arXiv subjects

Daniel Suchet

Publications and source records attributed to Daniel Suchet.

13 recordsLinked to original sources

arXiv2026

R{\'e}flexions sur la puissance motrice du Soleil

A quintessential source of heat, the Sun radiates toward the Earth a power ten thousand times greater than humanity's energy needs. Harnessing this energy bounty, however, requires capturing and converting sunlight. Today, this conversion can be achieved through several families of technologies at varying stages of maturity: photovoltaic solar, thermal, concentrated solar power, and more. While their applications differ, all these technologies must meet common fundamental constraints, and as Carnot proposed, one can 'consider in all its generality the principle of producing motion through heat' from the Sun. However, unlike traditional 'heat engines,' the coupling with the hot source here is radiative, introducing specific constraints that must be accounted for. In this presentation dedicated to radiative machines, you will encounter familiar terms as well as particular expressions that will provide the keys to understanding solar technologies

physics.pop-ph↗

arXiv2023

The Role of Nonequilibrium LO Phonons, Pauli Exclusion, and Intervalley Pathways on the Relaxation of Hot Carriers in InGaAs Multi-Quantum-Well Structures

Under continuous-wave laser excitation in an InGaAs multi-quantum-well (MQW) structure, the carrier temperature extracted from photoluminescence rises faster for 405 nm excitation compared with 980 nm excitation, as the injected carrier density increases. Ensemble Monte Carlo simulation of the carrier dynamics in the MQW system shows that this carrier temperature rise is dominated by nonequilibrium LO phonon effects, with the Pauli exclusion having a significant effect at high carrier densities. Further, we find a significant fraction of carriers reside in the satellite L-valleys for 405 nm excitation due to strong intervalley transfer, leading to a cooler steady-state electron temperature in the central valley compared with the case when intervalley transfer is excluded from the model. Good agreement between experiment and simulation has been shown, and a detailed analysis has been presented. This study expands our knowledge of the dynamics of the hot carrier population in semiconductors, which can be applied to further limit energy loss in solar cells.

cond-mat.mes-hall↗

arXiv2022

Applicability of Hubbert model to global mining industry: Interpretations and insights

The Hubert's model has been introduced in 1956 as a phenomenological description of the time evolution of US oil fields production. It has since then acquired a vast notoriety as a conceptual approach to resource depletion. It is often invoked nowadays in the context of the energy transition to question the limitations induced by the finitude of mineral stocks. Yet, its validity is often controversial despite its popularity. This paper offers a pedagogical introduction to the model, assesses its ability to describe the current evolution of 20 mining elements, and discusses the nature and robustness of conclusions drawn from Hubbert's model considered either as a for cast or as a foresight tool. We propose a novel way to represent graphically these conclusions as a "Hubbert's map" which offers direct visualization of their main features.

physics.soc-ph↗

arXiv2022

Enhancement of Hot Carrier Effects and Signatures of Confinement in Terms of Thermalization Power in Quantum Well Solar Cells

A theoretical model using electron-phonon scattering rate equations is developed for assessing carrier thermalization under steady-state conditions in two-dimensional systems. The model is applied to investigate the hot carrier effect in III-V hot-carrier solar cells with a quantum well absorber. The question underlying the proposed investigation is: what is the power required to maintain two populations of electron and hole carriers in a quasi-equilibrium state at fixed temperatures and quasi-Fermi level splitting? The obtained answer is that the thermalization power density is reduced in two-dimensional systems compared to their bulk counterpart, which demonstrates a confinement-induced enhancement of the hot carrier effect in quantum wells. This power overall increases with the well thickness, and it is moreover shown that the intra-subband contribution dominates at small thicknesses while the inter-subband contribution increases with thickness and dominates in the bulk limit. Finally, the effects of the thermodynamic state of phonons and screening are clarified. In particular, the two-dimensional thermalization power density exhibits a non-monotonic dependence on the thickness of the quantum well layer, when both out-of-equilibrium longitudinal optical phonons and screening effects are taken into account. Our theoretical and numerical results provide tracks to interpret intriguing experimental observations in quantum well physics. They will also offer guidelines to increase the yield of photovoltaic effect based on the hot carrier effect using quantum well heterostructures, a result critical to the research toward high-efficiency solar cell devices.

