arXiv subjects

Daniele Sanvitto

Publications and source records attributed to Daniele Sanvitto.

At least 19 recordsLinked to original sources

arXiv2026

Dynamical stabilisation of a quantum fluid using a single topological defect

The size and shape of a quantum fluid in equilibrium is strongly influenced by the inter-particle interactions. In the attractive interaction regime, atomic quantum fluids ultimately collapse in a violent process that expels most of the particles from the macroscopically occupied state. Here, we use a quantum fluid of light in propagating geometry as an analogue to a two-dimensional Bose-Einstein condensate (BEC) with large attractive interactions to show that non-trivial topology significantly alters the dynamical behaviour of the collapse, enhancing the BEC stability and delaying the collapse time by an order of magnitude. We measure direct experimental signatures of topology affecting quantum hydrodynamics, unveiling the inherent competition between attractive nonlinearities, that lead to the collapse, and the preservation of topological charge from a multi-charged vortex. We fully characterise the collapse process in coordinate space and the eventual `solitonification' of the system and connect it to the mode structure of the excitation spectrum.

cond-mat.quant-gas↗

arXiv2026

Geometric control of hyperbolic exciton-polariton condensate dimers

Coupled many-body quantum systems exhibit rich emergent physics with diverse stationary and dynamical behaviors. By engineering platforms with tunable and distinct coupling mechanisms, new insights emerge into the collective behavior of coupled many body systems. Particles can be exchanged via evanescent or ballistic coupling: the former, based on proximity, yields large spectral splitting, while the latter requires strict phase-matching, analogous to phase-coupled harmonic oscillators, and has a smaller impact on the energy landscape. We demonstrate an all-optically tunable quantum fluid dimer based on exciton-polariton condensates in a photonic crystal waveguide with hyperbolic (saddle-like) dispersion. Varying the dimer's angle relative to the grating tunes the coupling from evanescent to ballistic. We directly observe spectral features and mass flow shaped by the saddle dispersion. This work highlights photonic crystals as powerful platforms to explore condensed matter phenomena lying at the interface between delay-coupled nonlinear oscillators and tight binding physics.

physics.optics↗

arXiv2026

Dynamical development of long-range spatial coherence in non-equilibrium bosonic condensation

Development of spontaneous coherence is one of the hallmarks of bosonic condensation in a variety of physical systems, such as cold atoms, confined photons, and hybrid light-matter quasiparticles like exciton polaritons in semiconductors. While spatial coherence is well understood once a steady-state condensate has been established, its temporal evolution as the condensate forms is largely unexplored. Here, we explore the dynamical formation of a non-equilibrium, driven-dissipative exciton-polariton condensate through both time-resolved experiments and numerical modeling. Our study reveals that the spatial coherence is established through two distinct stages. The early-time stage is interaction-driven and features transient oscillations in spatial coherence. This stage is followed by a steady-state regime characterized by a spatially-uniform high degree of coherence that extends over the entire size of the system and persists over time. These stages of spatial coherence development occur in both free flowing and confined exciton-polariton systems that undergo a quench - rapid growth of the condensate starting from two different initial settings. Our study offers a deep insight into the process by which long-range spatial coherence is established in a non-equilibrium bosonic condensate.

cond-mat.quant-gas↗

arXiv2026

Very strong light-matter coupling in patterned GaAs heterostructures

The very strong light-matter coupling regime enables the non-perturbative modification of matter properties via light. Using a patterned GaAs/AlGaAs waveguide with twelve wide quantum wells, we demonstrate hybridization of heavy- and light-hole excitons within a single polariton state and show that, at finite magnetic field, the presence of the light-hole exciton suppresses coupling to the heavy-hole Rydberg excitons and unbound scattering states. We develop a fully microscopic theory that accounts for the combined effects of the magnetic field and light-matter coupling on the excitons, providing an accurate description of the experimental results beyond a perturbative coupled-oscillator framework. This identifies quantum well width as a key control parameter for engineering the light-induced hybridization of matter wave functions in polaritons, which, in turn, can play a crucial role in the optical non-linearities.

cond-mat.mes-hall↗

arXiv2026

Magnetic-field driven hybridization of heavy- and light-hole Rydberg excitons in GaAs quantum wells

