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David C. Moore

Publications and source records attributed to David C. Moore.

At least 19 recordsLinked to original sources

Future directions in nuclear $\beta$ decay at FRIB and beyond

Motivated by the opportunities presented for studies relevant to nuclear structure, astrophysics, and fundamental symmetries with nuclear $\beta$ decay, the Facility for Rare Isotope Beams (FRIB) Theory Alliance topical program ``Future Directions in Nuclear $\beta$ Decays at FRIB'' was held in September of 2025. This white paper summarizes the main points of discussion over the two-week program, and it aims to provide a snapshot of the current status of the field while also highlighting important questions and opportunities for future work. We provide an overview of the experimental tools and techniques that enable modern $\beta$ decay studies, discuss the current state of nuclear many-body approaches used to study $\beta$ decays, and highlight the important science questions that can be addressed by weak decays.

nucl-th

Optomechanical Detection of Individual Gas Collisions

We experimentally demonstrate the detection of momentum transfers from individual collisions of Kr, Xe, and SF$_6$ with an optically levitated nanoparticle, finding good agreement with theoretical expectations. The observed event rates accurately measure the gas partial pressures, while the spectral shape provides a sensitive probe of the surface properties of the nanoparticle, including its temperature. The reconstruction of impulse signals as small as 200 keV/$c$ further establishes that levitated optomechanical sensors can reach the sensitivity required for precision measurements of fundamental particle interactions, and demonstrates a proof-of-principle for a primary pressure sensor based on the detection of individual gas particle collisions.

quant-ph

Decay-Resolved Charge Changes from Radioactive Decays in Levitated Microparticles

We measure event-by-event discrete changes in the net electric charge of an optically levitated silica microsphere arising from individual radioactive decays within the sphere, in coincidence with energy depositions in a nearby scintillation detector. The net charge of the levitated sphere is continuously monitored by measuring its driven response to an oscillating electric field, allowing individual charge-change events to be resolved on millisecond timescales with precision below an elementary charge. Simultaneously, $\alpha$ and $\beta$ particles emitted during decays of implanted $^{212}$Pb and its daughters are detected using a scintillator read out with an array of silicon photomultipliers. By correlating reconstructed charge-change times with the scintillator response, we can directly attribute abrupt changes in the sphere's net charge to individual nuclear decays, and identify differences in the distribution of charges ejected for $\alpha$ and $\beta$ decays. These results establish a new approach for studying low energy charged particles emitted by radioactive decays at the single-decay level, and identify showers of radiogenically produced low-energy electrons emitted by $\alpha$-decaying radon daughters implanted near solid surfaces.

physics.ins-det

Three-dimensional squeezing of optically levitated nanospheres

We propose a protocol to measure impulses beyond the standard quantum limit. The protocol reduces noise in all three spatial dimensions and consists of squeezing a mechanical system's state via a series of jumps in the frequency of the harmonic potential. We quantify how decoherence in a realistic system of an optically levitated, dielectric nanoparticle limits the ultimate sensitivity. We predict that $\sim$10 dB of squeezing is achievable with current technology, enabling quantum-enhanced detection of weak impulses.

quant-ph

A Spin-Based Pathway to Testing the Quantum Nature of Gravity

A key open problem in physics is the correct way to combine gravity (described by general relativity) with everything else (described by quantum mechanics). This problem suggests that general relativity and possibly also quantum mechanics need fundamental corrections. Most physicists expect that gravity should be quantum in character, but gravity is fundamentally different to the other forces because it alone is described by spacetime geometry. Experiments are needed to test whether gravity, and hence space-time, is quantum or classical. We propose an experiment to test the quantum nature of gravity by checking whether gravity can entangle two micron-sized crystals. A pathway to this is to create macroscopic quantum superpositions of each crystal first using embedded spins and Stern-Gerlach forces. These crystals could be nanodiamonds containing nitrogen-vacancy (NV) centres. The spins can subsequently be measured to witness the gravitationally generated entanglement. This is based on extensive theoretical feasibility studies and experimental progress in quantum technology. The eventual experiment will require a medium-sized consortium with excellent suppression of decoherence including vibrations and gravitational noise. In this white paper, we review the progress and plans towards realizing this. While implementing these plans, we will further explore the most macroscopic superpositions that are possible, which will test theories that predict a limit to this.

