arXiv subjects

Dao Xiang

Publications and source records attributed to Dao Xiang.

34 records · Page 2Linked to original sources

arXiv2021

Optical manipulation of electronic dimensionality in a quantum material

Exotic phenomenon can be achieved in quantum materials by confining electronic states into two dimensions. For example, relativistic fermions are realised in a single layer of carbon atoms, the quantized Hall effect can result from two-dimensional (2D) systems, and the superconducting transition temperature can be enhanced significantly in a one-atomic-layer material. Ordinarily, 2D electronic system can be obtained by exfoliating the layered materials, growing monolayer materials on substrates, or establishing interfaces between different materials. Herein, we use femtosecond infrared laser pulses to invert the periodic lattice distortion sectionally in a three-dimensional (3D) charge density wave material, creating macroscopic domain walls of transient 2D ordered electronic states with exotic properties. The corresponding ultrafast electronic and lattice dynamics are captured by time- and angle-resolved photoemission spectroscopy and MeV ultrafast electron diffraction. Surprisingly, a novel energy gap state, which might be a signature of light-induced superconductivity, is identified in the photoinduced 2D domain wall near the surface. Such optical modulation of atomic motion is a new path to realise 2D electronic states and will be a new platform for creating novel phases in quantum materials.

cond-mat.str-el↗

arXiv2021

Non-invasive time-sorting in radio-frequency compressed ultrafast electron diffraction

We demonstrate a non-invasive time-sorting method for ultrafast electron diffraction (UED) experiments with radio-frequency (rf) compressed electron beams. We show that electron beam energy and arrival time at the sample after rf compression are strongly correlated such that the arrival time jitter may be corrected through measurement of the beam energy. The method requires minimal change to the infrastructure of most of the UED machines and is applicable to both keV and MeV UED. In our experiment with ~3 MeV beam, the timing jitter after rf compression is corrected with 35 fs root-mean-square (rms) accuracy, limited by the 3x10^-4 energy stability. For keV UED with high energy stability, sub-10 fs accuracy in time-sorting should be readily achievable. This time-sorting technique allows us to retrieve the 2.5 THz oscillation related to coherent A1g phonon in laser excited Bismuth film and extends the temporal resolution of UED to a regime far beyond the 100-200 fs rms jitter limitation.

physics.acc-ph↗

arXiv2020

Achieving 50 femtosecond resolution in MeV ultrafast electron diffraction with a double bend achromat compressor

We propose and demonstrate a novel scheme to produce ultrashort and ultrastable MeV electron beam. In this scheme, the electron beam produced in a photocathode radio-frequency (rf) gun first expands under its own Coulomb force with which a positive energy chirp is imprinted in the beam longitudinal phase space. The beam is then sent through a double bend achromat with positive longitudinal dispersion where electrons at the bunch tail with lower energies follow shorter paths and thus catch up with the bunch head, leading to longitudinal bunch compression. We show that with optimized parameter sets, the whole beam path from the electron source to the compression point can be made isochronous such that the time of flight for the electron beam is immune to the fluctuations of rf amplitude. With a laser-driven THz deflector, the bunch length and arrival time jitter for a 20 fC beam after bunch compression are measured to be about 29 fs (FWHM) and 22 fs (FWHM), respectively. Such an ultrashort and ultrastable electron beam allows us to achieve 50 femtosecond (FWHM) resolution in MeV ultrafast electron diffraction where lattice oscillation at 2.6 THz corresponding to Bismuth A1g mode is clearly observed without correcting both the short-term timing jitter and long-term timing drift. Furthermore, oscillating weak diffuse scattering signal related to phonon coupling and decay is also clearly resolved thanks to the improved temporal resolution and increased electron flux. We expect that this technique will have a strong impact in emerging ultrashort electron beam based facilities and applications.

physics.acc-ph↗

arXiv2019

Femtosecond relativistic electron beam with reduced timing jitter from THz-driven beam compression

