arXiv subjects

David Novoa

Publications and source records attributed to David Novoa.

At least 19 recordsLinked to original sources

arXiv2026

High-Polarization-Extinction Raman Conversion in Gas-Filled Polarization-Maintaining Hollow-Core Fibers

Gas-filled hollow-core fibers (HCFs) have emerged as a versatile platform for high-power nonlinear optics, enabling phenomena from ultrafast pulse compression to broadband frequency generation. However, the lack of robust polarization control has remained a critical obstacle to the deployment of gas-based fiber sources. Here, we overcome this bottleneck by demonstrating the generation of highly-polarized Stokes light via stimulated Raman scattering (SRS) in a nitrogen-filled polarization-maintaining anti-resonant hollow-core fiber (PM-HCF). By exploiting the strong structural birefringence of the fiber, the Raman interaction becomes polarization-decoupled along the principal birefringence axes, leading to threshold-selective Raman amplification and an intrinsic polarization purification mechanism. As a result, the vibrational Raman Stokes emission exhibits a polarization extinction ratio (PER) of 35 dB, even when the incident pump PER is as low as ~2 dB. Through analytical theory and numerical modeling, we validate the underlying polarization-selective Raman dynamics and identify the fiber platform as the dominant factor governing the observed PER saturation. We further show that this high polarization purity and high conversion efficiency is maintained under tight bending conditions with radii down to 5 cm, in stark contrast to conventional non-PM-HCF. These results establish PM-HCFs as a robust and scalable architecture for generating polarization-stable, frequency-shifted light, and indicate that polarization may be treated as an actively engineerable degree of freedom in gas photonics, paving the way toward deployment-ready gas-based fiber sources for precision metrology, quantum communication, and coherent sensing.

physics.optics↗

arXiv2025

Scaling of nonlinear dynamics driven by stimulated Raman scattering in gas-filled hollow-core fibers

Optical systems are scalable under low-intensity illumination since their governing equations are linearly dependent of the optical signal strength. Nonetheless, in high-intensity regimes, the induced polarization becomes nonlinear, rendering the simple scalability of the previous systems invalid. Despite this, canonical nonlinear phenomena such as filamentation and high-harmonic generation in free space have recently been demonstrated to be scalable. Here we will discuss the extension of the scale-invariance paradigm to stimulated Raman scattering and molecular modulation in hollow anti-resonant fibers filled with Raman-active gases. We have found that the complex in-fiber dynamics can be accurately reproduced under very different conditions by keeping the so-called gain reduction factor, that accounts for the coupling of the interacting fields, as well as the dephasing time $T_2$ unaltered. Such scaling strategy enables access to equivalent nonlinear propagation scenarios without sacrificing performance, laying the foundations for to the design of nonlinear devices operating in exotic frequencies, like the ultraviolet, or quantum frequency convertors of non-classical light.

physics.optics↗

arXiv2024

Entanglement transfer during quantum frequency conversion in gas-filled hollow-core fibers

Quantum transduction is essential for the future hybrid quantum networks, connecting devices across different spectral ranges. In this regard, molecular modulation in hollow-core fibers has proven to be exceptional for efficient and tunable frequency conversion of arbitrary light fields down to the single-photon limit. However, insights on this conversion method for quantum light have remained elusive beyond standard semiclassical models. In this Letter, we employ a quantum Hamiltonian framework to characterize the behavior of entanglement during molecular modulation, while describing the quantum dynamics of both molecules and photons in agreement with recent experiments. In particular, apart from obtaining analytical expressions for the final opto-molecular states, our model predicts a close correlation between the evolution of the average photon numbers and the transfer of entanglement between the interacting parties. These results will contribute to the development of new fiber-based strategies to tackle the challenges associated with the upcoming generation of lightwave quantum technologies.

quant-ph↗

arXiv2024

Stimulated Raman Scattering and Molecular Modulation in Anti-resonant Hollow-core Fibres

Raman scattering is the inelastic process where photons bounce off molecules, losing energy and becoming red-shifted. This weak effect is unique to each molecular species, making it an essential tool in e.g. spectroscopy and label-free microscopy. The invention of the laser enabled a regime of stimulated Raman scattering (SRS), where the efficiency is greatly increased by inducing coherent molecular oscillations. However, this phenomenon required high intensities due to the limited interaction volumes, and this limitation was overcome by the emergence of anti-resonant fibres (ARFs) guiding light in a small hollow channel over long distances. Based on their unique properties, this Perspective reviews the transformative impact of ARFs on modern SRS-based applications ranging from development of light sources and convertors for spectroscopy and materials science, to quantum technologies for the future quantum networks, providing insights into future trends and the expanding horizons of the field.

