arXiv subjects

Daniel Koller

Publications and source records attributed to Daniel Koller.

8 recordsLinked to original sources

arXiv2010

Plasmonic crystal demultiplexer and multiports

Artificially built periodic optical structures in dielectric and metallic media have generated considerable interest due to their potential for optical device miniaturization. In this context plasmonics, i.e., optics based on surface plasmon polaritons (SPPs) offers new exciting prospects. SPPs are hybrid light/electron surface waves at the interface between a dielectric and a metal and as such hold the potential for 2D optical functionality. Indeed, SPP elements as mirrors, splitters and interferometers have been recently demonstrated. However, for plasmonics to qualify at the information technology level requires necessarily the realization of wavelength division (demultiplexing) which constitutes a fundamental ingredient of optical communication. In the following we experimentally demonstrate 2D SPP demultiplexing in the visible spectral range by using photonic crystals for SPPs (plasmonic crystals). In addition, we demonstrate that plasmonic crystal are capable of realizing integrated linear multiports which could constitute building blocks of analog or quantum optical computing.

physics.optics↗

arXiv2010

Surface Plasmon Polariton microscope with Parabolic Reflectors

We report the realization of a two--dimensional optical microscope for surface plasmons polaritons (SPPs) based on parabolic Bragg mirrors. These mirrors are built from lithographically fabricated gold nanostructures on gold thin films. We show by direct imaging by leakage radiation microscopy that the magnification power of the SPP microscope follows basic predictions of geometrical optics. Spatial resolution down to the value set by the diffraction limit is demonstrated.

physics.optics↗

arXiv1996

Energy gap in superconducting fullerides: optical and tunneling studies

Tunneling and optical transmission studies have been performed on superconducting samples of Rb3C60. At temperatures much below the superconducting transition temperature Tc the energy gap is 2 Delta=5.2 +- 0.2meV, corresponding to 2 Delta/kB Tc = 4.2. The low temperature density of states, and the temperature dependence of the optical conductivity resembles the BCS behavior, although there is an enhanced ``normal state" contribution. The results indicate that this fulleride material is an s-wave superconductor, but the superconductivity cannot be described in the weak coupling limit.

cond-mat↗

arXiv1995

Polymeric alkali fullerides are stable in air

Infrared transmission, electron spin resonance, and X-ray diffraction measurements show unambiguously that RbC$_{60}$ and KC$_{60}$ are stable in air, in contrast to Rb$_{6}$C$_{60}$ which decomposes rapidly upon exposure. The specimens studied transform into pure C$_{60}$ and other byproducts when heated above $100\dd $C, approximately the temperature of the orthorhombic-fcc phase transition. The stability of these compounds raises the possibility of applying them as protective layers for the superconducting fullerides.

cond-mat↗

arXiv1994

Infrared and Raman Evidence for Dimers and Polymers in Rb1C60

The infrared- and Raman-active vibrational modes of C60 were measured in the various structural states of Rb1C60. According to earlier studies, Rb1C60 has an $fcc$ structure at temperatures above ~100C, a linear chain polymer orthorhombic structure when slowly cooled, and an as yet undetermined structure when very rapidly cooled ("quenched"). We show that the spectra obtained in the polymer state are consistent with each C60 molecule having bonds to two diametrically opposite neighbors. In the quenched state, we find evidence for further symmetry breaking, implying a lower symmetry structure than the polymer state. The spectroscopic data of the quenched phase are shown to be consistent with Rb2(C60)2, a dimerization of C60.

cond-mat↗

arXiv1994

Infrared Spectroscopic Study of Phase Transisions in A1c60 Compounds (a=K,Rb,Cs)

Optical measurements on doped C$_{60}$ films provide evidence for a transition from a high temperature conducting phase to a low temperature insulating phase in quenched Rb$_1$C$_{60}$ and K$_1$C$_{60}$ compounds, while Cs$_1$C$_{60}$ did not exhibit this behavior. For slow cooled samples our study confirms earlier results indicating phase separation of K$_1$C$_{60}$ to K$_3$C$_{60}$ and C$_{60}$, and the formation of a new Rb$_1$C$_{60}$ phase at low temperatures. Upon slow cooling Cs$_1$C$_{60}$ behaves similar to Rb$_1$C$_{60}$.

cond-mat↗

arXiv1994

Insulating and Conducting Phases of RbC60

Optical measurements were performed on thin films of Rb$_{x}$C$_{60}$, identified by X-ray diffraction as mostly $x=1$ material. The samples were subjected to various heat treatments, including quenching and slow cooling from 400K. The dramatic increase in the transmission of the quenched samples, and the relaxation towards the transmission observed in slow cooled samples provides direct evidence for the existence of a metastable insulating phase. Slow cooling results in a phase transition between two electrically conducting phases.

cond-mat↗

arXiv1993

In-Situ Infrared Transmission Study of Rb- and K-Doped Fullerenes

We have measured the four IR active $C_{60}$ molecular vibrations in $M_{x}C_{60}$ $(M = K, Rb)$ as a function of doping $x$. We observe discontinuous changes in the vibrational spectra showing four distinct phases (presumably $x = 0, 3, 4$, and 6). The $1427cm^{-1}$ and $576cm^{-1}$ modes show the largest changes shifting downward in frequency in four steps as the doping increases. Several new very weak modes are visible in the $x=6$ phase and are possibly Raman modes becoming weakly optically active. We present quantitative fits of the data and calculate the electron-phonon coupling of the $1427cm^{-1}$ IR mode.

cond-mat↗