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Daniel Podolsky

Publications and source records attributed to Daniel Podolsky.

At least 19 recordsLinked to original sources

Bulk Superconductivity driven by Disorder-Induced Delocalization in 4Hb-Ta(S$_{1-x}$Se$_x$)$_2$

The unconventional superconductor 4Hb-TaS$_2$ is a natural heterostructure that can be broadly understood as interleaving Mott-like and metallic layers. We study the properties of this material as a function of quenched disorder in the form of Se/S substitution and find that while disordered samples show bulk superconductivity, clean samples do not. We show that a disorder-driven delocalization of carriers in the Mott-like ($1T$-) layer forms a new Fermi surface that is absent in the cleanest samples. This suggests that one of the primary drivers for superconductivity is the fragility of the Mott state, whose delocalization brings to life a sea of strongly correlated electrons.

cond-mat.supr-con

Charge-Informed Quantum Error Correction

We investigate the statistical physics of quantum error correction in ${\rm U}(1)$ symmetry-enriched topological quantum memories. Starting from a phenomenological error model of charge-conserving noise, we study the optimal decoder assuming the local charges of each anyon can be measured. The error threshold of the optimal decoder corresponds to a continuous phase transition in a disordered two-dimensional integer loop model on the Nishimori line. Using an effective replica field theory analysis and Monte Carlo numerics, we show that the optimal decoding transition exhibits Berezinskii-Kosterlitz-Thouless universality with a modified universal jump in winding number variance. We further generalize the model beyond the Nishimori line, which defines a large class of suboptimal decoders. At low nonzero temperatures and strong disorder, we find numerical evidence of a disorder-dominated loop-glass phase which corresponds to a "confidently incorrect" decoder. The zero-temperature limit defines the minimum-cost flow decoder, which serves as the ${\rm U}(1)$ analog of minimum-weight perfect matching in $\mathbb{Z}_2$ topological codes. Both the optimal and minimum-cost flow decoders are shown to dramatically outperform the charge-agnostic optimal decoder in symmetry-enriched topological codes.

quant-ph

Quadrupolar and dipolar phases of excitons in transition-metal dichalcogenide trilayer heterostructures

Recent experiments on trilayer transition-metal dichalcogenide heterostructures have revealed the rich behavior of dipolar excitons. Motivated by these experimental observations, we investigate the collective dynamics of planar quantum dipoles whose orientation fluctuates due to charge tunneling between the outer layers. Using large-scale quantum Monte Carlo simulations, we map out the low-temperature phase diagram as a function of experimentally tunable parameters. We uncover a diverse landscape of phases driven by dipolar correlations. Under strong dipole fluctuations, a quadrupolar superfluid emerges. Suppressing charge tunneling nucleates a droplet state stabilized by the attractive interaction between antiparallel dipoles. At high exciton densities, the system gives way to a partially fragmented condensate, characterized by competing quadrupolar and dipolar superfluid states. Furthermore, at a large exciton mass and high density, we find a staggered dipolar crystal. Our detailed study of the dependence of exciton energy shifts on an external electric field directly interprets existing experimental data and underscores the crucial role of the antiparallel dipolar configuration. Our results provide a guide for future experimental explorations of quantum phases of trilayer excitons.

cond-mat.mes-hall

Breakdown of chiral anomaly and emergent phases in Weyl semimetals under orbital magnetic fields

An external orbital magnetic field applied perpendicular to the separation vector of a pair of Weyl points can couple them and induce a gap in the electronic spectrum. In this work, we investigate the gap-opening behavior in the presence of a lattice, revealing rich phenomenology absent in the continuum picture. Specifically, we address the emergence of layered Chern insulating states, examining how the anisotropy of the Weyl cone dispersion influences the sequence of phase transitions, and establishing connections to the continuum limit. We analyze the evolution of surface Fermi-arc states across these regimes, highlighting their distinct behaviors during the gap-opening transitions.

cond-mat.mes-hall

Sideband Spectroscopy in the Strong Driving Regime: Volcano Transparency and Sideband Anomaly

