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David Gershoni

Publications and source records attributed to David Gershoni.

At least 19 recordsLinked to original sources

Temporal CW polarization-tomography of photon pairs from the biexciton radiative cascade: theory and experiment

We study, experimentally and theoretically, temporal correlations between the polarization of photon pairs emitted during the biexciton-exciton radiative cascade from a single semiconductor quantum dot, optically excited by a continuous-wave light source. The system is modeled by a Lindbladian coupled to two Markovian baths: One bath represents the continuous light source, and a second represents the emitted radiation. Very good agreement is obtained between the theoretical model that we constructed and a set of 36 different time resolved, polarization correlation measurements between cascading photon pairs.

quant-ph

Eliminating the confined dark-exciton qubit precession using an externally applied magnetic field

We investigate experimentally and theoretically the behavior of the confined dark exciton in an InAs/GaAs semiconductor quantum dot, under the application of an external magnetic field in Voigt configuration. We show that by varying the magnitude and direction of the external field one can accurately control the dark-exciton fine-structure splitting. In addition, we show that the dark-exciton spin state is approximately polarized along the cubic crystallographic directions [100] or equivalents. By comparing our experimental results with a model for the exchange and Zeeman interactions, we find the conditions for nullifying the fine-structure splitting between the two eigenstates of the dark exciton, thereby stopping its qubit precession.

cond-mat.mes-hall

Continuous and deterministic all-photonic cluster state of indistinguishable photons

Cluster states are key resources for measurement-based quantum information processing. Photonic cluster and graph states, in particular, play indispensable roles in quantum network and quantum metrology. We demonstrate a semiconductor quantum dot based device in which the confined hole spin acts as a needle in a quantum knitting machine producing continuously and deterministically at sub-Gigahertz repetition rate single indistinguishable photons which are all polarization entangled to each other and to the spin in a one dimensional cluster state. By projecting two nonadjacent photons onto circular polarization bases we disentangle the spin from the photons emitted in between, thus continuously and deterministically preparing all-photonic cluster states for the first time. We use polarization tomography on four sequentially detected photons to demonstrate and to directly quantify the robustness of the cluster's entanglement and the determinism in its photon generation.

quant-ph

Magneto-optics of a charge-tunable quantum dot: Observation of a negative diamagnetic shift

We present magneto-optical studies of a self-assembled semiconductor quantum dot in neutral and positively charged states. The diamagnetic shifts and Zeeman splitting of many well-identified optical transitions are precisely measured. Remarkably, a pronounced negative diamagnetic shift is observed for spectral lines resulting from a doubly positively charged excitonic complex. We use the Hartree - Fock approximation for describing the direct Coulomb and exchange interactions between the quantum dot confined carriers in various configurations. A simple harmonic potential model, which we extend to capture the influence of an externally applied magnetic field in Faraday configuration, is then used to quantitatively account for all the measured diamagnetic shifts. We show that the negative shift is due to the change in the hole-hole exchange interaction energy induced by the magnetic field. Using this model and the measured shifts we extract the dielectric constant of the quantum dot material and get a decent estimate of the quantum dot dimensions. Further, the measured Zeeman splitting of the various spectral lines are also explained by a simple model using algebraic sums and differences of the $g$-factors of the confined charge carriers in their respective first and second discrete energy levels. Finally, the obtained values of the electronic $g$-factor and that of the dielectric constant are independently used to determine the effective composition (x) of the ternary In$_{x}$Ga$_{1-x}$As quantum dot. Both agree to within the experimental uncertainties.

cond-mat.mes-hall

Quantum dot molecule devices with optical control of charge status and electronic control of coupling

