arXiv subjects

Dario Gerace

Publications and source records attributed to Dario Gerace.

At least 55 records · Page 3Linked to original sources

arXiv2020

Quantum computers as universal quantum simulators: state-of-art and perspectives

The past few years have witnessed the concrete and fast spreading of quantum technologies for practical computation and simulation. In particular, quantum computing platforms based on either trapped ions or superconducting qubits have become available for simulations and benchmarking, with up to few tens of qubits that can be reliably initialized, controlled, and measured. The present review aims at giving a comprehensive outlook on the state of art capabilities offered from these near-term noisy devices as universal quantum simulators, i.e. programmable quantum computers potentially able to calculate the time evolution of many physical models. First, we give a pedagogic overview on the basic theoretical background pertaining digital quantum simulations, with a focus on hardware-dependent mapping of spin-type Hamiltonians into the corresponding quantum circuit model as a key initial step towards simulating more complex models. Then, we review the main experimental achievements obtained in the last decade regarding the digital quantum simulation of such spin models, mostly employing the two leading quantum architectures. We compare their performances and outline future challenges, also in view of prospective hybrid technologies, towards the ultimate goal of reaching the long sought quantum advantage for the simulation of complex many body models in the physical sciences.

quant-ph↗

arXiv2020

Selective tuning of optical modes in a silicon comb-like photonic crystal cavity

Realizing multiply resonant photonic crystal cavities with large free spectral range is key to achieve integrated devices with highly efficient nonlinear response, such as frequency conversion, four-wave mixing, and parametric oscillation. This task is typically difficult owing to the cavity modes' sensitivity to fabrication disorder, which makes it hard to reliably achieve a comb-like spectrum of equally spaced modes even when a perfect matching is theoretically predicted. Here we show that a comb-like spectrum of up to 8 modes with very high quality factor and diffraction limited volumes can be engineered in the bichromatic-type potential of a two-dimensional photonic crystal cavity fabricated in a thin silicon membrane. To cope with the tight tolerance in terms of frequency spacings and resonance linewidths, we develop a permanent post-processing technique that allows the selective tuning of individual confined modes, thus achieving an almost perfect frequency matching of high Q resonances with record finesse in silicon microresonators. Our experimental results are extremely promising in view of ultra-low power nonlinear photonics in silicon.

physics.optics↗

arXiv2020

Inverse design of photonic crystals through automatic differentiation

Gradient-based inverse design in photonics has already achieved remarkable results in designing small-footprint, high-performance optical devices. The adjoint variable method, which allows for the efficient computation of gradients, has played a major role in this success. However, gradient-based optimization has not yet been applied to the mode-expansion methods that are the most common approach to studying periodic optical structures like photonic crystals. This is because, in such simulations, the adjoint variable method cannot be defined as explicitly as in standard finite-difference or finite-element time- or frequency-domain methods. Here, we overcome this through the use of automatic differentiation, which is a generalization of the adjoint variable method to arbitrary computational graphs. We implement the plane-wave expansion and the guided-mode expansion methods using an automatic differentiation library, and show that the gradient of any simulation output can be computed efficiently and in parallel with respect to all input parameters. We then use this implementation to optimize the dispersion of a photonic crystal waveguide, and the quality factor of an ultra-small cavity in a lithium niobate slab. This extends photonic inverse design to a whole new class of simulations, and more broadly highlights the importance that automatic differentiation could play in the future for tracking and optimizing complicated physical models.

physics.optics↗

arXiv2020

Tailoring dispersion of room temperature exciton-polaritons with perovskite-based subwavelength metasurfaces

Exciton-polaritons, elementary excitations arising from the strong coupling regime between photons and excitons in insulators or semiconductors, represent a promising platform for studying quantum fluids of light and realizing prospective all-optical devices. Among different materials for room temperature polaritonic devices, two-dimensional (2D) layered perovskites have recently emerged as one of the promising candidates thanks to their prominent excitonic features at room temperature. Here we report on the experimental demonstration of exciton-polaritons at room temperature in resonant metasurfaces made from a subwavelength 2D lattice of perovskite pillars. These metasurfaces are obtained via spincoating, followed by crystallization of the perovskite solution in a pre-patterned glass backbone. The strong coupling regime is revealed by both angular-resolved reflectivity and photoluminescence measurements, showing anticrossing between photonic modes and the exciton resonance with a Rabi splitting in the 200 meV range. Moreover, we show that the polaritonic dispersion can be engineered by tailoring the photonic Bloch mode to which perovskite excitons are coupled. Linear, parabolic, and multi-valley polaritonic dispersions are experimentally demonstrated. All of our results are perfectly reproduced by both numerical simulations based on a rigorous coupled wave analysis and an elementary model based on a quantum theory of radiation-matter interaction. Our results suggest a new approach to study exciton-polaritons and pave the way towards large-scale and low-cost integrated polaritonic devices operating at room temperature.