cond-mat.mes-hall↗

arXiv2021

Impact of excitation energy on hot carrier properties in InGaAs MQW structure

Hot carrier solar cells aim to overcome the theoretical limit of single-junction photovoltaic devices by suppressing the thermalization of hot carriers and extracting them through energy selective contacts. Designing efficient hot carrier absorbers requires further investigation on hot carrier properties in materials. Although the thermalization of hot carriers is responsible for a large portion of energy loss in solar cells, it is still one of the least understood phenomena in semiconductors. Here, the impact of excitation energy on the properties of photo-generated hot carriers in an InGaAs multi-quantum well (MQW) structure at various lattice temperatures and excitation powers is studied. Photoluminescence (PL) emission of the sample is detected by a hyperspectral luminescence imager, which creates spectrally and spatially resolved PL maps. The thermodynamic properties of hot carriers, such as temperature and quasi-Fermi level splitting, are carefully determined via applying full PL spectrum fitting, which solves the Fermi-Dirac integral and considers the band-filling effect in the nanostructured material. In addition, the impact of thermalized power density and carrier scattering with longitudinal optical phonons on the spectral linewidth broadening under two excitation energies is studied.

physics.app-ph↗

arXiv2019

Quasi-thermalization of collisionless particles in quadrupole potentials

We analyze several puzzling features of a recent experiment with a noninteracting gas of atoms in a quadrupole trap. After an initial momentum kick, the system reaches a stationary, quasi-thermal state even without collisions, due to the dephasing of individual particle trajectories. Surprisingly, the momentum distribution remains anisotropic at long times, characterized by different "temperatures" along the different directions. In particular, there is no transfer of the kick energy between the axial and radial trap directions. To understand these effects we discuss and solve two closely related models: a spherically symmetric trap $V(r)\simeq r^\alpha$ and a strongly confined gas along one direction (a "pancake" trap). We find that in the isotropic trap, the gas unexpectedly also preserves the anisotropy of the kick at long times, which we are able to explain using the conservation of angular momentum and the virial theorem. Depending on the value of $\alpha$ we find that the kick can cool or heat the orthogonal directions. The pancake trap case is quantitatively similar to the quadrupole one. We show that for the former, the temperature anisotropy and memory of the kick direction are due to the change in the 2D effective potential resulting from the kick, thereby also explaining the quadrupole experimental results.

cond-mat.quant-gas↗

arXiv2019

Impact of electron-phonon scattering on optical properties of CH$_3$NH$_3$PbI$_3$ hybrid perovskite material

We investigate numerically the impact of the electron-phonon scattering on the optical properties of a perovskite material (CH3NH3PbI3). Using non-equilibrium Green functions formalism, we calculate the local density-of-states for several values of the electron-phonon scattering strength as well as in the case of ballistic transport. We report an Urbach-like penetration of the density-of-states in the bandgap due to scattering. The density-of-states expands deeper in the bandgap with the scattering strength. We determine the electronic current contributions relative to photon absorption and photon emission. This allows to estimate the Urbach energy from the absorption coefficient below the bandgap. Values of Urbach energy up to 9.5 meV are obtained, meaning that scattering contribution to the total experimental Urbach energy of 15meV is quite important. The Urbach tail is generally attributed to the disorder of the system, leaving hope for further improvement. Yet, we show in this work that a significant contribution to the Urbach tail comes from carriers-phonon interactions, an intrinsic properties of the material which thus set a lower bound on the improvement margin. Finally, we estimate the open-circuit voltage Voc for a solar cell assuming such a material as an absorber. Voc losses increase with the scattering strength, up to 41 mV. This study then confirms that scattering of electrons in perovskite material modifies the optical behaviour.

cond-mat.mes-hall↗

arXiv2018

Voltage preservation in Intermediate Band Solar Cells

Intermediate Band Solar Cell is an advanced concept for solar energy conversion in which two low-energy photons can promote an electron to the conduction band through a so-called intermediate band. To limit recombination and preserve the photo-generated voltage, generation to- and from the intermediate band should be matched. However, all practical realizations experienced a significant voltage degradation as compared to a single junction without intermediate band. In this work, we develop a novel analytical optimization method based on Lagrange multipliers. We demonstrate that an Intermediate Band Solar Cell under solar spectrum cannot meet voltage preservation and current matching at the same time. By contrast, we show that the implementation of an energy shift (\emph{electronic ratchet}) in any of the bands allows those two criteria to be filled simultaneously. Additional insights are provided by the numerical study of the short circuit current and fill factor of the systems at stake, which show that a system with ratchet benefits from the same current increase as a standard Intermediate Band Solar Cell (same short-circuit current), while maintaining I-V properties of a single junction (same open-voltage circuit, same fill factor).

