arXiv subjects

Daniel W. Savin

Publications and source records attributed to Daniel W. Savin.

At least 19 recordsLinked to original sources

arXiv2026

A Point-Spread Function for the Extreme Ultraviolet High-Resolution Imager on board Solar Orbiter

We present the point-spread function (PSF) of the Extreme Ultraviolet High-Resolution Imager (HRIEUV) onboard Solar Orbiter, which observes the Sun at 174 Angstrom. This PSF provides a quantitative description of light diffracted by the mesh and mounting supporting the entrance filter, light diffracted by the mesh supporting the filter-wheel filter, as well as light that is diffusely scattered by the microroughness of the mirrors. Deconvolution with this PSF corrects the images for instrumental scattered light, substantially improving image quality and photometric accuracy. First, we determine the diffraction component of the PSF from mechanical drawings of the instrument. We find that 26% of the incoming light is diffracted, predominantly by the entrance-filter mounting and mesh. Second, we fit the diffuse scattered light using partial image occultations during the 2023-Jan-03 Mercury transit. We find that the diffuse scattered light is well described by a softened power law, which scatters 42% of light over the detector. Combined, 57% of the incoming light is redistributed over the detector by diffraction and scattering. Correcting for these effects markedly enhances the dynamic range and contrast of the observations. The intensity in bright structures intensifies by up to 40% and the intensity in dark structures decreases by up to 85 %. All images features become much clearer, facilitating a more precise scientific analysis of HRIEUV observations.

astro-ph.SR↗

arXiv2026

Theoretical Ion Sputtering Yields from Loose Powders using a Multiscale Monte Carlo Approach

Ion sputtering from loose powders remains poorly understood despite its relevance to planetary science and industry. We developed a multiscale Monte Carlo model to simulate sputtering from powders, using a higher-fidelity approach for the target geometry compared to voxel-based methods. Simulating Kr+ ions impacting Cu powders and flat slabs, we show that sputtering from loose powders differs markedly from that of flat slabs or rough surfaces. The main differences are: (1) for incident angles a > 0 degree relative to the bulk normal, the escaping sputtering yield is dominated by backward-directed ejecta for all ion energies; (2) for a < 60 degrees, the yield peaks toward the ion-beam origin, similar to the opposition effect seen in optical observations of airless bodies; (3) the angular distribution peak is half or less than that of a flat slab; (4) as ion energy increases, no evolution occurs from primary to secondary knock-on sputtering in the ejecta angular distribution. We attribute these behaviors to the powders interconnected voids. Ions penetrate these voids and sputter underlying grains; the ejecta then preferentially escape toward the ion-beam origin, where shadowing is minimal. We derive two fitting functions: 1) relating the escaping sputtering yield of a powder to that of a flat surface, depending only on porosity, incident angle, mean local incidence angle, and the corresponding flat slab yield; 2) providing the double-differential angular distribution of the escaping ejecta for porosities > 0.49. These provide a potentially universal fitting function of the absolute doubly-differential escaping sputtering yield from loose powders.

physics.app-ph↗

arXiv2025

Formation of a Coronal Hole by a quiet-Sun Filament Eruption

A coronal hole formed as a result of a quiet-Sun filament eruption close to the solar disk center on 2014 June 25. We studied this formation using images from the Atmospheric Imaging Assembly (AIA), magnetograms from the Helioseismic and Magnetic Imager (HMI), and a differential emission measure (DEM) analysis derived from the AIA images. The coronal hole developed in three stages: (1) formation, (2) migration, and (3) stabilization. In the formation phase, the emission measure (EM) and temperature started to decrease six hours before the filament erupted. Then, the filament erupted and a large coronal dimming formed over the following three hours. Subsequently, in a phase lasting $15.5$~hours, the coronal dimming migrated by 150" from its formation site to a location where potential field source surface extrapolations indicate the presence of open magnetic field lines, marking the transition into a coronal hole. During this migration, the coronal hole drifted across quasi-stationary magnetic elements in the photosphere, implying the occurrence of magnetic interchange reconnection at the boundaries of the coronal hole. In the stabilization phase, the magnetic properties and area of the coronal hole became constant. The EM of the coronal hole decreased, which we interpret as a reduction in plasma density due to the onset of plasma outflow into interplanetary space. As the coronal hole rotated towards the solar limb, it merged with a nearby pre-existing coronal hole. At the next solar rotation, the coronal hole was still apparent, indicating a lifetime of >1 solar rotation.

