arXiv subjects

Darrick Chang

Publications and source records attributed to Darrick Chang.

At least 19 recordsLinked to original sources

arXiv2026

Neural network modeling of many-body super- and sub-radiant dynamics

There is significant interest in exploring novel phenomena in quantum light-matter interfaces, which are driven by the combination of structured dissipation and long-range interactions that are typical in such systems. To this end, it is important to develop new general numerical simulation techniques, which can access large system sizes and are not based on semi-classical approaches. Here, we report the first application of neural quantum states to obtain the dissipative dynamics of light-matter-coupled systems beyond what is accessible with exact and tensor-network calculations. We specifically apply this method to simulate the many-body emission dynamics of approximately 40 atoms, arranged in dense arrays in one and two dimensions. These systems have been chosen because they can support prominent subradiant dynamics at late times and could be realized with cold atomic quantum simulators.

quant-ph↗

arXiv2025

Is Lindblad for me?

The Lindblad master equation is a foundational tool for modeling the dynamics of open quantum systems. As its use has extended far beyond its original domain, the boundaries of its validity have grown opaque. In particular, the rise of new research areas including open quantum many-body systems, non-equilibrium condensed matter, and the possibility to test its limits in driven-open quantum simulators, call for a critical revision of its regimes of applicability. In this pedagogical review, we re-examine the folklore surrounding its three standard approximations (Born, Markov, and Rotating Wave Approximation), as we build our narrative by employing a series of examples and case studies accessible to any reader with a solid background on the fundamentals of quantum mechanics. As a synthesis of our work, we offer a checklist that contrasts common lore with refined expectations, offering a practical guideline for assessing the breakdown of the Lindblad framework in the problem at hand.

quant-ph↗

arXiv2024

Collective optical properties of moir\'e excitons

We propose that excitons in moir\'e transition metal dichalcogenide bilayers offer a promising platform for investigating collective radiative properties. While some of these optical properties resemble those of cold atom arrays, moir\'e excitons extend to the deep subwavelength limit, beyond the reach of current optical lattice experiments. Remarkably, we show that the collective optical properties can be exploited to probe certain correlated electron states without requiring subwavelength spatial resolution. Specifically, we illustrate that the Wigner crystal states of electrons doped into these bilayers act as an emergent periodic potential for excitons. Moreover, the collective dissipative excitonic bands and their associated Berry curvature can reveal various charge orders that emerge at the corresponding electronic doping. Our study provides a promising pathway for future research on the interplay between collective effects and strong correlations involving moir\'e excitons.

cond-mat.mes-hall↗

arXiv2024

Selective Radiance in Super-Wavelength Atomic Arrays

A novel way to create efficient atom-light interfaces is to engineer collective atomic states that selectively radiate into a target optical mode by suppressing emission into undesired modes through destructive interference. While it is generally assumed that this approach requires dense atomic arrays with sub-wavelength lattice constants, here we show that selective radiance can also be achieved in arrays with super-wavelength spacing. By stacking multiple two-dimensional arrays we find super-wavelength mirror configurations where one can eliminate emission into unwanted diffraction orders while enhancing emission into the desired specular mode, leading to near-perfect reflection of weak resonant light. These super-wavelength arrays can also be functionalized into efficient quantum memories, with error probabilities on the order of ~1 for a trilayer with only around ~100 atoms per layer. Relaxing the previous constraint of sub-wavelength spacing could potentially ease the technical requirements for realizing efficient atom-light interfaces, such as enabling the use of tweezer arrays.

quant-ph↗

arXiv2023

Valley-hybridized gate-tunable 1D exciton confinement in MoSe2

Controlling excitons at the nanoscale in semiconductor materials represents a formidable challenge in the fields of quantum photonics and optoelectronics. Achieving this control holds great potential for unlocking strong exciton-exciton interaction regimes, enabling exciton-based logic operations, exploring exotic quantum phases of matter, facilitating deterministic positioning and tuning of quantum emitters, and designing advanced optoelectronic devices. Monolayers of transition metal dichalcogenides (TMDs) offer inherent two-dimensional confinement and possess significant binding energies, making them particularly promising candidates for achieving electric-field-based confinement of excitons without dissociation. While previous exciton engineering strategies have predominantly focused on local strain gradients, the recent emergence of electrically confined states in TMDs has paved the way for novel approaches. Exploiting the valley degree of freedom associated with these confined states further broadens the prospects for exciton engineering. Here, we show electric control of light polarization emitted from one-dimensional (1D) quantum confined states in MoSe2. By employing non-uniform in-plane electric fields, we demonstrate the in-situ tuning of the trapping potential and reveal how gate-tunable valley-hybridization gives rise to linearly polarized emission from these localized states. Remarkably, the polarization of the localized states can be entirely engineered through either the spatial geometry of the 1D confinement potential or the application of an out-of-plane magnetic field.