quant-ph

Search for Dark Matter Scattering from Optically Levitated Nanoparticles

The development of levitated optomechanics has enabled precise force sensors that operate in the quantum measurement regime, opening up unique opportunities to search for new physics whose weak interactions may have evaded existing sensors. We demonstrate the detection of impulsive forces acting on optically levitated nanoparticles, where the dominant noise source is provided by measurement backaction. Using these sensors, we search for momentum transfers that may originate from scattering of passing particlelike dark matter. For dark matter that couples to Standard Model neutrons via a generic long-range interaction, this search constrains a range of models in the mass range $1$-$10^7~\mathrm{GeV/}c^2$, placing upper limits on single neutron coupling strength as low as $\leq 1 \times 10^{-7}$ at the 95% confidence level. We also demonstrate the ability of using the inherent directional sensitivity of these sensors to separate possible dark matter signals from backgrounds. Future extensions of the techniques developed here can enable searches for light dark matter and massive neutrinos that can reach sensitivity several orders of magnitude beyond existing searches.

hep-ex

Kilobyte-Scale, Selector-Free, Temperature-Hard AlScN Ferroelectric Diode Crossbar Arrays

We report the fabrication and characterization of kilobyte-scale, selector-free, ferroelectric (FE) diode crossbar memory arrays based on aluminum scandium nitride (AlScN). Utilizing a fully CMOS back-end-of-line (BEOL) compatible process, we fabricated 2-kilobyte (128 $\times$ 128) arrays with device diameters down to 5 $\mu$m, achieving memory densities up to 2500 bits/mm$^2$. Large-scale electrical characterization across 1000 randomly selected devices reveals a yield rate of 95.2%, a tight switching voltage distribution with a coefficient of variation (CV) of 0.003, and consistent on/off ratios of around 10 with a CV of 0.27. We demonstrate selector-free read and program operations of the array, enabled by the high nonlinearity, rectification, and uniform switching behavior of the FE diodes. Furthermore, we verified consistent ferroelectric switching during array operation at temperatures up to 600 $^\circ$C. Our results highlight the potential of AlScN FE diode arrays for energy-efficient, high-density memory applications and lay the groundwork for future integration in compute-near-memory, high-temperature memory, and analog compute-in-memory systems.

cond-mat.mes-hall

Optical Levitation of Arrays of Microspheres

Levitated optomechanical systems are rapidly becoming leading tools for precision sensing of forces and accelerations acting on particles in the femtogram to nanogram mass range. These systems enable a high level of control over the sensor's center-of-mass motion, rotational degrees of freedom, and electric charge state. For many sensing applications, extending these techniques to arrays of sensors enables rejection of correlated noise sources and increases sensitivity to interactions that may be too rare or weak to detect with a single particle. Here we present techniques capable of trapping defect free, two-dimensional arrays of more than 25 microspheres in vacuum. These techniques provide independent control of the optical potential for each sphere. Simultaneous imaging of the motion of all spheres in the array is demonstrated using camera-based imaging, with optimized object tracking algorithms reaching a displacement sensitivity below 1 nm/$\surd$Hz. Such arrays of levitated microspheres may find applications ranging from inertial sensing to searches for weakly interacting particles such as dark matter.

physics.optics

Al0.68Sc0.32N/SiC based metal-ferroelectric-semiconductor capacitors operating up to 1000 {\deg}C

Ferroelectric (Fe) materials-based devices show great promise for non-volatile memory applications, yet few demonstrate reliable operation at elevated temperatures. In this work, we demonstrate Ni/Al0.68Sc0.32N/4H-SiC metal-ferroelectric-semiconductor capacitors for high-temperature non-volatile memory applications. Our 30-nm thick ferroelectric Al0.68Sc0.32N film grown on SiC exhibits stable and robust ferroelectric switching up to 1000{\deg}C. The coercive field decreases linearly from -6.4/+11.9 MV cm-1 at room temperature to -3.1/+7.8 MV cm-1 at 800{\deg}C, further reducing to -2.5 MV cm-1 at 1000{\deg}C. At 600{\deg}C, the devices achieve remarkable reliability with ~2000 endurance cycles and over at least 100 hours of retention with negligible polarization loss. At 800{\deg}C, the devices retain data for at least 10,000 seconds and exceed 400 write cycles. Our results further highlight the potential for ferroelectric AlScN thin-films particularly when paired with SiC semiconductor substrates for high-temperature non-volatile memory.