physics.optics↗

arXiv2023

Shortcuts to Adiabatic Soliton Compression in Active Nonlinear Kerr Media

We implement variational shortcuts to adiabaticity for optical pulse compression in an active nonlinear Kerr medium with distributed amplification and spatially varying dispersion and nonlinearity. Starting with the hyperbolic secant ansatz, we employ a variational approximation to systematically derive dynamical equations, establishing analytical relationships linking the amplitude, width, and chirp of the pulse. Through the inverse engineering approach, we manipulate the distributed gain/loss, nonlinearity and dispersion profiles to efficiently compress the optical pulse over a reduced distance with high fidelity. In addition, we explore the dynamical stability of the system to illustrate the advantage of our protocol over conventional adiabatic approaches. Finally, we analyze the impact of tailored higher-order dispersion on soliton self-compression and derive physical constraints on the final soliton width for the complementary case of soliton expansion. The broader implications of our findings extend beyond optical systems, encompassing areas such as cold-atom and magnetic systems highlighting the versatility and relevance of our approach in various physical contexts.

physics.optics↗

arXiv2023

Generation of THz radiation through molecular modulation in hydrogen-filled hybrid anti-resonant fibers

We study the generation of narrowband terahertz (THz) pulses by stimulated Raman scattering and molecular modulation in hydrogen-filled hybrid hollow-core fibers. Using a judicious combination of materials and transverse structures, this waveguide design enables simultaneous confinement of optical and THz signals with reasonably low attenuation, as well as high nonlinear overlap. The THz pulses are then generated as the second Stokes band of a ns-long near-infrared pump pulse, aided by Raman coherence waves excited in the gaseous core by the beat-note created by the pump and its first Stokes band. Optimization of the fiber characteristics facilitates phase matching between the corresponding transitions and coherence waves while avoiding coherent gain suppression, resulting in optical-to-THz conversion efficiencies up to 60%, as confirmed by rigorous numerical modelling under ideal conditions. When the current optical material constraints are considered, however, the attainable efficiencies relax to 0.2%, a still competitive value compared to other systems. The approach is in principle power and energy scalable, as well as tunable in the 1 - 10 THz range without any spectral gaps, thereby opening new pathways to the development of fiber-based THz sources complementary to other mature technologies such as quantum cascade lasers.

physics.optics↗

arXiv2022

High-quality 8-fold self-compression of ultrashort near-UV pulses in Ar-filled ultrathin-walled photonic crystal fiber

We demonstrate generation of 7.6 fs near-UV pulses centered at 400 nm via 8-fold soliton-effect self-compression in an Ar-filled hollow-core kagom\'e-style photonic crystal fiber with ultrathin core walls. Analytical calculations of the effective compression length and soliton order permit adjustment of the experimental parameters, and numerical modelling of the nonlinear pulse dynamics in the fiber accurately predict the spectro-temporal profiles of the self-compressed pulses. After compensation of phase distortion introduced by the optical elements along the beam path from the fiber to the diagnostics, 71% of the pulse energy was in the main temporal lobe, with peak powers in excess of 0.2 GW. The convenient set-up opens up new opportunities for time-resolved studies in spectroscopy, chemistry and materials science.

physics.optics↗

arXiv2021

Efficient self-compression of ultrashort UV pulses in air-filled hollow-core photonic crystal fiber

We report generation of ultrashort UV pulses by soliton self-compression in kagom\'e-style hollow-core photonic crystal fiber filled with ambient air. Pump pulses with energy 2.6 uJ and duration 54 fs at 400 nm were compressed temporally by a factor of 5, to a duration of ~11 fs. The experimental results are supported by numerical simulations, showing that both Raman and Kerr effects play a role in the compression dynamics. The convenience of using ambient air, and the absence of glass windows that would distort the compressed pulses, makes the setup highly attractive as the basis of an efficient table-top UV pulse compressor.

physics.optics↗

arXiv2020

High-brightness seven-octave carrier envelope phase-stable light source

High-brightness sources of coherent and few-cycle-duration light waveforms with spectral coverage from the UV to the THz would offer unprecedented versatility and opportunities for a spectacular range of applications from bio-chemical sensing, to time-resolved and nonlinear spectroscopy, to attosecond light-wave electronics. Combinations of various sources with frequency conversion and supercontinuum generation can provide relatively large spectral coverage, but many applications require much broader spectral range and low-jitter synchronization for time-domain measurements. Here, we present a carrier-envelope-phase stable light source, seeded by a mid-IR frequency comb, with simultaneous spectral coverage across 7 optical octaves, from the UV (340 nm) into the THz (40,000 nm). Combining soliton self-compression and dispersive wave generation in an anti-resonant-reflection photonic crystal fibre with intra-pulse difference frequency generation in BaGa2GeSe6, the spectral brightness is 2-5 orders of magnitude above synchrotron sources. This enables high-dynamic-range spectroscopies and provides enticing prospects for attosecond physics and material sciences.

