arXiv subjects

Daniel Bedau

Publications and source records attributed to Daniel Bedau.

18 recordsLinked to original sources

arXiv2026

Improved selector behavior in ultrathin chromium-doped V$_2$O$_3$ films

Devices based on the negative differential resistance effect in chromium doped V$_2$O$_3$ are considered to be promising as selector elements for use in emerging memory technologies, as well as for neuromorphic applications. It is shown by electrical measurements, that the switching effect is maintained for very thin films down to 5 nm, and even improved properties such as a low leakage current and an abrupt transition are observed. For these thicknesses, the behavior of crystalline and amorphous films becomes very similar; most strikingly, a forming step is required in both. Transmission electron microscopy reveals this to be likely due to a thin amorphous layer that forms at the interface to the TiN electrode. Elemental mapping further shows a complex distribution of the chromium dopants, as well as a diffusion of Ti into the layer from the electrode, which might be responsible for the improved properties.

cond-mat.str-el↗

arXiv2024

A Method for Fabricating CMOS Back-End-of-Line-Compatible Solid-State Nanopore Devices

Solid-state nanopores, nm-sized holes in thin, freestanding membranes, are powerful single-molecule sensors capable of interrogating a wide range of target analytes, from small molecules to large polymers. Interestingly, due to their high spatial resolution, nanopores can also identify tags on long polymers, making them an attractive option as the reading element for molecular information storage strategies. To fully leverage the compact and robust nature of solid-state nanopores, however, they will need to be packaged in a highly parallelized manner with on-chip electronic signal processing capabilities to rapidly and accurately handle the data generated. Additionally, the membrane itself must have specific physical, chemical, and electrical properties to ensure sufficient signal-to-noise ratios are achieved, with the traditional membrane material being SiNX . Unfortunately, the typical method of deposition, low-pressure vapour deposition, requires temperatures beyond the thermal budget of CMOS back-end-of-line integration processes, limiting the potential to generate an on-chip solution. To this end, we explore various lower-temperature deposition techniques that are BEOL-compatible to generate SiNx membranes for solid-state nanopore use, and successfully demonstrate the ability for these alternative methods to generate low-noise nanopores that are capable of performing single-molecule experiments.

physics.app-ph↗

arXiv2024

Electronic vs. phononic thermal transport in Cr-doped V2O3 thin films across the Mott transition

Understanding the thermal conductivity of chromium doped V2O3 is crucial for optimizing the design of selectors for memory and neuromorphic devices. We utilized the time-domain thermoreflectance technique to measure the thermal conductivity of chromium doped V2O3 across varying concentrations, spanning the doping induced metal-insulator transition. In addition, different oxygen stoichiometries and film thicknesses were investigated in their crystalline and amorphous phases. Chromium doping concentration (0%-30%) and the degree of crystallinity emerged as the predominant factors influencing the thermal properties, while the effect of oxygen flow (600-1400 ppm) during deposition proved to be negligible. Our observations indicate that even in the metallic phase of V2O3, the lattice contribution is the dominant factor in thermal transport with no observable impact from the electrons on heat transport. Finally, the thermal conductivity of both amorphous and crystalline V2O3 was measured at cryogenic temperatures (80-450 K). Our thermal conductivity measurements as a function of temperature reveal that both phases exhibit behavior similar to amorphous materials, indicating pronounced phonon scattering effects in the crystalline phase of V2O3.

cond-mat.str-el↗

arXiv2024

Bulk-like Mott-Transition in ultrathin Cr-doped V2O3 films and the influence of its variability on scaled devices

The pressure driven Mott-transition in Chromium doped V2O3 films is investigated by direct electrical measurements on polycrystalline films with thicknesses down to 10 nm, and doping concentrations of 2%, 5% and 15%. A change in resistivity of nearly two orders of magnitude is found for 2% doping. A simulation model based on a scaling law description of the phase transition and percolative behavior in a resistor lattice is developed. This is used to show that despite significant deviations in the film structure from single crystals, the transition behavior is very similar. Finally, the influence of the variability between grains on the characteristics of scaled devices is investigated and found to allow for scaling down to at least 50 nm device width.

