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Dante M. Kennes

Publications and source records attributed to Dante M. Kennes.

At least 19 recordsLinked to original sources

Symmetry Rules for Cavity Materials Engineering with Linearly Polarized Vacuum Fields

Cavity materials engineering, aiming to manipulate material properties by coupling to vacuum fluctuations inside a cavity, is a rapidly advancing field. Despite significant progress, most studies to date have focused on specific materials and cavity configurations. Here, through a comprehensive group-theoretical analysis, we establish general symmetry rules for cavity materials engineering with linearly polarized cavity photon modes. By analyzing the symmetry of the effective photon-free quantum-electrodynamics Hamiltonian, we provide a complete classification of the symmetry-breaking patterns induced by cavity modes for all crystallographic point groups. The power of this framework is then demonstrated by quantum-electrodynamical density functional theory calculations. In particular, we explain the distinct cavity-induced lifting of band degeneracies in cubic BaTiO$_3$ for different cavity mode configurations, and the cavity-modified infrared and Raman spectra of monolayer MoS$_2$ due to symmetry breaking. Our results highlight the central role of symmetry in cavity materials engineering and provide general guidelines for future studies in this field.

cond-mat.mtrl-sci↗

Extended s-wave superconductivity in M-point twisted bilayer SnSe2

We investigate the emergence of electronic order and unconventional superconductivity in M-valley moiré materials. Starting from a first-principles Wannier model of AB-stacked twisted SnSe2, we tackle the (gate-screened) long-ranged Coulomb interaction with functional renormalization group simulations resolving the momentum structure and energy scales of the leading Fermi surface instabilities. Upon doping an antiferromagnetic stripe state at half-filling ($ν=3$ electrons per moiré unit cell) of the moiré flat bands, magnetic order gives way to unconventional superconductivity mediated by valley-selective spin fluctuations: Large hole doping ($ν\approx1$) leads to weak-coupling superconductors with various pairing symmetries, while slight electron- and hole-doping ($ν\approx2,4$) stabilizes a spin-singlet, extended s-wave state that benefits from scattering between virtual particle and hole states that are detuned from the Fermi level. These findings establish M-point moiré materials as a quantum simulation platform with phenomenological parallels to the class of iron pnictide superconductors.

cond-mat.supr-con↗

Cavity Control of Strongly Correlated Electrons Beyond Resonant Coupling

Interfacing materials with electromagnetic cavities offers a route to modify equilibrium properties through structured vacuum fluctuations. The coupling between light and correlated electrons lacks a characteristic energy scale, making vacuum induced ground state modifications of such systems inherently off-resonant and sensitive to the full photon mode structure. We develop a consistent cavity-QED formalism for dispersive electromagnetic environments in the Coulomb gauge, capturing both dynamical dressing via the vector potential and static screening by the dielectric. With this formalism, we perform a non-perturbative study of the cavity-induced modification of magnetism in the Hubbard model close to half-filling, including all cavity modes and with parameters determined from first principles. At half-filling, we show that the modification of the magnetic exchange interaction $J$ is controlled by a generalized Purcell factor, proportional to the frequency integrated photonic density of states relative to free space. This result identifies polaritonic surface cavities as promising platforms to modify correlated systems. For the surface cavity a competition between static screening and dynamical dressing via the vector potential leads to a net enhancement of $J$, directly observable in two-magnon Raman spectroscopy. The inclusion of screening is essential to obtain even qualitatively correct results. At weak doping, a variational exact diagonalization of the cavity-coupled $t$-$J$ polaron reveals that a low-frequency surface cavity can reverse the nodal-antinodal dichotomy of the bare polaron dispersion. This effect lies beyond mean field theory and is observable via ARPES measurements. Our framework establishes a concrete design principle linking cavity geometry to material response in the off-resonant regime, which will guide future experimental and theoretical explorations.

