arXiv subjects

Dario Ballarini

Publications and source records attributed to Dario Ballarini.

At least 19 recordsLinked to original sources

arXiv2026

Dynamical stabilisation of a quantum fluid using a single topological defect

The size and shape of a quantum fluid in equilibrium is strongly influenced by the inter-particle interactions. In the attractive interaction regime, atomic quantum fluids ultimately collapse in a violent process that expels most of the particles from the macroscopically occupied state. Here, we use a quantum fluid of light in propagating geometry as an analogue to a two-dimensional Bose-Einstein condensate (BEC) with large attractive interactions to show that non-trivial topology significantly alters the dynamical behaviour of the collapse, enhancing the BEC stability and delaying the collapse time by an order of magnitude. We measure direct experimental signatures of topology affecting quantum hydrodynamics, unveiling the inherent competition between attractive nonlinearities, that lead to the collapse, and the preservation of topological charge from a multi-charged vortex. We fully characterise the collapse process in coordinate space and the eventual `solitonification' of the system and connect it to the mode structure of the excitation spectrum.

cond-mat.quant-gas↗

arXiv2026

Geometric control of hyperbolic exciton-polariton condensate dimers

Coupled many-body quantum systems exhibit rich emergent physics with diverse stationary and dynamical behaviors. By engineering platforms with tunable and distinct coupling mechanisms, new insights emerge into the collective behavior of coupled many body systems. Particles can be exchanged via evanescent or ballistic coupling: the former, based on proximity, yields large spectral splitting, while the latter requires strict phase-matching, analogous to phase-coupled harmonic oscillators, and has a smaller impact on the energy landscape. We demonstrate an all-optically tunable quantum fluid dimer based on exciton-polariton condensates in a photonic crystal waveguide with hyperbolic (saddle-like) dispersion. Varying the dimer's angle relative to the grating tunes the coupling from evanescent to ballistic. We directly observe spectral features and mass flow shaped by the saddle dispersion. This work highlights photonic crystals as powerful platforms to explore condensed matter phenomena lying at the interface between delay-coupled nonlinear oscillators and tight binding physics.

physics.optics↗

arXiv2026

Dynamical development of long-range spatial coherence in non-equilibrium bosonic condensation

Development of spontaneous coherence is one of the hallmarks of bosonic condensation in a variety of physical systems, such as cold atoms, confined photons, and hybrid light-matter quasiparticles like exciton polaritons in semiconductors. While spatial coherence is well understood once a steady-state condensate has been established, its temporal evolution as the condensate forms is largely unexplored. Here, we explore the dynamical formation of a non-equilibrium, driven-dissipative exciton-polariton condensate through both time-resolved experiments and numerical modeling. Our study reveals that the spatial coherence is established through two distinct stages. The early-time stage is interaction-driven and features transient oscillations in spatial coherence. This stage is followed by a steady-state regime characterized by a spatially-uniform high degree of coherence that extends over the entire size of the system and persists over time. These stages of spatial coherence development occur in both free flowing and confined exciton-polariton systems that undergo a quench - rapid growth of the condensate starting from two different initial settings. Our study offers a deep insight into the process by which long-range spatial coherence is established in a non-equilibrium bosonic condensate.

cond-mat.quant-gas↗

arXiv2026

Very strong light-matter coupling in patterned GaAs heterostructures

The very strong light-matter coupling regime enables the non-perturbative modification of matter properties via light. Using a patterned GaAs/AlGaAs waveguide with twelve wide quantum wells, we demonstrate hybridization of heavy- and light-hole excitons within a single polariton state and show that, at finite magnetic field, the presence of the light-hole exciton suppresses coupling to the heavy-hole Rydberg excitons and unbound scattering states. We develop a fully microscopic theory that accounts for the combined effects of the magnetic field and light-matter coupling on the excitons, providing an accurate description of the experimental results beyond a perturbative coupled-oscillator framework. This identifies quantum well width as a key control parameter for engineering the light-induced hybridization of matter wave functions in polaritons, which, in turn, can play a crucial role in the optical non-linearities.