Tunnel-coupled pairs of optically active quantum dots - quantum dot molecules (QDMs) - offer the possibility to combine excellent optical properties such as strong light-matter coupling with two-spin singlet-triplet ($S-T_0$) qubits having extended coherence times. The $S-T_0$ basis formed using two spins is inherently protected against electric and magnetic field noise. However, since a single gate voltage is typically used to stabilize the charge occupancy of the dots and control the inter-dot orbital couplings, operation of the $S-T_0$ qubits under optimal conditions remains challenging. Here, we present an electric field tunable QDM that can be optically charged with one (1h) or two holes (2h) on demand. We perform a four-phase optical and electric field control sequence that facilitates the sequential preparation of the 2h charge state and subsequently allows flexible control of the inter-dot coupling. Charges are loaded via optical pumping and electron tunnel ionization. We achieve one- and two-hole charging efficiencies of 93.5 $\pm$ 0.8 % and 80.5 $\pm$ 1.3 %, respectively. Combining efficient charge state preparation and precise setting of inter-dot coupling allows control of few-spin qubits, as would be required for on-demand generation of two-dimensional photonic cluster states or quantum transduction between microwaves and photons.

cond-mat.mes-hall

A deterministic source of indistinguishable photons in a cluster state

Measurement-based quantum communication relies on the availability of highly entangled multi-photon cluster states. The inbuilt redundancy in the cluster allows communication between remote nodes using repeated local measurements, compensating for photon losses and probabilistic Bell-measurements. For feasible applications, the cluster generation should be fast, deterministic, and its photons - indistinguishable. We present a novel source based on a semiconductor quantum-dot device. The dot confines a heavy-hole, precessing in a finely tuned external weak magnetic field while periodically excited by a sequence of optical pulses. Consequently, the dot emits indistinguishable polarization-entangled photons, where the field strength optimizes the entanglement. We demonstrate Gigahertz rate deterministic generation of >90% indistinguishable photons in a cluster state with more than 10 photons characteristic entanglement-length.

quant-ph

Quantum tomography of entangled spin-multi-photon states

We present a novel method for quantum tomography of multi-qubit states. We apply the method to spin-multi-photon states, which we produce by periodic excitation of a semiconductor quantum-dot- confined spin every 1/4 of its coherent precession period. These timed excitations lead to the deterministic generation of strings of entangled photons in a cluster state. We show that our method can be used for characterizing the periodic process map, which produces the photonic cluster. From the measured process map, we quantify the robustness of the entanglement in the cluster. The 3-fold enhanced generation rate over previous demonstrations reduces the spin decoherence between the pulses and thereby increases the entanglement.

quant-ph

The coherence of quantum dot confined electron- and hole-spin in low external magnetic field

We investigate experimentally and theoretically the temporal evolution of the spin of the conduction band electron and that of the valence band heavy hole, both confined in the same semiconductor quantum dot. In particular, the coherence of the spin purity in the limit of a weak externally applied magnetic field, comparable in strength to the Overhauser field due to fluctuations in the surrounding nuclei spins. We use an all-optical pulse technique to measure the spin evolution as a function of time after its initialization. We show for the first time that the spin purity performs complex temporal oscillations which we quantitatively simulate using a central spin model. Our model encompasses the Zeeman and the hyperfine interactions between the spin and the external and Overhauser fields, respectively. Our novel studies are essential for the design and optimization of quantum-dot-based entangled multi-photon sources. Specifically, cluster and graph states, which set stringent limitations on the magnitude of the externally applied field.

cond-mat.mes-hall

Selective Noise Resistant Gate

Realizing individual control on single qubits in a spin-based quantum register is an ever-increasing challenge due to the close proximity of the qubits resonance frequencies. Current schemes typically suffer from an inherent trade-off between fidelity and qubits selectivity. Here, we report on a new scheme which combines noise protection by dynamical decoupling and magnetic gradient based selectivity, to enhance both the fidelity and the selectivity. With a single nitrogen-vacancy center in diamond, we experimentally demonstrate quantum gates with fidelity = 0.9 $\pm$ 0.02 and a 50 kHz spectral bandwidth, which is almost an order of magnitude narrower than the unprotected bandwidth. Our scheme will enable selective control of an individual nitrogen-vacancy qubit in an interacting qubits array using relatively moderate gradients of about 1 mG/nm.

quant-ph

Optical Phase Measurement Using a Deterministic Source of Entangled Multi-photon States

