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Dante M. Kennes

Publications and source records attributed to Dante M. Kennes.

139 records · Page 8Linked to original sources

Blockade of vortex flow by thermal fluctuations in atomically thin clean-limit superconductors

Resistance in superconductors arises from the motion of vortices driven by flowing supercurrents or external electromagnetic fields and may be strongly affected by thermal or quantum fluctuations. The common expectation borne out in previous experiments is that as the temperature is lowered, vortex motion is suppressed, leading to a decreased resistance. A new generation of materials provides access to the previously inaccessible regime of clean-limit superconductivity in atomically thin superconducting layers. We show experimentally that for few-layer 2H-NbSe$_2$ the resistance below the superconducting transition temperature may be non-monotonic, passing through a minimum and then increasing again as temperature is decreased further. The effects exists over a wide range of current and magnetic fields, but is most pronounced in monolayer devices at intermediate currents. Analytical and numerical calculations confirm that the findings can be understood in a two-fluid vortex model, in which a fraction of vortices flow in channels while the rest are pinned but thermally fluctuating in position. We show theoretically that the pinned, fluctuating vortices effectively control the mobility of the free vortices. The findings provide a new perspective on fundamental questions of vortex mobility and dissipation in superconductors.

cond-mat.mes-hall↗

Floquet-engineered light-cone spreading of correlations in a driven quantum chain

We investigate the light-cone-like spread of electronic correlations in a laser-driven quantum chain. Using the time-dependent density matrix renormalization group, we show that high-frequency driving leads to a Floquet-engineered spread velocity that determines the enhancement of density-density correlations when the ratio of potential and kinetic energies is effectively increased both by either a continuous or a pulsed drive. For large times we numerically show the existence of a Floquet steady state at not too long distances on the lattice with minimal heating. Intriguingly, we find a discontinuity of dynamically scaled correlations at the edge of the light cone, akin to the discontinuity known to exist for quantum quenches in Luttinger liquids. Our work demonstrates the potential of pump-probe experiments for investigating light-induced correlations in low-dimensional materials and puts quantitative speed limits on the manipulation of long-ranged correlations through Floquet engineering.

cond-mat.str-el↗

Universal Optical Control of Chiral Superconductors and Majorana Modes

Chiral superconductors are a novel class of unconventional superconductors that host topologically protected chiral Majorana fermions at interfaces and domain walls, elusive quasiparticles that could serve as a platform for topological quantum computing. Here we show that, in analogy to a qubit, the out-of-equilibrium superconducting state in such materials can be described by a Bloch vector and controlled on ultrafast time scales. The all-optical control mechanism is universal, permitting arbitrary rotations of the order parameter, and can induce a dynamical change of handedness of the condensate. It relies on transient breaking of crystal symmetries via choice of pulse polarization to enable arbitrary rotations of the Bloch vector. The mechanism extends to ultrafast time scales, and importantly the engineered state persists after the pump is switched off. We demonstrate that these phenomena should appear in graphene or magic-angle twisted bilayer graphene (TBG), as well as Sr$_2$RuO$_4$, as candidate chiral $d+id$ and $p+ip$ superconductors, respectively. Furthermore, we show that chiral superconductivity can be detected in time-resolved pump-probe measurements. This paves the way towards a robust mechanism for ultrafast control and measurement of chirally-ordered phases and Majorana modes.