cond-mat.mes-hall↗

arXiv2026

Magnetic-field driven hybridization of heavy- and light-hole Rydberg excitons in GaAs quantum wells

We present a combined theoretical and experimental study of ground and excited Rydberg exciton states in wide GaAs quantum wells exposed to a magnetic field in the Faraday geometry. We employ a multiband exciton model based on the Luttinger Hamiltonian, which captures valence-band mixing between heavy- and light-hole states induced by both the quantum well confinement and the magnetic field, and we develop an efficient numerical approach to solve for both ground- and excited-state excitons. The method treats Coulomb interactions, magnetic confinement, and band mixing on an equal footing, enabling a systematic characterization of exciton energies, oscillator strengths, and orbital composition. We show that band hybridization increases with magnetic field and is significantly more pronounced for higher excited states, where it sets in at lower fields and strongly modifies their properties. The theoretical predictions are validated by polarization-resolved magneto-reflectance measurements up to 9 T on GaAs/Al$_{0.4}$Ga$_{0.6}$As quantum wells of 20 nm width. We find excellent agreement for both the diamagnetic shift and Zeeman splitting of the ground state and the first four Rydberg excitons. Our results demonstrate that valence-band mixing plays a crucial role in determining the magnetic-field dependence of excited exciton states and must be properly included for a quantitative description of magneto-excitons in wide GaAs quantum wells.

cond-mat.mes-hall↗

arXiv2026

Exciton-Tunable Phase Control and Superstrong Coupling Through Multimode Polariton Engineering in Planar Waveguides

Strong light-matter coupling in optical waveguides provides a versatile platform for engineering hybrid polaritonic modes and their dispersion. Here we investigate multimode exciton-photon coupling in visible semiconductor waveguides supporting several transverse electric modes. Using rigorous coupled-wave analysis combined with a coupled-oscillator model, we show that the photonic band structure can be engineered across a range of regimes, from conventional multimode strong coupling to the superstrong coupling regime, where the Rabi splitting becomes comparable to the spacing between adjacent photonic modes. In the latter regime, hybridization between orthogonal electromagnetic modes is enabled by restricting the active material to a subregion of the mode volume where the photonic modes exhibit strong mutual overlap. This breaking of the orthogonality leads to polaritonic branches whose composition can be tuned among several photonic modes and the exciton. We demonstrate that small shifts of the exciton resonance produce pronounced changes in the propagation constants of different polariton branches, enabling exciton-controlled phase modulation through modal interference and, in the superstrong coupling regime, direct modal switching across a continuous S-shaped dispersion. The resulting figures of merit predict $π$ phase shifts for exciton energy shifts of only a few meV over propagation lengths of tens of micrometers, while larger shifts are still required for mode switching. These results establish multimode waveguide polaritons as a versatile platform spanning multiple coupling regimes, for compact phase and intensity control in integrated photonic architectures.

physics.optics↗

arXiv2026

Pulse, polarization and topology shaping of polariton fuids

Here we present different approaches to ultrafast pulse and polarization shaping, based on a ``quantum fluid'' platform of polaritons. Indeed we exploit the normal modes of two dimensional polariton fluids made of strong coupled quantum well excitons and microcavity photons, by rooting different polarization and topological states into their sub-picosecond Rabi oscillations. Coherent control of two resonant excitation pulses allows us to prepare the desired state of the polariton, taking benefit from its four-component features given by the combination of the two normal modes with the two degrees of polarization. An ultrafast imaging based on the digital off-axis holography technique is implemented to study the polariton complex wavefunction with time and space resolution. We show in order coherent control of the polariton state on the Bloch sphere, an ultrafast polarization sweeping of the Poincaré sphere, and the dynamical twist of full Poincaré states such as the skyrmion on the sphere itself. Finally, we realize a new kind of ultrafast swirling vortices by adding the angular momentum degree of freedom to the two-pulse scheme. These oscillating topology states are characterized by one or more inner phase singularities tubes which spirals around the axis of propagation. The mechanism is devised in the splitting of the vortex into the upper and lower polaritons, resulting in an oscillatory exchange of energy and angular momentum and in the emitted time and space structured photonic packets.