cond-mat.mtrl-sci

Materials for High Temperature Digital Electronics

Silicon microelectronics, consisting of complementary metal oxide semiconductor (CMOS) technology, have changed nearly all aspects of human life from communication to transportation, entertainment, and healthcare. Despite the widespread and mainstream use, current silicon-based devices suffer significant reliability issues at temperatures exceeding 125 C. The emergent technological frontiers of space exploration, geothermal energy harvesting, nuclear energy, unmanned avionic systems, and autonomous driving will rely on control systems, sensors, and communication devices which operate at temperatures as high as 500 C and beyond. At these extreme temperatures, active (heat exchanger, phase change cooling) or passive (fins and thermal interface materials) cooling strategies add significant mass and complication which is often infeasible. Thus, new material solutions beyond conventional silicon CMOS devices are necessary for high temperature, resilient electronic systems. Accomplishing this will require a united effort to explore development, integration, and ultimately manufacturing of non-silicon-based logic and memory technologies, non-traditional metals for interconnects, and ceramic packaging technology.

cond-mat.mtrl-sci

Mechanical detection of nuclear decays

We report the detection of individual nuclear $\alpha$ decays through the mechanical recoil of the entire micron-sized particle in which the decaying nuclei are embedded. Momentum conservation ensures that such measurements are sensitive to any particles emitted in the decay, including neutral particles that may otherwise evade detection with existing techniques. Detection of the minuscule recoil of an object more than $10^{12}$ times more massive than the emitted particles is made possible by recently developed techniques in levitated optomechanics, which enable high-precision optical control and measurement of the mechanical motion of optically trapped particles. Observation of a change in the net charge of the particle coincident with the recoil allows decays to be identified with background levels at the micro-Becquerel level. The techniques developed here may find use in fields ranging from nuclear forensics to dark matter and neutrino physics.

physics.ins-det

Quantum Sensors for High Energy Physics

Strong motivation for investing in quantum sensing arises from the need to investigate phenomena that are very weakly coupled to the matter and fields well described by the Standard Model. These can be related to the problems of dark matter, dark sectors not necessarily related to dark matter (for example sterile neutrinos), dark energy and gravity, fundamental constants, and problems with the Standard Model itself including the Strong CP problem in QCD. Resulting experimental needs typically involve the measurement of very low energy impulses or low power periodic signals that are normally buried under large backgrounds. This report documents the findings of the 2023 Quantum Sensors for High Energy Physics workshop which identified enabling quantum information science technologies that could be utilized in future particle physics experiments, targeting high energy physics science goals.

hep-ex

Scalable and Stable Ferroelectric Non-Volatile Memory at > 500 $^\circ$C

Non-volatile memory (NVM) devices that reliably operate at temperatures above 300 $^\circ$C are currently non-existent and remains a critically unmet challenge in the development of high-temperature (T) resilient electronics, necessary for many emerging, complex computing and sensing in harsh environments. Ferroelectric Al$_x$Sc$_{1-x}$N exhibits strong potential for utilization in NVM devices operating at very high temperatures (> 500 $^\circ$C) given its stable and high remnant polarization (PR) above 100 $μ$C/cm$^2$ with demonstrated ferroelectric transition temperature (TC) > 1000 $^\circ$C. Here, we demonstrate an Al$_{0.68}$Sc$_{0.32}$N ferroelectric diode based NVM device that can reliably operate with clear ferroelectric switching up to 600 $^\circ$C with distinguishable On and Off states. The coercive field (EC) from the Pulsed I-V measurements is found to be -5.84 (EC-) and +5.98 (EC+) (+/- 0.1) MV/cm at room temperature (RT) and found to decrease with increasing temperature up to 600 $^\circ$C. The devices exhibit high remnant polarizations (> 100 $μ$C/cm$^2$) which are stable at high temperatures. At 500 $^\circ$C, our devices show 1 million read cycles and stable On-Off ratio above 1 for > 6 hours. Finally, the operating voltages of our AlScN ferrodiodes are < 15 V at 600 $^\circ$C which is well matched and compatible with Silicon Carbide (SiC) based high temperature logic technology, thereby making our demonstration a major step towards commercialization of NVM integrated high-T computers.