astro-ph.SR↗

arXiv2025

Elemental Abundances at Coronal Hole Boundaries as a Means to Investigate Interchange Reconnection and the Solar Wind

The origin of the slow solar wind is not well understood, unlike the fast solar wind which originates from coronal holes. In-situ elemental abundances of the slow solar wind suggest that it originates from initially closed field lines that become open. Coronal hole boundary regions are a potential source of slow solar wind as there open field lines interact with the closed loops through interchange reconnection. Our primary aim is to quantify the role of interchange reconnection at the boundaries of coronal holes. To this end, we have measured the relative abundances of different elements at these boundaries. Reconnection is expected to modulate the relative abundances through the first ionization potential (FIP) effect. For our analysis we used spectroscopic data from the extreme ultraviolet imaging spectrometer (EIS) on board Hinode. To account for the temperature structure of the observed region we computed the differential emission measure (DEM). Using the DEM we were able to infer the ratio between coronal and photospheric abundances, known as the FIP bias. By examining the variation of the FIP bias moving from the coronal hole to the quiet Sun, we have been able to constrain models of interchange reconnection. The FIP bias variation in the boundary region around the coronal hole has an approximate width of 30-50 Mm, comparable to the size of supergranules. This boundary region is also a source of open flux into interplanetary space. We find that there is an additional ~30% open flux that originates from this boundary region.

astro-ph.SR↗

arXiv2024

High-Resolution Laboratory Measurements of M-shell Fe EUV Line Emission using EBIT-I

Solar physicists routinely utilize observations of Ar-like Fe IX and Cl-like Fe X emission to study a variety of solar structures. However, unidentified lines exist in the Fe IX and Fe X spectra, greatly impeding the spectroscopic diagnostic potential of these ions. Here, we present measurements using the Lawrence Livermore National Laboratory EBIT-I electron beam ion trap in the wavelength range 238-258 A. These studies enable us to unambiguously identify the charge state associated with each of the observed lines. This wavelength range is of particular interest because it contains the Fe IX density diagnostic line ratio 241.74 A/244.91 A, which is predicted to be one of the best density diagnostics of the solar corona, as well as the Fe X 257.26 A magnetic-field-induced transition. We compare our measurements to the Fe IX and Fe X lines tabulated in CHIANTI v10.0.1, which is used for modeling the solar spectrum. In addition, we have measured previously unidentified Fe X lines that will need to be added to CHIANTI and other spectroscopic databases.

astro-ph.SR↗

arXiv2024

Dissociative recombination of rotationally cold ArH$^+$

We have experimentally studied dissociative recombination (DR) of electronically and vibrationally relaxed ArH$^+$ in its lowest rotational levels, using an electron--ion merged-beams setup at the Cryogenic Storage Ring. We report measurements for the merged-beams rate coefficient of ArH$^+$ and compare it to published experimental and theoretical results. In addition, by measuring the kinetic energy released to the DR fragments, we have determined the internal state of the DR products after dissociation. At low collision energies, we find that the atomic products are in their respective ground states, which are only accessible via non-adiabatic couplings to neutral Rydberg states. Published theoretical results for ArH$^+$ have not included this DR pathway. From our measurements, we have also derived a kinetic temperature rate coefficient for use in astrochemical models.

physics.atom-ph↗

arXiv2023

Absolute Doubly Differential Angular Sputtering Yields for 20 keV Kr+ on Polycrystalline Cu

We have measured the absolute doubly differential angular sputtering yield for 20 keV Kr+ impacting a polycrystalline Cu slab at an incidence angle of θi = 45° relative to the surface normal. Sputtered Cu atoms were captured using collectors mounted on a half dome above the sample, and the sputtering distribution was measured as a function of the sputtering polar, θs, and azimuthal, phi, angles. Absolute results of the sputtering yield were determined from the mass gain of each collector, the ion dose, and the solid angle subtended, after irradiation to a total fluence of ~ 1 x 10^18 ions/cm^2. Our approach overcomes shortcomings of commonly used methods that only provide relative yields as a function of θs in the incidence plane (defined by the ion velocity and the surface normal). Our experimental results display an azimuthal variation that increases with increasing θs and is clearly discrepant with simulations using binary collision theory. We attribute the observed azimuthal anisotropy to ion-induced formation of micro- and nano-scale surface features that suppress the sputtering yield through shadowing and redeposition effects, neither of which are accounted for in the simulations. Our experimental results demonstrate the importance of doubly differential angular sputtering studies to probe ion sputtering processes at a fundamental level and to explore the effect of ion-beam-generated surface roughness.