Precision measurements of optical phases have many applications in science and technology. Entangled multi-photon states have been suggested for performing such measurements with precision that significantly surpasses the shot-noise limit. Until recently, such states have been generated mainly using spontaneous parametric down-conversion -- a process which is intrinsically probabilistic, counteracting the advantages that the entangled photon states might have. Here, we use a semiconductor quantum dot to generate entangled multi-photon states in a deterministic manner, using periodic timed excitation of a confined spin. This way we entangle photons one-by-one at a rate which exceeds 300 MHz. We use the resulting multi-photon state to demonstrate super-resolved optical phase measurement. Our results open up a scalable way for realizing genuine quantum enhanced super-sensitive measurements in the near future.

cond-mat.mes-hall

Complete state tomography of a quantum dot confined spin qubit

Semiconductor quantum dots are probably the preferred choice for interfacing anchored, matter spin qubits and flying photonic qubits. While full tomography of a flying qubit or light polarization is in general straightforward, matter spin tomography is a challenging and resource-consuming task. Here we present a novel all-optical method for conducting full tomography of quantum-dot-confined spins. Our method is applicable for electronic spin configurations such as the conduction-band electron, the valence-band hole, and for electron-hole pairs such as the bright and the dark exciton. We excite the spin qubit using short resonantly tuned, polarized optical pulse, which coherently converts the qubit to an excited qubit that decays by emitting a polarized single-photon. We perform the tomography by using two different orthogonal, linearly polarized excitations, followed by time-resolved measurements of the degree of circular polarization of the emitted light from the decaying excited qubit. We demonstrate our method on the dark exciton spin state with fidelity of 0.94, mainly limited by the accuracy of our polarization analyzers.

quant-ph

Depolarization of Electronic Spin Qubits Confined in Semiconductor Quantum Dots

Quantum dots are arguably the best interface between matter spin qubits and flying photonic qubits. Using quantum dot devices to produce joint spin-photonic states requires the electronic spin qubits to be stored for extended times. Therefore, the study of the coherence of spins of various quantum dot confined charge carriers is important both scientifically and technologically. In this study we report on spin relaxation measurements performed on five different forms of electronic spin qubits confined in the very same quantum dot. In particular, we use all optical techniques to measure the spin relaxation of the confined heavy hole and that of the dark exciton - a long lived electron-heavy hole pair with parallel spins. Our measured results for the spin relaxation of the electron, the heavy-hole, the dark exciton, the negative and the positive trions, in the absence of externally applied magnetic field, are in agreement with a central spin theory which attributes the dephasing of the carriers' spin to their hyperfine interactions with the nuclear spins of the atoms forming the quantum dots. We demonstrate that the heavy hole dephases much slower than the electron. We also show, both experimentally and theoretically, that the dark exciton dephases slower than the heavy hole, due to the electron-hole exchange interaction, which partially protects its spin state from dephasing.

cond-mat.mes-hall

Accessing the dark exciton spin in deterministic quantum-dot microlenses

The dark exciton state in semiconductor quantum dots constitutes a long-lived solid-state qubit which has the potential to play an important role in implementations of solid-state based quantum information architectures. In this work, we exploit deterministically fabricated QD microlenses with enhanced photon extraction, to optically prepare and readout the dark exciton spin and observe its coherent precession. The optical access to the dark exciton is provided via spin-blockaded metastable biexciton states acting as heralding state, which are identified deploying polarization-sensitive spectroscopy as well as time-resolved photon cross-correlation experiments. Our experiments reveal a spin-precession period of the dark exciton of $(0.82\pm0.01)\,$ns corresponding to a fine-structure splitting of $(5.0\pm0.7)\,μ$eV between its eigenstates $\left|\uparrow\Uparrow\pm\downarrow\Downarrow\right\rangle$. By exploiting microlenses deterministically fabricated above pre-selected QDs, our work demonstrates the possibility to scale up implementations of quantum information processing schemes using the QD-confined dark exciton spin qubit, such as the generation of photonic cluster states or the realization of a solid-state-based quantum memory.