physics.app-ph

Collision-resolved pressure sensing

Heat and pressure are ultimately transmitted via quantized degrees of freedom, like gas particles and phonons. While a continuous Brownian description of these noise sources is adequate to model measurements with relatively long integration times, sufficiently precise measurements can resolve the detailed time dependence coming from individual bath-system interactions. We propose the use of nanomechanical devices operated with impulse readout sensitivity around the ``standard quantum limit'' to sense ultra-low gas pressures by directly counting the individual collisions of gas particles on a sensor. We illustrate this in two paradigmatic model systems: an optically levitated nanobead and a tethered membrane system in a phononic bandgap shield.

quant-ph

Searches for massive neutrinos with mechanical quantum sensors

The development of quantum optomechanics now allows mechanical sensors with femtogram masses to be controlled and measured in the quantum regime. If the mechanical element contains isotopes that undergo nuclear decay, measuring the recoil of the sensor following the decay allows reconstruction of the total momentum of all emitted particles, including any neutral particles that may escape detection in traditional detectors. As an example, for weak nuclear decays the momentum of the emitted neutrino can be reconstructed on an event-by-event basis. We present the concept that a single nanometer-scale, optically levitated sensor operated with sensitivity near the standard quantum limit can search for heavy sterile neutrinos in the keV-MeV mass range with sensitivity significantly beyond existing constraints. We also comment on the possibility that mechanical sensors operated well into the quantum regime might ultimately reach the sensitivities required to provide an absolute measurement of the mass of the light neutrino states.

hep-ex

Coherent scattering of low mass dark matter from optically trapped sensors

We propose a search for low mass dark matter particles through momentum recoils caused by their scattering from trapped, nm-scale objects. Our projections show that even with a modest array of fg-mass sensors, parameter-space beyond the reach of existing experiments can be explored. The case of smaller, ag-mass sensors is also analyzed - where dark matter can coherently scatter from the entire sensor - enabling a large enhancement in the scattering cross-section relative to interactions with single nuclei. Large arrays of such sensors have the potential to explore new parameter space down to dark matter masses as low as 10 keV. If recoils from dark matter are detected by such sensors, their inherent directional sensitivity would allow an unambiguous identification of a dark matter signal.

physics.ins-det

MAQRO -- BPS 2023 Research Campaign Whitepaper

The objective of the proposed MAQRO mission is to harness space for achieving long free-fall times, extreme vacuum, nano-gravity, and cryogenic temperatures to test the foundations of physics in macroscopic quantum experiments. This will result in the development of novel quantum sensors and a means to probe the foundations of quantum physics at the interface with gravity. Earlier studies showed that the proposal is feasible but that several critical challenges remain, and key technologies need to be developed. These new technologies will open up the potential for achieving additional science objectives. The proposed research campaign aims to advance the state of the art and to perform the first macroscopic quantum experiments in space. Experiments on the ground, in micro-gravity, and in space will drive the proposed research campaign during the current decade to enable the implementation of MAQRO within the subsequent decade.

quant-ph

Control and measurement of electric dipole moments in levitated optomechanics

Levitated optomechanical systems are rapidly becoming leading tools for precision sensing, enabling a high level of control over the sensor's center of mass motion, rotation and electric charge state. Higher-order multipole moments in the charge distribution, however, remain a major source of backgrounds. By applying controlled precessive torques to the dipole moment of a levitated microsphere in vacuum, we demonstrate cancellation of dipole-induced backgrounds by 2 orders of magnitude. We measure the dipole moments of ng-mass spheres and determine their scaling with sphere size, finding that the dominant torques arise from induced dipole moments related to dielectric-loss properties of the SiO$_2$ spheres. Control of multipole moments in the charge distribution of levitated sensors is a key requirement to sufficiently reduce background sources in future applications.

physics.optics