quant-ph↗

Organizing Principles for Moiré Quantum Matter

Moiré flat bands in van der Waals bilayers are usually discussed through a small set of mechanisms associated with the $Γ$ and $K$ valleys of hexagonal crystals, and more recently with $M$-valleys systems. Here we show that this view is incomplete. The momentum-space location and effective local orbital character of the monolayer's band edge, in conjunction with the moiré symmetry and the symmetry representations of the resulting bands, provide a general set of organizing variables for the emergent low-energy moiré Hamiltonian. Applying fully relaxed first-principles calculations, band unfolding and symmetry-representation analysis to more than 600 commensurate twisted bilayers spanning all 2D lattice classes, we identify several routes to moiré quantum matter beyond the conventional single-orbital paradigm. The resulting flat bands realize trigonal, honeycomb, square, checkerboard and kagome-like Hubbard models with single-orbital, multi-orbital and multi-site Hilbert spaces; spin-orbit-coupled multi-orbital flat bands exhibit symmetry-indicated topology beyond the conventional $K$-valley setting; and nonsymmorphic moiré symmetries enforce semimetallic flat-band connectivity. Analogous quasi-one-dimensional flat-band structures are found in $M$-valley hexagonal systems and $X$-valley square or rectangular systems resulting from emergent momentum-space nonsymmorphic symmetries. Separately, coupled multi-valley manifolds with kagome-like connectivity are identified in several systems whose parent band edges lie at non-high-symmetry points. These results establish a valley-orbital-symmetry framework for connecting parent-material electronic structure to emergent moiré Hamiltonians relevant to correlated, topological and symmetry-enforced moiré phases.

cond-mat.mtrl-sci↗

Macroscopic Polarization and Magnetization from Cavity Vacuum Fluctuations

Cavity light-matter interaction has recently emerged as a new avenue for manipulating material properties without driving fields. Here, we demonstrate that cavity vacuum fluctuations can induce macroscopic polarization (magnetization), even in materials that lack spontaneous polarization (net magnetization) in free space. Starting from the effective photon-free quantum-electrodynamics Hamiltonian, we identify all crystallographic (magnetic) point groups that allow such cavity-induced responses. We derive the form of the corresponding response tensors based on symmetry analysis, whose elements can be obtained by quantum electrodynamical density functional theory (QEDFT) calculations. As representative examples, we show that the cavity-induced polarization in $α$-quartz can be continuously controlled by rotating the cavity. For antiferromagnetic Mn$_3$Sn, we demonstrate that cavity-induced symmetry breaking generates an out-of-plane magnetization, accompanied by an anomalous Hall conductivity component that is forbidden outside the cavity. Our work establishes symmetry as a guiding principle for cavity materials engineering and provides a route for controlling polarization and magnetization through quantum vacuum fluctuations, i.e., cavity materials engineering.

cond-mat.mtrl-sci↗

Disorder-enhanced compressibility of Floquet random quantum circuits

Current quantum hardware is limited by noise and decoherence, which restrict the depth of unitary circuits that can be implemented with high fidelity. We investigate how the compressibility of time-evolution operators depends on the dynamical regime of the underlying many-body system. As a testbed, we study a one-dimensional Floquet random circuit with a tunable competition between interactions and on-site disorder. Using tensor-network simulations, we characterize operator growth through the operator-entanglement entropy of the Floquet unitary as well as of out-of-time-ordered correlators (OTOCs). We find rapid operator scrambling at weak disorder, while strong disorder leads to slow OTOC-front propagation and logarithmic or near-logarithmic operator-entanglement growth over the accessible time window. We then optimize shallow brickwall circuits to approximate the Floquet evolution and show that strong-disorder circuits can be compressed to substantially smaller depths than weak-disorder circuits at fixed logarithmic fidelity density. These results suggest that localized or slowly scrambling dynamics provide a favorable regime for compressed quantum simulation on noisy devices.

quant-ph↗

Many-body correlations in Floquet steady-states: Frequency-resolved renormalization group of the driven Anderson impurity

We introduce a functional renormalization group framework formulated directly in the Floquet steady-state that systematically incorporates frequency-dependent interaction effects. By retaining the frequency structure of the two-particle vertex up to second order in interaction strength, our approach provides controlled access to dynamical response functions and nonequilibrium transport in driven, interacting systems. Using the periodically driven single-impurity Anderson model as a paradigmatic example, we benchmark our results against state-of-the-art Floquet Green's function methods and find quantitative agreement for finite-frequency observables up to intermediate interaction strengths. Remarkably, we also show that static properties are often captured reliably by much simpler approximations, suggesting practical pathways for modeling driven quantum materials. Finally, we demonstrate that although periodic driving of the dot strongly broadens the Kondo resonance through inelastic scattering, it leaves the many-body Kondo cloud largely intact. This robustness suppresses Floquet replicas of the Kondo peak and leads to a partial persistence of Kondo pinning, highlighting the resilience of emergent many-body correlations under local periodic driving.