physics.optics↗

arXiv2020

Generation of sub-40 fs pulses at 1.8 \mu m by chirp-assisted Raman scattering in hydrogen-filled hollow-core fibre

The possibility of performing time-resolved spectroscopic studies in the molecular fingerprinting region or extending the cut-off wavelength of high-harmonic generation has recently boosted the development of efficient mid-infrared ultrafast lasers. In particular, fibre lasers based on active media such as thulium or holmium are a very active area of research since they are robust, compact and can operate at high repetition rates. These systems, however, are still complex, are unable to deliver pulses shorter than 100 fs and are not yet as mature as their near-infrared counterparts. Here we report generation of sub-40 fs pulses at 1.8 microns, with quantum efficiencies of 50% and without need for post-compression, in hydrogen-filled hollow-core photonic crystal fibre pumped by a commercial 300-fs fibre laser at 1030 nm. This is achieved by pressure-tuning the dispersion and avoiding Raman gain suppression by adjusting the chirp of the pump pulses and the proportion of higher order modes launched into the fibre. The system is optimized using a physical model that incorporates the main linear and nonlinear contributions to the optical response. The approach is average power-scalable, permits adjustment of the pulse shape and can potentially allow access to much longer wavelengths.

physics.optics↗

arXiv2020

Narrowband vacuum ultraviolet light via cooperative Raman scattering in dual-pumped gas-filled photonic crystal fiber

Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do not simultaneously fulfill those two requirements, and few if any are truly compact, cost-effective and easy to use by non-specialists. Here we introduce a novel approach that goes a long way to meeting this challenge. It is based on hydrogen-filled hollow-core photonic crystal fiber pumped simultaneously by two spectrally distant pulses. Stimulated Raman scattering enables the generation of coherence waves of collective molecular motion in the gas, which together with careful dispersion engineering and control over the modal content of the pump light, facilitates cooperation between the two separate Raman combs, resulting in a spectrum that reaches deep into the VUV. Using this system, we demonstrate the generation of a dual Raman comb of narrowband lines extending down to 141 nm using only 100 mW of input power delivered by a commercial solid-state laser. The approach may enable access to tunable VUV light to any laboratory and therefore boost progress in many research areas across multiple disciplines.

physics.optics↗

arXiv2018

Thresholdless deep and vacuum ultraviolet Raman frequency conversion in H$_2$-filled photonic crystal fiber

Coherent ultraviolet (UV) light has many uses, for example in the study of molecular species relevant in biology and chemistry. Very few if any laser materials offer UV transparency along with damage-free operation at high photon energies and laser power. Here we report efficient generation of deep and vacuum UV light using hydrogen-filled hollow-core photonic crystal fiber (HC-PCF). Pumping above the stimulated Raman threshold at 532 nm, coherent molecular vibrations are excited in the gas, permitting highly efficient thresholdless wavelength conversion in the UV. The system is uniquely pressure-tunable, allows spatial structuring of the out-coupled radiation, and shows excellent performance in the vacuum UV. It can also in principle operate at the single-photon level, when all other approaches are extremely inefficient.

physics.optics↗

arXiv2018

UV soliton dynamics and Raman-enhanced supercontinuum generation in photonic crystal fiber

Ultrafast broadband ultraviolet radiation is of importance in spectroscopy and photochemistry, since high photon energies enable single-photon excitations and ultrashort pulses allow time-resolved studies. Here we report the use of gas-filled hollow-core photonic crystal fibers (HC-PCFs) for efficient ultrafast nonlinear optics in the ultraviolet. Soliton self-compression of 400 nm pulses of (unprecedentedly low) ~500 nJ energies down to sub-6-fs durations is achieved, as well as resonant emission of tunable dispersive waves from these solitons. In addition, we discuss the generation of a flat supercontinuum extending from the deep ultraviolet to the visible in a hydrogen-filled HC-PCF. Comparisons with argon-filled fibers show that the enhanced Raman gain at high frequencies makes the hydrogen system more efficient. As HC-PCF technology develops, we expect these fiber-based ultraviolet sources to lead to new applications.

physics.optics↗

arXiv2018

Dominance of backward stimulated Raman scattering in gas-filled hollow-core photonic crystal fibers

