arXiv subjects

Daniel Kaplan

Publications and source records attributed to Daniel Kaplan.

At least 37 records · Page 2Linked to original sources

arXiv2024

Real-Space Imaging of the Band Topology of Transition Metal Dichalcogenides

The topological properties of Bloch bands are intimately tied to the structure of their electronic wavefunctions within the unit cell of a crystal. Here, we show that scanning tunneling microscopy (STM) measurements on the prototypical transition metal dichalcogenide (TMD) semiconductor WSe$_2$ can be used to unambiguously fix the location of the Wannier center of the valence band. Using site-specific substitutional doping, we first determine the position of the atomic sites within STM images, establishing that the maximum electronic density of states at the $K$-point lies between the atoms. In contrast, the maximum density of states at the $Γ$ point is at the atomic sites. This signifies that WSe$_2$ is a topologically obstructed atomic insulator, which cannot be adiabatically transformed to the trivial atomic insulator limit.

cond-mat.mtrl-sci↗

arXiv2024

Topological superconductivity from repulsive interactions in twisted WSe$_2$

The recent observation of superconductivity in twisted bilayer WSe$_2$ raises intriguing questions concerning the origin and the properties of superconducting states realized in bands with non-trivial topological properties and repulsive electron-electron interactions. Using a continuum band structure model, we analyze a mechanism for Coulomb interaction-driven superconductivity in twisted bilayers of WSe$_2$. We discuss the symmetries and the phenomenological properties of the resulting superconducting phases and their evolution with interlayer potential difference, tunable via an out of plane electric field. The pairing strength is a non-monotonic function of interlayer potential, being larger at intermediate values due to mixing of singlet and triplet pairing. In contrast, at larger interlayer potential, the pairing tendency is suppressed due to enhanced Coulomb repulsion. The superconducting state is chiral in a large regime of parameters and undergoes a transition to a nodal nematic superconductor at a critical potential difference. The chiral state, characterized by an intervalley-symmetric superposition of triplet and singlet pairs, is classified as a topological superconductor within the Altland-Zirnbauer class C. At zero interlayer potential difference, the superconducting state is instead of class D, which hosts Majorana zero modes, making it a promising candidate for applications in quantum computation.

cond-mat.supr-con↗

arXiv2024

Crepant resolutions of stratified varieties via gluing

Let $X$ be a variety with a stratification $\mathcal{S}$ into smooth locally closed subvarieties such that $X$ is locally a product along each stratum (e.g., a symplectic singularity). We prove that assigning to each open subset $U \subset X$ the set of isomorphism classes of locally projective crepant resolutions of $U$ defines an $\mathcal{S}$-constructible sheaf of sets. Thus, for each stratum $S$ and basepoint $s \in S$, the fundamental group acts on the set of germs of projective crepant resolutions at $s$, leaving invariant the germs extending to the entire stratum. Global locally projective crepant resolutions correspond to compatible such choices for all strata. For example, if the local projective crepant resolutions are unique, they automatically glue uniquely. We give criteria for a locally projective crepant resolution $ρ: \tilde X \to X$ to be globally projective. We show that the sheafification of the presheaf $U \mapsto \text{Pic}(ρ^{-1}(U)/U)$ of relative Picard classes is also constructible. The resolution is globally projective only if there exist local relatively ample bundles whose classes glue to a global section of this sheaf. The obstruction to lifting this section to a global ample line bundle is encoded by a gerbe on the singularity $X$. We show the gerbes are automatically trivial if $X$ is a symplectic quotient singularity. Our main results hold in the more general setting of partial crepant resolutions, that need not have smooth source. We apply the theory to symmetric powers and Hilbert schemes of surfaces with du Val singularities, finite quotients of tori, multiplicative and Nakajima quiver varieties, as well as to canonical threefold singularities.

math.AG↗

arXiv2024

Even-integer Quantum Hall Effect in an Oxide Caused by Hidden Rashba Effect

In the presence of high magnetic field, quantum Hall systems usually host both even- and odd-integer quantized states because of lifted band degeneracies. Selective control of these quantized states is challenging but essential to understand the exotic ground states and manipulate the spin textures. Here, we study the quantum Hall effect in Bi2O2Se thin films. In magnetic fields as high as 50 T, we observe only even-integer quantum Hall states, but no sign of odd-integer states. However, when reducing the thickness of the epitaxial Bi2O2Se film to one unit cell, we observe both odd- and even-integer states in this Janus (asymmetric) film grown on SrTiO3. By means of a Rashba bilayer model based on ab initio band structures of Bi2O2Se thin films, we can ascribe the absence of odd-integer states in thicker films to the hidden Rasbha effect, where the local inversion symmetry breaking in two sectors of the [Bi2O2]2+ layer yields opposite Rashba spin polarizations, which compensate with each other. In the one unit cell Bi2O2Se film grown on SrTiO3, the asymmetry introduced by top surface and bottom interface induces a net polar field. The resulting global Rashba effect lifts the band degeneracies present in the symmetric case of thicker films.

