arXiv subjects

David P. Lake

Publications and source records attributed to David P. Lake.

At least 19 recordsLinked to original sources

arXiv2024

Optical Switching of $\chi^{(2)}$ in Diamond Photonics

Diamond's unique physical properties make it a versatile material for a wide range of nonlinear and quantum photonic technologies. However, unlocking diamond's full potential as a nonlinear photonic material with non-zero second-order susceptibility $\chi^{(2)}\neq0$ requires symmetry breaking. In this work, we use a nanoscale cavity to demonstrate second-harmonic generation (SHG) in diamond, and demonstrate, for the first time, that the magnitude of the diamond's effective $\chi^{(2)}$ strongly depends on the electronic configuration of defects in the diamond crystal, such as nitrogen-vacancy centres. The modification of $\chi^{(2)}$ arises from photoionisation from the negative to neutral charge-state, and is manifested by quenching of SHG upon green illumination. Toggling the green illumination allows for optical switching of the device's $\chi^{(2)}$. Optical control of $\chi^{(2)}$ by defect engineering opens the door for second-order nonlinear processes in diamond.

physics.optics↗

arXiv2024

Nonlinear optical charge state switching and pumping to a diamond NV center dark state

The photodynamics of diamond nitrogen-vacancy (NV) centers limits their performance in many quantum technologies. Quenching of photoluminescence, which degrades NV readout, is commonly ascribed to a dark state that is not fully understood. Using a nanoscale cavity to generate intense infrared fields that quench NV emission nonlinearly with field intensity, we show that the dark state is accessed by two-photon pumping into the $^4\!A_2$ quartet state of the neutrally charged NV (NV$^0$). We constrain this state's energy relative to the NV$^0$ ground-state ($^2\!E$) to ${<}0.58$\,eV and the recombination energy threshold to the NV$^-$ ground state ($^3\!A_2$) to $\leq2.33\,\text{eV}$. Furthermore, we estimate the intrinsic lifetime of $^4\!A_2$ state to be $1.78-6.06\,\mu\text{s}$ and show that accessing this state allows sensing of local infrared fields. This new understanding will allow predictions of the limits of NV technologies reliant upon intense fields, including levitated systems, spin--optomechanical devices, and absorption--based magnetometers.

quant-ph↗

arXiv2023

In-situ tuning of optomechanical crystals with nano-oxidation

Optomechanical crystals are a promising device platform for quantum transduction and sensing. Precise targeting of the optical and acoustic resonance frequencies of these devices is crucial for future advances on these fronts. However, fabrication disorder in these wavelength-scale nanoscale devices typically leads to inhomogeneous resonance frequencies. Here we achieve in-situ, selective frequency tuning of optical and acoustic resonances in silicon optomechanical crystals via electric field-induced nano-oxidation using an atomic-force microscope. Our method can achieve a tuning range >2 nm (0.13%) for the optical resonance wavelength in the telecom C-band, and >60 MHz (1.2%) for the acoustic resonance frequency at 5 GHz. The tuning resolution of 1.1 nm for the optical wavelength, and $150$ kHz for the acoustic frequency allows us to spectrally align multiple optomechanical crystal resonators using optimal oxidation patterns determined via an inverse design protocol. Our results establish a method for precise post-fabrication tuning of optomechancical crystals. This technique can enable coupled optomechanical resonator arrays, scalable resonant optomechanical circuits, and frequency matching of microwave-optical quantum transducers.

physics.optics↗

arXiv2023

Fiber-taper collected emission from NV centers in high-$Q/V$ diamond microdisks

Fiber-coupled microdisks are a promising platform for enhancing the spontaneous emission from color centers in diamond. The measured cavity-enhanced emission from the microdisk is governed by the effective volume ($V$) of each cavity mode, the cavity quality factor ($Q$), and the coupling between the microdisk and the fiber. Here we observe photoluminescence from an ensemble of nitrogen-vacancy centers into high $Q/V$ microdisk modes, which when combined with coherent spectroscopy of the microdisk modes, allows us to elucidate the relative contributions of these factors. The broad emission spectrum acts as an internal light source facilitating mode identification over several cavity free spectral ranges. Analysis of the fiber-taper collected microdisk emission reveals spectral filtering both by the cavity and the fiber-taper, the latter of which we find preferentially couples to higher-order microdisk modes. Coherent mode spectroscopy is used to measure $Q\sim 1\times10^{5}$ -- the highest reported values for diamond microcavities operating at visible wavelengths. With realistic optimization of the microdisk dimensions, we predict that Purcell factors of $\sim 50$ are within reach.