physics.optics↗

arXiv2019

Quantum implementation of an artificial feed-forward neural network

Artificial intelligence algorithms largely build on multi-layered neural networks. Coping with their increasing complexity and memory requirements calls for a paradigmatic change in the way these powerful algorithms are run. Quantum computing promises to solve certain tasks much more efficiently than any classical computing machine, and actual quantum processors are now becoming available through cloud access to perform experiments and testing also outside of research labs. Here we show in practice an experimental realization of an artificial feed-forward neural network implemented on a state-of-art superconducting quantum processor using up to 7 active qubits. The network is made of quantum artificial neurons, which individually display a potential advantage in storage capacity with respect to their classical counterpart, and it is able to carry out an elementary classification task which would be impossible to achieve with a single node. We demonstrate that this network can be equivalently operated either via classical control or in a completely coherent fashion, thus opening the way to hybrid as well as fully quantum solutions for artificial intelligence to be run on near-term intermediate-scale quantum hardware.

quant-ph↗

arXiv2019

Optimal efficiency of the Q-cycle mechanism around physiological temperatures from an open quantum systems approach

The Q-cycle mechanism entering the electron and proton transport chain in oxygenic photosynthesis is an example of how biological processes can be efficiently investigated with elementary microscopic models. Here we address the problem of energy transport across the cellular membrane from an open quantum system theoretical perspective. We model the cytochrome $b_6f$ protein complex under cyclic electron flow conditions starting from a simplified kinetic model, which is hereby revisited in terms of a quantum master equation formulation and spin-boson Hamiltonian treatment. We apply this model to theoretically demonstrate an optimal thermodynamic efficiency of the Q-cycle around ambient and physiologically relevant temperature conditions. Furthermore, we determine the quantum yield of this complex biochemical process after setting the electrochemical potentials to values well established in the literature. The present work suggests that the theory of quantum open systems can successfully push forward our theoretical understanding of complex biological systems working close to the quantum/classical boundary.

quant-ph↗

arXiv2019

Doubly-resonant $χ^{(2)}$ nonlinear photonic crystal cavity based on a bound state in the continuum

Photonic nanostructures simultaneously maximizing spectral and spatial overlap between fundamental and second-harmonic confined modes are highly desirable for enhancing second-order nonlinear effects in nonlinear media. These conditions have thus far remained challenging to satisfy in photonic crystal cavities because of the difficulty in designing a band gap at the second-harmonic frequency. Here, we solve this issue by using instead a bound state in the continuum at that frequency, and we design a doubly-resonant photonic crystal slab cavity with strongly improved figures of merit for nonlinear frequency conversion when compared to previous photonic crystal designs. Furthermore, we show that the far-field emission at both frequencies is highly collimated around normal incidence, which allows for simultaneously efficient pump excitation and collection of the generated nonlinear signal. Our results could lead to unprecedented conversion efficiencies in both parametric down conversion and second harmonic generation in an extremely compact architecture.

physics.optics↗

arXiv2018

An Artificial Neuron Implemented on an Actual Quantum Processor

Artificial neural networks are the heart of machine learning algorithms and artificial intelligence protocols. Historically, the simplest implementation of an artificial neuron traces back to the classical Rosenblatt's `perceptron', but its long term practical applications may be hindered by the fast scaling up of computational complexity, especially relevant for the training of multilayered perceptron networks. Here we introduce a quantum information-based algorithm implementing the quantum computer version of a perceptron, which shows exponential advantage in encoding resources over alternative realizations. We experimentally test a few qubits version of this model on an actual small-scale quantum processor, which gives remarkably good answers against the expected results. We show that this quantum model of a perceptron can be used as an elementary nonlinear classifier of simple patterns, as a first step towards practical training of artificial quantum neural networks to be efficiently implemented on near-term quantum processing hardware.

