arXiv subjects

Daniele De Bernardis

Publications and source records attributed to Daniele De Bernardis.

At least 19 recordsLinked to original sources

arXiv2026

Enabling Deterministic Passive Quantum State Transfer with Giant Atoms

Achieving quantum state transfer in passive ways can become a powerful asset for scalable quantum networks. Here, we demonstrate how giant atoms coupled to 1D waveguides provide a platform for such a passive, deterministic transfer. Specifically, we show that when the giant atom's extent is comparable to the width of the emitted wavepacket, this wavepacket can be designed to be time-reversal-symmetric by engineering the positions and strengths of atom-waveguide coupling points. We first derive general analytical conditions under which arbitrary qubit decays can be mapped to wavevector-dependent couplings that guarantee perfect state transfer in the continuum limit of infinitely many coupling points. Then, for experimentally relevant configurations with a finite number of coupling points, we optimize the coupling positions and values. We demonstrate that the transfer fidelity can be boosted well beyond the value for a single coupling point (54%), reaching 87% with only two coupling points and exceeding 99% with ten or more. We further analyze the robustness of the protocol against disorder in the coupling points as well as frequency variations of the qubits and extend the formalism to environments with nonlinear dispersion, showing that dispersion-induced distortions can be fully compensated by judiciously chosen setups. Our results establish giant atoms as a powerful platform for realizing high-fidelity quantum state transfer and demonstrate how time-dependent control can be instead encoded into the device design.

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arXiv2026

Electrostatics-induced breakdown of the integer quantum Hall effect in cavity QED

We address the prevailing theoretical explanation of the recently observed breakdown of the integer quantum Hall effect in a two-dimensional electron gas embedded in a metallic split-ring resonator. Within the same single-particle description of quantized Hall conductance, we compare previously proposed vacuum-induced transport modifications against an alternative mechanism that explains this breakdown in terms of non-chiral edge channels arising solely from electrostatic boundary effects. This direct comparison shows that for experimentally relevant parameters, the electrostatic contribution exceeds that of any vacuum-induced conductance modifications by many orders of magnitude and yields characteristic transport signatures and energy scales that align well with experimental observations. This finding sheds new light on this puzzling phenomenon, supporting an electrostatic rather than a vacuum-related interpretation that can be directly tested in experiments.

cond-mat.mes-hall↗

arXiv2026

Breakdown of the optical saturation regime in molecular single-photon emitters

Solid-state single organic molecules, such as dibenzoterrylene (DBT) in organic matrices, are prominent deterministic single-photon sources, usually modeled as effective two-level systems (TLS). We show that single DBT molecules in anthracene nanocrystals, under strong continuous-wave driving, depart from this picture: instead of the expected saturation, fluorescence is strongly suppressed at high resonant pump power, while the linewidth broadens beyond the TLS prediction -- an \emph{anomalous saturation} regime. Comparing coherent and incoherent excitation and independently calibrating temperature via phonon-induced dephasing rules out laser-induced heating and intersystem crossing. Instead, a model of intensity-dependent excited-state absorption (ESA) toward a short-lived dark state quantitatively reproduces both the fluorescence suppression and the linewidth broadening. We further show that matrix quality mitigates this quenching, and that pulsed excitation schemes are strategic toward full population inversion, with direct implications for quantum nanophotonics and molecular optomechanics.

quant-ph↗

arXiv2026

Giant-atom-enabled quantum optics with valley-polarized photons

Valleytronics and valley photonics exploit the valley degree of freedom to encode and manipulate information. Here we show that photonic valleys can be selectively addressed in quantum optics using a simple two-level emitter, provided it is coupled nonlocally to the field, thereby realizing a so-called giant atom. Specifically, we consider a qubit coupled at multiple points to an engineered honeycomb lattice of resonators with detuned sublattice frequencies. By tailoring the geometry of the coupling points, the giant atom can be made to emit selectively into a single valley. The emitted photons thereby acquire a well-defined valley character and inherit the associated Berry curvature. By placing the qubit near a domain wall between regions of opposite sublattice detuning, whose interface supports valley-polarized edge modes, emission becomes chiral along the domain wall. This provides a promising route toward implementation of single-photon disorder-robust chiral emission without breaking time-reversal symmetry of the electromagnetic medium in platforms such as circuit QED.