cond-mat.mes-hall↗

arXiv2024

Even Integer Quantum Hall Effect in Materials with Hidden Spin Texture

Because spin-orbit coupling (SOC) is invisible in the band structure when inversion symmetry exists, whether spins are trivially degenerate or strongly coupled to momentum due to SOC is presumed to make little difference in transport measurements, such as magnetoresistance and quantum oscillations. In this work, however, we show that hidden Rashba SOC in a centrosymmetric two-dimensional material can lead to the quantum Hall effect with only even-integer plateaus, unlike a spinless electron gas. Here, two Rashba layers that are degenerate but with opposite SOC due to inversion symmetry, hybridize with each other and create two doubly-degenerate bands with hidden spin texture. Correspondingly, two branches of Landau levels interact, resulting in significant suppression of spin splitting due to the balancing of intralayer SOC and interlayer hybridization. Furthermore, we show that breaking inversion symmetry restores the ordinary quantum Hall fluid by introducing spin-split Fermi surfaces. Our theory can apply to centrosymmetric materials with strong SOC, as demonstrated in a recent experiment on the two-dimensional semiconductor Bi$_2$O$_2$Se.

cond-mat.mes-hall↗

arXiv2024

Electrical control of intrinsic nonlinear Hall effect in antiferromagnetic topological insulator sandwiches

Nonlinear Hall effect (NHE) can originate from the quantum metric mechanism in antiferromagnetic topological materials with PT symmetry, which has been experimentally observed in MnBi2Te4. In this work, we propose that breaking PT symmetry via external electric fields can lead to a dramatic enhancement of NHE, thus allowing for an electric control of NHE. Microscopically, this is because breaking PT symmetry can lift spin degeneracy of a Kramers' pair, giving rise to additional contributions within one Kramers' pair of bands. We demonstrate this enhancement through a model Hamiltonian that describes an antiferromagnetic topological insulator sandwich structure.

cond-mat.mes-hall↗

arXiv2024

Ultralow-Noise Optical Parametric Amplifier for Stimulated Raman Scattering Imaging

We present a 40-MHz ultrafast optical parametric amplifier (OPA), tunable from 0.8 to 1 $μ$m, with a relative intensity noise (RIN) matching the shot-noise floor (-160 dB/Hz) above 2 MHz. The OPA is pumped by a 20-W Kerr-lens mode-locked Ytterbium laser and seeded by a a supercontinuum generated in an all-normal-dispersion (ANDi) fiber. With an average output power >1.5 W, this compact and simple scheme is an attractive alternative to synchronously-pumped optical parametric oscillators, especially within the context of stimulated Raman scattering (SRS) imaging. To illustrate the latter, we perform chemical imaging of vinegar droplets in oil by SRS microscopy.

physics.optics↗

arXiv2023

Hidden non-collinear spin-order induced topological surface states

Rare-earth monopnictides are a family of materials simultaneously displaying complex magnetism, strong electronic correlation, and topological band structure. The recently discovered emergent arc-like surface states in these materials have been attributed to the multi-wave-vector antiferromagnetic order, yet the direct experimental evidence has been elusive. Here we report the observation of non-collinear antiferromagnetic order with multiple modulations using spin-polarized scanning tunneling microscopy. Moreover, we discover a hidden spin-rotation transition of single-to-multiple modulations 2 K below the Neel temperature. The hidden transition coincides with the onset of the surface states splitting observed by our angle-resolved photoemission spectroscopy measurements. Single modulation gives rise to a band inversion with induced topological surface states in a local momentum region while the full Brillouin zone carries trivial topological indices, and multiple modulation further splits the surface bands via non-collinear spin tilting, as revealed by our calculations. The direct evidence of the non-collinear spin order in NdSb not only clarifies the mechanism of the emergent topological surface states, but also opens up a new paradigm of control and manipulation of band topology with magnetism.

cond-mat.str-el↗

arXiv2023

Unification of Nonlinear Anomalous Hall Effect and Nonreciprocal Magnetoresistance in Metals by the Quantum Geometry