physics.optics↗

arXiv2023

Feedback Enhanced Phonon Lasing of a Microwave Frequency Resonator

The amplitude of self-oscillating mechanical resonators in cavity optomechanical systems is typically limited by nonlinearities arising from the cavity's finite optical bandwidth. We propose and demonstrate a feedback technique for increasing this limit. By modulating the cavity input field with a signal derived from its output intensity, we increase the amplitude of a self-oscillating GHz frequency mechanical resonator by $22\%$ (increase in coherent phonon number of $50\%$) limited only by the achievable optomechanical cooperativity of the system. This technique will advance applications dependent on high dynamic mechanical stress, such as coherent spin-phonon coupling, as well as implementations of sensors based on self-oscillating resonators.

physics.optics↗

arXiv2022

High frequency torsional motion transduction using optomechanical coupled oscillators

Using light to measure an object's motion is central to operating mechanical sensors that probe forces and fields. Cavity optomechanical systems embed mechanical resonators inside optical resonators. This enhances the sensitivity of optomechanical measurements, but only if the mechanical resonator does not spoil the properties of the optical cavity. For example, cavity optomechanical detection of resonators made from optically absorbing materials, or whose geometry does not possess suitable spatial symmetry, is challenging. Here we demonstrate a system that overcomes challenges in measuring high-frequency twisting motion of a nanodisk by converting them to vibrations of a photonic crystal cavity. Optomechanical readout of the cavity then enables measurement of the nanodisk's torsional resonances with sensitivity $5.1\times 10^{-21}-1.2\times 10^{-19}\,\text{Nm}/\sqrt{\text{Hz}}$ for a mechanical frequency range of 5--800 MHz. The nanodisk can be outfitted with magnetic nanostructures or metasurfaces without affecting the optical properties of the cavity, making the system suitable for torque magnetometry and structured light sensing.

physics.optics↗

arXiv2022

Nonlinear optics in gallium phosphide cavities: simultaneous second and third harmonic generation

We demonstrate the simultaneous generation of second and third harmonic signals from a telecom wavelength pump in a gallium phosphide (GaP) microdisk. Using analysis of the power scaling of both the second and third harmonic outputs and calculations of nonlinear cavity mode coupling factors, we study contributions to the third harmonic signal from direct and cascaded sum frequency generation processes. We find that despite the relatively high material absorption in gallium phosphide at the third harmonic wavelength, both of these processes can be significant, with relative magnitudes that depend closely on the detuning between the second harmonic wavelength of the cavity modes.

physics.optics↗

arXiv2021

Demonstration of hybrid high-Q hexagonal boron nitride microresonators

Hexagonal boron nitride (hBN) is a wide bandgap van der Waals material that is emerging as a powerful platform for quantum optics and nanophotonics. In this work, we demonstrate whispering gallery mode silica microresonators hybridized with thin layers of epitaxially grown hBN that exhibit high optical quality factor $> 7 \times 10^5$. Measurements of the effect of hBN thickness on optical $Q$ and comparison with a theoretical model allows the linear optical absorption coefficient of the hBN films to be estimated. These high-$Q$ devices will be useful for applications in quantum and nonlinear optics, and their hybridized geometry provides a sensitive platform for evaluating losses in hBN and other 2D materials.

physics.optics↗

arXiv2021

Tunable amplification and cooling of a diamond resonator with a microscope

Controlling the dynamics of mechanical resonators is central to many quantum science and metrology applications. Optomechanical control of diamond resonators is attractive owing to diamond's excellent physical properties and its ability to host electronic spins that can be coherently coupled to mechanical motion. Using a confocal microscope, we demonstrate tunable amplification and damping of a diamond nanomechanical resonator's motion. Observation of both normal mode cooling from room temperature to 80K, and amplification into self--oscillations with $60\,μ\text{W}$ of optical power is observed via waveguide optomechanical readout. This system is promising for quantum spin-optomechanics, as it is predicted to enable optical control of stress-spin coupling with rates of $\sim$ 1 MHz (100 THz) to ground (excited) states of diamond nitrogen vacancy centers.