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arXiv2026

Cavity modification of magnetoplasmon mode through coupling with intersubband polaritons

We investigate the coupling of a multi-mode metal-insulator-metal cavity to a two-dimensional electron gas (2DEG) in a quantum well in the presence of a strong magnetic field. The TM cavity mode is strongly hybridized with an intersubband transition of the 2DEG, forming a polaritonic mode in the ultrastrong coupling regime, while the TE mode remains an almost purely cavity mode. The magnetoplasmon excitation emerging from the presence of the magnetic field couples with both TM and TE modes, exhibiting different coupling strengths and levels of spatial field inhomogeneity. While the strong homogeneity of the bare TE mode gives rise to the standard anticrossing of strong coupling, the inhomogeneous polaritonic TM mode is shown to activate an observable Coulombic effect in the spectral response, often referred to as non-locality. This experiment demonstrates a cavity-induced modification of the 2DEG response and offers a new route to probing the effect of Coulomb interactions in ultrastrongly coupled systems via reshaping of their cavity mode profiles.

cond-mat.mes-hall↗

arXiv2025

Superstrong Dynamics and Directional Emission of a Giant Atom in a Structured Bath

Quantum emitters coupled to waveguides with nonlinear dispersion show rich quantum dynamics with the promise of implementing non-trivial non-Markovian quantum models. Recent advances in engineered photonic environments now allow the realization of discrete-site waveguides with tailored dispersion, yet most implementations of waveguide QED remain limited to a local qubit-waveguide coupling. Here, we study a transmon qubit non-locally coupled to a high-impedance coupled cavity array (CCA), thus implementing a \emph{giant atom} in a structured photonic environment. The non-local coupling produces interference with the CCA modes, selectively enhancing interaction with even and long-wavelength modes, while suppressing coupling to odd and short-wavelength modes. For a subset of symmetric, long-wavelength modes, we reach the superstrong coupling regime. In this regime, measurements of the atomic participation ratio reveal strongly hybridized eigenmodes on a par with a strongly reduced qubit participation at the frequency of maximum hybridization with the qubit, in agreement with theory. Time-domain measurements of the qubit dynamics show clear deviations from the single-mode Jaynes--Cummings model, marked by the emergence of mode--mode interactions. By breaking spatial inversion symmetry of the CCA, the qubit seeds dressed eigenmodes confined to either the right or left of the qubit, which we exploit to implement and characterize a directional photon-emission protocol. These results demonstrate precise control over multimode light--matter interaction in a structured photonic environment.

quant-ph↗

arXiv2025

Hybrid interfaces at the single quantum level in fluorescent molecules

We theoretically investigate a single fluorescent molecule as a hybrid quantum optical device, in which multiple external laser sources exert control of the vibronic states. In the high-saturation regime, a coherent interaction is established between the vibrational and electronic degrees of freedom, and molecules can simulate several cavity QED models, whereby a specific vibrational mode plays the role of the cavity mode. Focusing on the specific example where the system is turned into an analogue simulator of the quantum Rabi model, the steady state exhibits vibrational bi-modality resulting in a statistical mixture of highly non-classical vibronic cat states. Applying our paradigm to molecules with prominent spatial asymmetry and combining an optical excitation with a THz(IR) driving, the system can be turned into a single photon transducer. Two possible implementations are discussed based on the coupling to a subwavelength THz patch antenna or a resonant metamaterial. In a nutshell, this work assesses the role of molecules as an optomechanical quantum toolbox for creating hybrid entangled states of electrons, photons, and vibrations, hence enabling frequency conversion over very different energy scales.

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arXiv2025

Non-Markovian dynamics of a qubit due to accelerated light in a lattice

We investigate the emission of a qubit weakly coupled to a one-band coupled-cavity array where, due to an engineered gradient in the cavity frequencies, photons are effectively accelerated by a synthetic force F. For strong F, a reversible emission described by an effective Jaynes-Cummings model occurs, causing a chiral time-periodic excitation of an extensive region of the array, either to the right or to the left of the qubit depending on its frequency. For weak values of F instead, a complex non-Markovian decay with revivals shows up. This is reminiscent of dynamics induced by mirrors in standard waveguides, despite the absence of actual mirrors, and can be attributed to the finite width of the energy band which confines the motion of the emitted photon. In a suitable regime, the decay is well described by a delay differential equation formally analogous to the one governing the decay of an atom in a multi-mode cavity where the cavity length and time taken by a photon to travel between the two mirrors are now embodied by the amplitude and period of Bloch oscillations, respectively.

