arXiv subjects

David Cesar

Publications and source records attributed to David Cesar.

16 recordsLinked to original sources

arXiv2026

Mutually phase-stable tunable attosecond soft X-ray attosecond pulses from a free-electron laser

We demonstrate the production of mutually phase-stable attosecond X-ray pulse pairs with tunable relative time delays and phases in a cascaded X-ray free-electron laser. We showcase the method in an experiment at the LCLS-II, in which a shaped electron beam is used in a split undulator configuration to generate the two attosecond pulses. We achieve mutual phase stability by reusing microbunching generated in the first undulator in order to seed the FEL process in the second at a detuned frequency. We measure controllable temporal delays between the two pulses directly in the time domain using angular streaking of photoelectrons, with a step size of 250 attoseconds. We then show that the behavior of the X-ray spectrum is consistent with phase stability between the two pulses, with a relative phase that can be easily tuned using inter-undulator phase shifters. This method is particularly well-suited to few to ten eV energy separations and sub to few femtosecond time delays, which are ideal for experiments in the soft X-ray regime for pushing the limits of our models for molecular dynamics and exerting direct coherent control over quantum systems.

physics.acc-ph↗

arXiv2026

Broadband hard X-ray attosecond pulses from extremely chirped electron beams

Attosecond pulses from free-electron lasers have opened the doors to atomic site-specific studies of bound electronic dynamics on their natural, sub-femtosecond timescales. Key to their success has been electron beam shaping techniques enabling the generation of sub-femtosecond current spikes with peak currents on the order of 10 kA. We demonstrate in an RF linac the generation of current spikes with extreme chirps on the order of 350 MeV/micron, directly competitive with the chirps expected from beam-driven plasma wakefield accelerators. Leveraging chirp-taper compensation, we use these highly chirped beams to generate hard X-ray attosecond pulses with bandwidths exceeding 30 eV, a factor of two beyond previous demonstrations. We simultaneously present the first explicit experimental evidence of chirp-taper compensation in an attosecond XFEL, finding that optimal tapering improves the bandwidth and pulse energy by factors of two and five, respectively, for our conditions. In addition to the immediate utility of such broadband hard X-ray pulses, electron beams with such extreme chirps can be utilized for unique new experimental modalities by performing further compression after the undulators. Such post-lasing compression can enable subsequent superradiant light emission at longer wavelengths, or direct excitation of quantum systems with the beam's intense space-charge field for unique attosecond pump-probe possibilities.

physics.acc-ph↗

arXiv2026

Advanced Control of Electron Beams: Tailoring X-ray Production with Programmable Laser Shaping

Leveraging the full scientific capabilities of next-generation high-repetition-rate free-electron lasers requires programmable control over electron-beam properties at their source. The photoinjector drive laser defines the electron beam's initial six-dimensional phase-space distribution, yet has historically been limited to Gaussian or static flat-top profiles, with most manipulation occurring downstream. Here we demonstrate software-programmable ultraviolet pulse shaping at the LCLS-II photoinjector as a source-level actuator that complements traditional accelerator controls. Using a coupled architecture combining dispersion-controlled nonlinear frequency conversion with spatial-light-modulator spectral shaping, we generate user-defined temporal structures and observe their imprint on electron bunches through high-resolution time-domain diagnostics. Laser-imposed multi-peaked modulation persists through acceleration, magnetic compression, and undulator transport with shot-to-shot repeatability, producing clearly resolved current structure in the compressed beam. Variance-based reconstruction from transverse deflecting cavity measurements reveals structured X-ray emission profiles exhibiting temporal features consistent with the programmed laser waveform. By providing rapid, software-controlled reconfiguration of electron-beam initial conditions, this source-level control approach establishes a programmable upstream actuator for future adaptive optimization and autonomous facility operation at high-repetition-rate light sources.