cond-mat.supr-con↗

Magic Angle Spectroscopy

The electronic properties of heterostructures of atomically-thin van der Waals (vdW) crystals can be modified substantially by Moiré superlattice potentials arising from an interlayer twist between crystals. Moiré-tuning of the band structure has led to the recent discovery of superconductivity and correlated insulating phases in twisted bilayer graphene (TBLG) near the so-called "magic angle" of $\sim$1.1°, with a phase diagram reminiscent of high T$_c$ superconductors. However, lack of detailed understanding of the electronic spectrum and the atomic-scale influence of the Moiré pattern has so far precluded a coherent theoretical understanding of the correlated states. Here, we directly map the atomic-scale structural and electronic properties of TBLG near the magic angle using scanning tunneling microscopy and spectroscopy (STM/STS). We observe two distinct van Hove singularities (vHs) in the LDOS which decrease in separation monotonically through 1.1° with the bandwidth (t) of each vHs minimized near the magic angle. When doped near half Moiré band filling, the conduction vHs shifts to the Fermi level and an additional correlation-induced gap splits the vHs with a maximum size of 7.5 meV. We also find that three-fold (C$_3$) rotational symmetry of the LDOS is broken in doped TBLG with a maximum symmetry breaking observed for states near the Fermi level, suggestive of nematic electronic interactions. The main features of our doping and angle dependent spectroscopy are captured by a tight-binding model with on-site (U) and nearest neighbor Coulomb interactions. We find that the ratio U/t is of order unity, indicating that electron correlations are significant in magic angle TBLG. Rather than a simple maximization of the DOS, superconductivity arises in TBLG at angles where the ratio U/t is largest, suggesting a pairing mechanism based on electron-electron interactions.

cond-mat.mes-hall↗

Multi-flat bands and strong correlations in Twisted Bilayer Boron Nitride

In a groundbreaking experimental advance it was recently shown that by stacking two sheets of graphene atop of each other at a twist angle close to one of the so called "magic angles", an effective two-dimensional correlated system emerges. In this system the kinetic energy of the low-energy electrons is much reduced and consequently interactions become very relevant, providing a new platform into the physics of two-dimensional correlated materials. Evidence of a proposed Mott insulating as well as superconducting state in these highly tunable systems has spurred much attention as they could pave the way to understanding long-standing questions of high-$T_c$ superconductivity or provide candidate systems for topological chiral superconductors; key to highly relevant quantum technologies. Here, we demonstrate that twisted bilayer boron nitride (TBBN) is an exciting and even richer alternative to twisted bilayer graphene (TBG). Crucially, we show that in TBBN multiple flat bands emerge without having to fine tuning close to a "magic angle" that upon doping lead to correlated phases of matter (insulating and superconducting). TBBN could thus be much less sensitive to small deviations in the twist angle and therefore provide a particularly suited experimental platform to study correlation physics in two dimensions. Furthermore, we find that in marked contrast to TBG at small twist angle families of 2,4 and 6-fold degenerate, well separated, bands emerge within the gap, considerably broadening the addressable physics.

cond-mat.mes-hall↗

Dynamics of the Anderson impurity model: benchmarking a non-adiabatic exchange-correlation potential in time-dependent density functional theory

In this comparative study we benchmark a recently developed non-adiabatic exchange-correlation potential within time-dependent density functional theory (TDDFT) (Phys.\ Rev.\ Lett.\ {\bf 120}, 157701 (2018)) by (a) validating the transient dynamics using a numerically exact density matrix renormalization group approach as well as by (b) comparing the $RC$-time, a typical linear response quantity, to upto second order perturbation theory results. As a testbed we use the dynamics of the single impurity Anderson model. These benchmarks show that the non-adiabatic functional yields quantitatively accurate results for the transient dynamics for temperatures of the order of the hybridization strength while the TDDFT $RC$-times quantitatively agree with those from second-order perturbation theory for temperatures which are large compared to the hybridization strength. Both results are particularly intriguing given the relatively low numerical cost of a TDDFT calculation (at least compared to exact approaches).

cond-mat.stat-mech↗

Light-induced d-wave superconductivity through Floquet-engineered Fermi surfaces in cuprates

We introduce a mechanism for light-induced Floquet engineering of the Fermi surface to dynamically tip the balance between competing instabilities in correlated condensed matter systems in the vicinity of a van-Hove singularity. We first calculate how the Fermi surface is deformed by an off-resonant, high-frequency light field and then determine the impact of this deformation on the ordering tendencies using an unbiased functional renormalization group approach. As a testbed, we investigate Floquet engineering in cuprates driven by light. We find that the $d$-wave superconducting ordering tendency in this system can be strongly enhanced over the Mott insulating one. This gives rise to extended regions of induced $d$-wave superconductivity in the effective phase diagram in the presence of a light field.