cond-mat.other↗

arXiv2026

Dynamical universality in a driven quantum fluid of light

Universal scaling near phase transitions is one of the central ideas of physics, linking the growth of spatial correlations to the slowing down of dynamics. So far, direct experimental access to this critical behavior has remained largely confined to equilibrium many-body systems, and especially to static critical behavior. Here we probe how universality emerges in a driven quantum fluid of light formed by exciton--polaritons in a semiconductor microcavity. By probing the fluctuation-dominated disordered phase below the condensation threshold, we directly measure both the static growth of the correlation length $ξ$ and the dynamical slowing down of the relaxation time $τ$. We find that these quantities obey the universal relation $τ\propto ξ^{z}$ with dynamical exponent $z \approx 2$, revealing diffusive dynamics of a non-conserved order parameter. Our results extend the physics of critical dynamics from equilibrium matter to driven optical systems, bridging quantum condensates and lasers.

cond-mat.quant-gas↗

arXiv2025

Fully Integrated Perovskite Polaritonic Circuits with Tunable Lasing and Nonlinear Amplification

Photonic integrated circuits are emerging as a key technology for compact and energy-efficient optical information processing. Yet, their practical implementation remains limited by the intrinsically weak optical nonlinearities of conventional materials, which demand high power and large footprints to achieve significant nonlinear responses. Exciton-polaritons, hybrid light-matter excitations of semiconducting materials, offer a promising solution by combining strong optical nonlinearities with the high speed and large scalability typical of photonic devices. However, despite their potential, working on-chip polaritonic elements demonstrating room temperature coherent lasing, controllable nonlinear propagation, or amplification have remained elusive. Here we demonstrate a fully integrated perovskite polaritonic circuit that overcomes these limitations. Using a single-step microfluidic lithographic technique, we realize waveguide circuits with integrated gratings that simultaneously act as couplers and mirrors, forming in-plane Fabry-Pérot cavities. These structures support robust in-plane polariton lasing between gratings, yielding coherent emission along the waveguide. Furthermore, we observe clear signatures of strong nonlinear self-phase modulation and, for the first time, optical amplification of guided polaritons at room temperature. Our simple, scalable platform opens the way to low-power, highly nonlinear optical circuits for integrated photonics and neuromorphic architectures operating at room temperature.

physics.optics↗

arXiv2025

Topological Pathways to Two-Dimensional Quantum Turbulence

We present a combined experimental and theoretical investigation of the formation and decay kinetics of vortices in two dimensional, compressible quantum turbulence. We follow the temporal evolution of a quantum fluid of exciton polaritons, hybrid light matter quasiparticles, and measure both phase and modulus of the order parameter in the turbulent regime. Fundamental topological conservation laws require that the formation and annihilation of vortices also involve critical points of the velocity field, namely nodes and saddles. Identifying the simplest mechanisms underlying these processes enables us to develop an effective kinetic model that closely aligns with the experimental observations, and shows that different processes are responsible for vortex number growth and decay. These findings underscore the crucial role played by topological constraints in shaping nonlinear, turbulent evolution of two dimensional quantum fluids.

cond-mat.quant-gas↗

arXiv2025

Microfluidic-Assisted Growth of Perovskite Microwires for Room-Temperature All-Optical Switching Based on Total Internal Reflection

The development of efficient integrated photonic circuits is fundamental for ongoing research in information processing and computer science. The greatest challenge in strong light-matter regime facing photonic systems is achieving strong nonlinearities, which are exploitable in strongly coupled systems, leading to the formation of exciton-polaritons. In this context, the use of hybrid organic-inorganic perovskites offers a promising alternative, exhibiting robust interactions at Room Temperature (RT). However, the development of perovskite-based integrated devices requires both the ability to achieve long in-plane propagation, and the development of alternative fabrication approaches tailored to perovskite materials, designed to preserve their optical properties and prevent degradation. Herein, we present the realization of a proof-of-concept all-optical switch using propagating polaritons confined in Total Internal Reflection (TIR), which ensures long in-plane propagation and limited optical losses. We realized an efficient injection/extraction of the TIR-confined waveguide polariton modes by employing gold grating couplers prepatterned on the substrate.