We propose and demonstrate a novel method to reduce the pulse width and timing jitter of a relativistic electron beam through THz-driven beam compression. In this method the longitudinal phase space of a relativistic electron beam is manipulated by a linearly polarized THz pulse in a dielectric tube such that the bunch tail has a higher velocity than the bunch head, which allows simultaneous reduction of both pulse width and timing jitter after passing through a drift. In this experiment, the beam is compressed by more than a factor of four from 130 fs to 28 fs with the arrival time jitter also reduced from 97 fs to 36 fs, opening up new opportunities in using pulsed electron beams for studies of ultrafast dynamics. This technique extends the well known rf buncher to the THz frequency and may have a strong impact in accelerator and ultrafast science facilities that require femtosecond electron beams with tight synchronization to external lasers.

physics.acc-ph↗

arXiv2019

Terahertz oscilloscope for recording time information of ultrashort electron beams

We propose and demonstrate a Terahertz (THz) oscilloscope for recording time information of an ultrashort electron beam. By injecting a laser-driven THz pulse with circular polarization into a dielectric tube, the electron beam is swept helically such that the time information is uniformly encoded into the angular distribution that allows one to characterize both the temporal profile and timing jitter of an electron beam. The dynamic range of the measurement in such a configuration is significantly increased compared to deflection with a linearly polarized THz pulse. With this THz oscilloscope, nearly 50-fold longitudinal compression of a relativistic electron beam to about 15 fs (rms) is directly visualized with its arrival time determined with 3 fs accuracy. This technique bridges the gap between streaking of photoelectrons with optical lasers and deflection of relativistic electron beams with radio-frequency deflectors, and should have wide applications in many ultrashort electron beam based facilities.

physics.acc-ph↗

arXiv2018

Few-femtosecond Electron Beam with THz-frequency Wakefield-driven Compression

We propose and demonstrate a novel method to produce few-femtosecond electron beam with relatively low timing jitter. In this method a relativistic electron beam is compressed from about 150 fs (rms) to about 7 fs (rms, upper limit) with the wakefield at THz frequency produced by a leading drive beam in a dielectric tube. By imprinting the energy chirp in a passive way, we demonstrate through laser-driven THz streaking technique that no additional timing jitter with respect to an external laser is introduced in this bunch compression process, a prominent advantage over the conventional method using radio-frequency bunchers. We expect that this passive bunching technique may enable new opportunities in many ultrashort-beam based advanced applications such as ultrafast electron diffraction and plasma wakefield acceleration.

physics.acc-ph↗

arXiv2018

Terahertz streaking of few-femtosecond relativistic electron beams

Streaking of photoelectrons with optical lasers has been widely used for temporal characterization of attosecond extreme ultraviolet pulses. Recently, this technique has been adapted to characterize femtosecond x-ray pulses in free-electron lasers with the streaking imprinted by farinfrared and Terahertz (THz) pulses. Here, we report successful implementation of THz streaking for time-stamping of an ultrashort relativistic electron beam of which the energy is several orders of magnitude higher than photoelectrons. Such ability is especially important for MeV ultrafast electron diffraction (UED) applications where electron beams with a few femtosecond pulse width may be obtained with longitudinal compression while the arrival time may fluctuate at a much larger time scale. Using this laser-driven THz streaking technique, the arrival time of an ultrashort electron beam with 6 fs (rms) pulse width has been determined with 1.5 fs (rms) accuracy. Furthermore, we have proposed and demonstrated a non-invasive method for correction of the timing jitter with femtosecond accuracy through measurement of the compressed beam energy, which may allow one to advance UED towards sub-10 fs frontier far beyond the ~100 fs (rms) jitter.

physics.acc-ph↗

arXiv2018

Imaging nanoscale spatial modulation of a relativistic electron beam with a MeV ultrafast electron microscope

Accelerator-based MeV ultrafast electron microscope (MUEM) has been proposed as a promising tool to study structural dynamics at the nanometer spatial scale and picosecond temporal scale. Here we report experimental tests of a prototype MUEM where high quality images with nanoscale fine structures were recorded with a pulsed 3 MeV picosecond electron beam. The temporal and spatial resolution of the MUEM operating in single-shot mode is about 4 ps (FWHM) and 100 nm (FWHM), corresponding to a temporal-spatial resolution of 4e-19 s*m, about 2 orders of magnitude higher than that achieved with state-of-the-art single-shot keV UEM. Using this instrument we offer the demonstration of visualizing the nanoscale periodic spatial modulation of an electron beam, which may be converted into longitudinal density modulation through emittance exchange to enable production of high-power coherent radiation at short wavelengths. Our results mark a great step towards single-shot nanometer-resolution MUEMs and compact intense x-ray sources that may have wide applications in many areas of science.

