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Daniel Wirtitsch

Publications and source records attributed to Daniel Wirtitsch.

5 recordsLinked to original sources

Exploiting ionization dynamics in the nitrogen vacancy center for rapid, high-contrast spin and charge state initialization

We propose and experimentally demonstrate a method to strongly increase the sensitivity of spin measurements on nitrogen-vacancy (NV) centers in diamond, which can be readily implemented in existing quantum sensing experiments. While charge state transitions of this defect are generally considered a parasitic effect to be avoided, we show here that these can be used to significantly increase the NV center's spin contrast, a key quantity for high sensitivity magnetometry and high fidelity state readout. The protocol consists of a two-step procedure, in which the charge state of the defect is first purified by a strong laser pulse, followed by weak illumination to obtain high spin polarization. We observe a relative improvement of the readout contrast by 17 %, and infer a reduction of the initialization error of more than 50 %. The contrast enhancement is accompanied by a beneficial increase of the readout signal. For long sequence durations, typically encountered in high-resolution magnetometry, a measurement speedup by a factor of >1.5 is extracted, and we find that the technique is beneficial for sequences of any duration. Additionally, our findings give detailed insight into the charge and spin polarization dynamics of the NV center, and provide actionable insights for direct optical, spin-to-charge, and electrical readout of solid-state spin centres.

quant-ph

Microelectronic readout of a diamond quantum sensor

Quantum sensors based on the nitrogen-vacancy (NV) centre in diamond are rapidly advancing from scientific exploration towards the first generation of commercial applications. While significant progress has been made in developing suitable methods for the manipulation of the NV centre spin state, the detection of the defect luminescence has so far limited the performance of miniaturized sensor architectures. The recent development of photoelectric detection of the NV centre's spin state offers a path to circumvent these limitations, but has to-date required research-grade low current amplifiers to detect the picoampere-scale currents obtained from these systems. Here we report on the photoelectric detection of magnetic resonance (PDMR) with NV ensembles using a complementary metal-oxide semiconductor (CMOS) device. The integrated circuit delivers a digitized output of the diamond sensor with low noise and 50 femtoampere resolution. This integration provides the last missing component on the path to a compact, diamond-based quantum sensor. The device is suited for continuous wave (CW) as well as pulsed operation. We demonstrate its functionality with DC and AC magnetometry up to several megahertz, coherent spin rotation and multi-axial decoupling sequences for quantum sensing.

quant-ph

Room-temperature control and electrical readout of individual nitrogen-vacancy nuclear spins

Nuclear spins in semiconductors are leading candidates for quantum technologies, including quantum computation, communication, and sensing. Nuclear spins in diamond are particularly attractive due to their extremely long coherence lifetime. With the nitrogen-vacancy (NV) centre, such nuclear qubits benefit from an auxiliary electronic qubit, which has enabled entanglement mediated by photonic links. The transport of quantum information by the electron itself, via controlled transfer to an adjacent centre or via the dipolar interaction, would enable even faster and smaller processors, but optical readout of arrays of such nodes presents daunting challenges due to the required sub-diffraction inter-site distances. Here, we demonstrate the electrical readout of a basic unit of such systems - a single 14N nuclear spin coupled to the NV electron. Our results provide the key ingredients for quantum gate operations and electrical readout of nuclear qubit registers, in a manner compatible with nanoscale electrode structures. This demonstration is therefore a milestone towards large-scale diamond quantum devices with semiconductor scalability.

cond-mat.mes-hall

Scalable spin-photon entanglement by time-to-polarization conversion

Spin-photon interfaces are strong candidates for building blocks of future quantum networks and quantum computers. Several systems currently under examination present promising features, but none of them yet fulfil all requirements for these aims. A particularly attractive strategy for the realization of these applications is the creation of strings of entangled photons, where quantum correlations among the photons are mediated by operations on the spin of the emitter. Here, we demonstrate for the first time the creation of spin-photon entanglement within the fundamental unit of a novel, scalable protocol based on time-to-polarization conversion. This principle allows us to bypass many of the imperfections of currently available photon sources and can therefore be utilized with a large variety of emitters. We execute the protocol using a nitrogen-vacancy centre in diamond, which possesses a long coherence lifetime and multiple spin degrees of freedom, thereby offering an outlook towards the creation of large entangled states.

quant-ph

Collective Strong Coupling with Homogeneous Rabi Frequencies using a 3D Lumped Element Microwave Resonator

We design and implement 3D lumped element microwave cavities for the coherent and uniform coupling to electron spins hosted by nitrogen vacancy centers in diamond. Our design spatially focuses the magnetic field to a small mode volume. We achieve large homogeneous single spin coupling rates, with an enhancement of the single spin Rabi frequency of more than one order of magnitude compared to standard 3D cavities with a fundamental resonance at \SI{3}{GHz}. Finite element simulations confirm that the magnetic field component is homogeneous throughout the entire sample volume, with a RMS deviation of 1.54\%. With a sample containing $10^{17}$ nitrogen vacancy electron spins we achieve a collective coupling strength of $Ω=\SI{12}{MHz}$, a cooperativity factor $C=27$ and clearly enter the strong coupling regime. This allows to interface a macroscopic spin ensemble with microwave circuits, and the homogeneous Rabi frequency paves the way to manipulate the full ensemble population in a coherent way.

quant-ph