quant-ph

Deterministic Generation of a Cluster State of Entangled Photons

We use semiconductor quantum dots, "artificial atoms," to implement a scheme for deterministic generation of long strings of entangled photons in a cluster state, an important resource for quantum information processing. We demonstrate a prototype device which produces strings of a few hundred photons in which the entanglement persists over 5 sequential photons. The implementation follows a proposal by Lindner and Rudolph (Phys. Rev. Lett. 2009) which suggested periodic timed excitation of a precessing electron spin as a mechanism for entangling the electron spin with the polarization of the sequentially emitted photons. In our realization, the entangling qubit is a quantum dot confined dark exciton. By performing full quantum process tomography, we obtain the process map which fully characterizes the evolution of the system, containing the dark exciton and n photons after n applications of the periodic excitations. Our implementation may greatly reduce the resources needed for quantum information processing.

quant-ph

Local probing of nuclear bath polarization with a single electronic spin

We demonstrate experimentally that a polarized nuclear spin modifies the dynamic behavior of a neighboring electronic spin. Specifically, an out-of-phase component appears in the electronic spin-echo signal. This component is proportional to the nuclear spin degree of polarization and strongly depends on the nuclear polarization direction. When the electronic spin is surrounded by a polarized nuclear spin bath, the spin-echo quadrature manifests a characteristic frequency related only to the nuclear spins abundance and their collective polarization. We use this analysis to propose a novel measurement method for the local nuclear spin bath of a single electronic spin. We quantify the realistic experimental regimes at which the scheme is efficient. Our proposal has potential applications for quantum sensing schemes, and opens a route for a systematic study of polarized mesoscopical-systems.

quant-ph

Local and bulk 13C hyperpolarization in NV-centered diamonds at variable fields and orientations

Polarizing nuclear spins is of fundamental importance in biology, chemistry and physics. Methods for hyperpolarizing 13C nuclei from free electrons in bulk, usually demand operation at cryogenic temperatures. Room-temperature approaches targeting diamonds with nitrogen-vacancy (NV) centers could alleviate this need, but hitherto proposed strategies lack generality as they demand stringent conditions on the strength and/or alignment of the magnetic field. We report here an approach for achieving efficient electron->13C spin alignment transfers, compatible with a broad range of magnetic field strengths and field orientations with respect to the diamond crystal. This versatility results from combining coherent microwave- and incoherent laser-induced transitions between selected energy states of the coupled electron-nuclear spin manifold. 13C-detected Nuclear Magnetic Resonance (NMR) experiments demonstrate that this hyperpolarization can be transferred via first-shell or via distant 13Cs, throughout the nuclear bulk ensemble. This method opens new perspectives for applications of diamond NV centers in NMR, and in quantum information processing.

quant-ph

Optically Detected Magnetic Resonance Imaging

Optically detected magnetic resonance (ODMR) provides ultrasensitive means to detect and image a small number of electron and nuclear spins, down to the single spin level with nanoscale resolution. Despite the significant recent progress in this field, it has never been combined with the power of pulsed magnetic resonance imaging (MRI) techniques. Here, we demonstrate for the first time how these two methodologies can be integrated using short pulsed magnetic field gradients to spatially-encode the sample. This results in what we denote as an "optically detected magnetic resonance imaging" (ODMRI) technique. It offers the advantage that the image is acquired in parallel from all parts of the sample, with well-defined three-dimensional point-spread function, and without any loss of spectroscopic information. In addition, this approach may be used in the future for parallel but yet spatially-selective efficient addressing and manipulation of the spins in the sample. Such capabilities are of fundamental importance in the field of quantum spin-based devices and sensors.

cond-mat.mes-hall

Time-Optimal Universal Control of Two-Level Systems under Strong Driving

We experimentally study the time-optimal construction of arbitrary single-qubit rotations under a single strong driving field of finite amplitude. Using radiation-dressed states of nitrogen vacancy centers in diamond, we realize a strongly-driven two-level system and achieve driving frequencies four times larger than its Larmor frequency. We implement time optimal universal rotations on this system, characterize their performance using quantum process tomography, and demonstrate a dual-axis ac magnetometry sequence with pulses at sub-Larmor time scales. Our results pave the way for applying fast qubit control and high-density pulse schemes in the fields of quantum information processing and quantum metrology.

quant-ph