We study the response of a spin to two crossed magnetic fields: a strong and fast transverse field, and a weak and slow longitudinal field. We characterize the sideband response at the sum and the difference of driving frequencies over a broad range of parameters. In the strong transverse driving regime, the emission spectrum has a characteristic volcano lineshape with a narrow central transparency region surrounded by asymmetric peaks. Next, we couple the spin to a nonlinear cavity that both drives and measures it. In a sufficiently slow longitudinal field, the emission spectrum exhibits anomalous behavior, where the resonances in both the right and left sidebands lie on the same side of the central resonance. The theoretical results are compared to the experimental measurement of the emission of substitutional nitrogen P1 and nitrogen-vacancy NV$^-$ defects in diamond.

cond-mat.other

Ion Coulomb crystals: an exotic form of condensed matter

Ion Coulomb crystals are ordered structures formed by laser-cooled ions in traps that are characterized by interparticle distances of several micrometers and energy scales on the order of $\mu$eV. Their crystalline structure emerges from the interplay between Coulomb repulsion and the external confining potential, which can be readily tuned. Moreover, individual ions can be precisely manipulated with lasers and imaged via resonance fluorescence. These unusual and unique properties make ion crystals a powerful platform for studying phases of matter in the strongly correlated regime and at low temperatures where their dynamics is manifestly quantum mechanical. This review examines the theoretical framework and experimental characterization of ion Coulomb crystals from a condensed-matter perspective. We discuss their dynamical and thermodynamic properties in one, two, and three dimensions, and review recent investigations into their out-of-equilibrium behavior. We provide outlooks on future directions for exploring novel condensed matter phenomena with trapped ion crystals, as well as for exploiting these features for scientific and technical applications.

physics.atom-ph

Defect-Mediated Melting of Square-Lattice Solids

The Kosterlitz-Thouless-Halperin-Nelson-Young (KTHNY) theory successfully explains the melting mechanism of two-dimensional isotropic lattices as a two-step process driven by the unbinding of topological defects. By considering the elastic theory of the square lattice, we extend the KTHNY theory to melting of square lattice solids. In addition to the familiar elastic constants that govern the theory -- the Young's modulus and the Poisson ratio -- a third constant controlling the anisotropy of the medium emerges. This modifies both the logarithmic and angular interactions between the topological defects. Despite this modification, the extended theory retains the qualitative features of the isotropic case, predicting a two-step melting with an intermediate tetratic phase. However, some subtle differences arise, including a modified bound on the translational correlation exponent and the absence of universal values for the Young's modulus at the solid-to-tetratic phase transition.

cond-mat.soft

Improved Actions using The Renormalization Group

We introduce a numerical method to study critical properties near classical and quantum phase transitions. Our method applies ideas of the Tensor Renormalization Group to obtain an improved action which is used to extract critical properties by performing Monte Carlo simulations on relatively small system sizes. We demonstrate this method on the XY model in three dimensions. Our method may provide a framework with which to efficiently study universal properties in a large class of phase transitions.

cond-mat.stat-mech

Computational Phase Transitions in Two-Dimensional Antiferromagnetic Melting

A computational phase transition in a classical or quantum system is a non-analytic change in behavior of an order parameter which can only be observed with the assistance of a nontrivial classical computation. Such phase transitions, and the computational observables which detect them, play a crucial role in the optimal decoding of quantum error-correcting codes and in the scalable detection of measurement-induced phenomena. In this work we show that computational phase transitions and observables can also provide important physical insight on the phase diagram of a classical statistical physics system, specifically in the context of the dislocation-mediated melting of a two-dimensional antiferromagnetic (AF) crystal. In the solid phase, elementary dislocations disrupt the bipartiteness of the underlying square lattice, and as a result, pairs of dislocations are linearly confined by string-like AF domain walls. It has previously been argued that a novel AF tetratic phase can arise when double dislocations proliferate while elementary dislocations remain bound. However, since elementary dislocations carry AF Ising gauge flux, no local order parameter can distinguish between AF and paramagnetic (PM) tetratic regimes, and consequently there is no thermodynamic phase transition separating the two regimes. Nonetheless, we demonstrate that it is possible to algorithmically construct a staggered magnetization which distinguishes the AF and PM tetratic regimes by "pairing" dislocations, which requires an increasingly nontrivial classical computation as elementary dislocation pairs increase in density and unbind. We discuss both algorithm-dependent and "intrinsic" algorithm-independent computational phase transitions in this setting, the latter of which includes a transition in one's ability to consistently sort atoms into two sublattices to construct a well-defined staggered magnetization.