cond-mat.str-el↗

Cavity-enhanced superconducting response in an underdoped cuprate

Superconductors carry electrical current without resistance when paired electrons condense into a coherent macroscopic quantum state. In underdoped cuprates, evidence suggests that pairing-related correlations and superconducting fluctuations can survive above the temperature at which global coherence is lost, pointing to phase fluctuations as a key limitation on superconductivity in this regime. Motivated by recent demonstrations of cavity-modified collective states in quantum materials, we investigate whether superconducting coherence can be stabilized by engineering the electromagnetic environment of the superconductor. We study an underdoped YBa$_2$Cu$_3$O$_{7-δ}$ thin film in a tunable terahertz cavity formed with a semi-transparent gold mirror. From temperature-dependent terahertz transmission measurements, we find that the cavity enhances the superconducting response below the critical temperature, with an increase of the inferred superfluid weight. The effect becomes more pronounced at smaller cavity lengths and is accompanied by an upward shift of the superconducting onset temperature. Calculations based on a cavity-coupled model for phase-fluctuating superconductors capture these trends and support an interpretation in terms of cavity-enhanced phase stiffness. These results showcase the potential of cavity engineering for designing emergent functionalities in correlated systems.

cond-mat.supr-con↗

Divergent Coherent Phonon Responses Across the Metal-Insulator Crossover

Ultrafast laser control of material properties hinges on understanding light-matter interactions. We use two experimentally accessible response functions, laser fluence induced phonon softening and the amplitude of coherent reflectance oscillations, to compare how strongly different materials respond to ultrafast photoexcitation. Comparing a diverse set of materials, we find that only a narrow class, including Sb, GeTe, and Bi2Te3, shows exceptional responses such as pronounced phonon softening and a giant increase of reflectance oscillations with increasing fluence. These response functions peak in an intermediate conductivity regime of about 102 - 104 S/cm, at the crossover between localized and delocalized electronic states. The corresponding class of solids also shows other unconventional properties including high dielectric constants, enhanced Born effective charges, coordination numbers exceeding the 8-N rule and uncommon bond rupture. This suggests that these materials employ a unique bonding mechanism, coined metavalent bonding. Frozen-phonon DFT calculations show that the strong fluence dependence arises from Peierls-like instabilities, leading to large deformation potentials and anharmonic double-well potentials. These findings identify metavalent bonding as a design principle for enhanced coherent phonon control and provide a quantitative framework for identifying materials with exceptional ultrafast responses.

cond-mat.mtrl-sci↗

Feasibility study of continuous electronic Pomeranchuk cooling with a flavor-degenerate Wigner crystal

Achieving sub-millikelvin electron temperatures in nanoelectronic devices could unveil new transport phenomena, extend quantum coherence times, and enhance the precision of quantum metrology. However, maintaining such low temperatures continuously remains a long-standing challenge. Here, we propose and simulate an on-chip cooling cycle that harnesses the entropy difference between an electron liquid (EL) and a Wigner crystal (WC) in flavor-degenerate flat-band materials. Cooling is driven by a current through a device with a locally gated region. Within this region, the charge carrier density is tuned such that a WC forms beneath the gate. As carriers transition from an EL to WC phase, their entropy increases, extracting heat and the sliding WC advects this heat along the device. The heat is then released when carriers transition back to the EL phase, which establishes distinct hot and cold regions and a steady temperature gradient over the device. Simulations show net cooling for sufficiently low current densities, typically below $1~\mathrm{nA}/μ\mathrm{m}$, whereas Joule heating dominates at higher currents. Within the gated region, we estimate cooling powers of up to $8.4~\mathrm{aW}/μ\mathrm{m}$ at a bath temperature of $4~\mathrm{mK}$. Our approach can achieve electron temperatures well below $1~\mathrm{mK}$ under suitable conditions, promising a route towards continuous on-chip cooling in this temperature regime. Our approach applies to any flat-band material with low-energy flavor degeneracy (valley and/or orbital) and low disorder, including gapped Bernal-stacked bilayer graphene, rhombohedral-stacked multilayer graphene, and magic-angle twisted bilayer graphene.