cond-mat.str-el↗

Strong Correlations and d+id Superconductivity in Twisted Bilayer Graphene

We compute the phase diagram of twisted bilayer graphene near the magic angle where the occurrence of flat bands enhances the effects of electron-electron interactions and thus unleashes strongly-correlated phenomena. Most importantly, we find a crossover between d+id superconductivity and Mott insulating behavior near half-filling of the lowest electron band when the temperature is increased. This is consistent with recent experiments. Our results are obtained using unbiased many-body renormalization group techniques combined with a mean-field analysis of the effective couplings.

cond-mat.str-el↗

Non-equilibrium Optical Conductivity: General Theory and Application to Transient Phases

A non-equilibrium theory of optical conductivity of dirty-limit superconductors and commensurate charge density wave is presented. We discuss the current response to different experimentally relevant light-field probe pulses and show that a single frequency definition of the optical conductivity $σ(ω)\equiv j(ω)/E(ω)$ is difficult to interpret out of the adiabatic limit. We identify characteristic time domain signatures distinguishing between superconducting, normal metal and charge density wave states. We also suggest a route to directly address the instantaneous superfluid stiffness of a superconductor by shaping the probe light field.

cond-mat.supr-con↗

Transport in quasiperiodic interacting systems: from superdiffusion to subdiffusion

Using a combination of numerically exact and renormalization-group techniques we study the nonequilibrium transport of electrons in an one-dimensional interacting system subject to a quasiperiodic potential. For this purpose we calculate the growth of the mean-square displacement as well as the melting of domain walls. While the system is nonintegrable for all studied parameters, there is no on finite region default of parameters for which we observe diffusive transport. In particular, our model shows a rich dynamical behavior crossing over from superdiffusion to subdiffusion. We discuss the implications of our results for the general problem of many-body localization, with a particular emphasis on the rare region Griffiths picture of subdiffusion.

cond-mat.dis-nn↗

Transient superconductivity from electronic squeezing of optically pumped phonons

Advances in light sources and time resolved spectroscopy have made it possible to excite specific atomic vibrations in solids and to observe the resulting changes in electronic properties but the mechanism by which phonon excitation causes qualitative changes in electronic properties, has remained unclear. Here we show that the dominant symmetry-allowed coupling between electron density and dipole active modes implies an electron density-dependent squeezing of the phonon state which provides an attractive contribution to the electron-electron interaction, independent of the sign of the bare electron-phonon coupling and with a magnitude proportional to the degree of laser-induced phonon excitation. Reasonable excitation amplitudes lead to non-negligible attractive interactions that may cause significant transient changes in electronic properties including superconductivity. The mechanism is generically applicable to a wide range of systems, offering a promising route to manipulating and controlling electronic phase behavior in novel materials.

cond-mat.supr-con↗

The quench dynamics of a dissipative quantum system: a renormalization group study

We study dissipation in a small quantum system coupled to an environment held in thermodynamic equilibrium. The relaxation dynamics of a system subject to an abrupt quench in the parameters of the underlying Hamiltonian is investigated using two complementary renormalization group approaches. The methods are applied to the Ohmic spin-boson model close to the coherent-to-incoherent transition. In particular, the role of non-Markovian memory for the relaxation before and after the quench of the spin-boson coupling and the Zeeman splitting of the up and down spin is investigated.

cond-mat.mes-hall↗

Quench dynamics of correlated quantum dots

We study the relaxation dynamics of a quantum dot with local Coulomb correlations coupled to two noninteracting leads which are held in grandcanonical equilibrium. Only charge degrees of freedom are considered and the dot is described by a model which in the scaling limit becomes equivalent to the interacting resonant level model. The time evolution of the current and dot occupancy resulting out of changes of the dot-lead coupling, the dots onsite energy, or the charging energy are studied. Abrupt and smooth parameter changes as well as setups with and without driving bias voltage are considered. For biased dots we investigate the often studied response after turning on the dot-lead coupling but also the experimentally more relevant case in which the voltage is turned on. We identify and explain a variety of interesting many-body effects and clarify the role of initial correlations.

cond-mat.str-el↗