cond-mat.stat-mech

Motion from Measurement: The Role of Symmetry of Quantum Measurements

In quantum mechanics, measurements are dynamical processes and thus they should be capable of inducing currents. The symmetries of the Hamiltonian and measurement operator provide an organizing principle for understanding the conditions for such currents to emerge. The central role is played by the inversion and time-reversal symmetries. We classify the distinct behaviors that emerge from single and repeated measurements, with and without coupling to a dissipative bath. While the breaking of inversion symmetry alone is sufficient to generate currents through measurements, the breaking of time-reversal symmetry by the measurement operator leads to a dramatic increase in the magnitude of the currents. We consider the dependence on the measurement rate and find that the current is non-monotonic. Furthermore, nondegenerate measurements can lead to current loops within the steady state even in the Zeno limit.

quant-ph

Free electron topological bound state induced by light beam with a twisted wavefront

Recent advances in ultrafast electron emission, microscopy, and diffraction have demonstrated a remarkable ability to manipulate free electrons with quantum coherence using light beams. Here, we present a framework for exploring free electron quantum number in ultrafast electron-light interactions. We derive an explicit Jackiw-Rebbi solution for a low-energy free electron wavefunction subjected to a spatiotemporally twisted laser field, resulting in a flying topologically protected bound state with a quantum number of e/2 - termed a "half-electron". This flying bound state is dispersion-free due to its topological nature. We demonstrate the topological confinement and pair generation mechanism of half-electrons in free space, expanding their domain beyond the topological states typically found in solids and photonics. This advancement enhances our understanding of emulating exotic quantum and topological effects with low-energy free electrons.

quant-ph

Low-energy Free-electron Rabi oscillation and its applications

We propose free-electron Rabi oscillation by creating an isolated two-level system in a synthetic energy space induced by laser. The {\pi}/2-pulse and {\pi}-pulse in synthetic Rabi dynamics can function as 'beam splitters' and 'mirrors' for free-electron interferometry, allowing us to detect local electromagnetic fields and plasmonic excitations. When the coupling field is quantized, we can observe quantum and vacuum Rabi oscillations of the two-level electron, which can be used to investigate the quantum statistics of optical excitations and electron-photon entanglement. Recent advances in laser control of electron microscopes and spectroscopes makes the experimental detection of synthetic Rabi oscillations possible. However, observing the quantum Rabi oscillation of electrons remains challenging. Our work has the potential to advance various fundamentals and applications of resonant light-matter interactions between low-energy electrons and quatum light.

quant-ph

Synthetic dimensions using ultrafast free electrons

We propose a synthetic dimension for ultrafast free electrons based on the discrete energy sidebands in photon-induced near-field electron microscopy (PINEM). The PINEM synthetic dimension can offer a powerful way to coherently shape or modulate free-electron wavefunctions in systems such as ultrafast transmission electron microscopes, dielectric laser accelerators, and quantum free-electron lasers. As examples of this paradigm, we demonstrate Bloch oscillations, diffraction management, and linear optics effects such as Talbot self-imaging in the PINEM lattice. These effects show the potential of PINEM synthetic dimensions as a novel quantum simulation platform.

quant-ph

Phonon-induced modification of quantum criticality

We study the effect of acoustic phonons on the quantum phase transition in the O($N$) model. We develop a renormalization group analysis near (3+1) space-time dimensions and derive the RG equations using an $\epsilon$-expansion. Our results indicate that when the number of flavors of the underlying O($N$) model exceeds a critical number $N_c=4$, the quantum transition remains second-order of the Wilson-Fisher type while, for $N\le 4$, it is a weakly first-order transition. We characterize this weakly first-order transition by a length-scale $\xi^*$, below which the behavior appears to be critical. At finite temperatures for $N\le 4$, a tricritical point separates the weakly first-order and second-order transitions.