physics.acc-ph↗

arXiv2026

Upstream Laser-based Longitudinal Enhancement of Relativistic Photoelectrons

Controlling the longitudinal phase space of high-brightness relativistic electron beams is crucial for advancing a broad spectrum of charged-particle-based instrumentation and scientific frontiers. A generalized method for achieving this control involves manipulating the photoemission laser's temporal distribution at the picosecond level, a long-standing technical challenge. Recent developments in laser shaping have enabled the creation of high-power, picosecond-scale symmetrical and asymmetrical temporal profiles, capable of fine-tuning complex space-charge dynamics and external field effects in relativistic charged-particle beams. Here, we demonstrate that rather than deviations from theorized, idealized laser distributions, a controlled asymmetry can be harnessed to counteract accelerator-induced distortions. By implementing spatiotemporal shaping of the ultraviolet photocathode laser at the LCLS-II superconducting injector, we achieve deterministic control over the longitudinal phase space without downstream corrections. We find that this optical asymmetry induces a self-linearizing effect across both low (40 pC) and high (80 pC) charge regimes, effectively suppressing nonlinear compression and energy chirp. Consequently, this approach is expected to preserve a low emittance comparable to that of ideal flattop or regular Gaussian profiles, while delivering superior current uniformity and shot-to-shot stability. These results establish spatiotemporal laser shaping as a compact, generalizable tool for directly optimizing beam brightness at the source.

physics.optics↗

arXiv2025

Beam Halo Formation via Longitudinal-Transverse Coupling in Continuous-Wave Photoinjectors

Beam halo formation poses a critical challenge for high-repetition-rate continuous-wave (CW) free-electron lasers (FELs), directly affecting beam quality and machine protection, as observed during the LCLS-II commissioning. We identify and experimentally validate a previously unrecognized three-step mechanism for halo generation in the photoinjector, arising from coupled longitudinal-transverse dynamics in the low-energy beam. Theoretical analysis reveals that (i) the RF buncher induces an energy-radius correlation, (ii) velocity bunching transforms this correlation into hollowed density structures in the bunch head and tail, and (iii) differential overfocusing of these hollowed regions by downstream focusing forms the observed halo. This mechanism is confirmed by particle-in-cell simulations and direct experimental measurements, including controlled formation of a core-ring profile via solenoid tuning. The results establish the physical origin of the halo and demonstrate a mitigation via buncher compression tuning that reduces halo and downstream loss, supporting sustained high-repetition-rate FEL operation.

physics.acc-ph↗

arXiv2025

Nonlinear reversal of photo-excitation on the attosecond time scale improves ultrafast x-ray diffraction images

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to visualize non-equilibrium dynamics in systems beyond few atoms. However, extreme x-ray intensities introduce significant electronic damage, limiting material contrast and spatial resolution. Here we show that newly available intense subfemtosecond (sub-fs) x-ray FEL pulses can outrun most ionization cascades and partially reverse x-ray damage through stimulated x-ray emission in the vicinity of a resonance. In our experiment, we compared thousands of coherent x-ray diffraction patterns and simultaneously recorded ion spectra from individual Ne nanoparticles injected into the FEL focus. Our experimental results and theoretical modeling reveal that x-ray diffraction increases and the average charge state decreases in particles exposed to sub-fs pulses compared to those illuminated with 15-femtosecond pulses. Sub-fs exposures outrun most Auger decays and impact ionization processes, and enhance nonlinear effects such as stimulated emission, which cycle bound electrons between different states. These findings demonstrate that intense sub-fs x-ray FEL pulses are transformative for advancing high-resolution imaging and spectroscopy in chemical and material sciences, and open the possibilities of coherent control of the interaction between x-rays and complex specimen beyond few atoms.

physics.optics↗

arXiv2025

Experimental demonstration of attosecond hard X-ray pulses

We present the first direct experimental confirmation of attosecond pulse generation in the hard X-ray regime with a free-electron laser. Our experiment is based on measurements of a nonlinear optical phenomenon known as amplified spontaneous emission (ASE) from 3d transition metals. By analyzing the yield of the collective X-ray fluorescence induced by ultrashort pulses at the Linac Coherent Light Source, we identify the generation of attosecond pulses and shot-to-shot fluctuations in their duration, ranging from 100 as to 400 as. The observed product of bandwidth and pulse duration for 100 as pulses is approximately 2 fs$\cdot$eV, indicating the generation of nearly transform-limited pulses. Our results extend the photon energy reach of attosecond techniques by one order of magnitude, providing the ability to simultaneously probe matter on the time-scales of electronic phenomena and with atomic spatial resolution. Furthermore, attosecond hard X-ray pulses can outrun the fastest radiation damage processes, paving the way to single-shot damage-free X-ray measurements.