cond-mat.mes-hall↗

arXiv2023

Dynamics of inhomogeneous spin ensembles with all-to-all interactions: breaking permutational invariance

We investigate the consequences of introducing non-uniform initial conditions in the dynamics of spin ensembles characterized by all-to-all interactions. Specifically, our study involves the preparation of a set of semi-classical spin ensembles with varying orientations. Through this setup, we explore the influence of such non-uniform initial states on the disruption of permutational invariance. Comparing this approach to the traditional scenario of initializing with spins uniformly aligned, we find that the dynamics of the spin ensemble now spans a more expansive effective Hilbert space. This enlargement arises due to the inclusion of off-diagonal coherences between distinct total angular momentum subspaces - an aspect typically absent in conventional treatments of all-to-all spin dynamics. Conceptually, the dynamic evolution can be understood as a composite of multiple homogeneous sub-ensembles navigating through constrained subspaces. Notably, observables that are sensitive to the non-uniformity of initial conditions exhibit discernible signatures of these off-diagonal coherences. We adopt this fresh perspective to reexamine the relaxation phenomena exhibited by the Dicke model, as well as a prototypical example of a boundary time crystal. Intriguingly, ensembles initialized with inhomogeneous initial conditions can show distinctive behaviors when contrasted with canonical instances of collective dynamics. These behaviors encompass the emergence of novel gapless excitations, the manifestation of limit-cycles featuring dressed frequencies due to superradiance, instances of frequency locking or beating synchronizations, and even the introduction of ``extra'' dimensions within the dynamics. In closing, we provide a brief overview of the potential implications of our findings in the context of modern cavity quantum electrodynamics (QED) platforms.

quant-ph↗

arXiv2021

Extensible quantum simulation architecture based on atom-photon bound states in an array of high-impedance resonators

Engineering the electromagnetic environment of a quantum emitter gives rise to a plethora of exotic light-matter interactions. In particular, photonic lattices can seed long-lived atom-photon bound states inside photonic band gaps. Here we report on the concept and implementation of a novel microwave architecture consisting of an array of compact, high-impedance superconducting resonators forming a 1 GHz-wide pass band, in which we have embedded two frequency-tuneable artificial atoms. We study the atom-field interaction and access previously unexplored coupling regimes, in both the single- and double-excitation subspace. In addition, we demonstrate coherent interactions between two atom-photon bound states, in both resonant and dispersive regimes, that are suitable for the implementation of SWAP and CZ two-qubit gates. The presented architecture holds promise for quantum simulation with tuneable-range interactions and photon transport experiments in nonlinear regime.

quant-ph↗

arXiv2021

Many-body localization in waveguide QED

At the quantum many-body level, atom-light interfaces generally remain challenging to solve for or understand in a non-perturbative fashion. Here, we consider a waveguide quantum electrodynamics model, where two-level atoms interact with and via propagating photons in a one-dimensional waveguide, and specifically investigate the interplay of atomic position disorder, multiple scattering of light, quantum nonlinear interactions and dissipation. We develop qualitative arguments and present numerical evidence that such a system exhibits a many-body localized~(MBL) phase, provided that atoms are less than half excited. Interestingly, while MBL is usually formulated with respect to closed systems, this system is intrinsically open. However, as dissipation originates from transport of energy to the system boundaries and the subsequent radiative loss, the lack of transport in the MBL phase makes the waveguide QED system look essentially closed and makes applicable the notions of MBL. Conversely, we show that if the system is initially in a delocalized phase due to a large excitation density, rapid initial dissipation can leave the system unable to efficiently transport energy at later times, resulting in a dynamical transition to an MBL phase. These phenomena can be feasibly realized in state-of-the-art experimental setups.

quant-ph↗

arXiv2020

Transient dynamics of the quantum light retrieved from Rydberg polaritons

We study the photon statistics of weak coherent pulses propagating through a cold Rydberg atomic ensemble in the regime of Rydberg electromagnetically induced transparency. We show experimentally that the value of the second-order autocorrelation function of the transmitted light strongly depends on the position within the pulse and heavily varies during the transients of the pulse. In particular, we show that the falling edge of the transmitted pulse displays much lower values than the rest of the pulse. We derive a theoretical model that quantitatively predicts our results and explains the physical behavior involved. Finally, we use this effect to generate single photons localized within a pulse from the atomic ensemble. We show that by selecting only the last part of the transmitted pulse, the single photons show an antibunching parameter as low as 0.12 and a generation efficiency per trial larger than possible with probabilistic generation schemes with atomic ensembles.