physics.app-ph↗

arXiv2023

Automated Graph-Based Detection of Quantum Control Schemes: Application to Molecular Laser Cooling

One of the demanding frontiers in ultracold quantum science is identifying laser cooling schemes for complex atoms and molecules out of their vast spectra of internal states. Motivated by the prospect of expanding the set of available ultracold molecules for applications in fundamental physics, chemistry, astrochemistry, and quantum simulation, we propose and demonstrate an automated graph-based search approach for viable laser cooling schemes. The method is time efficient, reproduces the results of previous manual searches, and reveals a plethora of new potential laser cooling schemes. We discover laser cooling schemes for YO, C$_2$, OH$^+$, CN, and CO$_2$, including surprising schemes that start from highly excited states or do not rely on a strong main transition. A central insight of this work is that the reinterpretation of quantum states and transitions between them as a graph can dramatically enhance the ability to identify new quantum control schemes for complex quantum systems. As such, this approach will also apply to complex atoms and, in fact, any complex many-body quantum system with a discrete spectrum of internal states.

quant-ph↗

arXiv2023

Dissociative Recombination of Rotationally Cold OH$^+$ and Its Implications for the Cosmic Ray Ionization Rate in Diffuse Clouds

Observations of OH$^+$ are used to infer the interstellar cosmic ray ionization rate in diffuse atomic clouds, thereby constraining the propagation of cosmic rays through and the shielding by interstellar clouds, as well as the low energy cosmic ray spectrum. In regions where the H$_2$ to H number density ratio is low, dissociative recombination (DR) is the dominant destruction process for OH$^+$ and the DR rate coefficient is important for predicting the OH$^+$ abundance and inferring the cosmic ray ionization rate. We have experimentally studied DR of electronically and vibrationally relaxed OH$^+$ in its lowest rotational levels, using an electron--ion merged-beams setup at the Cryogenic Storage Ring. From these measurements, we have derived a kinetic temperature rate coefficient applicable to diffuse cloud chemical models, i.e., for OH$^+$ in its electronic, vibrational, and rotational ground level. At typical diffuse cloud temperatures, our kinetic temperature rate coefficient is a factor of $\sim 5$ times larger than the previous experimentally derived value and a factor of $\sim 33$ times larger than the value calculated by theory. Our combined experimental and modelling results point to a significant increase for the cosmic ray ionization rate inferred from observations of OH$^+$ and H$_2$O$^+$, corresponding to a geometric mean of $(6.6 \pm 1.0) \times 10^{-16}\,\mathrm{s}^{-1}$, which is more than a factor of two larger than the previously inferred values of the cosmic ray ionization rate in diffuse atomic clouds. Combined with observations of diffuse and dense molecular clouds, these findings indicate a greater degree of cosmic ray shielding in interstellar clouds than has been previously inferred.

astro-ph.GA↗

arXiv2023

Laser Scheme for Doppler Cooling of the Hydroxyl Cation (OH$^+$)

We report on a cycling scheme for Doppler cooling of trapped OH$^+$ ions using transitions between the electronic ground state $X^3Σ^-$ and the first excited triplet state $A^3Π$. We have identified relevant transitions for photon cycling and repumping, have found that coupling into other electronic states is strongly suppressed, and have calculated the number of photon scatterings required to cool OH$^+$ to a temperature where Raman sideband cooling can take over. In contrast to the standard approach, where molecular ions are sympathetically cooled, our scheme does not require co-trapping of another species and opens the door to the creation of pure samples of cold molecular ions with potential applications in quantum information, quantum chemistry, and astrochemistry. The laser cooling scheme identified for OH$^+$ is efficient despite the absence of near-diagonal Franck-Condon factors, suggesting that broader classes of molecules and molecular ions are amenable to laser cooling than commonly assumed.

physics.atom-ph↗

arXiv2022

Experimental determination of the dissociative recombination rate coefficient for rotationally-cold CH$^{+}$ and its implications for the diffuse cloud chemistry