physics.acc-ph↗

arXiv2018

Coulomb-driven relativistic electron beam compression

Coulomb interaction between charged particles is a well-known phenomenon in many areas of researches. In general the Coulomb repulsion force broadens the pulse width of an electron bunch and limits the temporal resolution of many scientific facilities such as ultrafast electron diffraction and x-ray free-electron lasers. Here we demonstrate a scheme that actually makes use of Coulomb force to compress a relativistic electron beam. Furthermore, we show that the Coulomb-driven bunch compression process does not introduce additional timing jitter, which is in sharp contrast to the conventional radio-frequency buncher technique. Our work not only leads to enhanced temporal resolution in electron beam based ultrafast instruments that may provide new opportunities in probing material systems far from equilibrium, but also opens a promising direction for advanced beam manipulation through self-field interactions.

physics.acc-ph↗

arXiv2016

Measurements of Terahertz Radiation Generated using a Metallic, Corrugated Pipe

A method for producing narrow-band THz radiation proposes passing an ultra-relativistic beam through a metallic pipe with small periodic corrugations. We present results of a measurement of such an arrangement at Brookhaven's Accelerator Test Facility (ATF). Our pipe was copper and was 5 cm long; the aperture was cylindrically symmetric, with a 1 mm (radius) bore and a corrugation depth (peak-to-peak) of 60 um. In the experiment we measured both the effect on the beam of the structure wakefield and the spectral properties of the radiation excited by the beam. We began by injecting a relatively long beam compared to the wavelength of the radiation, but with short rise time, to excite the structure, and then used a downstream spectrometer to infer the radiation wavelength. This was followed by injecting a shorter bunch, and then using an interferometer (also downstream of the corrugated pipe) to measure the spectrum of the induced THz radiation. For the THz pulse we obtain and compare with calculations: the central frequency, the bandwidth, and the spectral power---compared to a diffraction radiation background signal.

physics.acc-ph↗

arXiv2016

Time-resolved Measurement of Quadrupole Wakefields in Corrugated Structures

Corrugated structures have recently been widely used for manipulating electron beam longitudinal phase space and for producing THz radiation. Here we report on time-resolved measurements of the quadrupole wakefields in planar corrugated structures. It is shown that while the time- dependent quadrupole wakefield produced by a planar corrugated structure causes significant growth in beam transverse emittance, it can be effectively canceled with a second corrugated structure with orthogonal orientation. The strengths of the time-dependent quadrupole wakefields for various corrugated structure gaps are also measured and found to be in good agreement with theories. Our work should forward the applications of corrugated structures in many accelerator based scientific facilities.

physics.acc-ph↗

arXiv2015

Demonstration of nonlinear-energy-spread compensation in relativistic electron bunches with corrugated structures

High quality electron beams with flat distributions in both energy and current are critical for many accelerator-based scientific facilities such as free-electron lasers and MeV ultrafast electron diffraction and microscopes. In this Letter we report on using corrugated structures to compensate for the beam nonlinear energy chirp imprinted by the curvature of the radio-frequency field, leading to a significant reduction in beam energy spread. By using a pair of corrugated structures with orthogonal orientations, we show that the quadrupole wake fields which otherwise increase beam emittance can be effectively canceled. This work also extends the applications of corrugated structures to the low beam charge (a few pC) and low beam energy (a few MeV) regime and may have a strong impact in many accelerator-based facilities.

physics.acc-ph↗

arXiv2014

A Multi-length Bunches Design for Electron Storage Rings with Odd Buckets

A scheme with two superconducting RF cavities (sc-cavities) is designed to upgrade electron storage rings with odd buckets into multi-length bunches. In this paper, Hefei Light Source II (HLS II) is given as an example for odd buckets. In accordance with 45 buckets, which is multiples of 3, three different length of bunches generated simultaneously is proposed in the presently applied user optics. The final result is to, without low-alpha optics, fill HLS II with long bunches of 50 ps length, medium bunches of 23 ps and short bunches of 6 ps. Each third buckets can be filled with short bunches, of which the current limit is up to 6.6 mA, more than 60 times the value of low-alpha mode. Moreover, particles tracking about beam dynamics performed by ELEGANT and calculations about beam instabilities are presented in this paper.