We present a combined theoretical and experimental study of ground and excited Rydberg exciton states in wide GaAs quantum wells exposed to a magnetic field in the Faraday geometry. We employ a multiband exciton model based on the Luttinger Hamiltonian, which captures valence-band mixing between heavy- and light-hole states induced by both the quantum well confinement and the magnetic field, and we develop an efficient numerical approach to solve for both ground- and excited-state excitons. The method treats Coulomb interactions, magnetic confinement, and band mixing on an equal footing, enabling a systematic characterization of exciton energies, oscillator strengths, and orbital composition. We show that band hybridization increases with magnetic field and is significantly more pronounced for higher excited states, where it sets in at lower fields and strongly modifies their properties. The theoretical predictions are validated by polarization-resolved magneto-reflectance measurements up to 9 T on GaAs/Al$_{0.4}$Ga$_{0.6}$As quantum wells of 20 nm width. We find excellent agreement for both the diamagnetic shift and Zeeman splitting of the ground state and the first four Rydberg excitons. Our results demonstrate that valence-band mixing plays a crucial role in determining the magnetic-field dependence of excited exciton states and must be properly included for a quantitative description of magneto-excitons in wide GaAs quantum wells.

cond-mat.mes-hall↗

arXiv2026

Exciton-Tunable Phase Control and Superstrong Coupling Through Multimode Polariton Engineering in Planar Waveguides

Strong light-matter coupling in optical waveguides provides a versatile platform for engineering hybrid polaritonic modes and their dispersion. Here we investigate multimode exciton-photon coupling in visible semiconductor waveguides supporting several transverse electric modes. Using rigorous coupled-wave analysis combined with a coupled-oscillator model, we show that the photonic band structure can be engineered across a range of regimes, from conventional multimode strong coupling to the superstrong coupling regime, where the Rabi splitting becomes comparable to the spacing between adjacent photonic modes. In the latter regime, hybridization between orthogonal electromagnetic modes is enabled by restricting the active material to a subregion of the mode volume where the photonic modes exhibit strong mutual overlap. This breaking of the orthogonality leads to polaritonic branches whose composition can be tuned among several photonic modes and the exciton. We demonstrate that small shifts of the exciton resonance produce pronounced changes in the propagation constants of different polariton branches, enabling exciton-controlled phase modulation through modal interference and, in the superstrong coupling regime, direct modal switching across a continuous S-shaped dispersion. The resulting figures of merit predict $π$ phase shifts for exciton energy shifts of only a few meV over propagation lengths of tens of micrometers, while larger shifts are still required for mode switching. These results establish multimode waveguide polaritons as a versatile platform spanning multiple coupling regimes, for compact phase and intensity control in integrated photonic architectures.

physics.optics↗

arXiv2026

Modeling the Quantum Photon Statistics in Hybrid Light-Matter Integrated Circuits

Strong light-matter coupling between a guided electromagnetic mode and an excitonic semiconductor transition gives rise to exciton-polaritons with optical nonlinearities far exceeding those of conventional photonic platforms. Utilizing these nonlinearities in the few-particle regime, where quantum signatures such as photon antibunching, sub-Poissonian statistics and non-trivial inter-mode correlations become accessible, is a central goal of integrated quantum photonics. Yet, a quantitative theoretical framework connecting realistic waveguide parameters to measurable non-classical photonic output is absent. Here, we present a comprehensive framework for predicting and benchmarking quantum photon statistics in polaritonic integrated circuits, using state-of-the-art experimentally achieved device parameters for (Al)GaAs waveguide platforms. By mapping the pulsed nonlinear waveguide dynamics onto a bosonic quantum circuit representation that explicitly incorporates dissipation, we identify experimentally accessible quantum signatures across two circuit configurations: a single waveguide in a free-space interferometric configuration and a fully integrated multimode coupled-waveguide circuit. We further show that slow-light engineering of the polariton dispersion offers a practical route to amplifying the effective nonlinearity, pushing quantum signatures beyond Gaussian statistics.