physics.optics↗

arXiv2025

Directional optical parametric amplification in a hyperbolic metamaterial

Optical parametric amplification (OPA) comprises essentially a nonlinear four-wave mixing process in which a "pump" and a "signal" field give rise to an "idler" field under certain phase-matching conditions. Here we use a photonic crystal waveguide strongly-coupled with an excitonic reservoir to generate this process between different guided modes at optical wavelengths. Differently from classical nonlinear optical crystals, where the pump and idler photons travel almost collinearly, our exciton-polaritons are naturally separated in the waveguide due to their opposite group velocities. Due to the high efficiency of the process we can generate the idler field of the parametric process by pumping with a continuous wave laser and choose its direction of propagation in the waveguide by adjusting the angle of incidence of the seed laser. We show the OPA process to be robust against surface defects of the waveguide and can lead to simple-to-fabricate devices compared to microcavities that take advantage of strong signal-idler correlations in a propagating geometry. Our results closely agree with mean-field numerical simulations.

physics.optics↗

arXiv2024

Condensation dynamics in a two-dimensional photonic crystal waveguide

Exciton-polariton condensation occurs at the extrema of the underlying dispersion where the density of states diverges and carriers can naturally accumulate. The existence of multiple such points leads to coupling and competition between the associated modes and dynamical redistribution of the carriers in the dispersion. Here, we directly engineer the above situation via subwavelength periodic patterning of a two-dimensional nanostructure. This leads to multimode condensation into a pair of symmetric condensates that form at high-momenta, accidental-coupling points, and a high-symmetry $Γ$-point with a bound-in-the-continuum (BiC) state. The dynamical behaviour of the system reveals the non-simultaneous appearance of these condensates and the interplay of non-trivial gain and relaxation mechanisms. We fully characterise the quasi-static and dynamical regime of this artificial crystal and the properties of the different condensates. This understanding is necessary when band-structure engineering techniques are used to achieve precise control of condensate formation with given energy and momentum.

physics.optics↗

arXiv2024

Enhanced polariton interactions in suspended WS2 monolayer microcavity

Transition-metal dichalcogenides monolayers exhibit strong exciton resonances that enable intense light-matter interactions at room temperature (RT). However, the sensitivity of these materials to the surrounding environment and their intense interactions with the sustaining substrate result in the enhancement of excitonic losses through scattering, dissociation and defects formation, hindering their full potential for the excitation of optical nonlinearities in exciton-polariton platforms. From this point of view, the use of suspended monolayers holds the potential to completely eliminate substrate-induced losses, offering unique advantages for the investigation and exploitation of intrinsic electronic, mechanical, and optical properties of 2D materials based polaritonic systems, without any influence of proximity effects of all sort. In this work, we report a novel fabrication approach enabling the realization of a planar λ/2 microcavity filled with a suspended WS2 monolayer in its centre. In such a system, we experimentally demonstrate a 2-fold enhancement of the strong coupling at RT, due to reduced overall losses as compared to similar systems based on dielectric-filled microcavities. Moreover, as a result of minimized losses, spin-dependent polaritonic interactions in our platform are significantly amplified, leading to achievement of a record exciton interaction constant approaching the theoretically predicted value at RT, without making use of theoretical hypothesis on the effective polariton densities. This approach holds promises for pushing 2D materials-based polaritonic systems to their intrinsic limits, paving the way for the realization of novel polaritonic devices with superior performance.