physics.optics↗

arXiv2024

Attosecond Coherent Electron Motion in a Photoionized Aromatic Molecule

In molecular systems, the ultrafast motion of electrons initiates the process of chemical change. Tracking this electronic motion across molecules requires coupling attosecond time resolution to atomic-scale spatial sensitivity. In this work, we employ a pair of attosecond x-ray pulses from an x-ray free-electron laser to follow electron motion resulting from the sudden removal of an electron from a prototypical aromatic system, para-aminophenol. X-ray absorption enables tracking this motion with atomic-site specificity. Our measurements are compared with state-of-the-art computational modeling, reproducing the observed response across multiple timescales. Sub-femtosecond dynamics are assigned to states undergoing non-radiative decay, while few-femtosecond oscillatory motion is associated with electronic wavepacket motion in stable cation states, that will eventually couple to nuclear motion. Our work provides insight on the ultrafast charge motion preceding and initiating chemical transformations in moderately complex systems, and provides a powerful benchmark for computational models of ultrafast charge motion in matter.

physics.chem-ph↗

arXiv2024

"Beam `a la carte": laser heater shaping for attosecond pulses in a multiplexed x-ray free-electron laser

Electron beam shaping allows the control of the temporal properties of x-ray free-electron laser pulses from femtosecond to attosecond timescales. Here we demonstrate the use of a laser heater to shape electron bunches and enable the generation of attosecond x-ray pulses. We demonstrate that this method can be applied in a selective way, shaping a targeted subset of bunches while leaving the remaining bunches unchanged. This experiment enables the delivery of shaped x-ray pulses to multiple undulator beamlines, with pulse properties tailored to specialized scientific applications.

physics.acc-ph↗

arXiv2024

Spectrotemporal shaping of attosecond x-ray pulses with a fresh-slice free-electron laser

We propose a scheme allowing coherent shaping, i.e., controlling both the amplitude and phase, of attosecond x-ray pulses at free-electron lasers. We show that by seeding an FEL with a short coherent seed that overfills the amplification bandwidth, one can shape the Wigner function of the pulse by controlling the undulator taper profile. The examples of controllable pulse pairs and trains, as well as isolated spectrotemporally shaped pulses with very broad bandwidths are examined in detail. Existing attosecond XFELs can achieve these experimental conditions in a two-stage cascade, in which the seed is generated by a short current spike in an electron bunch and shaped in an unspoiled region within the same bunch. We experimentally demonstrate the production and control of phase-stable pulse trains using this method at the Linac Coherent Light Source II.

physics.acc-ph↗

arXiv2024

Attosecond X-ray Core-level Chronoscopy of Aromatic Molecules

Attosecond photoemission or photoionization delays are a unique probe of the structure and the electronic dynamics of matter. However, spectral congestion and spatial delocalization of valence electron wave functions set fundamental limits to the complexity of systems that can be studied and the information that can be retrieved, respectively. Using attosecond X-ray pulses from LCLS, we demonstrate the key advantages of measuring core-level delays: the photoelectron spectra remain atom-like, the measurements become element specific and the observed scattering dynamics originate from a point-like source. We exploit these unique features to reveal the effects of electronegativity and symmetry on attosecond scattering dynamics by measuring and calculating the photoionization delays between N-1s and C-1s core shells of a series of aromatic azabenzene molecules. Remarkably, the delays increase with the number of nitrogen atoms in the molecule and reveal multiple resonances. We identify two previously unknown mechanisms regulating the associated attosecond dynamics, namely the enhanced confinement of the trapped wavefunction with increasing electronegativity of the atoms and the decrease of the coupling strength among the photoemitted partial waves with increasing symmetry. This study demonstrates the unique opportunities opened by measurements of core-level photoionization delays for unraveling attosecond electron dynamics in complex matter.

