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Daniel A. Bustamante Lopez

Publications and source records attributed to Daniel A. Bustamante Lopez.

7 recordsLinked to original sources

Phonon angular momentum transfer torque

Angular momentum in solids is carried by (quasi)particles such as magnons, plasmons, and phonons, and coupling between these reservoirs enables diverse hybrid phenomena. Here, we introduce the transfer of angular momentum from lattice vibrations to magnetic order through the phonon angular momentum transfer torque (PAMTT), generated by a polarized phonon bath. We identify thermal routes for generating phonon angular momentum: a phonon Edelstein accumulation in noncentrosymmetric crystals and temperature-gradient-induced PAM currents with longitudinal Seebeck-like and transverse Hall components. Using realistic order-of-magnitude estimates, we find that PAMTT could produce measurable ferromagnetic-resonance frequency shifts and, for favorable interfacial coupling, drive magnetization reversal on nanosecond timescales.

cond-mat.other↗

Precessional modes of phonon angular momentum

Magnons are collective precessional excitations of electron spins and are ubiquitous in emerging information technologies. Here, we show that the crystal lattice can support an analogous precessional mode of phonon angular momentum. Superposition of a circularly polarized phonon and a linearly polarized phonon normal to the circular-motion plane generates a transverse angular-momentum component that rotates at their difference frequency and decays on a timescale set by the participating phonon linewidths, defining a mode with its own resonance and lifetime. Coupling between spin and phonon angular momentum hybridizes this precessional mode with a magnon near resonance. Our results establish phonon angular momentum precessional modes as lattice analogues of magnons and identify their spectroscopic and time-domain signatures.

cond-mat.mtrl-sci↗

Ferron Hall effect: Transverse accumulation of polarization driven by thermal gradients in ferroelectrics

The phonon Hall effect describes the generation of a transverse heat current in response to a longitudinal thermal gradient in a magnetic field. Here, we theoretically demonstrate that, when the lattice excitations deflected by the Hall effect carry electric dipole moments, their transverse motion produces an accumulation of electric polarization in ferroelectric materials. This accumulation is driven by lattice excitations that carry polarization, known as ferrons, and we therefore call the mechanism the ferron Hall effect. Using atomistic lattice dynamics with parameters obtained from density functional theory, we illustrate the effect in the prototypical ferroelectric BaTiO3. Our results identify ferrons as the electric-polarization analogues of magnons in transverse transport and provide a route toward thermal and magnetic manipulation of ferroic order.

cond-mat.mtrl-sci↗

Atomistic theory of the phonon angular momentum Hall effect

The spin and orbital Hall effects convert longitudinal charge currents into transverse flows of electronic angular momentum. Here we develop an atomistic theory of the recently proposed lattice-vibrational analogue, in which a longitudinal heat current driven by a thermal gradient is converted into a transverse current of phonon angular momentum. We derive a microscopic real-space expression for this current and show that it originates from thermally induced mixing of polarized vibrational motion, leading to a characteristic edge accumulation of phonon angular momentum. We demonstrate the effect in minimal square- and honeycomb-lattice models and compute the resulting phonon angular momentum accumulations for a range of example materials using input from first-principles calculations. Our results confirm that the phonon angular momentum Hall effect is a universal response of crystalline solids and our framework is generically applicable to all materials.

cond-mat.mtrl-sci↗

Electro-phononic and magneto-phononic frequency conversion

Nonlinear frequency conversion by optical rectification, as well as difference- and sum-frequency generation are fundamental processes for producing electromagnetic radiation at different frequencies. Here, we demonstrate that coherently excited infrared-active phonons can be used as transducers for generating nonlinear electric polarizations and magnetizations via phonon-phonon and phonon-magnon interactions, in a way similar to nonlinear optical frequency conversion. We derive analytical solutions for the time-dependent polarizations and magnetizations for the second-order response to the electric field component of an ultrashort laser pulse. These allow us to define second-order nonlinear electric and magneto-electric susceptibilities that capture the rectification, as well as the impulsive and sum-frequency excitation of coherent phonons and magnons. Our theoretical framework naturally incorporates existing mechanisms and further leads to the prediction of a hybrid magneto-opto-phononic inverse Faraday effect involving photon-phonon-magnon scattering. Our work demonstrates nonlinear phononics as a pathway to controlling the electric polarization and magnetization in solids.

physics.optics↗

Ultrafast simultaneous manipulation of multiple ferroic orders through nonlinear phonon excitation

Recent experimental studies have demonstrated the possibility of utilizing strong terahertz pulses to manipulate individual ferroic orders on pico- and femtosecond timescales. Here, we extend these findings and showcase the simultaneous manipulation of multiple ferroic orders in BiFeO$_3$, a material that is both ferroelectric and antiferromagnetic at room temperature. We find a concurrent enhancement of ferroelectric and antiferromagnetic second-harmonic generation (SHG) following the resonant excitation of a high-frequency fully-symmetric phonon mode. Based on first-principles calculations and phenomenological modeling, we ascribe this observation to the inherent coupling of the two ferroic orders to the nonequilibrium distortions induced in the crystal lattice by nonlinearly driven phonons. Our finding highlights the potential of nonlinear phononics as a technique for manipulating multiple ferroic order parameters at once. In addition, this approach provides a promising avenue to studying the dynamical magnetization and polarization behavior, as well as their intrinsic coupling, on ultrashort timescales.

cond-mat.str-el↗

Light-induced weak ferromagnetism through nonlinear magnonic rectification

Rectification describes the generation of a quasistatic component from an oscillating field, such as an electric polarization in optical rectification, or a structural distortion in nonlinear phononic rectification. Here, we present a third fundamental process for magnetization, in which spin precession is rectified along the coordinates of a nonlinearly driven magnon mode in an antiferromagnet. We demonstrate theoretically that a quasistatic magnetization can be induced by transient spin canting in response to the coherent excitation of a chiral phonon mode that produces an effective magnetic field for the spins. This mechanism, which we call nonlinear magnonic rectification, is generally applicable to magnetic systems that exhibit infrared-active chiral phonon modes. Our results serve as an example of light-induced weak ferromagnetism and open a promising avenue towards creating dynamical spin configurations that are not accessible in equilibrium.

cond-mat.mtrl-sci↗