physics.optics↗

arXiv2020

Processing light with an optically tunable mechanical memory

Mechanical systems are one of the promising platforms for classical and quantum information processing and are already widely-used in electronics and photonics. Cavity optomechanics offers many new possibilities for information processing using mechanical degrees of freedom; one of them is storing optical signals in long-lived mechanical vibrations by means of optomechanically induced transparency. However, the memory storage time is limited by intrinsic mechanical dissipation. More over, in-situ control and manipulation of the stored signals--processing--has not been demonstrated. Here, we address both of these limitations using a multi-mode cavity optomechanical memory. An additional optical field coupled to the memory modifies its dynamics through time-varying parametric feedback. We demonstrate that this can extend the memory decay time by an order of magnitude, decrease its effective mechanical dissipation rate by two orders of magnitude, and deterministically shift the phase of a stored field by over 2$π$. This further expands the information processing toolkit provided by cavity optomechanics.

physics.optics↗

arXiv2020

Two-colour interferometry and switching through optomechanical dark mode excitation

Efficient switching and routing of photons of different wavelengths is a requirement for realizing a quantum internet. Multimode optomechanical systems can solve this technological challenge and enable studies of fundamental science involving widely separated wavelengths that are inaccessible to single-mode optomechanical systems. To this end, we demonstrate interference between two optomechanically induced transparency processes in a diamond on-chip cavity. This system allows us to directly observe the dynamics of an optomechanical dark mode that interferes photons at different wavelengths via their mutual coupling to a common mechanical resonance. This dark mode does not transfer energy to the dissipative mechanical reservoir and is predicted to enable quantum information processing applications that are insensitive to mechanical decoherence. Control of the dark mode is also utilized to demonstrate all-optical, two-colour switching and interference with light separated by over 5 THz in frequency.

physics.optics↗

arXiv2019

Optomechanically amplified wavelength conversion in diamond microcavities

Efficient, low noise conversion between different colors of light is a necessary tool for interfacing quantum optical technologies that have different operating wavelengths. Optomechanically mediated wavelength conversion and amplification is a potential method for realizing this technology, and is demonstrated here in microdisks fabricated from single crystal diamond--a material that can host a wide range of quantum emitters. Frequency up--conversion is demonstrated with internal conversion efficiency of $\sim$45% using both narrow and broadband probe fields, and optomechanical frequency conversion with amplification is demonstrated in the optical regime for the first time.

physics.optics↗

arXiv2019

Realizing $Q$ > 300,000 in diamond microdisks for optomechanics via etch optimization

Nanophotonic structures in single--crystal diamond (SCD) that simultaneously confine and co-localize photons and phonons are highly desirable for applications in quantum information science and optomechanics. Here we describe an optimized process for etching SCD microdisk structures designed for optomechanics applications. This process allows the optical quality factor, $Q$, of these devices to be enhanced by a factor of 4 over previous demonstrations to $Q \sim 335,000$, which is sufficient to enable sideband resolved coherent cavity optomechanical experiments. Through analysis of optical loss and backscattering rates we find that $Q$ remains limited by surface imperfections. We also describe a technique for altering microdisk pedestal geometry which could enable reductions in mechanical dissipation.

physics.app-ph↗

arXiv2018

Hexagonal boron nitride cavity optomechanics

Hexagonal boron nitride (hBN) is an emerging layered material that plays a key role in a variety of two-dimensional devices, and has potential applications in nanophotonics and nanomechanics. Here, we demonstrate the first cavity optomechanical system incorporating hBN. Nanomechanical resonators consisting of hBN beams with predicted thickness between 8 nm and 51 nm were fabricated using electron beam induced etching and positioned in the optical nearfield of silicon microdisk cavities. A 160 fm/$\sqrt{\text{Hz}}$ sensitivity to the hBN nanobeam motion is demonstrated, allowing observation of thermally driven mechanical resonances with frequencies between 1 and 23 MHz, and mechanical quality factors reaching 1100 at room temperature in high vacuum. In addition, the role of air damping is studied via pressure dependent measurements. Our results constitute an important step towards realizing integrated optomechanical circuits employing hBN.