cond-mat.mes-hall↗

Ballistic Exciton Flow Driven by Intertwined Exciton-Electron Orders in a Moiré Superlattice

Moiré superlattices of transition-metal dichalcogenides (TMDs) host strongly interacting Bose-Fermi mixtures in which bosonic excitons coexist with correlated electron lattices. Using ultrafast, time- and energy-resolved photoluminescence (PL) and reflectance microscopy, we show that strong exciton-electron and exciton-exciton repulsion can enable collective ballistic exciton transport in a WSe$_2$/WS$_2$ heterobilayer. The ballistic transport is energy-selective: repulsive interactions drive excitons into a higher moiré exciton band, where enhanced intersite hopping enables rapid spatial expansion. Correspondingly, the exciton mean-squared displacement (MSD) exhibits a quadratic time dependence ($\propto t^2$). This ballistic expansion is enhanced at fractional electron fillings where the electrons form generalized Wigner-crystal (GWC) orders. Afterwards, the system transitions into a mixed electron-exciton Mott state as Auger recombination and density depletion conclude the ballistic expansion. A one-dimensional Bose-Fermi Hubbard model solved using density-matrix renormalization group (DMRG) qualitatively reproduces the measured exciton transport and time-dependent response. It further confirms that strong cross-species interactions allow the electron crystal to perforate the exciton Mott background, accelerating its melting and enhancing exciton motion. Our results establish moiré TMDs as highly tunable platforms for realizing strongly interacting Bose-Fermi mixtures, which we employ here to demonstrate real-time control of intertwined bosonic and electronic order and to establish a route to the exciton insulator-fluid transition.

cond-mat.str-el↗

Surface Functional Renormalization Group for Layered Quantum Materials

We present an extension to the two-dimensional functional renormalization group to efficiently treat interactions on the surface or at interfaces of three-dimensional systems. As an application, we consider a semi-infinite stack of two-dimensional square lattices, including a Hubbard interaction on the surface layer and an alternating interlayer coupling. We investigate how strongly correlated states of the decoupled two-dimensional Hubbard model on the surface evolve under inclusion of such an SSH-like interlayer coupling. For large parts of the phase diagram as a function of the interlayer hopping parameters, the physics of the two-dimensional system prevails, with antiferromagnetic, superconducting $d$-wave, and ferromagnetic correlations taking center stage. However, for intermediate interlayer couplings the superconducting state at intermediate interaction strengths separates into two regimes by a small region of incommensurate spin-density-wave and spin-bond order, enabling the potential realization of chiral spin-bond order.

cond-mat.str-el↗

Supercurrent Growth in Nonequilibrium Superconductors

In ultrafast experiments on superconductors, a pump laser pulse often heats up the electronic system and suppresses the density of superfluid electrons. Subsequently, the electrons undergo a cooling process because of electron-phonon thermalization so that the superfluid density recovers in time. We study the nonequilibrium electromagnetic response of the system in this cooling process. We show that if a supercurrent is initiated by a probe electric field pulse, an intriguing phenomenon of `supercurrent growth' occurs, meaning that the net current grows in time with the increasing superfluid density. Using the Boltzmann kinetic equation, we uncover its microscopic origin as the momentum-relaxing scattering of Bogoliubov quasiparticles by impurities and phonons, in stark contrast to the widely accepted intuition that impurities always attenuate currents. We further show that supercurrent growth has important experimental manifestations, including the ultrafast Meissner effect and an optical reflectivity exceeding unity.

cond-mat.supr-con↗

Tailoring spontaneous symmetry breaking in engineered van der Waals superlattices