cond-mat.str-el

Topological Order in an Antiferomagnetic Tetratic

We study lattice melting in two dimensional antiferromagnets. We argue that, for strong enough magnetic interactions, single lattice dislocations are prohibitive due to magnetic frustration. This leads to a melting scenario in which a tetratic phase, composed of free dislocation pairs and bound disclinations, separates the solid from the liquid phases. We demonstrate this phase numerically in a system of hard spheres confined between parallel plates, where spins are represented by the the heights of the spheres. We find that, in the tetratic phase, the spins are as antiferromagnetically ordered as allowed by their spatial configuration.

cond-mat.stat-mech

Generalized Fresnel-Floquet equations for driven quantum materials

Optical drives at terahertz and mid-infrared frequencies in quantum materials are increasingly used to reveal the nonlinear dynamics of collective modes in correlated many-body systems and their interplay with electromagnetic waves. Recent experiments demonstrated several surprising optical properties of transient states induced by driving, including the appearance of photo-induced edges in the reflectivity in cuprate superconductors, observed both below and above the equilibrium transition temperature. Furthermore, in other driven materials, reflection coefficients larger than unity have been observed. In this paper we demonstrate that unusual optical properties of photoexcited systems can be understood from the perspective of a Floquet system; a system with periodically modulated system parameters originating from pump-induced oscillations of a collective mode. We present a general phenomenological model of reflectivity from Floquet materials, which takes into account parametric generation of excitation pairs. We find a universal phase diagram of drive induced features in reflectivity which evidence a competition between driving and dissipation. To illustrate our general analysis we apply our formalism to two concrete examples motivated by recent experiments: a single plasmon band, which describes Josephson plasmons in layered superconductors, and a phonon-polariton system, which describes upper and lower polaritons in materials such as insulating SiC. Finally we demonstrate that our model can be used to provide an accurate fit to results of phonon-pump - terahertz-probe experiments in the high temperature superconductor $\rm{YBa_2Cu_3O_{6.5}}$. Our model explains the appearance of a pump-induced edge, which is higher in energy than the equilibrium Josephson plasmon edge, even if the interlayer Josephson coupling is suppressed by the pump pulse.

cond-mat.str-el

Multi-scale dynamical symmetries and selection rules in nonlinear optics

Symmetries and their associated selection rules are extremely useful in all fields of science. In particular, for system that include electromagnetic (EM) fields interacting with matter, it has been shown that both of symmetries of matter and EM field's time-dependent polarization play a crucial role in determining the properties of linear and nonlinear responses. The relationship between the system's symmetry and the properties of its excitations facilitate precise control over light emission and enable ultrafast symmetry-breaking spectroscopy of variety of properties. Here. we formulate the first general theory that describes the macroscopic dynamical symmetries (including quasicrystal-like symmetries) of an EM vector field, revealing many new symmetries and selection rules in light-matter interactions. We demonstrate an example of multi-scale selection rules experimentally in the framework of high harmonic generation (HHG). This work waves the way for novel spectroscopic techniques in multi-scale system as well as for imprinting complex structures in EUV-X-ray beams, attosecond pulses, or the interacting medium itself.

physics.optics

Periodic dynamics in superconductors induced by an impulsive optical quench

A number of experiments have evidenced signatures of enhanced superconducting correlations after photoexcitation. Initially, these experiments were interpreted as resulting from quasi-static changes in the Hamiltonian parameters, for example, due to lattice deformations or melting of competing phases. Yet, several recent observations indicate that these conjectures are either incorrect or do not capture all the observed phenomena, which include reflectivity exceeding unity, large shifts of Josephson plasmon edges, and appearance of new peaks in terahertz reflectivity. These observations can be explained from the perspective of a Floquet theory involving a periodic drive of system parameters, but the origin of the underlying oscillations remains unclear. In this paper, we demonstrate that following incoherent photoexcitation, long-lived oscillations are generally expected in superconductors with low-energy Josephson plasmons, such as in cuprates or fullerene superconductor K$_3$C$_{60}$. These oscillations arise from the parametric generation of plasmon pairs due to pump-induced perturbation of the superconducting order parameter. We show that this bi-plasmon response can persist even above the transition temperature as long as strong superconducting fluctuations are present. Our analysis offers a robust framework to understand light-induced superconducting behavior, and the predicted bi-plasmon oscillations can be directly detected using available experimental techniques.

cond-mat.supr-con