physics.optics↗

arXiv2017

Optomechanically induced transparency and cooling in thermally stable diamond microcavities

Diamond cavity optomechanical devices hold great promise for quantum technology based on coherent coupling between photons, phonons and spins. These devices benefit from the exceptional physical properties of diamond, including its low mechanical dissipation and optical absorption. However the nanoscale dimensions and mechanical isolation of these devices can make them susceptible to thermo-optic instability when operating at the high intracavity field strengths needed to realize coherent photon--phonon coupling. In this work, we overcome these effects through engineering of the device geometry, enabling operation with large photon numbers in a previously thermally unstable regime of red-detuning. We demonstrate optomechanically induced transparency with cooperativity > 1 and normal mode cooling from 300 K to 60 K, and predict that these device will enable coherent optomechanical manipulation of diamond spin systems.

physics.optics↗

arXiv2016

Single-crystal diamond low-dissipation cavity optomechanics

Single-crystal diamond cavity optomechanical devices are a promising example of a hybrid quantum system: by coupling mechanical resonances to both light and electron spins, they can enable new ways for photons to control solid state qubits. However, realizing cavity optomechanical devices from high quality diamond chips has been an outstanding challenge. Here we demonstrate single-crystal diamond cavity optomechanical devices that can enable photon-phonon-spin coupling. Cavity optomechanical coupling to $2\,\text{GHz}$ frequency ($f_\text{m}$) mechanical resonances is observed. In room temperature ambient conditions, these resonances have a record combination of low dissipation (mechanical quality factor, $Q_\text{m} > 9000$) and high frequency, with $Q_\text{m}\cdot f_\text{m} \sim 1.9\times10^{13}$ sufficient for room temperature single phonon coherence. The system exhibits high optical quality factor ($Q_\text{o} > 10^4$) resonances at infrared and visible wavelengths, is nearly sideband resolved, and exhibits optomechanical cooperativity $C\sim 3$. The devices' potential for optomechanical control of diamond electron spins is demonstrated through radiation pressure excitation of mechanical self-oscillations whose 31 pm amplitude is predicted to provide 0.6 MHz coupling rates to diamond nitrogen vacancy center ground state transitions (6 Hz / phonon), and $\sim10^5$ stronger coupling rates to excited state transitions.

quant-ph↗

arXiv2016

Efficient telecom to visible wavelength conversion in doubly resonant GaP microdisks

Resonant second harmonic generation between 1550 nm and 775 nm with outside efficiency $> 4.4\times10^{-4}\, \text{mW}^{-1}$ is demonstrated in a gallium phosphide microdisk cavity supporting high-$Q$ modes at visible ($Q \sim 10^4$) and infrared ($Q \sim 10^5$) wavelengths. The double resonance condition was satisfied through intracavity photothermal temperature tuning using $\sim 360\,μ$W of 1550 nm light input to a fiber taper and resonantly coupled to the microdisk. Above this pump power efficiency was observed to decrease. The observed behavior is consistent with a simple model for thermal tuning of the double resonance condition.

physics.optics↗

arXiv2015

Single crystal diamond nanobeam waveguide optomechanics

Optomechanical devices sensitively transduce and actuate motion of nanomechanical structures using light. Single--crystal diamond promises to improve the performance of optomechanical devices, while also providing opportunities to interface nanomechanics with diamond color center spins and related quantum technologies. Here we demonstrate dissipative waveguide--optomechanical coupling exceeding 35 GHz/nm to diamond nanobeams supporting both optical waveguide modes and mechanical resonances, and use this optomechanical coupling to measure nanobeam displacement with a sensitivity of $9.5$ fm/$\sqrt{\text{Hz}}$ and optical bandwidth $>150$nm. The nanobeams are fabricated from bulk optical grade single--crystal diamond using a scalable undercut etching process, and support mechanical resonances with quality factor $2.5 \times 10^5$ at room temperature, and $7.2 \times 10^5$ in cryogenic conditions (5K). Mechanical self--oscillations, resulting from interplay between photothermal and optomechanical effects, are observed with amplitude exceeding 200 nm for sub-$μ$W absorbed optical power, demonstrating the potential for optomechanical excitation and manipulation of diamond nanomechanical structures.

physics.optics↗