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Daniel K. Pratt

Publications and source records attributed to Daniel K. Pratt.

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Neutron-scattering measurements of the spin excitations in LaFeAsO and Ba(Fe$_{0.953}$Co$_{0.047}$)$_{2}$As$_{2}$: Evidence for a sharp enhancement of spin fluctuations by nematic order

Inelastic neutron scattering was employed to investigate the impact of electronic nematic order on the magnetic spectra of LaFeAsO and Ba(Fe$_{0.953}$Co$_{0.047}$)$_{2}$As$_{2}$. These materials are ideal to study the paramagnetic-nematic state, since the nematic order, signaled by the tetragonal-to-orthorhombic transition at $T_{\rm S}$, sets in well above the stripe antiferromagnetic ordering at $T_{\rm N}$. We find that the temperature-dependent dynamic susceptibility displays an anomaly at $T_{\rm S}$ followed by a sharp enhancement in the spin-spin correlation length, revealing a strong feedback effect of nematic order on the low-energy magnetic spectrum. Our findings can be consistently described by a model that attributes the structural/nematic transition to magnetic fluctuations, and unveils the key role played by nematic order in promoting the long-range stripe antiferromagnetic order in iron pnictides.

cond-mat.str-el

Neutron Scattering Studies of the Ferroelectric Distortion and Spin Dynamics in the Type-1 Multiferroic Perovskite Sr0.56Ba0.44MnO3

The magnetic order, spin dynamics, and crystal structure of the multiferroic Sr0.56Ba0.44MnO3 have been investigated using neutron and x-ray scattering. Ferroelectricity develops at TC=305 K with a polarization of 4.2 microC/cm2 associated with the displacements of the Mn ions, while the Mn4+ spins order below TN = 200 K into a simple G-type commensurate magnetic structure. Below TN the ferroelectric order decreases dramatically demonstrating that the two order parameters are strongly coupled. The ground state spin dynamics are characterized by a spin gap of 4.6(5) meV and the magnon density of states peaking at 43 meV. Detailed spin wave simulations with a gap and isotropic exchange of J=4.8(2) meV describe the excitation spectrum well. Above TN strong spin correlations coexist with robust ferroelectric order.

cond-mat.mtrl-sci