quant-ph↗

arXiv2018

Photon propagation through dissipative Rydberg media at large input rates

We study the dissipative propagation of quantized light in interacting Rydberg media under the conditions of electromagnetically induced transparency (EIT). Rydberg blockade physics in optically dense atomic media leads to strong dissipative interactions between single photons. The regime of high incoming photon flux constitutes a challenging many-body dissipative problem. We experimentally study in detail for the first time the pulse shapes and the second-order correlation function of the outgoing field and compare our data with simulations based on two novel theoretical approaches well-suited to treat this many-photon limit. At low incoming flux, we report good agreement between both theories and the experiment. For higher input flux, the intensity of the outgoing light is lower than that obtained from theoretical predictions. We explain this discrepancy using a simple phenomenological model taking into account pollutants, which are nearly-stationary Rydberg excitations coming from the reabsorption of scattered probe photons. At high incoming photon rates, the blockade physics results in unconventional shapes of measured correlation functions.

quant-ph↗

arXiv2017

Integrated nanoplasmonic quantum interfaces for room temperature single photon sources

We describe a general analytical framework of a nanoplasmonic cavity-emitter system interacting with a dielectric photonic waveguide. Taking into account emitter quenching and dephasing, our model directly reveals the single photon extraction efficiency, $η$, as well as the indistinguishability, $I$, of photons coupled into the waveguide mode. Rather than minimizing the cavity modal volume, our analysis predicts an optimum modal volume to maximize $η$ that balances waveguide coupling and spontaneous emission rate enhancement. Surprisingly, our model predicts that near-unity indistinguishability is possible, but this requires a much smaller modal volume, implying a fundamental performance trade-off between high $η$ and $I$ at room temperature. Finally, we show that maximizing $ηI$ requires that the system has to be driven in the weak coupling regime because quenching effects and decreased waveguide coupling drastically reduce $η$ in the strong coupling regime.

physics.optics↗

arXiv2016

Self-organization of atoms coupled to a chiral reservoir

Tightly confined modes of light, as in optical nanofibers or photonic crystal waveguides, can lead to large optical coupling in atomic systems, which mediates long-range interactions between atoms. These one-dimensional systems can naturally possess couplings that are asymmetric between modes propagating in different directions. Strong long-range interaction among atoms via these modes can drive them to a self-organized periodic distribution. In this paper, we examine the self-organizing behavior of atoms in one dimension coupled to a chiral reservoir. We determine the solution to the equations of motion in different parameter regimes, relative to both the detuning of the pump laser that initializes the atomic dipole-dipole interactions and the degree of reservoir chirality. In addition, we calculate possible experimental signatures such as reflectivity from self-organized atoms and motional sidebands.

quant-ph↗

arXiv2016

Atom-field dressed states in slow-light waveguide QED

We discuss the properties of atom-photon bound states in waveguide QED systems consisting of single or multiple atoms coupled strongly to a finite-bandwidth photonic channel. Such bound states are formed by an atom and a localized photonic excitation and represent the continuum analog of the familiar dressed states in single-mode cavity QED. Here we present a detailed analysis of the linear and nonlinear spectral features associated with single- and multi-photon dressed states and show how the formation of bound states affects the waveguide-mediated dipole-dipole interactions between separated atoms. Our results provide a both qualitative and quantitative description of the essential strong-coupling processes in waveguide QED systems, which are currently being developed in the optical and the microwave regime.

quant-ph↗

arXiv2015

Electro-mechanical control of an optical emitter using graphene

Active, in situ control of light at the nanoscale remains a challenge in modern physics and in nanophotonics in particular. A promising approach is to take advantage of the technological maturity of nano-electromechanical systems (NEMS) and to combine it with on-chip optics. However, in scaling down the dimensions of such integrated devices, the coupling of a NEMS to optical fields becomes challenging. Despite recent progress in nano-optomechanical coupling, active control of optical fields at the nanoscale has not been achieved with an on-chip NEMS thus far. Here, we show a new type of hybrid system, which consists of an on-chip graphene NEMS suspended a few tens of nanometers above nitrogen-vacancy centres (NVC), which are stable single photon emitters embedded in nano-diamonds. Electromechanical control of the photons emitted by the NVC is provided by electrostatic tuning of the graphene NEMS position, which is transduced to a modulation of NVC emission intensity. The optomechanical coupling between the graphene displacement and the NVC emission is based on near-field dipole-dipole interaction. This class of optomechanical coupling increases strongly for smaller distances, making it suitable for devices with nanoscale dimensions. These achievements hold promise for the selective control of single-emitter arrays on chip, optical spectroscopy of individual nano-objects, integrated optomechanical information processing and quantum optomechanics.