quant-ph↗

arXiv2024

Quantum nonlinear optics on the edge of a few-particle fractional quantum Hall fluid in a small lattice

We study the quantum dynamics in response to time-dependent external potentials of the edge modes of a small fractional quantum Hall fluid composed of few particles on a lattice in a bosonic Laughlin-like state at filling ν = 1/2. We show that the nonlinear chiral Luttinger liquid theory provides a quantitatively accurate description even for the small lattices that are available in state-of-the-art experiments, away from the continuum limit. Experimentally-accessible data related to the quantized value of the bulk transverse Hall conductivity are identified both in the linear and the non-linear response to an external excitation. The strong nonlinearity induced by the open boundaries is responsible for sizable quantum blockade effects, leading to the generation of nonclassical states of the edge modes.

cond-mat.mes-hall↗

arXiv2024

Enhanced control of single-molecule emission frequency and spectral diffusion

The Stark effect provides a powerful method to shift the spectra of molecules, atoms and electronic transitions in general, becoming one of the simplest and most straightforward way to tune the frequency of quantum emitters by means of a static electric field. At the same time, in order to reduce the emitter sensitivity to charge noise, inversion symmetric systems are typically designed, providing a stable emission frequency, with a quadratic-only dependence on the applied field. However, such nonlinear behaviour might reflect in correlations between the tuning ability and unwanted spectral fluctuations. Here, we provide experimental evidence of this trend, using molecular quantum emitters in the solid state cooled down to liquid helium temperatures. We finally combine the electric field generated by electrodes, which results parallel to the molecule induced dipole, to optically excite long-lived charge states, acting in the perpendicular direction. Based on the anisotropy of the molecule's polarizability, our two-dimensional control of the local electric field allows not only to tune the emitter's frequency but also to sensibly suppress the spectral instabilities associated to field fluctuations.

quant-ph↗

arXiv2024

Light-matter interactions in the vacuum of ultra-strongly coupled systems

We theoretically study how the peculiar properties of the vacuum state of an ultra-strongly coupled system can affect basic light-matter interaction processes. In this unconventional electromagnetic environment, an additional emitter no longer couples to the bare cavity photons, but rather to the polariton modes emerging from the ultra-strong coupling. As such, the effective light-matter interaction strength is sensitive to the properties of the distorted vacuum state. Different interpretations of our predictions in terms of modified quantum fluctuations in the vacuum state and of radiative reaction in classical electromagnetism are critically discussed. Whereas our discussion is focused on the experimentally most relevant case of intersubband polaritons in semiconductor devices, our framework is fully general and applies to generic material systems.

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arXiv2024

Nonperturbative cavity quantum electrodynamics: is the Jaynes-Cummings model still relevant?

In this tutorial review, we briefly discuss the role that the Jaynes-Cummings model occupies in present-day research in cavity quantum electrodynamics with a particular focus on the so-called ultrastrong coupling regime. We start by critically analyzing the various approximations required to distill such a simple model from standard quantum electrodynamics. We then discuss how many of those approximations can, and often have been broken in recent experiments. The consequence of these failures has been the need to abandon the Jaynes-Cummings model for more complex models. In this, the quantum Rabi model has the most prominent role and we will rapidly survey its rich and peculiar phenomenology. We conclude the paper by showing how the Jaynes-Cummings model still plays a crucial role even in non-perturbative light-matter coupling regimes.

