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David A. Dahlbom

Publications and source records attributed to David A. Dahlbom.

5 recordsLinked to original sources

Tunable Skyrmions in a Topological Wigner Crystal

In low density systems with strong interactions electrons are expected to crystallize into a Wigner solid. Recently, advances in two-dimensional systems where electrons carry Berry curvature have added a topological dimension to Wigner crystallization. Using a model for pseudospin interactions in a topological Wigner crystal, here we show that the competition between ferromagnetic Heisenberg exchange $J$ and the chiral interaction $γ$ on the triangular lattice stabilizes a zero-field skyrmion crystal whose density is continuously tunable through the ratio $γ/J$. The chiral interaction originates from finite Berry curvature in an underlying time-reversal broken Wigner crystal. In the continuum limit, the chiral interaction acts as a chemical potential for skyrmions, while higher-order gradient terms beyond the nonlinear sigma model select the skyrmion density. At large chiral coupling, we uncover a 24-site tetra-skyrmion crystal carrying four units of topological charge per magnetic unit cell, which becomes degenerate with four-sublattice tetrahedral order as $J \to 0$. We characterize the magnon structure for these phases and discuss the transition between the tunable skyrmion crystal to these states at large $γ/J$. Our results establish the phase diagram of ferromagnetic topological Wigner crystals.

cond-mat.str-el

The 6H-Perovskite Dimer Lattice with Antiferromagnetic Interactions: Ba$_3$ARu$_2$O$_9$

We investigate the magnetic behavior of the 6H-perovskite dimer lattice Ba$_3$Zn$_{1-x}$Ca$_x$Ru$_2$O$_9$ using analytical theory, density functional theory, inelastic neutron scattering, and modeling of historical magnetization and neutron-scattering data. A dimer mean-field theory built upon classical Luttinger-Tisza analysis generates a phase diagram revealing a transition from a nonmagnetic singlet to a finite-moment ground state as interdimer couplings increase. A (generalized) linear spin-wave theory captures multiplet mixing, excitation gap closing, and fluctuation-induced moment suppression. Density functional theory on select compounds and neutron spectroscopy on dilute Ba$_3$Zn(Ru$_{1-x}$Sb$_x$)$_2$O$_9$ confirm the exchange hierarchy, enabling quantification of previously published experiments within this framework. Our results identify three mechanisms for magnetic moment suppression: quantum fluctuations, ligand hybridization, and nonmagnetic-singlet/magnetic-multiplet mixing.

cond-mat.str-el

Quantum entanglement of XY-type spin dimers in Shastry-Sutherland lattice

We report a comprehensive study on the origin of the enigmatic disordered ground state within the Shastry-Sutherland lattice, BaCe$_2$ZnS$_5$, at low temperatures. The magnetization and heat capacity data show a lack of magnetic ordering down to 73 mK. We deploy a localized spin dimer model which can accurately reproduce the dynamic structure factor of the neutron data, magnetization and heat capacity data. Remarkably, the intra-dimer exchange interaction shows strong XY-type anisotropy and the ground state of BaCe$_2$ZnS$_5$ is in an entangled state $(|\uparrow\uparrow> - |\downarrow\downarrow>)/\sqrt{2}$. This is in contrast to the singlet dimer state that is obtained for Heisenberg interactions. These results confirm that BaCe$_2$ZnS$_5$ is in a quantum paramagnet state consisting of entangled spin dimer states.

cond-mat.str-el

Classical dynamics of the antiferromagnetic Heisenberg $S=1/2$ spin ladder

We employ a classical limit grounded in SU(4) coherent states to investigate the temperature-dependent dynamical spin structure factor of the $S = 1/2$ ladder consisting of weakly coupled dimers. By comparing the outcomes of this classical approximation with density matrix renormalization group and exact diagonalization calculations in finite size ladders, we demonstrate that the classical dynamics offers an accurate approximation across the entire temperature range when the interdimer coupling is weak and a good approximation in the high temperature regime even when the interdimer coupling is strong. This agreement is achieved after appropriately rescaling the temperature axis and renormalizing expectation values to satisfy a quantum sum rule, following D. Dahlbom et al. [Phys. Rev. B 109, 014427 (2024)]. We anticipate the method will be particularly effective when applied to 2D and 3D lattices composed of weakly-coupled dimers, situations that remain challenging for alternative numerical methods.

cond-mat.str-el

Understanding temperature-dependent SU($3$) spin dynamics in the $S=1$ antiferromagnet Ba$_2$FeSi$_2$O$_7$

Quantum magnets admit more than one classical limit and $N$-level systems with strong single-ion anisotropy are expected to be described by a classical approximation based on SU($N$) coherent states. Here we test this hypothesis by modeling finite temperature inelastic neutron scattering (INS) data of the effective spin-one antiferromagnet \bfso{}. The measured dynamic structure factor is calculated with a generalized Landau-Lifshitz dynamics for SU($3$) spins. Unlike the traditional classical limit based on SU($2$) coherent states, the results obtained with classical SU($3$) spins are in good agreement with the measured temperature-dependent spectrum. The SU($3$) approach developed here provides a general framework to understand the broad class of materials comprising weakly coupled antiferromagnetic dimers, trimers, or tetramers, and magnets with strong single-ion anisotropy.

cond-mat.str-el