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David Hofman

Publications and source records attributed to David Hofman.

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In-situ total scattering investigation of crystalline ordering in amorphous ion-beam sputtered thin films for interferometric gravitational wave detectors

Amorphous tantala is an important optical material used in a number of high-precision optical applications, including gravitational wave interferometry. In this paper, we study in-situ the structural changes that occur in amorphous ion-beam sputtered coatings during an annealing treatment by means of a synchrotron radiation scattering experiment. The scattering signal is measured as a function of time on a large range of the Q-space. X-Ray diffraction and Rietveld analysis are used to study crystallization during the annealing treatment, whereas pair distribution function analysis allows to inspect the structural changes occurring during the amorphous to crystalline transition. Our findings indicate that several structural rearrangements occur in parallel, namely a first quick establishment of a backbone structure in the cationic substructure appearing on a rather extended range (up to 100 Angstrom), followed by a progressive rearrangement of the oxygen atoms environment which gradually increases the crystallinity of the structure.

cond-mat.mtrl-sci

Elastic and structural anisotropy in silica thin films for gravitational-wave detectors

The thermal noise of mirror coatings for gravitational-wave detectors critically depends on the elastic properties of the constituent materials. Data analyses and theoretical models typically assume each material is homogeneous and isotropic, but isotropy has never been explicitly verified. Using Brillouin light scattering (BLS), we demonstrate for the first time that ion-beam-sputtered SiO2 -- a material still viable for future mirror coatings -- exhibits cylindrical elastic symmetry, with in-plane isotropy but a notable 6% compressive anisotropy along the film normal. This anisotropy remains unchanged after the post-deposition heat treatment currently used in ground-based detectors (500 $^\circ$C, 10 h) but is nearly eliminated at 900 $^\circ$C. Infrared reflectivity experiments support these findings by directly revealing heterogeneities in the distribution of bridging and non-bridging oxygen structures along the growth axis. While BLS measures the real part of the elastic constants at GHz frequencies, the data reveal negligible contributions from mechanical relaxations in the kHz-GHz range, making BLS a valid substitute for low-frequency properties obtained from standard anisotropy-insensitive techniques. Our results highlight that restoring isotropy through heat treatment -- by softening the material, enabling more than 7% out-of-plane expansion, and smoothing out structural heterogeneities -- may play a key role in reducing thermal noise. This proof-of-concept study extends beyond silica, providing critical insights for the design of future coatings.

physics.optics

Comparison of arm cavity optical losses for the two wavelengths of the Einstein Telescope gravitational wave detector

A new generation of gravitational wave detectors is currently being designed with the likely use of a different laser wavelength compared to current instruments. The estimation of the optical losses for this new wavelength is particularly relevant to derive the detector sensitivity and also to anticipate the optical performances of future instruments. In this article, we measured the absorption and angle-resolved scattering of several mirror samples in order to compare optical losses at a wavelength of 1064 and 1550\ nm. In addition, we have carried out simulations of the Einstein Telescope arm cavities at 1064 and 1550\ nm taking into account losses due to surface low-spatial frequency flatness. Our results suggest that optical losses as measured at 1064\ nm are about twice as large as those at 1550\ nm as predicted with a simple model.

physics.optics