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Daniel R. Spiegel

Publications and source records attributed to Daniel R. Spiegel.

2 recordsLinked to original sources

Amplitude Modulation and Relaxation-Oscillation of Counterpropagating Rolls within a Broken-Symmetry Laser-Induced Electroconvection Strip

We report a liquid-crystal pattern-formation experiment in which we break the lateral (translational) symmetry of a nematic medium with a laser-induced thermal gradient. The work is motivated by an improved measurement (reported here) of the temperature dependence of the electroconvection threshold voltage in planar-nematic 4-methoxybenzylidene-4-butylaniline (MBBA). In contrast with other broken-symmetry-pattern studies that report a uniform drift, we observe a strip of counterpropagating rolls that collide at a sink point, and a strong temporally periodic amplitude modulation within a width of 3-4 rolls about the sink point. The time dependence of the amplitude at a fixed position is periodic but displays a nonsinusoidal relaxation-oscillation profile. After reporting experimental results based on spacetime contours and wavenumber profiles, along with a measurement of the change in the drift frequency with applied voltage at a fixed control parameter, we propose some potential guidelines for a theoretical model based on saddle-point solutions for Eckhaus-unstable states and coupled complex Ginzburg-Landau equations. Published in PRE 73, 036317 (2006).

cond-mat.soft

Forced Rayleigh Scattering Studies of Tracer Diffusion in a Nematic Liquid Crystal: The Relevance of Complementary Gratings

We have employed forced Rayleigh scattering (FRS) to study the diffusion of an azo tracer molecule (methyl red) through a nematic liquid crystal (5CB). This system was first investigated in an important study by Hara et al. (Japan. J. Appl. Phys. 23, 1420 [1984]). Since that time, it has become clear that the presence of complementary ground-state and photoproduct FRS gratings can result in nonexponential profiles, and that complementary-grating effects are significant even when "minor" deviations from exponential decay are observed. We have investigated the methyl red/5CB system in order to evaluate the possible effects of complementary gratings. In the isotropic phase, we find that the presence of complementary gratings results in a nonmonotonic FRS signal, which significantly changes the values inferred for the isotropic diffusion coefficients. As a result, the previously reported discontinuity at the nematic/isotropic transition temperature (TNI) is not present in the new data. On the other hand, in the nematic phase, the new experiments largely confirm the previous observations of single-exponential FRS decay and the non-Arrhenius temperature dependence of the nematic diffusion coefficients close to TNI. Finally, we have also observed that the decrease in the diffusion anisotropy with increasing temperature can be correlated with the 5CB nematic order parameter S(T) over the full nematic temperature range.

cond-mat.soft