cond-mat.str-el↗

arXiv2024

Magnetization dynamics driven by displacement currents across a magnetic tunnel junction

Understanding the high-frequency transport characteristics of magnetic tunnel junctions (MTJs) is crucial for the development of fast-operating spintronics memories and radio frequency devices. Here, we present the study of frequency-dependent capacitive current effect in CoFeB/MgO-based MTJs and its influence on magnetization dynamics using time-resolved magneto-optical Kerr effect technique. In our device operating at gigahertz frequencies, we find a large displacement current of the order of mA's, which does not break the tunnel barrier of the MTJ. Importantly, this current generates an Oersted field and spin-orbit torque, inducing magnetization dynamics. Our discovery holds promise for building robust MTJ devices operating under high current conditions, also highlighting the significance of capacitive impedance in high frequency magnetotransport techniques.

cond-mat.mes-hall↗

arXiv2024

Synaptogen: A cross-domain generative device model for large-scale neuromorphic circuit design

We present a fast generative modeling approach for resistive memories that reproduces the complex statistical properties of real-world devices. To enable efficient modeling of analog circuits, the model is implemented in Verilog-A. By training on extensive measurement data of integrated 1T1R arrays (6,000 cycles of 512 devices), an autoregressive stochastic process accurately accounts for the cross-correlations between the switching parameters, while non-linear transformations ensure agreement with both cycle-to-cycle (C2C) and device-to-device (D2D) variability. Benchmarks show that this statistically comprehensive model achieves read/write throughputs exceeding those of even highly simplified and deterministic compact models.

cs.NE↗

arXiv2023

A Compact Model of Threshold Switching Devices for Efficient Circuit Simulations

In this paper, we present a new compact model of threshold switching devices which is suitable for efficient circuit-level simulations. First, a macro model, based on a compact transistor based circuit, was implemented in LTSPICE. Then, a descriptive model was extracted and implemented in MATLAB, which is based on the macro model. This macro model was extended to develop a physical model that describes the processes that occur during the threshold switching. The physical model derived comprises a delay structure with few electrical components adjacent to the second junction. The delay model incorporates an internal state variable, which is crucial to transform the descriptive model into a compact model and to parameterize it in terms of electrical parameters that represent the component's behavior. Finally, we applied our model by fitting measured i-v data of an OTS device manufactured by Western Digital Research.

cond-mat.mes-hall↗

arXiv2022

Fabrication of highly resistive NiO thin films for nanoelectronic applications

Thin films of the prototypical charge transfer insulator NiO appear to be a promising material for novel nanoelectronic devices. The fabrication of the material is challenging however, and mostly a p-type semiconducting phase is reported. Here, the results of a factorial experiment are presented that allow optimization of the film properties of thin films deposited using sputtering. A cluster analysis is performed, and four main types of films are found. Among them, the desired insulating phase is identified. From this material, nanoscale devices are fabricated, which demonstrate that the results carry over to relevant length scales. Initial switching results are reported.

cond-mat.mtrl-sci↗

arXiv2020

Non-Volatile Memory Array Based Quantization- and Noise-Resilient LSTM Neural Networks

In cloud and edge computing models, it is important that compute devices at the edge be as power efficient as possible. Long short-term memory (LSTM) neural networks have been widely used for natural language processing, time series prediction and many other sequential data tasks. Thus, for these applications there is increasing need for low-power accelerators for LSTM model inference at the edge. In order to reduce power dissipation due to data transfers within inference devices, there has been significant interest in accelerating vector-matrix multiplication (VMM) operations using non-volatile memory (NVM) weight arrays. In NVM array-based hardware, reduced bit-widths also significantly increases the power efficiency. In this paper, we focus on the application of quantization-aware training algorithm to LSTM models, and the benefits these models bring in terms of resilience against both quantization error and analog device noise. We have shown that only 4-bit NVM weights and 4-bit ADC/DACs are needed to produce equivalent LSTM network performance as floating-point baseline. Reasonable levels of ADC quantization noise and weight noise can be naturally tolerated within our NVMbased quantized LSTM network. Benchmark analysis of our proposed LSTM accelerator for inference has shown at least 2.4x better computing efficiency and 40x higher area efficiency than traditional digital approaches (GPU, FPGA, and ASIC). Some other novel approaches based on NVM promise to deliver higher computing efficiency (up to 4.7x) but require larger arrays with potential higher error rates.