Superlattice engineering in van der Waals heterostructures (e.\,g.\ by moiré engineering) provides a powerful platform for designing electronic bands and realising correlated and topological quantum phenomena. Here, we pioneer a scheme to tailor superpotentials based on intrinsic substrate electronic orders. We show that this establishes a robust, self-aligned, and highly versatile route to band-structure control as we demonstrate in graphene by engineering two distinct, nearly commensurate superlattices using the charge density waves of 1T-NbSe$_2$. In these superlattices the graphene's Dirac cones are folded either to the $Γ$-point or to the K-points of the mini-Brillouin zone. Using scanning tunnelling microscopy, we observe that the $Γ$-folded system preserves C$_3$ symmetry, while the K-folded system exhibits spontaneous symmetry breaking. Combining density functional theory with an interlayer interaction model, we reveal that this difference is not electronically driven but originates from a structural instability. Our work establishes superlattice engineering for designer quantum states and unveils a structural mechanism for controlled emergent symmetry breaking.

cond-mat.mes-hall↗

Continuous unitary transformations using tensor network representations access the full many-body localized spectrum

We develop variational continuous unitary transformations (VCUTs), which integrate Wegner-Wilson flow equations with tensor network techniques to approximately diagonalize many-body localized (MBL) Hamiltonians. The diagonalizing unitary is represented as a matrix product operator whose bond dimension controls the accuracy. For the disordered Heisenberg chain, VCUTs accurately reproduces the full spectrum across the ergodic-to-MBL crossover at small system sizes and scales to $L = 48$ sites. Beyond eigenenergies, the method can track the spatial entanglement structure of the diagonalizing unitary $U(l)$ at each flow step, enabling identification of local integrals of motion deep in the MBL phase.

cond-mat.dis-nn↗

Floquet Engineering Magnetism and Superconductivity in the Square-Lattice Hubbard Model

We study the interplay of magnetic order and superconductivity in the square-lattice Hubbard model under periodic driving with circularly polarized light. Formulating diagrammatic techniques based on the random-phase approximation in terms of Floquet Green's functions, allows us to analyze fluctuation-driven unconventional pairing for weak-to-moderate interactions. The interplay of repulsive interactions and photo-assisted hopping of electrons gives rise to a rich magnetic phase diagram featuring an antiferromagnetic-to-ferromagnetic transition prior to a Floquet Lifshitz transition. Close to the antiferromagnetic transition, topological $d+id$-wave superconductivity prevails in the phase diagram for a wide range of drive parameters. At intermediate-to-high frequency driving near the Floquet Lifshitz transition, superconducting orders are tuned from spin-singlet $d$-wave to spin-triplet $p$-wave character, providing an effective protocol for Floquet engineering topological superconductivity.

cond-mat.str-el↗

Cavity control of multiferroic order in single-layer NiI$_2$

Controlling materials through their interactions with electromagnetic vacuum fluctuations is an emergent frontier in material engineering. Although recent experiments have demonstrated dark cavity effects for electronic material phases, like superconductivity, ferroelectricity and charge density waves, a smoking gun experiment for magnetic systems is lacking. Largely, this comes from the focus on phase transitions, where a large critical light-matter coupling is needed to observe cavity modifications. Here, we propose spiral magnets, where even a small cavity-mediated change in magnetic interactions is reflected in a change of the spiral wavelength, as a promising platform to observe cavity effects. We focus on the single-layer multiferroic NiI$_2$, interacting with electric field fluctuations from surface phonon polaritons of the paraelectric substrate SrTiO$_3$. With decreasing substrate-material distance, the ratio of nearest and third nearest neighbor exchange interactions reduces, leading to an increase of the spiral wavelength and an eventual transition into a ferromagnetic state. Our work identifies a realistic platform to observe cavity vacuum renormalization effects in magnetic systems.

cond-mat.mtrl-sci↗

Tree tensor networks for many-body localization in two dimensions

We investigate the disordered spin-$\frac12$Heisenberg model in two dimensions and employ tree tensor networks (TTNs) with a physics-informed structural optimization of the tree layout, to simulate dynamics in the many-body localization problem. We find that TTNs are able to capture two-dimensional entanglement patterns more effectively than matrix product states (MPS) while being more efficient to contract than projected entangled pair states (PEPS) to probe larger systems and longer times. Structural optimization of the trees based on time evolution of the entanglement in the system allows to keep the necessary bond dimensions low and to maximally exploit the increased expressiveness of TTNs over MPS. In this way, we achieve more accurate results in all considered parameter regimes both below and above the ergodicity-to-localization crossover at a comparable compute-time cost.

cond-mat.dis-nn↗