physics.acc-ph↗

arXiv2014

Beam by design: laser manipulation of electrons in modern accelerators

Accelerator-based light sources such as storage rings and free-electron lasers use relativistic electron beams to produce intense radiation over a wide spectral range for fundamental research in physics, chemistry, materials science, biology and medicine. More than a dozen such sources operate worldwide, and new sources are being built to deliver radiation that meets with the ever increasing sophistication and depth of new research. Even so, conventional accelerator techniques often cannot keep pace with new demands and, thus, new approaches continue to emerge. In this article, we review a variety of recently developed and promising techniques that rely on lasers to manipulate and rearrange the electron distribution in order to tailor the properties of the radiation. Basic theories of electron-laser interactions, techniques to create micro- and nano-structures in electron beams, and techniques to produce radiation with customizable waveforms are reviewed. We overview laser-based techniques for the generation of fully coherent x-rays, mode-locked x-ray pulse trains, light with orbital angular momentum, and attosecond or even zeptosecond long coherent pulses in free-electron lasers. Several methods to generate femtosecond pulses in storage rings are also discussed. Additionally, we describe various schemes designed to enhance the performance of light sources through precision beam preparation including beam conditioning, laser heating, emittance exchange, and various laser-based diagnostics. Together these techniques represent a new emerging concept of "beam by design" in modern accelerators, which is the primary focus of this article

physics.acc-ph↗

arXiv2013

Slippage effect on laser phase error amplification in seeded harmonic generation free-electron lasers

Free-electron lasers (FELs) seeded with external lasers hold great promise for generating high power radiation with nearly transform-limited bandwidth in soft x-ray region. However, it has been pointed out that the initial seed laser noise will be amplified by the frequency up-conversion process, which may degrade the quality of the output radiation produced by a harmonic generation scheme. In this paper, theoretical and simulation studies for laser phase error amplification in seeded FEL schemes with slippage effect taken into account are presented. It is found that, the seed laser imperfection experienced by the electron beam can be significantly smoothed by the slippage effect in the modulator when the slippage length is comparable to the laser pulse length. This smoothing effect allows one to preserve the excellent temporal coherence of seeded FELs in presence of large laser phase errors. For ultra-short UV seed lasers with FWHM around 16 fs, the slippage length in a modulator with ~30 undulator periods is typically comparable to the laser width; for longer seed laser pulses with FWHM around 80 fs, the slippage length can be made comparable to the laser width using a modulator tuned at the sub-harmonic of the UV seed laser. Three-dimensional simulations have been carried out for a soft x-ray facility using seed laser pulses with large frequency chirp and the results show that the sensitivity of the bandwidth of the seeded FEL to the initial frequency chirp can be significantly reduced by a proper design of the modulator such that the slippage length is comparable to the laser width. Our studies show that the tolerance on laser phase error for generating nearly transform-limited soft x-ray pulses in seeded FELs is much looser than previously thought and fully coherent radiation at nanometer wavelength may be reached with current technologies.

physics.acc-ph↗

arXiv2012

Reversible electron beam heating for suppression of microbunching instabilities at free-electron lasers

The presence of microbunching instabilities due to the compression of high-brightness electron beams at existing and future X-ray free-electron lasers (FELs) results in restrictions on the attainable lasing performance and renders beam imaging with optical transition radiation impossible. The instability can be suppressed by introducing additional energy spread, i.e., "heating" the electron beam, as demonstrated by the successful operation of the laser heater system at the Linac Coherent Light Source. The increased energy spread is typically tolerable for self-amplified spontaneous emission FELs but limits the effectiveness of advanced FEL schemes such as seeding. In this paper, we present a reversible electron beam heating system based on two transverse deflecting radio-frequency structures (TDSs) up and downstream of a magnetic bunch compressor chicane. The additional energy spread is introduced in the first TDS, which suppresses the microbunching instability, and then is eliminated in the second TDS. We show the feasibility of the microbunching gain suppression based on calculations and simulations including the effects of coherent synchrotron radiation. Acceptable electron beam and radio-frequency jitter are identified, and inherent options for diagnostics and on-line monitoring of the electron beam's longitudinal phase space are discussed.

physics.acc-ph↗