physics.app-ph↗

arXiv2018

Beneficial impact of tunneling in nano-structured intermediate-band solar cell

Using the non equilibrium Green functions formalism we propose a study of the electronic excitation and collection in nano-structured intermediate-band solar cell. We demonstrate that a thin tunnel barrier between the nano-objects and the host material is beneficial for both current and voltage. For the current, the confinement generated by such a thin barrier favors the intersubband optical coupling in the nano-objects and then improves the excitation-collection trade-off. We also show that a broadened density-of-state in the nano-objects increases the radiative recombination and then degrades the voltage. Using a detailed balance model we propose a broadening factor for this Voc degradation which decreases when a tunnel barrier enhances the life-time in the nano-objects.

physics.app-ph↗

arXiv2018

An electronic ratchet is required in nanostructured intermediate band solar cells

We investigate in this letter the intrinsic properties that have limited the efficiency of nanostructured intermediate band solar cells. Those devices take advantage of intra-band transitions, which occur on narrow energy width, and present low radiative recombination efficiency. We derive the minimum requirements in terms of those two characteristics to achieve efficiencies in excess of the Shockley-Queisser limit, and show that compatible nanostructures are challenging to obtain. Especially, we evidence that currently experimentally considered materials cannot overcome the best single junction cells. In order to solve those issues, we consider devices including an electronic ratchet mechanism. Firstly, such devices are shown to be much less sensitive on the limitations of the nanostructures characteristics, so that requirements for high efficiencies can be met. Secondly, we show that quantum well devices present advantages over their quantum dots counterparts, although they have attracted much less interest so far.

physics.app-ph↗

arXiv2017

Long range mediated interactions in a mixed dimensional system

We present a mixed-dimensional atomic gas system to unambiguously detect and systematically probe mediated interactions. In our scheme, fermionic atoms are confined in two parallel planes and interact via exchange of elementary excitations in a three-dimensional background gas. This interaction gives rise to a frequency shift of the out-of-phase dipole oscillations of the two clouds, which we calculate using a strong coupling theory taking the two-body mixed-dimensional scattering into account exactly. The shift is shown to be easily measurable for strong interactions and can be used as a probe for mediated interactions.

cond-mat.quant-gas↗

arXiv2016

Analog Simulation of Weyl Particles with Cold Atoms

We study theoretically, numerically, and experimentally the relaxation of a collisionless gas in a quadrupole trap after a momentum kick. The non-separability of the potential enables a quasi thermalization of the single particle distribution function even in the absence of interactions. Suprinsingly, the dynamics features an effective decoupling between the strong trapping axis and the weak trapping plane. The energy delivered during the kick is redistributed according to the symmetries of the system and satisfies the Virial theorem, allowing for the prediction of the final temperatures. We show that this behaviour is formally equivalent to the relaxation of massless relativistic Weyl fermions after a sudden displacement from the center of a harmonic trap.

cond-mat.quant-gas↗

arXiv2015

Simultaneous sub-Doppler laser cooling of fermionic $^6$Li and $^{40}$K on the D$_1$ line: Theory and Experiment

We report on simultaneous sub-Doppler laser cooling of fermionic $^6$Li and $^{40}$K using the D$_1$ optical transitions. We compare experimental results to a numerical simulation of the cooling process applying a semi-classical Monte Carlo wavefunction method. The simulation takes into account the three dimensional optical molasses setup and the dipole interaction between atoms and the bichromatic light field driving the D$_1$ transitions. We discuss the physical mechanisms at play, we identify the important role of coherences between the ground state hyperfine levels and compare D$_1$ and D$_2$ sub-Doppler cooling. In 5 ms, the D$_1$ molasses phase largely reduces the temperature for both $^6$Li and $^{40}$K at the same time, with a final temperature of 44 $μ$K and 11 $μ$K, respectively. For both species this leads to a phase-space density close to $10^{-4}$. These conditions are well suited to directly load an optical or magnetic trap for efficient evaporative cooling to quantum degeneracy.

physics.atom-ph↗