By contrast, for an array with half-integer-wavelength spacing, destructive interference of scattering amplitudes yields a non-monotonic, sub-radiant cavity intensity versus $N$. By analyzing the polarization of light emitted from the cavity, we find that Rayleigh scattering can be collectively enhanced or suppressed with respect to Raman scattering. We observe also that atom-induced shifts and broadenings of the cavity resonance are precisely tuned by varying the atom number and positions. Altogether, tweezer arrays provide exquisite control of atomic cavity QED spanning from the single- to the many-body regime.

quant-ph↗

Autonomous feedback stabilization of a cavity-coupled spin oscillator

We report out-of-equilibrium stabilization of the collective spin of an atomic ensemble through autonomous feedback by a driven optical cavity. For a magnetic field applied at an angle to the cavity axis, dispersive coupling to the cavity provides sensitivity to a combination of the longitudinal and transverse spin. Coherent backaction by cavity light onto the atoms, conditioned by the optical cavity susceptibility, stabilizes the collective spin state at an arbitrary energy. The set point tracking and closed-loop gain spectrum of the feedback system are characterized and found to agree closely with analytic predictions.

physics.atom-ph↗

Optical Telecommunications-Band Clock based on Neutral Titanium Atoms

We propose an optical clock based on narrow, spin-forbidden M1 and E2 transitions in laser-cooled neutral titanium. These transitions exhibit much smaller black body radiation shifts than those in alkaline earth atoms, small quadratic Zeeman shifts, and have wavelengths in the S, C, and L-bands of fiber-optic telecommunication standards, allowing for integration with robust laser technology. We calculate lifetimes; transition matrix elements; dynamic scalar, vector, and tensor polarizabilities; and black body radiation shifts of the clock transitions using a high-precision relativistic hybrid method that combines a configuration interaction and coupled cluster approaches. We also calculate the line strengths and branching ratios of the transitions used for laser cooling. To identify magic trapping wavelengths, we have completed the largest-to-date direct dynamical polarizability calculations. Finally, we identify new challenges that arise in precision measurements due to magnetic dipole-dipole interactions and describe an approach to overcome them. Direct access to a telecommunications-band atomic frequency standard will aid the deployment of optical clock networks and clock comparisons over long distances.

physics.atom-ph↗

Mid-circuit cavity measurement in a neutral atom array

Subsystem readout during a quantum process, or mid-circuit measurement, is crucial for error correction in quantum computation, simulation, and metrology. Ideal mid-circuit measurement should be faster than the decoherence of the system, high-fidelity, and nondestructive to the unmeasured qubits. Here, we use a strongly coupled optical cavity to read out the state of a single tweezer-trapped 87Rb atom within a small tweezer array. Measuring either atomic fluorescence or the transmission of light through the cavity, we detect both the presence and the state of an atom in the tweezer, within only tens of microseconds, with state preparation and measurement infidelities of roughly 0.5% and atom loss probabilities of around 1%. Using a two-tweezer system, we find measurement on one atom within the cavity causes no observable hyperfine-state decoherence on a second atom located tens of microns from the cavity volume. This high-fidelity mid-circuit readout method is a substantial step towards quantum error correction in neutral atom arrays.

quant-ph↗

Superresolution microscopy of optical fields using tweezer-trapped single atoms

We realize a scanning probe microscope using single trapped $^{87}$Rb atoms to measure optical fields with subwavelength spatial resolution. Our microscope operates by detecting fluorescence from a single atom driven by near-resonant light and determining the ac Stark shift of an atomic transition from other local optical fields via the change in the fluorescence rate. We benchmark the microscope by measuring two standing-wave Gaussian modes of a Fabry-Pérot resonator with optical wavelengths of 1560 nm and 781 nm. We attain a spatial resolution of 300 nm, which is superresolving compared to the limit set by the 780 nm wavelength of the detected light. Sensitivity to short length scale features is enhanced by adapting the sensor to characterize an optical field via the force it exerts on the atom.

physics.atom-ph↗

Tracking evaporative cooling of a mesoscopic atomic quantum gas in real time

The fluctuations in thermodynamic and transport properties in many-body systems gain importance as the number of constituent particles is reduced. Ultracold atomic gases provide a clean setting for the study of mesoscopic systems; however, the detection of temporal fluctuations is hindered by the typically destructive detection, precluding repeated precise measurements on the same sample. Here, we overcome this hindrance by utilizing the enhanced light--matter coupling in an optical cavity to perform a minimally invasive continuous measurement and track the time evolution of the atom number in a quasi two-dimensional atomic gas during evaporation from a tilted trapping potential. We demonstrate sufficient measurement precision to detect atom number fluctuations well below the level set by Poissonian statistics. Furthermore, we characterize the non-linearity of the evaporation process and the inherent fluctuations of the transport of atoms out of the trapping volume through two-time correlations of the atom number. Our results establish coupled atom--cavity systems as a novel testbed for observing thermodynamics and transport phenomena in mesosopic cold atomic gases and, generally, pave the way for measuring multi-time correlation functions of ultracold quantum gases.

cond-mat.quant-gas↗