Backward stimulated Raman scattering in gases provides a promising route to compression and amplification of a Stokes seed-pulse by counter-propagating against a pump-pulse, as has been already demonstrated in various platforms, mainly in free-space. However, the dynamics governing this process when seeded by noise has not yet been investigated in a fully controllable collinear environment. Here we report the first unambiguous observation of efficient noise-seeded backward stimulated Raman scattering in a hydrogen-filled hollow-core photonic crystal fiber. At high gas pressures, when the backward Raman gain is comparable with, but lower than, the forward gain, we report quantum conversion efficiencies exceeding 40% to the backward Stokes at 683 nm from a narrowband 532-nm-pump. The efficiency increases to 65% when the backward process is seeded by a small amount of back-reflected forward-generated Stokes light. At high pump powers the backward Stokes signal, emitted in a clean fundamental mode and spectrally pure, is unexpectedly always stronger than its forward-propagating counterpart. We attribute this striking observation to the unique temporal dynamics of the interacting fields, which cause the Raman coherence (which takes the form of a moving fine-period Bragg grating) to grow in strength towards the input end of the fiber. A good understanding of this process, together with the rapid development of novel anti-resonant-guiding hollow-core fibers, may lead to improved designs of efficient gas-based Raman lasers and amplifiers operating at wavelengths from the ultraviolet to the mid-infrared.

physics.optics↗

arXiv2017

Effect of anti-crossings with cladding resonances on ultrafast nonlinear dynamics in gas-filled PCFs

Spectral anti-crossings between the fundamental guided mode and core wall resonances alter the dispersion in hollow-core anti-resonant-reflection photonic crystal fibers. Here we study the effect of this dispersion change on the nonlinear propagation and dynamics of ultrashort pulses. We find that it causes emission of narrow spectral peaks through a combination of four-wave mixing and dispersive wave emission. We further investigate the influence of the anti-crossings on nonlinear pulse propagation and show that their impact can be minimized by adjusting the core-wall thickness in such a way that the anti-crossings lie spectrally distant from the pump wavelength.

physics.optics↗

arXiv2017

Enhanced Control of Transient Raman Scattering Using Buffered Hydrogen in Hollow-Core PCF

Many reports on stimulated Raman scattering in mixtures of Raman-active and noble gases indicate that the addition of a dispersive buffer gas increases the phase-mismatch to higher-order Stokes and antiStokes sidebands, resulting in preferential conversion to the first few Stokes lines, accompanied by a significant reduction in Raman gain due to collisions with buffer gas molecules. Here we report that, provided the dispersion can be precisely controlled, the effective Raman gain in gas-filled hollow-core photonic crystal fiber (PCF) can actually be significantly enhanced when a buffer gas is added. This counterintuitive behavior occurs when the nonlinear coupling between the interacting fields is strong, and can result in a performance similar to that of a pure Raman-active gas, but at much lower total gas pressure, allowing competing effects such as Raman backscattering to be suppressed. We report high modal purity in all the emitted sidebands, along with anti-Stokes conversion efficiencies as high as 5% in the visible and 2% in the ultraviolet. The results point to a new class of gas-based waveguide device in which the pressure-tunable nonlinear optical response is beneficially adjusted by the addition of other gases.

physics.optics↗

arXiv2017

Coherent control of flexural vibrations in dual-nanoweb fibers using phase-modulated two-frequency light

Coherent control of the resonant response in spatially extended optomechanical structures is complicated by the fact that the optical drive is affected by the back-action from the generated phonons. Here we report a new approach to coherent control based on stimulated Raman-like scattering, in which the optical pressure can remain unaffected by the induced vibrations even in the regime of strong optomechanical interactions. We demonstrate experimentally coherent control of flexural vibrations simultaneously along the whole length of a dual-nanoweb fiber, by imprinting steps in the relative phase between the components of a two-frequency pump signal,the beat frequency being chosen to match a flexural resonance. Furthermore, sequential switching of the relative phase at time intervals shorter than the lifetime of the vibrations reduces their amplitude to a constant value that is fully adjustable by tuning the phase-modulation depth and switching rate. The results may trigger new developments in silicon photonics, since such coherent control uniquely decouples the amplitude of optomechanical oscillations from power-dependent thermal effects and nonlinear optical loss.

physics.optics↗

arXiv2017

Generation of Broadband Mid-IR and UV Light in Gas-Filled Single-Ring Hollow-Core PCF

We report generation of an ultrafast supercontinuum extending into the mid- infrared in gas-filled single-ring hollow-core photonic crystal fiber (SR-PCF) pumped by 1.7 $\mu$m light from an optical parametric amplifier. The simple fiber structure offers shallow dispersion and flat transmission in the near and mid-infrared, enabling the generation of broadband spectra extending from 300 nm to 3.1 $\mu$m, with a total energy of a few $\mu$J. In addition, we report the emission of ultraviolet dispersive waves whose frequency can be tuned simply by adjusting the pump wavelength. SR-PCF also provides an effective means of compressing and delivering tunable ultrafast pulses in the near and mid-infrared spectral regions.

physics.optics↗