physics.optics↗

arXiv2024

Exciton-polariton ring Josephson junction

Macroscopic coherence in quantum fluids allows the observation of interference effects in their wavefunctions, and enables applications such as superconducting quantum interference devices based on Josephson tunneling. The Josephson effect manifests in both fermionic and bosonic systems, and has been well studied in superfluid helium and atomic Bose-Einstein condensates. In exciton-polariton condensates - that offer a path to integrated semiconductor platforms - creating weak links in ring geometries has so far remained challenging. In this work, we realize a Josephson junction in a polariton ring condensate. Using optical control of the barrier, we induce net circulation around the ring and demonstrate both superfluid-hydrodynamic and the Josephson regime characterized by a sinusoidal tunneling current. Our theory in terms of the free-energy landscapes explains the appearance of these regimes using experimental values. These results show that weak links in ring condensates can be explored in optical integrated circuits and hold potential for room-temperature applications.

cond-mat.mes-hall↗

arXiv2024

Reconfigurable quantum fluid molecules of bound states in the continuum

Topological bound states in the continuum are confined wave-mechanical objects that offer advantageous ways to enhance light-matter interactions in compact photonic devices. In particular, their large quality factor in the strong-coupling regime has recently enabled the demonstration of Bose-Einstein condensation of bound-state-in-the-continuum polaritons. Here, we show that condensation into a negative-mass bound state in the continuum exhibits interaction-induced state confinement, opening opportunities for optically reprogrammable molecular arrays of quantum fluids of light. We exploit this optical trapping mechanism to demonstrate that such molecular complexes show hybridization with macroscopic modes with unusual topological charge multiplicity. Additionally, we demonstrate the scalability of our technique by constructing extended mono- and diatomic chains of bound-state-in-the-continuum polariton fluids that display non-Hermitian band formation and the opening of a minigap. Our findings offer insights into large-scale, reprogrammable, driven, dissipative many-body systems in the strong-coupling regime.

physics.optics↗

arXiv2024

Emerging supersolidity from a polariton condensate in a photonic crystal waveguide

A supersolid is a counter-intuitive phase of matter where its constituent particles are arranged into a crystalline structure, yet they are free to flow without friction. This requires the particles to share a global macroscopic phase while being able to reduce their total energy by spontaneous, spatial self-organisation. This exotic state of matter has been achieved in different systems using Bose-Einstein condensates coupled to cavities, possessing spin-orbit coupling, or dipolar interactions. Here we provide experimental evidence of a new implementation of the supersolid phase in a novel non-equilibrium context based on exciton-polaritons condensed in a topologically non-trivial, bound-in-the-continuum state with exceptionally low losses. We measure the density modulation of the polaritonic state indicating the breaking of translational symmetry with a remarkable precision of a few parts in a thousand. Direct access to the phase of the wavefunction allows us to additionally measure the local coherence of the superfluid component. We demonstrate the potential of our synthetic photonic material to host phonon dynamics and a multimode excitation spectrum.

cond-mat.mes-hall↗

arXiv2023

Room temperature polariton condensation from Whispering gallery modes in CsPbBr3 microplatelets

Room temperature (RT) polariton condensate holds exceptional promise for revolutionizing various fields of science and technology, encompassing optoelectronics devices to quantum information processing. Using perovskite materials like all-inorganic CsPbBr3 single crystal provides additional advantages, such as ease of synthesis, cost-effectiveness, and compatibility with existing semiconductor technologies. In this work, we show the formation of whispering gallery modes (WGM) in CsPbBr3 single crystals with controlled geometry, synthesized using a lowcost and efficient capillary bridge method. Through the implementation of microplatelets geometry, we achieve enhanced optical properties and performance thanks to the presence of sharp edges and a uniform surface, effectively avoiding non-radiative scattering losses caused by defects. This allows us not only to observe strong light matter coupling and formation of whispering gallery polaritons, but also to demonstrate the onset of polariton condensation at RT. This investigation not only contributes to the advancement of our knowledge concerning the exceptional optical properties of perovskite-based polariton systems, but also unveils prospects for the exploration of WGM polariton condensation within the framework of a 3D perovskite-based platform, working at RT. The unique characteristics of polariton condensate, including low excitation thresholds and ultrafast dynamics, open up unique opportunities for advancements in photonics and optoelectronics devices.

physics.optics↗