The quantum geometry has significant consequences in determining transport and optical properties in quantum materials. Here, we use a semiclassical formalism coupled with perturbative corrections unifying the nonlinear anomalous Hall effect (NLAHE) and nonreciprocal magnetoresistance (NMR, longitudinal resistance) from the quantum geometry. In the dc limit, both transverse and longitudinal nonlinear conductivities include a term due to the normalized quantum metric dipole. The quantum metric contribution is intrinsic and does not scale with the quasiparticle lifetime. We demonstrate the coexistence of a NLAHE and NMR in films of the doped antiferromagentic topological insulator MnBi$_2$Te$_4$. Our work indicates that both longitudinal and transverse nonlinear transport provide a sensitive probe of the quantum geometry in solids.

cond-mat.mes-hall↗

arXiv2023

Quantum metric-induced nonlinear transport in a topological antiferromagnet

The Berry curvature and quantum metric are the imaginary part and real part, respectively, of the quantum geometric tensor which characterizes the topology of quantum states. The former is known to generate a zoo of important discoveries such as quantum Hall effect and anomalous Hall effect (AHE), while the consequences of the quantum metric have rarely been probed by transport. In this work, we observed quantum metric induced nonlinear transport, including both nonlinear AHE and diode-like nonreciprocal longitudinal response, in thin films of a topological antiferromagnet, MnBi$_2$Te$_4$. Our observation reveals that the transverse and longitudinal nonlinear conductivities reverse signs when reversing the antiferromagnetic order, diminish above the Néel temperature, and are insensitive to disorder scattering, thus verifying their origin in the band structure topology. They also flip signs between electron and hole-doped regions, in agreement with theoretical calculations. Our work provides a pathway to probe the quantum metric through nonlinear transport and to design magnetic nonlinear devices.

cond-mat.mes-hall↗

arXiv2023

Can ChatGPT be used to generate scientific hypotheses?

We investigate whether large language models can perform the creative hypothesis generation that human researchers regularly do. While the error rate is high, generative AI seems to be able to effectively structure vast amounts of scientific knowledge and provide interesting and testable hypotheses. The future scientific enterprise may include synergistic efforts with a swarm of "hypothesis machines", challenged by automated experimentation and adversarial peer reviews.

cs.CL↗

arXiv2023

Emergent topological quantum orbits in the charge density wave phase of kagome metal CsV$_3$Sb$_5$

The recently discovered kagome materials $A$V$_3$Sb$_5$ ($A$ = K, Rb, Cs) attract intense research interest in intertwined topology, superconductivity, and charge density waves (CDW). Although the in-plane $2\times2$ CDW is well studied, its out-of-plane structural correlation with the Fermi surface properties is less understood. In this work, we advance the theoretical description of quantum oscillations and investigate the Fermi surface properties in the three-dimensional CDW phase of CsV$_3$Sb$_5$. We derived Fermi-energy-resolved and layer-resolved quantum orbits that agree quantitatively with recent experiments in the fundamental frequency, cyclotron mass, and topology. We reveal a complex Dirac nodal network that would lead to a $π$ Berry phase of a quantum orbit in the spinless case. However, the phase shift of topological quantum orbits is contributed by the orbital moment and Zeeman effect besides the Berry phase in the presence of spin-orbital coupling (SOC). Therefore, we can observe topological quantum orbits with a $π$ phase shift in otherwise trivial orbits without SOC, contrary to common perception. Our work reveals the rich topological nature of kagome materials and paves a path to resolve different topological origins of quantum orbits.

cond-mat.str-el↗

arXiv2023

Exceptional Collections for Mirrors of Invertible Polynomials

We prove the existence of a full exceptional collection for the derived category of equivariant matrix factorizations of an invertible polynomial with its maximal symmetry group. This proves a conjecture of Hirano--Ouchi. In the Gorenstein case, we also prove a stronger version of this conjecture due to Takahashi. Namely, that the full exceptional collection is strong.

math.AG↗

arXiv2022

Unifying semiclassics and quantum perturbation theory at nonlinear order

Nonlinear electrical response permits a unique window into effects of band structure geometry. It can be calculated either starting from a Boltzmann approach for small frequencies, or using Kubo's formula for resonances at finite frequency. However, a precise connection between both approaches has not been established. Focusing on the second order nonlinear response, here we show how the semiclassical limit can be recovered from perturbation theory in the velocity gauge, provided that finite quasiparticle lifetimes are taken into account. We find that matrix elements related to the band geometry combine in this limit to produce the semiclassical nonlinear conductivity. We demonstrate the power of the new formalism by deriving a quantum contribution to the nonlinear conductivity which is of order $τ^{-1}$ in the relaxation time $τ$, which is principally inaccessible within the Boltzmann approach. We outline which steps can be generalized to higher orders in the applied perturbation, and comment about potential experimental signatures of our results.

