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Dang-Khoa D. Le

Publications and source records attributed to Dang-Khoa D. Le.

3 recordsLinked to original sources

A Direct Algebraic Approach to Normal Ordering of Exponential Bosonic Operators with Applications to Two-Dimensional Excitonic Form Factors

We develop a systematic algebraic approach, based on the Wei--Norman factorization method, to the normal ordering of exponential bosonic operators and apply it to derive analytical excitonic form factors in two-dimensional semiconducting materials. By introducing an auxiliary parameter, the normal-ordering problem is reduced to a system of ordinary differential equations determined by the commutation relations of the underlying closed Lie algebra. The approach is first illustrated for exponential operators associated with the Heisenberg--Weyl and $su(1,1)$ algebras, and is then extended to two-mode bosonic operators involving $su(2)$ and a six-generator closed algebra that contains two coupled $su(1,1)$ subalgebras. For the excitonic application, the Levi--Civita transformation maps the two-dimensional exciton problem onto an oscillator representation, providing a natural formulation in terms of bosonic creation and annihilation operators. Combined with the Laplace and Fourier representations of the Rytova--Keldysh potential, this formulation reduces the interaction matrix elements to the evaluation of exponential bosonic form factors. The isotropic problem is governed by a three-generator $su(1,1)$ algebra, whereas the anisotropic case requires the full six-generator algebra together with an additional $su(2)$ factorization. Explicit analytical expressions for both form factors, $\langle e^{-rt}\rangle$ and $\langle e^{i\mathbf q\cdot\mathbf r}\rangle$, are obtained, providing useful building blocks for matrix-element calculations in two-dimensional excitonic systems and potentially in other quantum problems involving exponential bosonic operators.

cond-mat.mtrl-sci↗

Anisotropic two-dimensional magnetoexciton with exact center-of-mass separation

Excitons in anisotropic two-dimensional (2D) materials, defined by direction-dependent effective masses, are of pronounced interest for their roles in excitonic and magneto-optical phenomena. A perpendicular magnetic field complicates the separation of center-of-mass (c.m.) and relative motions, especially when electron and hole masses are comparable. Conventional theories often employ an approximate c.m. separation using factorized wave functions, modifying magnetic Hamiltonian terms and possibly introducing inaccuracies in magnetoexciton energy predictions. This work develops an exact analytical framework for c.m. and relative motion separation in anisotropic 2D magnetoexcitons, without resorting to the stationary-c.m. approximation. Starting from the full electron-hole Hamiltonian in a homogeneous magnetic field, the formalism uses the conserved pseudomomentum to derive a relative-motion Hamiltonian, revealing new anisotropy-dependent couplings and magnetic coefficients absent in approximate models. The resulting Schrödinger equation is treated via the Feranchuk-Komarov operator method and Levi-Civita transformation, allowing non-perturbative, systematically convergent solutions. Application to monolayer black phosphorus and titanium trisulfide, both freestanding and encapsulated in hexagonal boron nitride, yields magnetoexciton energies, diamagnetic coefficients, and probability densities for the ten lowest states across considerable magnetic-field ranges. The results demonstrate the significant influence of anisotropy-dependent coupling on magnetic response in systems with strong mass anisotropy. This formalism is generalizable to other anisotropic 2D semiconductors, establishing a foundation for advanced magneto-optical studies.

cond-mat.mes-hall↗

Retrieval of fundamental material parameters of monolayer transition metal dichalcogenides from experimental exciton energies: An analytical approach

We propose a straightforward and highly accurate method for extracting material parameters such as screening length, bandgap energy, exciton reduced mass, and the dielectric constant of the surrounding medium from experimental magnetoexciton energies available for monolayer transition metal dichalcogenides (TMDCs). Our approach relies on analytical formulations that allow us to calculate the screening length $r_0$ and bandgap energy $E_g$ directly from the experimental $s$-state exciton energies $E_{1s}$, $E_{2s}$, and $E_{3s}$. We also establish a relationship between the surrounding dielectric constant $κ$ and the exciton reduced mass $μ$. This relationship simplifies the Schr{ö}dinger equation for a magnetoexciton in a TMDC monolayer, transforming it into a one-parameter equation that depends solely on the single material parameter $μ$. Furthermore, we develop an analytical formula with high accuracy for magnetoexciton energies as a function of the exciton reduced mass: $E(B,μ)$. Then, the inverse of this formula allows us to calculate the exciton reduced mass from experimental data on magnetoexciton energies. By applying this method, we extract key material parameters, $E_g$, $r_0$, $μ$, and $κ$, from the magnetoexciton energies of monolayer TMDCs, including WSe$_2$, WS$_2$, MoSe$_2$, and MoS$_2$, encapsulated by hexagonal boron nitride (hBN) slabs in various current experiments. The material properties we retrieve complement and correct existing experimental and theoretical data. Additionally, we develop an analytical method for calculating diamagnetic coefficients and exciton radii with high accuracy compared to numerical calculations. Based on this method, we provide diamagnetic coefficients and exciton radii computed using the extracted material parameters.

cond-mat.mes-hall↗