physics.chem-ph↗

arXiv2024

Experimental Demonstration of Attosecond Pump-Probe Spectroscopy with an X-ray Free-Electron Laser

Pump-probe experiments with sub-femtosecond resolution are the key to understanding electronic dynamics in quantum systems. Here we demonstrate the generation and control of sub-femtosecond pulse pairs from a two-colour X-ray free-electron laser (XFEL). By measuring the delay between the two pulses with an angular streaking diagnostic, we characterise the group velocity of the XFEL and demonstrate control of the pulse delay down to 270 as. We demonstrate the application of this technique to a pump-probe measurement in core-excited para-aminophenol. These results demonstrate the ability to perform pump-probe experiments with sub-femtosecond resolution and atomic site specificity.

physics.acc-ph↗

arXiv2021

SHarD: A beam dynamics simulationcode for dielectric laser acceleratorsbased on spatial harmonic field expansion

In order to demonstrate acceleration of electrons to relativistic scales by an on chipdielectric laser accelerator (DLA), a ponderomotive focusing scheme capable of capturingand transporting electrons through nanometer-scale apertures over extended interactionlengths has been proposed. We present a Matlab-based numerical code (SHarD) utilizinga spatial harmonic expansion of the fields within the dielectric structure to simulate theevolution of the beam phase space distribution in this scheme. The code can be usedto optimize key-parameters for the accelerator performance such as the final energy,transverse spot size evolution and total number of electrons accelerated through currentlyfabricated structures. Eventually, the simulation model will be applied to inform thephase mask profile to be added to a pulse front tilt drive laser pulse using a liquid crystalmask in the experimental setup being assembled at UCLA Pegasus Laboratory.

physics.acc-ph↗

arXiv2019

All Optical Control of Beam Dynamics in a DLA

Dielectric laser acceleration draws upon nano-fabrication techniques to build photonic structures for high gradient electron acceleration. At the small spatial scales characteristic of these structures conventional accelerator techniques become ineffective at stabilizing the beam dynamics. Instead we propose a scheme to stabilize the motion by directly modulating the drive laser, in analogy to a radio-frequency-quadrupole. Here we present a design for a programmable `lattice' being built at UCLA's Pegasus laboratory. The accelerator accepts an unmodulated 3.5 MeV electron beam and then bunches and accelerates the beam by 1.5 MeV over a distance of 2 cm.

physics.acc-ph↗

arXiv2019

Temporal magnification for streaked ultrafast electron diffraction and microscopy

One of the frontiers of modern electron scattering instrumentation is improving temporal resolution in order to enable the observation of dynamical phenomena at their fundamental time-scales. We analyze how a radiofrequency cavity can be used as an electron longitudinal lens in order to produce a highly magnified temporal replica of an ultrafast process, and, in combination with a deflecting cavity, enable streaked electron images of optical-frequency phenomena. We present start-to-end simulations of an MeV electron beamline for two variations of this idea (a `magnifying-glass' and a `point-projection' configuration) showing the feasibility for an electron probe to achieve single shot 1.4 fs(rms) temporal resolution.

physics.acc-ph↗

arXiv2016

Direct measurement of sub-10 fs relativistic electron beams with ultralow emittance

Ultralow emittance ($\leq20$ nm, normalized) electron beams with $10^5$ electrons per bunch are obtained by tightly focusing an ultrafast ($\sim$ 100 fs) laser pulse on the cathode of a 1.6 cell radiofrequency photoinjector. Taking advantage of the small initial longitudinal emittance, a downstream velocity bunching cavity is used to compress the beam to $<10$ fs rms bunch length. The measurement is performed using a thick high voltage deflecting cavity which is shown to be well-suited to measure ultrashort durations of bunching beams, provided that the beam reaches a ballistic longitudinal focus at the cavity center.

physics.acc-ph↗