cond-mat.mes-hall↗

arXiv2014

Harnessing vacuum forces for quantum sensing of graphene motion

Position measurements at the quantum level are vital for many applications, but also challenging. Typically, methods based on optical phase shifts are used, but these methods are often weak and difficult to apply to many materials. An important example is graphene, which is an excellent mechanical resonator due to its small mass and an outstanding platform for nanotechnologies, but is largely transparent. Here, we present a novel detection scheme based upon the strong, dispersive vacuum interactions between a graphene sheet and a quantum emitter. In particular, the mechanical displacement causes strong changes in the vacuum-induced shifts of the transition frequency of the emitter, which can be read out via optical fields. We show that this enables strong quantum squeezing of the graphene position on time scales short compared to the mechanical period.

quant-ph↗

arXiv2012

Mimicking interacting relativistic theories with stationary pulses of light

One of the most well known relativistic field theory models is the Thirring model (TM). Its realization can demonstrate the famous prediction for the renormalization of mass due to interactions. However, experimental verification of the latter requires complex accelerator experiments whereas analytical solutions of the model can be extremely cumbersome to obtain. In this work, following Feynman's original proposal, we propose a alternative quantum system as a simulator of the TM dynamics. Here the relativistic particles are mimicked, counter-intuitively, by polarized photons in a quantum nonlinear medium. We show that the entire set of regimes of the Thirring model -- bosonic or fermionic, and massless or massive -- can be faithfully reproduced using coherent light trapping techniques. The sought after correlations' scalings can be extracted by simple probing of the coherence functions of the light using standard optical techniques.

quant-ph↗

arXiv2010

Electromagnetically Induced Transparency and Slow Light with Optomechanics

Controlling the interaction between localized optical and mechanical excitations has recently become possible following advances in micro- and nano-fabrication techniques. To date, most experimental studies of optomechanics have focused on measurement and control of the mechanical subsystem through its interaction with optics, and have led to the experimental demonstration of dynamical back-action cooling and optical rigidity of the mechanical system. Conversely, the optical response of these systems is also modified in the presence of mechanical interactions, leading to strong nonlinear effects such as Electromagnetically Induced Transparency (EIT) and parametric normal-mode splitting. In atomic systems, seminal experiments and proposals to slow and stop the propagation of light, and their applicability to modern optical networks, and future quantum networks, have thrust EIT to the forefront of experimental study during the last two decades. In a similar fashion, here we use the optomechanical nonlinearity to control the velocity of light via engineered photon-phonon interactions. Our results demonstrate EIT and tunable optical delays in a nanoscale optomechanical crystal device, fabricated by simply etching holes into a thin film of silicon (Si). At low temperature (8.7 K), we show an optically-tunable delay of 50 ns with near-unity optical transparency, and superluminal light with a 1.4 microseconds signal advance. These results, while indicating significant progress towards an integrated quantum optomechanical memory, are also relevant to classical signal processing applications. Measurements at room temperature and in the analogous regime of Electromagnetically Induced Absorption (EIA) show the utility of these chip-scale optomechanical systems for optical buffering, amplification, and filtering of microwave-over-optical signals.

physics.optics↗

arXiv2010

Slowing and stopping light using an optomechanical crystal array

One of the major advances needed to realize all-optical information processing of light is the ability to delay or coherently store and retrieve optical information in a rapidly tunable manner. In the classical domain, this optical buffering is expected to be a key ingredient to managing the flow of information over complex optical networks. Such a system also has profound implications for quantum information processing, serving as a long-term memory that can store the full quantum information contained in an optical pulse. Here we suggest a novel approach to light storage involving an optical waveguide coupled to an optomechanical crystal array, where light in the waveguide can be dynamically and coherently transferred into long-lived mechanical vibrations of the array. Under realistic conditions, this system is capable of achieving large bandwidths and storage/delay times in a compact, on-chip platform.

quant-ph↗