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arXiv2023

Relaxation breakdown and resonant tunneling in ultrastrong-coupling cavity QED

We study the open relaxation dynamics of an asymmetric dipole that is ultrastrongly coupled to a single electromagnetic cavity mode. By using a thermalizing master equation for the whole interacting system we derive a phase diagram of the Liouvillian gap. It emerges that the ultrastrong coupling inhibits the system relaxation toward the equilibrium state due to an exponential suppression of the dipole tunneling rate. However, we find that polaronic multi-photon resonances restore fast relaxation by a cavity-mediated dipole resonant tunneling process. Aside of the numerical evidences, we develop a fully analytical description by diagonalizing the Rabi model through a generalized rotating-wave approximation, valid in the so-called polaron frame. The relaxation physics of such ultrastrong-coupling systems is then reduced to a multi-photon polaron version of the standard text-book dressed states picture. At the end we discuss an extension to a multi-well dipole that can set the basis of a cascaded resonant tunnelling setup in the ultrastrong coupling regime.

quant-ph↗

arXiv2023

Chiral quantum optics in the bulk of photonic quantum Hall systems

We study light-matter interactions in the bulk of a two-dimensional photonic lattice system, where photons are subject to the combined effect of a synthetic magnetic field and an orthogonal synthetic electric field. In this configuration, chiral waveguide modes appear in the bulk region of the lattice, in direct analogy to transverse Hall currents in electronic systems. By evaluating the non-Markovian dynamics of emitters that are coupled to those modes, we identify critical coupling conditions, under which the shape of the spontaneously emitted photons becomes almost fully symmetric. Combined with a directional, dispersionless propagation, this property enables a complete reabsorption of the photon by another distant emitter, without relying on any time-dependent control. We show that this mechanism can be generalized to arbitrary in-plane synthetic potentials, thereby enabling flexible realizations of re-configurable networks of quantum emitters with arbitrary chiral connectivity.

quant-ph↗

arXiv2023

Magnetic-field-induced cavity protection for intersubband polaritons

We analyse the effect of a strong perpendicular magnetic field on an intersubband transition in a disordered doped quantum well strongly coupled to an optical cavity. The magnetic field changes the lineshape of the intersubband optical transition due to the interface roughness of the quantum well from a Lorentzian to a Gaussian one. In this regime, a novel form of magnetic-field-induced cavity protection sets in, which strongly reduces the polariton linewidth to the cavity contribution only. Implications of our results for fundamental studies of nonlinear polariton dynamics and for technological applications to polariton lasers are finally highlighted.

cond-mat.mes-hall↗

arXiv2022

Optical-force-mediated coupling between levitated nanospheres can go ultrastrong

We theoretically investigate the effect of optical-force-mediated interactions onto the quantum dynamics of a pair of dielectric nanospheres optically trapped in two neighboring optical tweezers. Thanks to the interference between the tweezer beams and the elastically scattered light by the other nanosphere, the effective inter nanosphere coupling can reach the ultrastrong coupling regime. Experimentally accessible signatures of the entangled nature of the quantum ground state are highlighted, including entanglement witnesses based on position/momentum correlation functions and a sizable dynamical Casimir excitation upon a fast modulation of the tweezer's properties.

quant-ph↗

arXiv2021

The Vacua of Dipolar Cavity Quantum Electrodynamics

The structure of solids and their phases is mainly determined by static Coulomb forces while the coupling of charges to the dynamical, i.e., quantized degrees of freedom of the electromagnetic field plays only a secondary role. Recently, it has been speculated that this general rule can be overcome in the context of cavity quantum electrodynamics (QED), where the coupling of dipoles to a single field mode can be dramatically enhanced. Here we present a first exact analysis of the ground states of a dipolar cavity QED system in the non-perturbative coupling regime, where electrostatic and dynamical interactions play an equally important role. Specifically, we show how strong and long-range vacuum fluctuations modify the states of dipolar matter and induce novel phases with unusual properties. Beyond a purely fundamental interest, these general mechanisms can be important for potential applications, ranging from cavity-assisted chemistry to quantum technologies based on ultrastrongly coupled circuit QED systems.

quant-ph↗

arXiv2021

Light-matter interactions in synthetic magnetic fields: Landau-photon polaritons

We study light-matter interactions in two dimensional photonic systems in the presence of a spatially homogeneous synthetic magnetic field for light. Specifically, we consider one or more two-level emitters located in the bulk region of the lattice, where for increasing magnetic field the photonic modes change from extended plane waves to circulating Landau levels. This change has a drastic effect on the resulting emitter-field dynamics, which becomes intrinsically non-Markovian and chiral, leading to the formation of strongly coupled Landau-photon polaritons. The peculiar dynamical and spectral properties of these quasi-particles can be probed with state-of-the-art photonic lattices in the optical and the microwave domain and may find various applications for the quantum simulation of strongly interacting topological models.

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