cs.NE↗

arXiv2016

Template-Assisted Direct Growth of 1Td/in$^2$ Bit Patterned Media

We present a method for growing bit patterned magnetic recording media using directed growth of sputtered granular perpendicular magnetic recording media. The grain nucleation is templated using an epitaxial seed layer which contains Pt pillars separated by amorphous metal oxide. The scheme enables the creation of both templated data and servo regions suitable for high density hard disk drive operation. We illustrate the importance of using a process that is both topographically and chemically driven to achieve high quality media.

cond-mat.mtrl-sci↗

arXiv2015

Two-dimensional Decoding Algorithms and Recording Techniques for Bit Patterned Media Feasibility Demonstrations

Recording experiments and decoding algorithms are presented for evaluating the bit-error-rate of state-of-the-art magnetic bitpatterned media. The recording experiments are performed with a static tester and conventional hard-disk-drive heads. As the reader dimensions are larger than the bit dimensions in both the down-track and the cross-track directions, a two-dimensional bit decoding algorithm is required. Two such algorithms are presented in details together with the methodology implemented to accurately retrieve island positions during recording. Using these techniques, a 1.6 Td/in$^2$ magnetic bit pattern media is demonstrated to support 2D bit error rates below 1e-2 under shingled magnetic recording conditions.

cs.IT↗

arXiv2015

Bit Patterned Magnetic Recording: Theory, Media Fabrication, and Recording Performance

Bit Patterned Media (BPM) for magnetic recording provide a route to densities $>1 Tb/in^2$ and circumvents many of the challenges associated with conventional granular media technology. Instead of recording a bit on an ensemble of random grains, BPM uses an array of lithographically defined isolated magnetic islands, each of which stores one bit. Fabrication of BPM is viewed as the greatest challenge for its commercialization. In this article we describe a BPM fabrication method which combines e-beam lithography, directed self-assembly of block copolymers, self-aligned double patterning, nanoimprint lithography, and ion milling to generate BPM based on CoCrPt alloys. This combination of fabrication technologies achieves feature sizes of $<10 nm$, significantly smaller than what conventional semiconductor nanofabrication methods can achieve. In contrast to earlier work which used hexagonal close-packed arrays of round islands, our latest approach creates BPM with rectangular bitcells, which are advantageous for integration with existing hard disk drive technology. The advantages of rectangular bits are analyzed from a theoretical and modeling point of view, and system integration requirements such as servo patterns, implementation of write synchronization, and providing for a stable head-disk interface are addressed in the context of experimental results. Optimization of magnetic alloy materials for thermal stability, writeability, and switching field distribution is discussed, and a new method for growing BPM islands on a patterned template is presented. New recording results at $1.6 Td/in^2$ (teradot/inch${}^2$, roughly equivalent to $1.3 Tb/in^2$) demonstrate a raw error rate $<10^{-2}$, which is consistent with the recording system requirements of modern hard drives. Extendibility of BPM to higher densities, and its eventual combination with energy assisted recording are explored.

cond-mat.other↗

arXiv2013

Bimodal switching field distributions in all-perpendicular spin-valve nanopillars