Observations of CH$^+$ are used to trace the physical properties of diffuse clouds, but this requires an accurate understanding of the underlying CH$^+$ chemistry. Until this work, the most uncertain reaction in that chemistry was dissociative recombination (DR) of CH$^+$. Using an electron-ion merged-beams experiment at the Cryogenic Storage Ring, we have determined the DR rate coefficient of the CH$^+$ electronic, vibrational, and rotational ground state applicable for different diffuse cloud conditions. Our results reduce the previously unrecognized order-of-magnitude uncertainty in the CH$^+$ DR rate coefficient to $\sim \pm 20\%$ and are applicable at all temperatures relevant to diffuse clouds, ranging from quiescent gas to gas locally heated by processes such as shocks and turbulence. Based on a simple chemical network, we find that DR can be an important destruction mechanism at temperatures relevant to quiescent gas. As the temperature increases locally, DR can continue to be important up to temperatures of $ \sim 600\,\mathrm{K} $ if there is also a corresponding increase in the electron fraction of the gas. Our new CH$^+$ DR rate coefficient data will increase the reliability of future studies of diffuse cloud physical properties via CH$^+$ abundance observations.

astro-ph.GA↗

arXiv2021

Laser Cooling Scheme for the Carbon Dimer ($^{12}$C$_2$)

We report on a scheme for laser cooling of $^{12}$C$_2$. We have calculated the branching ratios for cycling and repumping transitions and calculated the number of photon scatterings required to achieve deflection and laser cooling of a beam of $C_2$ molecules under realistic experimental conditions. Our results demonstrate that C$_2$ cooling using the Swan ($d^3Π_\text{g} \leftrightarrow a^3Π_\text{u}$) and Duck ($d^3Π_\text{g} \leftrightarrow c^3Σ_\text{u}^+$) bands is achievable via techniques similar to state-of-the-art molecular cooling experiments. The Phillips ($A^1Π_\text{u} \leftrightarrow X^1Σ_\text{g}^+$) and Ballik-Ramsay ($b^3Σ_\text{g}^- \leftrightarrow a^3Π_\text{u}$) bands offer the potential for narrow-line cooling. This work opens up a path to cooling of molecules with carbon-carbon bonds and may pave the way toward quantum control of organic molecules.

physics.atom-ph↗

arXiv2019

Astro 2020: Astromineralogy of interstellar dust with X-ray spectroscopy

X-ray absorption fine structure (XAFS) in the 0.2-2 keV band is a crucial component in multi-wavelength studies of dust mineralogy, size, and shape -- parameters that are necessary for interpreting astronomical observations and building physical models across all fields, from cosmology to exoplanets. Despite its importance, many fundamental questions about dust remain open. What is the origin of the dust that suffuses the interstellar medium (ISM)? Where is the missing interstellar oxygen? How does iron, predominantly produced by Type Ia supernovae, become incorporated into dust? What is the main form of carbon in the ISM, and how does it differ from carbon in stellar winds? The next generation of X-ray observatories, employing microcalorimeter technology and $R \equiv λ/Δλ\geq 3000$ gratings, will provide pivotal insights for these questions by measuring XAFS in absorption and scattering. However, lab measurements of mineralogical candidates for astrophysical dust, with R > 1000, are needed to fully take advantage of the coming observations.

astro-ph.EP↗

arXiv2019

Experimental and theoretical studies of D + H$_3^+$ $\rightarrow$ H$_2$D$^+$ + H

Deuterated molecules are important chemical tracers of prestellar and protostellar cores. Up to now, the titular reaction has been assumed to contribute to the generation of these deuterated molecules. We have measured the merged-beams rate coefficient for this reaction as function of the relative collision energy in the range of about 10 meV to 10 eV. By varying the internal temperature of the reacting H$_3^+$ molecules, we found indications for the existence of a reaction barrier. We have performed detailed theoretical calculations for the zero-point-corrected energy profile of the reaction and determined a new value for the barrier height of $\approx$ 68 meV. Furthermore, we have calculated the tunneling probability through the barrier. Our experimental and theoretical results show that the reaction is essentially closed at astrochemically relevant temperatures. We derive a thermal rate coefficient of $<1\times 10^{-12}$ cm$^3$ s$^{-1}$ for temperatures below 75 K with tunneling effects included and below 155 K without tunneling.

astro-ph.IM↗

arXiv2018

Spectroscopic Measurements of the Ion Velocity Distribution at the Base of the Fast Solar Wind