cond-mat.mes-hall↗

arXiv2022

General nonlinear Hall current in magnetic insulators beyond the quantum anomalous Hall effect

Can a generic magnetic insulator exhibit a Hall current? The quantum anomalous Hall effect (QAHE) is one example of an insulating bulk carrying a quantized Hall conductivity and other insulators (with zero Chern number) present zero Hall conductance in the linear response regime. Here, we find that a general magnetic insulator possesses a nonlinear Hall conductivity quadratic to the electric field if the system breaks inversion symmetry. This conductivity originates from an induced orbital magnetization due to virtual interband transitions. We identify three contributions to the wavepacket motion, a velocity shift, a positional shift, and a Berry curvature renormalization. In contrast to the crystalline solid, we find that this nonlinear Hall conductivity vanishes for Landau levels of a 2D electron gas, indicating a fundamental difference between the QAHE and the Integer quantum Hall effect.

cond-mat.mes-hall↗

arXiv2022

Multiplicative preprojective algebras of Dynkin quivers

For a commutative ring $R$ and an ADE Dynkin quiver $Q$, we prove that the multiplicative preprojective algebra of Crawley-Boevey and Shaw, with parameter $q=1$, is isomorphic to the (additive) preprojective algebra as $R$-algebras if and only if the bad primes for $Q$ (2 in type D, 2 and 3 for $Q = E_{6}$, $E_{7}$ and 2, 3 and 5 for $Q= E_{8}$) are invertible in $R$. We construct an explicit isomorphism over $\mathbb{Z}[1/2]$ in type D, over $\mathbb{Z}[1/2, 1/3]$ for $Q = E_{6}$, $E_{7}$ and over $\mathbb{Z}[1/2, 1/3, 1/5]$ for $Q=E_{8}$. Conversely, if some bad prime is not invertible in $R$, we show that the additive and multiplicative preprojective algebras differ in zeroth Hochschild homology, and hence are not isomorphic. In fact, one only needs the vanishing of certain classes in zeroth Hochschild homology of the multiplicative preprojective algebra, utilizing a rigidification argument for isomorphisms that may be of independent interest. In the setting of Ginzburg dg-algebras, our obstructions are new in type E and give a more elementary proof of the negative result of Etgü--Lekili arXiv:1502.07922 in type D. Moreover, the zeroth Hochschild homology of the multiplicative preprojective algebra can be interpreted as the space of unobstructed deformations of the multiplicative Ginzburg dg-algebra by Van den Bergh duality. Finally, we observe that the multiplicative preprojective algebra is not symmetric Frobenius if $Q \neq A_1$, a departure from the additive preprojective algebra in characteristic 2 for $Q = D_{2n}$, $n \geq 2$ and $Q =E_{7}$, $E_{8}$.

math.RA↗

arXiv2022

Momentum-inversion symmetry breaking on the Fermi surface of magnetic topological insulators

Magnetic topological insulators (MnBi$_2$Te$_4$)(Bi$_2$Te$_3$)$_n$ were anticipated to exhibit magnetic energy gaps while recent spectroscopic studies did not observe them. Thus, magnetism on the surface is under debate. In this work, we propose another symmetry criterion to probe the surface magnetism. Because of both time-reversal symmetry-breaking and inversion symmetry-breaking, we demonstrate that the surface band structure violates momentum-inversion symmetry and leads to a three-fold rather than six-fold rotational symmetry on the Fermi surface if corresponding surface states couple strongly to the surface magnetism. Such a momentum-inversion symmetry violation is significant along the $Γ-K$ direction for surface bands on the (0001) plane.

cond-mat.mtrl-sci↗

arXiv2022

Twisted photovoltaics at terahertz frequencies from momentum shift current

The bulk photovoltaic effect (BPVE) converts light into a coherent dc current at zero bias, through what is commonly known as the shift current. This current has previously been attributed to the displacement of the electronic wave function center in real space, when the sample is excited by light. We reveal that materials like twisted bilayer graphene (TBG) with a flatband dispersion are uniquely suited to maximize the BPVE because they lead to an enhanced shift in the momentum space, unlike any previously known shift current mechanism. We identify properties of quantum geometry, which go beyond the quantum geometric tensor, and are unrelated to Berry charges, as the physical origin of the large BPVE we observe in TBG. Our calculations show that TBG with a band gap of several meV exhibits a giant BPVE in a range of 0.2-1 THz, which represents the strongest BPVE reported so far at this frequency in a two-dimensional material and partially persists even a room temperature. Our paper provides a design principle for shift current generation, which applies to a broad range of twisted heterostructures with the potential to overcome the so-called "terahertz gap" in THz sensing.

cond-mat.mes-hall↗