quant-ph↗

arXiv2016

Visible quantum plasmonics from metallic nanodimers

We report theoretical evidence that bulk nonlinear materials weakly interacting with highly localized plasmonic modes in ultra-sub-wavelength metallic nanostructures can lead to nonlinear effects at the single plasmon level in the visible range. In particular, the two-plasmon interaction energy in such systems is numerically estimated to be comparable with the typical plasmon linewidths. Localized surface plasmons are thus predicted to exhibit a purely nonclassical behavior, which can be clearly identified by a sub-Poissonian second-order correlation in the signal scattered from the quantized plasmonic field under coherent electromagnetic excitation. We explicitly show that systems sensitive to single-plasmon scattering can be experimentally realized by combining electromagnetic confinement in the interstitial region of gold nanodimers with local infiltration or deposition of ordinary nonlinear materials. We also propose configurations that could allow to realistically detect such an effect with state-of-the-art technology, overcoming the limitations imposed by the short plasmonic lifetime.

cond-mat.mes-hall↗

arXiv2016

Efficient continuous-wave nonlinear frequency conversion in high-Q Gallium Nitride photonic crystal cavities on Silicon

We report on nonlinear frequency conversion from the telecom range via second harmonic generation (SHG) and third harmonic generation (THG) in suspended gallium nitride slab photonic crystal (PhC) cavities on silicon, under continuous-wave resonant excitation. Optimized two-dimensional PhC cavities with augmented far-field coupling have been characterized with quality factors as high as 4.4$\times10^{4}$, approaching the computed theoretical values. The strong enhancement in light confinement has enabled efficient SHG, achieving normalized conversion efficiency of 2.4$\times10^{-3}$ $W^{-1}$, as well as simultaneous THG. SHG emission power of up to 0.74 nW has been detected without saturation. The results herein validate the suitability of gallium nitride for integrated nonlinear optical processing.

physics.optics↗

arXiv2016

Laser from a Manybody Correlated Medium

We consider a non-equilibrium system of interacting emitters described by the XXZ model, whose excitonic transitions are spatially and spectrally coupled to a single mode cavity. We demonstrate that the output radiation field is sensitive to an interplay between the hopping ($J$) and the interactions ($U$) of the excitons. Moderate values of the short-ranged interaction are shown to induce laser with maximal output at the Heisenberg point ($U=J$). In the laser regime, charge-charge correlations emerge and they are shown to strongly depend on the interaction-hopping ratio. In particular, the system shows charge-density correlations below the Heisenberg point and ferromagnetic correlations beyond the Heisenberg point. This contrast to the equilibrium behavior of the XXZ chain occurs since the laser explores highly excited states of the emitters.

quant-ph↗

arXiv2015

YBCO microwave resonators for strong collective coupling with spin ensembles

Coplanar microwave resonators made of 330 nm-thick superconducting YBCO have been realized and characterized in a wide temperature ($T$, 2-100 K) and magnetic field ($B$, 0-7 T) range. The quality factor $Q_L$ exceeds 10$^4$ below 55 K and it slightly decreases for increasing fields, remaining 90$\%$ of $Q_L(B=0)$ for $B=7$ T and $T=2$ K. These features allow the coherent coupling of resonant photons with a spin ensemble at finite temperature and magnetic field. To demonstrate this, collective strong coupling was achieved by using DPPH organic radical placed at the magnetic antinode of the fundamental mode: the in-plane magnetic field is used to tune the spin frequency gap splitting across the single-mode cavity resonance at 7.75 GHz, where clear anticrossings are observed with a splitting as large as $\sim 82$ MHz at $T=2$ K. The spin-cavity collective coupling rate is shown to scale as the square root of the number of active spins in the ensemble.

quant-ph↗

arXiv2015

Digital quantum simulators in a scalable architecture of hybrid spin-photon qubits

Resolving quantum many-body problems represents one of the greatest challenges in physics and physical chemistry, due to the prohibitively large computational resources that would be required by using classical computers. A solution has been foreseen by directly simulating the time evolution through sequences of quantum gates applied to arrays of qubits, i.e. by implementing a digital quantum simulator. Superconducting circuits and resonators are emerging as an extremely-promising platform for quantum computation architectures, but a digital quantum simulator proposal that is straightforwardly scalable, universal, and realizable with state-of-the-art technology is presently lacking. Here we propose a viable scheme to implement a universal quantum simulator with hybrid spin-photon qubits in an array of superconducting resonators, which is intrinsically scalable and allows for local control. As representative examples we consider the transverse-field Ising model, a spin-1 Hamiltonian, and the two-dimensional Hubbard model; for these, we numerically simulate the scheme by including the main sources of decoherence. In addition, we show how to circumvent the potentially harmful effects of inhomogeneous broadening of the spin systems.