quant-ph↗

arXiv2026

Pulse, polarization and topology shaping of polariton fuids

Here we present different approaches to ultrafast pulse and polarization shaping, based on a ``quantum fluid'' platform of polaritons. Indeed we exploit the normal modes of two dimensional polariton fluids made of strong coupled quantum well excitons and microcavity photons, by rooting different polarization and topological states into their sub-picosecond Rabi oscillations. Coherent control of two resonant excitation pulses allows us to prepare the desired state of the polariton, taking benefit from its four-component features given by the combination of the two normal modes with the two degrees of polarization. An ultrafast imaging based on the digital off-axis holography technique is implemented to study the polariton complex wavefunction with time and space resolution. We show in order coherent control of the polariton state on the Bloch sphere, an ultrafast polarization sweeping of the Poincaré sphere, and the dynamical twist of full Poincaré states such as the skyrmion on the sphere itself. Finally, we realize a new kind of ultrafast swirling vortices by adding the angular momentum degree of freedom to the two-pulse scheme. These oscillating topology states are characterized by one or more inner phase singularities tubes which spirals around the axis of propagation. The mechanism is devised in the splitting of the vortex into the upper and lower polaritons, resulting in an oscillatory exchange of energy and angular momentum and in the emitted time and space structured photonic packets.

cond-mat.other↗

arXiv2026

Dynamical universality in a driven quantum fluid of light

Universal scaling near phase transitions is one of the central ideas of physics, linking the growth of spatial correlations to the slowing down of dynamics. So far, direct experimental access to this critical behavior has remained largely confined to equilibrium many-body systems, and especially to static critical behavior. Here we probe how universality emerges in a driven quantum fluid of light formed by exciton--polaritons in a semiconductor microcavity. By probing the fluctuation-dominated disordered phase below the condensation threshold, we directly measure both the static growth of the correlation length $ξ$ and the dynamical slowing down of the relaxation time $τ$. We find that these quantities obey the universal relation $τ\propto ξ^{z}$ with dynamical exponent $z \approx 2$, revealing diffusive dynamics of a non-conserved order parameter. Our results extend the physics of critical dynamics from equilibrium matter to driven optical systems, bridging quantum condensates and lasers.

cond-mat.quant-gas↗

arXiv2026

Dynamic topological exciton-polaritons enabling ultrafast logic operations

Topological active materials have emerged as powerful paradigm bridging the discovery of exotic topological phases of matter with the development of functional topological devices. The recent extension of these material systems into dynamic regime, where topological properties can be actively manipulated at ultrafast timescales, promises unprecedented control over topological states and their functionalities. However, translating the static topological lasing signals into high-performance logic functions remain highly challenging, which imposes a far more stringent set of materials attributes. Here, leveraging the strong nonlinearity and pronounced spectral isolation of perovskite exciton-polaritons embedded in a Dirac vortex microcavity, we experimentally demonstrate the dynamic topological Majorana-like state polariton condensation with its ultrafast logic operations at room temperature. By actively coordinating pump and control beams in both spectral and temporal domain, we dynamically steer the topological polariton condensation process and demonstrate AND and NOT logic operations, achieving record extinction ratio (~20 dB), extremely low control fluence (~0.2 nJ/cm2) and sub-picosecond response time (~500 fs). Our results expand the frontier of dynamic topology and establish a novel pathway towards robust, ultrafast, and reconfigurable on-chip polaritonic logic circuits.

physics.optics↗

arXiv2025

Fully Integrated Perovskite Polaritonic Circuits with Tunable Lasing and Nonlinear Amplification

Photonic integrated circuits are emerging as a key technology for compact and energy-efficient optical information processing. Yet, their practical implementation remains limited by the intrinsically weak optical nonlinearities of conventional materials, which demand high power and large footprints to achieve significant nonlinear responses. Exciton-polaritons, hybrid light-matter excitations of semiconducting materials, offer a promising solution by combining strong optical nonlinearities with the high speed and large scalability typical of photonic devices. However, despite their potential, working on-chip polaritonic elements demonstrating room temperature coherent lasing, controllable nonlinear propagation, or amplification have remained elusive. Here we demonstrate a fully integrated perovskite polaritonic circuit that overcomes these limitations. Using a single-step microfluidic lithographic technique, we realize waveguide circuits with integrated gratings that simultaneously act as couplers and mirrors, forming in-plane Fabry-Pérot cavities. These structures support robust in-plane polariton lasing between gratings, yielding coherent emission along the waveguide. Furthermore, we observe clear signatures of strong nonlinear self-phase modulation and, for the first time, optical amplification of guided polaritons at room temperature. Our simple, scalable platform opens the way to low-power, highly nonlinear optical circuits for integrated photonics and neuromorphic architectures operating at room temperature.