Switching field measurements of the free layer element of 75 nm diameter spin-valve nanopillars reveal a bimodal distribution of switching fields at low temperatures (below 100 K). This result is inconsistent with a model of thermal activation over a single perpendicular anisotropy barrier. The correlation between antiparallel to parallel and parallel to antiparallel switching fields increases to nearly 50% at low temperatures. This reflects random fluctuation of the shift of the free layer hysteresis loop between two different magnitudes, which may originate from changes in the dipole field from the polarizing layer. The magnitude of the loop shift changes by 25% and is correlated to transitions of the spin-valve into an antiparallel configuration.

cond-mat.mes-hall↗

arXiv2013

Thermally assisted current-induced magnetization reversal in SrRuO3

We inject a sequence of 1 ms current pulses into uniformly magnetized patterns of the itinerant ferromagnet SrRuO3 until a magnetization reversal is detected. We detect the effective temperature during the pulse and find that the cumulative pulse time required to induce magnetization reversal depends exponentially on 1/T. In addition, we find that the cumulative pulse time also depends exponentially on the current amplitude. These observations indicate current-induced magnetization reversal assisted by thermal fluctuations.

cond-mat.mtrl-sci↗

arXiv2012

Current-induced magnetization reversal in SrRuO3

We inject current pulses into uniformly magnetized patterns of thin films of the itinerant ferromagnet SrRuO3, while monitoring the effective temperature of the patterns during the current injection. We gradually increase the amplitude of the pulses until magnetization reversal occurs. We observe magnetization reversal induced by current above a temperature-dependent threshold and show that this effect is not simply due to sample heating or Oersted fields. We discuss the applicability of the current-induced spin-wave instability scenario.

cond-mat.str-el↗

arXiv2012

Audio Cards for High-Resolution and Economical Electronic Transport Studies

We report on a technique for determining electronic transport properties using commercially available audio cards. Using a typical 24-bit audio card simultaneously as a sine wave generator and a narrow bandwidth ac voltmeter, we show the spectral purity of the analog-to-digital and digital-to-analog conversion stages, including an effective number of bits greater than 16 and dynamic range better than 110 dB. We present two circuits for transport studies using audio cards: a basic circuit using the analog input to sense the voltage generated across a device due to the signal generated simultaneously by the analog output; and a digitally-compensated bridge to compensate for nonlinear behavior of low impedance devices. The basic circuit also functions as a high performance digital lock-in amplifier. We demonstrate the application of an audio card for studying the transport properties of spin-valve nanopillars, a two-terminal device that exhibits Giant Magnetoresistance (GMR) and whose nominal impedance can be switched between two levels by applied magnetic fields and by currents applied by the audio card.

physics.ins-det↗

arXiv2011

Asymmetric switching behavior in perpendicularly magnetized spin-valve nanopillars due to the polarizer dipole field

We report the free layer switching field distributions of spin-valve nanopillars with perpendicular magnetization. While the distributions are consistent with a thermal activation model, they show a strong asymmetry between the parallel to antiparallel and the reverse transition, with energy barriers more than 50% higher for the parallel to antiparallel transitions. The inhomogeneous dipolar field from the polarizer is demonstrated to be at the origin of this symmetry breaking. Interestingly, the symmetry is restored for devices with a lithographically defined notch pair removed from the midpoint of the pillar cross-section along the ellipse long axis. These results have important implications for the thermal stability of perpendicular magnetized MRAM bit cells.

cond-mat.mes-hall↗

arXiv2010

Stability of 2pi domain walls in ferromagnetic nanorings

The stability of 2pi domain walls in ferromagnetic nanorings is investigated via calculation of the minimum energy path that separates a 2pi domain wall from the vortex state of a ferromagnetic nanoring. Trapped domains are stable when they exist between certain types of transverse domain walls, i.e., walls in which the edge defects on the same side of the magnetic strip have equal sign and thus repel. Here the energy barriers between these configurations and vortex magnetization states are obtained using the string method. Due to the geometry of a ring, two types of 2pi walls must be distinguished that differ by their overall topological index and exchange energy. The minimum energy path corresponds to the expulsion of a vortex. The energy barrier for annihilation of a 2pi wall is compared to the activation energy for transitions between the two ring vortex states.

cond-mat.mes-hall↗