quant-ph↗

arXiv2014

A quantum optical valve in a nonlinear-linear resonator junction

Electronic diodes, which enable the rectification of an electrical energy flux, have played a crucial role in the development of current microelectronics after the invention of semiconductor p-n junctions. Analogously, signal rectification at specific target wavelengths has recently become a key goal in optical communication and signal processing. Here we propose a genuinely quantum device with the essential rectifying features being demonstrated in a general model of a nonlinear-linear junction of coupled resonators. It is shown that such a surprisingly simple structure is a versatile valve and may be alternatively tuned to behave as: a photonic diode, a single or two-photon rectified source turning a classical input into a quantum output depending on the input frequency, or a quantum photonic splitter. Given the relevance of non-reciprocal operations in integrated circuits, the nonlinear-linear junction realises a crucial building component in prospective quantum photonic applications.

quant-ph↗

arXiv2014

Unconventional photon blockade in doubly resonant microcavities with second-order nonlinearity

It is shown that non-centrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably engineered coupled microcavities. The proposed scheme exploits the unconventional photon blockade of a coherent driving field at the input of a coupled cavity system, where one of the two cavities is engineered to resonate at both fundamental and second harmonic frequencies, respectively. Remarkably, the unconventional blockade mechanism occurs with reasonably low quality factors at both harmonics, and does not require a sharp doubly-resonant condition for the second cavity, thus proving its feasibility with current semiconductor technology.

cond-mat.mes-hall↗

arXiv2014

Room temperature Bloch surface wave polaritons

Polaritons are hybrid light-matter quasi-particles that have gathered a significant attention for their capability to show room temperature and out-of-equilibrium Bose-Einstein condensation. More recently, a novel class of ultrafast optical devices have been realized by using flows of polariton fluids, such as switches, interferometers and logical gates. However, polariton lifetimes and propagation distance are strongly limited by photon losses and accessible in-plane momenta in usual microcavity samples. In this work, we show experimental evidence of the formation of room temperature propagating polariton states arising from the strong coupling between organic excitons and a Bloch surface wave. This result, which was only recently predicted, paves the way for the realization of polariton devices that could allow lossless propagation up to macroscopic distances.

cond-mat.mes-hall↗

arXiv2013

Cooperativity of a few quantum emitters in a single-mode cavity

We theoretically investigate the emission properties of a single-mode cavity coupled to a mesoscopic number of incoherently pumped quantum emitters. We propose an operational measure for the medium cooperativity, valid both in the bad and in the good cavity regimes. We show that the opposite regimes of subradiance and superradiance correspond to negative and positive cooperativity, respectively. The lasing regime is shown to be characterized by nonnegative cooperativity. In the bad cavity regime we show that the cooperativity defines the transitions from subradiance to superradiance. In the good cavity regime it helps to define the lasing threshold, also providing distinguishable signatures indicating the lasing regime. Increasing the quality of the cavity mode induces a crossover from the solely superradiant to the lasing regime. Furthermore, we verify that lasing is manifested in a wide range of positive cooperative behavior, showing that stimulated emission and superradiance can coexist. The robustness of the cooperativity is studied with respect to experimental imperfections, such as inhomogeneous broadening and pure dephasing.

quant-ph↗

arXiv2013

Stimulated and spontaneous four-wave mixing in silicon-on-insulator coupled photonic wire nano-cavities

We report on four-wave mixing in coupled photonic crystal nano-cavities on a silicon-on-insulator platform. Three photonic wire cavities are side-coupled to obtain three modes equally separated in energy. The structure is designed to be self-filtering, and we show that the pump is rejected by almost two orders of magnitudes. We study both the stimulated and the spontaneous four-wave mixing processes: owing to the small modal volume, we find that signal and idler photons are generated with a hundred-fold increase in efficiency as compared to silicon micro-ring resonators.

cond-mat.mes-hall↗