physics.optics↗

arXiv2025

Low-power multi-mode fiber projector overcomes shallow neural networks classifiers

In the domain of disordered photonics, the characterization of optically opaque materials for light manipulation and imaging is a primary aim. Among various complex devices, multi-mode optical fibers stand out as cost-effective and easy-to-handle tools, making them attractive for several tasks. In this context, we cast these fibers into random hardware projectors, transforming an input dataset into a higher dimensional speckled image set. The goal of our study is to demonstrate that using such randomized data for classification by training a single logistic regression layer improves accuracy compared to training on direct raw images. Interestingly, we found that the classification accuracy achieved is higher than that obtained with the standard transmission matrix model, a widely accepted tool for describing light transmission through disordered devices. We conjecture that the reason for such improved performance could be due to the fact that the hardware classifier operates in a flatter region of the loss landscape when trained on fiber data, which aligns with the current theory of deep neural networks. These findings suggest that the class of random projections operated by multi-mode fibers generalize better to previously unseen data, positioning them as promising tools for optically-assisted neural networks. With this study, in fact, we want to contribute to advancing the knowledge and practical utilization of these versatile instruments, which may play a significant role in shaping the future of neuromorphic machine learning.

physics.optics↗

arXiv2025

Microfluidic-Assisted Growth of Perovskite Microwires for Room-Temperature All-Optical Switching Based on Total Internal Reflection

The development of efficient integrated photonic circuits is fundamental for ongoing research in information processing and computer science. The greatest challenge in strong light-matter regime facing photonic systems is achieving strong nonlinearities, which are exploitable in strongly coupled systems, leading to the formation of exciton-polaritons. In this context, the use of hybrid organic-inorganic perovskites offers a promising alternative, exhibiting robust interactions at Room Temperature (RT). However, the development of perovskite-based integrated devices requires both the ability to achieve long in-plane propagation, and the development of alternative fabrication approaches tailored to perovskite materials, designed to preserve their optical properties and prevent degradation. Herein, we present the realization of a proof-of-concept all-optical switch using propagating polaritons confined in Total Internal Reflection (TIR), which ensures long in-plane propagation and limited optical losses. We realized an efficient injection/extraction of the TIR-confined waveguide polariton modes by employing gold grating couplers prepatterned on the substrate.

physics.optics↗

arXiv2025

Directional optical parametric amplification in a hyperbolic metamaterial

Optical parametric amplification (OPA) comprises essentially a nonlinear four-wave mixing process in which a "pump" and a "signal" field give rise to an "idler" field under certain phase-matching conditions. Here we use a photonic crystal waveguide strongly-coupled with an excitonic reservoir to generate this process between different guided modes at optical wavelengths. Differently from classical nonlinear optical crystals, where the pump and idler photons travel almost collinearly, our exciton-polaritons are naturally separated in the waveguide due to their opposite group velocities. Due to the high efficiency of the process we can generate the idler field of the parametric process by pumping with a continuous wave laser and choose its direction of propagation in the waveguide by adjusting the angle of incidence of the seed laser. We show the OPA process to be robust against surface defects of the waveguide and can lead to simple-to-fabricate devices compared to microcavities that take advantage of strong signal-idler correlations in a propagating geometry. Our results closely agree with mean-field numerical simulations.

