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Daniel Hammerland

Publications and source records attributed to Daniel Hammerland.

3 recordsLinked to original sources

MHz to sub-kHz field detection with an all-dielectric potassium Rydberg-atom sensor

Rydberg sensors have significant promise as an alternative to the antenna systems used for sub-MHz frequency communications, where the scale of high-efficiency antennas is often impractically large, forcing the use of low-efficiency, electrically small antennas. The exploration of Rydberg sensors at these frequencies has been hampered by the low field transmission of the silicate vapor cells. We dramatically improve the low-frequency field transmission of silicate vapor cells by using potassium as the active medium instead of rubidium or cesium. The potassium Rydberg sensor can measure fields with frequencies down to 500 Hz in an all-dielectric sensor, effectively extending the low-frequency cutoff of the sensor by nearly four orders of magnitude compared to an equivalent rubidium vapor cell. With this simple substitution, experimentation with low-frequency sensing becomes dramatically more accessible to the community.

physics.atom-ph

Two-dimensional imaging of electromagnetic fields via light sheet fluorescence imaging with Rydberg atoms

The ability to image electromagnetic fields holds key scientific and industrial applications, including electromagnetic compatibility, diagnostics of high-frequency devices, and experimental scientific work involving field interactions. Generally electric and magnetic field measurements require conductive elements which significantly distort the field. However, electromagnetic fields can be measured without altering the field via the shift they induce on Rydberg states of alkali atoms in atomic vapor, which are highly sensitive to electric fields. Previous field measurements using Rydberg atoms utilized electromagnetically induced transparency to read out the shift on the states induced by the fields, but did not provide spatial resolution. In this work, we demonstrate that electromagnetically induced transparency can be spatially resolved by imaging the fluorescence of the atoms. We demonstrate that this can be used to image $\sim$ V/cm scale electric fields in the DC-GHz range and $\sim$ mT scale static magnetic fields, with minimal distortion to the fields. We also demonstrate the ability to image $\sim$ 5 mV/cm scale fields for resonant microwave radiation and measure standing waves generated by the partial reflection of the vapor cell walls in this regime. With additional processing techniques like lock-in detection, we predict that our sensitivities could reach down to nV/cm levels. We perform this field imaging with a spatial resolution of 160 $\mu$m, limited by our imaging system, and estimate the fundamental resolution limitation to be 5 $\mu$m.

physics.atom-ph

Attosecond X-ray Core-level Chronoscopy of Aromatic Molecules

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits to the complexity of systems that can be studied and the information that can be retrieved, respectively. Using attosecond X-ray pulses from LCLS, we demonstrate the key advantages of measuring core-level delays: the photoelectron spectra remain atom-like, the measurements become element specific and the observed scattering dynamics originate from a point-like source. We exploit these unique features to reveal the effects of electronegativity and symmetry on attosecond scattering dynamics by measuring and calculating the photoionization delays between N-1s and C-1s core shells of a series of aromatic azabenzene molecules. Remarkably, the delays increase with the number of nitrogen atoms in the molecule and reveal multiple resonances. We identify two previously unknown mechanisms regulating the associated attosecond dynamics, namely the enhanced confinement of the trapped wavefunction with increasing electronegativity of the atoms and the decrease of the coupling strength among the photoemitted partial waves with increasing symmetry. This study demonstrates the unique opportunities opened by measurements of core-level photoionization delays for unraveling attosecond electron dynamics in complex matter.

physics.chem-ph