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Darian Hall

Publications and source records attributed to Darian Hall.

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Strange Metal Hall Effect in Underdoped BaFe$_2$(As$_{1-x}$P$_x$)$_2$

The unusual transport properties of strange metals point to the breakdown of the quasiparticle picture, the understanding of which remains one of the most vexing problems in physics. Here, we report investigations of the electrical Hall effect of the strange metal superconductor BaFe$_2$(As$_{1-x}$P$_x$)$_2$. We show that a doping-independent contribution to the Hall effect exists within a fan shaped region above a putative quantum critical point. This `strange metal Hall' contribution echoes many of the properties of the antiferromangetic Hall response, but attains universal properties that distinguish it from the effects of Fermi surface reconstruction. This is consistent with an underlying origin connected to the presence of critical fluctuations, tying it to observations of $T$-linear resistivity and the appearance of unconventional superconductivity.

cond-mat.supr-con

Eclipsing Kitaev: off-diagonal exchange governs the correlated high-field phases of $\beta$-Li$_2$IrO$_3$

We report a high-field thermodynamic study of the hyperhoneycomb Kitaev material $\beta$-Li$_2$IrO$_3$, using magnetotropic susceptibility to resolve its low-temperature field-angle phase diagram across the principal crystallographic planes in magnetic fields up to $60$ T. Rather than evolving directly from the low-field incommensurate state into a polarized regime, the system exhibits a strongly direction-dependent sequence of correlated phases. Most notably, for fields in the $ac$-plane, we identify an additional high-field phase that is absent in the other principal planes and exists only within a restricted region of field-angle space. This phase structure is naturally explained by the competition between magnetic field and bond-directional exchange interactions. Using a symmetry-based description supported by microscopic calculations within the $J$-$K$-$\Gamma$ model, we show that off-diagonal $\Gamma$ exchange couples the ferromagnetic and staggered magnetic orders and thereby stabilizes the observed correlated high-field phases. The measured angular dependence of the critical fields is quantitatively captured by this theory, identifying $\Gamma$ exchange as the key interaction controlling the high-field response. These results clarify why the promise of a field-induced spin liquid -- the notion that suppressing magnetic order might reveal the underlying Kitaev physics -- remains unfulfilled in candidate materials: even when the Kitaev interaction is large, off-diagonal exchange stabilizes symmetry-constrained correlated phases that instead preempt the polarized state.

cond-mat.str-el

From Knots to Crystals: Machine-Learned Potentials for Self-Assembling Topological Solitons in Liquid Crystals

Knotted fields in classical and quantum systems have long been recognized for their non-trivial topologies and particle-like behavior, but practical applications have been limited by the difficulty of stabilizing them. Recently, stable knotted solitonic textures--heliknotons--were discovered in chiral liquid crystals, forming adaptive crystal assemblies via elastic distortion-mediated interactions. We use machine learning to develop single-site coarse-grained potentials that accurately capture these chiral anisotropic effective interactions. The resulting potentials accurately reproduce experimentally observed heliknoton assemblies and enable simulations at length and time scales far beyond the range of fine-grained continuum models. This general framework is readily transferable to other topological solitons, providing a powerful route to understand, predict, and ultimately control their collective behavior and dynamics.

cond-mat.soft

Fusion and Fission of Particle-like Chiral Nematic Vortex Knots

Vortex knots have been seen decaying in many physical systems. Here we describe topologically protected vortex knots, which remain stable and undergo fusion and fission while conserving a topological invariant analogous to that of baryon number. While the host medium, a chiral nematic liquid crystal, exhibits intrinsic chirality, cores of the vortex lines are structurally achiral regions where twist cannot be defined. We refer to them as "dischiralation" vortex lines, in analogy to dislocations and disclinations in ordered media where, respectively, positional and orientational order is disrupted. Fusion and fission of these vortex knots, which we reversibly switch by electric pulses, vividly reveal the physical embodiments of knot theory's concepts like connected sums of knots. Our findings provide insights into related phenomena in fields ranging from cosmology to particle physics and can enable applications in electro-optics and photonics, where such fusion and fission processes can be used for controlling light.

cond-mat.soft

Analysis of Hopf solitons as generalized fold maps

The Hopf index, a topological invariant that quantifies the linking of preimage fibers, is fundamental to the structure and stability of hopfions. In this work, we propose a new mathematical framework for modeling hopfions with high Hopf index, drawing on the language of singularity theory and the topology of differentiable maps. At the core of our approach is the notion of a generalized Hopf map of order $n$, whose structure is captured via fold maps and their Stein factorizations. We demonstrate that this theoretical construction not only aligns closely with recent experimental observations of high-Hopf-index hopfions, but also offers a precise classification of the possible configurations of fiber pairs associated to distinct points. Our results thus establish a robust bridge between the geometry of singular maps and the experimentally observed topology of complex field configurations of hopfions in materials and other physical systems.

cond-mat.soft