arXiv subjects

Danica Pavicevic

Publications and source records attributed to Danica Pavicevic.

4 recordsLinked to original sources

arXiv2025

Gap Inhomogeneity in Cuprates: a view from Two-Dimensional Josephson Echo Spectroscopy

Novel theoretical developments have allowed to connect microscopic disorder in bosonic collective excitations to the signatures in two-dimensional terahertz spectroscopy (Gómez Salvador et al. 2025). Here, we employ this framework to analyze the recently measured Josepshon echoes in optimally doped La$_{2-x}$Sr$_x$CuO$_4$ (Liu et al. 2024). We consider the spatial gap inhomogeneities -- observed in scanning tunneling microscopy -- as input for the disorder in the superfluid density, and compute the resulting echo peaks. The excellent agreement supports the interpretation that the gap inhomogeneity arises solely from pairing gap fluctuations, with no evidence for non-superconducting competing local orders. Finally, we study the microscopic origin of the inelastic processes, contributing to the damping of the Josephson plasmon at low temperatures, and conclude that it can be attributed to nodal quasiparticles.

cond-mat.supr-con↗

arXiv2025

Two-dimensional spectroscopy of bosonic collective excitations in disordered many-body systems

We present a novel theoretical approach for computing and analyzing two-dimensional spectroscopy of bosonic collective excitations in disordered many-body systems. Specifically, we employ the Keldysh formalism to derive, within a non-pertubative treatment of disorder effects, the third-order nonlinear response and obtain two-dimensional spectroscopy maps. In the weak nonlinear regime of our formalism, we demonstrate the ability of the echo peak to distinguish between elastic and inelastic scattering processes, in perfect agreement with the intuition developed in isolated two-level systems. Furthermore, we discuss unique many-body effects on the echo peak signature arising from interaction induced quantum fluctuations. In particular, we show that these quantum fluctuations induce a finite nonrephasable broadening and examine how the echo peak is influenced by the attractive or repulsive nature of the collective excitations.

cond-mat.str-el↗

arXiv2024

Principles of 2D terahertz spectroscopy of collective excitations: the case of Josephson plasmons in layered superconductors

Two-dimensional terahertz spectroscopy (2DTS), a terahertz analogue of nuclear magnetic resonance, is a new technique poised to address many open questions in complex condensed matter systems. The conventional theoretical framework used ubiquitously for interpreting multidimensional spectra of discrete quantum level systems is, however, insufficient for the continua of collective excitations in strongly correlated materials. Here, we develop a theory for 2DTS of a model collective excitation, the Josephson plasma resonance in layered superconductors. Starting from a mean-field approach at temperatures well below the superconducting phase transition, we obtain expressions for the multidimensional nonlinear responses that are amenable to intuition derived from the conventional single-mode scenario. We then consider temperatures near the superconducting critical temperature $T_c$, where dynamics beyond mean-field become important and conventional intuition fails. As fluctuations proliferate near $T_c$, the dominant contribution to nonlinear response comes from an optical parametric drive of counter-propagating Josephson plasmons, which gives rise to 2D spectra that are qualitatively different from the mean-field predictions. As such, and in contrast to one-dimensional spectroscopy techniques, such as third harmonic generation, 2DTS can be used to directly probe thermally excited finite-momentum plasmons and their interactions. Our theory provides a clear interpretation of recent 2DTS measurements on cuprates, and we discuss implications beyond the present context of Josephson plasmons.

cond-mat.supr-con↗

arXiv2023

Probing Inhomogeneous Cuprate Superconductivity by Terahertz Josephson Echo Spectroscopy

Inhomogeneities play a crucial role in determining the properties of quantum materials. Yet methods that can measure these inhomogeneities are few, and apply to only a fraction of the relevant microscopic phenomena. For example, the electronic properties of cuprate materials are known to be inhomogeneous over nanometer length scales, although questions remain about how such disorder influences supercurrents and their dynamics. Here, two-dimensional terahertz spectroscopy is used to study interlayer superconducting tunneling in near-optimally-doped La1.83Sr0.17CuO4. We isolate a 2 THz Josephson echo signal with which we disentangle intrinsic lifetime broadening from extrinsic inhomogeneous broadening. We find that the Josephson plasmons are only weakly inhomogeneously broadened, with an inhomogeneous linewidth that is three times smaller than their intrinsic lifetime broadening. This extrinsic broadening remains constant up to 0.7Tc, above which it is overcome by the thermally-increased lifetime broadening. Crucially, the effects of disorder on the Josephson plasma resonance are nearly two orders of magnitude smaller than the in-plane variations in the superconducting gap in this compound, which have been previously documented using Scanning Tunnelling Microscopy (STM) measurements. Hence, even in the presence of significant disorder in the superfluid density, the finite frequency interlayer charge fluctuations exhibit dramatically reduced inhomogeneous broadening. We present a model that relates disorder in the superfluid density to the observed lifetimes.

cond-mat.supr-con↗