physics.optics↗

arXiv2025

Supersolidity of polariton condensates in photonic crystal waveguides

Condensation of exciton-polaritons has been recently observed in one-dimensional photonic crystal waveguides, exploiting the interplay of long-lived gap confined eigenmodes and negative mass polariton branches. Here we focus on the theoretical emergence of a second emission threshold, in addition to the one associated with condensation at zero-momentum, due to the nonlinear polariton scattering from the condensate into finite momentum eigenmodes. The physics of this spatially modulated condensate is related to a spontaneous breaking of both phase and translational symmetries simultaneously, bearing strong similarities with the highly sought supersolid phase in Helium and ultracold atomic gases but with a novel mechanism typical of the driven-dissipative scenario. We then propose clear-cut and unequivocal experimental signatures that would allow to identify supersolidity phenomena in polariton condensates

cond-mat.quant-gas↗

arXiv2024

Condensation dynamics in a two-dimensional photonic crystal waveguide

Exciton-polariton condensation occurs at the extrema of the underlying dispersion where the density of states diverges and carriers can naturally accumulate. The existence of multiple such points leads to coupling and competition between the associated modes and dynamical redistribution of the carriers in the dispersion. Here, we directly engineer the above situation via subwavelength periodic patterning of a two-dimensional nanostructure. This leads to multimode condensation into a pair of symmetric condensates that form at high-momenta, accidental-coupling points, and a high-symmetry $Γ$-point with a bound-in-the-continuum (BiC) state. The dynamical behaviour of the system reveals the non-simultaneous appearance of these condensates and the interplay of non-trivial gain and relaxation mechanisms. We fully characterise the quasi-static and dynamical regime of this artificial crystal and the properties of the different condensates. This understanding is necessary when band-structure engineering techniques are used to achieve precise control of condensate formation with given energy and momentum.

physics.optics↗

arXiv2024

Room temperature spin-layer locking of exciton-polariton nonlinearities

Recent advancements in transition metal dichalcogenides (TMDs) have unveiled exceptional optical and electronic characteristics, opened up new opportunities, and provided a unique platform for exploring light-matter interactions under the strong coupling regime. The exploitation of exciton-polaritons, with their peculiar hybrid light-matter properties, for the development of spintronic customizable devices that enhance both the information capacity and functionality at ambient temperatures is often suggested as a promising route. However, although TMD polaritons have shown promising potential, the microscopic mechanisms leading to nonlinearities in TMD polaritons are complex and their spin-anisotropy, a crucial requirement for many proposed polaritonic devices, has been missing. Here, we demonstrate the absence of spin-anisotropic interaction in a monolayer WS2 microcavity (at room temperature) and show how spin-dependent interactions can be controlled and spin anisotropy recovered by engineering double WS2 layer structures with varied interlayer spacing. We attribute this phenomenon to a distinctive feature in exciton-polariton physics: layer-dependent polariton-phonon coupling. We use theoretical calculations of the phonon electrostatic potentials finding a drastically different coupling strength for single and double monolayer samples and discuss qualitatively how this explains the observed spin-anisotropic response. This is further consistent with experiments on multi WS2 layer samples and the identification of a critical separation distance, above which an effective single monolayer spin-anisotropic response is recovered, both in experiment and theory. Our work lays the groundwork for the development of spin-optronic polaritonic devices at room temperature.

physics.optics↗

arXiv2024

Enhanced polariton interactions in suspended WS2 monolayer microcavity

Transition-metal dichalcogenides monolayers exhibit strong exciton resonances that enable intense light-matter interactions at room temperature (RT). However, the sensitivity of these materials to the surrounding environment and their intense interactions with the sustaining substrate result in the enhancement of excitonic losses through scattering, dissociation and defects formation, hindering their full potential for the excitation of optical nonlinearities in exciton-polariton platforms. From this point of view, the use of suspended monolayers holds the potential to completely eliminate substrate-induced losses, offering unique advantages for the investigation and exploitation of intrinsic electronic, mechanical, and optical properties of 2D materials based polaritonic systems, without any influence of proximity effects of all sort. In this work, we report a novel fabrication approach enabling the realization of a planar λ/2 microcavity filled with a suspended WS2 monolayer in its centre. In such a system, we experimentally demonstrate a 2-fold enhancement of the strong coupling at RT, due to reduced overall losses as compared to similar systems based on dielectric-filled microcavities. Moreover, as a result of minimized losses, spin-dependent polaritonic interactions in our platform are significantly amplified, leading to achievement of a record exciton interaction constant approaching the theoretically predicted value at RT, without making use of theoretical hypothesis on the effective polariton densities. This approach holds promises for pushing 2D materials-based polaritonic systems to their intrinsic limits, paving the way for the realization of novel polaritonic devices with superior performance.

physics.optics↗