In situ measurements of the fast solar wind reveal non-thermal distributions of electrons, protons and, minor ions extending from $0.3$ AU to the heliopause. The physical mechanisms responsible for these non-thermal properties and the location where these properties originate remain open questions. Here we present spectroscopic evidence, from extreme ultraviolet spectroscopy, that the velocity distribution functions (VDFs) of minor ions are already non-Gaussian at the base of the fast solar wind in a coronal hole, at altitudes of $< 1.1 R_{\odot}$. Analysis of Fe, Si, and Mg spectral lines reveal a peaked line-shape core and broad wings that can be characteristed by a kappa VDF. A kappa distribution fit gives very small kappa indices off-limb of $κ\approx1.9-2.5$, indicating either (a) ion populations far from thermal equilibrium, (b) fluid motions such as non-Gaussian turbulent fluctuations or non-uniform wave motions, or (c) some combination of both. These observations provide important empirical constraints for the source region of the fast solar wind and for the theoretical models of the different acceleration, heating, and energy deposition processes therein. To the best of our knowledge, this is the first time that the ion VDF in the fast solar wind has been probed so close to its source region. The findings are also a timely precursor to the upcoming 2018 launch of the Parker Solar Probe, which will provide the closest in situ measurements of the solar wind at approximately $0.04$ AU ($8.5$ solar radii).

astro-ph.SR↗

arXiv2017

On the Energetics of the HCO$^+$ + C $\to$ CH$^+$ + CO Reaction and Some Astrochemical Implications

We explore the energetics of the titular reaction, which current astrochemical databases consider open at typical dense molecular (i.e., dark) cloud conditions. As is common for reactions involving the transfer of light particles, we assume that there are no intersystem crossings of the potential energy surfaces involved. In the absence of any such crossings, we find that this reaction is endoergic and will be suppressed at dark cloud temperatures. Updating accordingly a generic astrochemical model for dark clouds changes the predicted gas-phase abundances of 224 species by greater than a factor of 2. Of these species, 43 have been observed in the interstellar medium. Our findings demonstrate the astrochemical importance of determining the role of intersystem crossings, if any, in the titular reaction.

astro-ph.GA↗

arXiv2013

Observational Quantification of the Energy Dissipated by Alfvén Waves in a Polar Coronal Hole: Evidence that Waves Drive the Fast Solar Wind

We present a measurement of the energy carried and dissipated by Alfvén waves in a polar coronal hole. Alfvén waves have been proposed as the energy source that heats the corona and drives the solar wind. Previous work has shown that line widths decrease with height in coronal holes, which is a signature of wave damping, but have been unable to quantify the energy lost by the waves. This is because line widths depend on both the non-thermal velocity v_nt and the ion temperature T_i. We have implemented a means to separate the T_i and v_nt contributions using the observation that at low heights the waves are undamped and the ion temperatures do not change with height. This enables us to determine the amount of energy carried by the waves at low heights, which is proportional to v_nt. We find the initial energy flux density present was 6.7 +/- 0.7 x 10^5 erg cm^-2 s^-1, which is sufficient to heat the coronal hole and acccelerate the solar wind during the 2007 - 2009 solar minimum. Additionally, we find that about 85% of this energy is dissipated below 1.5 R_sun, sufficiently low that thermal conduction can transport the energy throughout the coronal hole, heating it and driving the fast solar wind. The remaining energy is roughly consistent with what models show is needed to provide the extended heating above the sonic point for the fast solar wind. We have also studied T_i, which we found to be in the range of 1 - 2 MK, depending on the ion species.

astro-ph.SR↗

arXiv2005

Cosmological Implications of the Uncertainty in H- Destruction Rate Coefficients

In primordial gas, molecular hydrogen forms primarily through associative detachment of H- and H, thereby destroying the H-. The H- anion can also be destroyed by a number of other reactions, most notably by mutual neutralization with protons. However, neither the associative detachment nor the mutual neutralization rate coefficients are well determined: both may be uncertain by as much as an order of magnitude. This introduces a corresponding uncertainty into the H2 formation rate, which may have cosmological implications. Here, we examine the effect that these uncertainties have on the formation of H2 and the cooling of protogalactic gas in a variety of situations. We show that the effect is particularly large for protogalaxies forming in previously ionized regions, affecting our predictions of whether or not a given protogalaxy can cool and condense within a Hubble time, and altering the strength of the ultraviolet background that is required to prevent collapse.

astro-ph↗