arXiv subjects

David R. M. Arvidsson-Shukur

Publications and source records attributed to David R. M. Arvidsson-Shukur.

At least 19 recordsLinked to original sources

arXiv2026

Superconducting-antiqubit simulation enables optimal phase estimation via unitary inversion

A positron is equivalent to an electron traveling backward through time. Casting transmon superconducting qubits as akin to electrons, we simulate a positron with a transmon subject to particular resonant and off-resonant drives. We call positron-like transmons "antiqubits." An antiqubit's effective gyromagnetic ratio equals the negative of a qubit's. This fact enables us to time-invert a unitary implemented on a transmon by its environment. We apply this platform-specific unitary inversion, with qubit--antiqubit entanglement, to achieve a quantum advantage in phase estimation: consider measuring the strength of a field that points in an unknown direction. An entangled qubit--antiqubit sensor offers the greatest possible sensitivity (amount of Fisher information), per qubit, per application of the field. We prove this result theoretically and observe it experimentally. This work shows how antimatter, whether real or simulated, can enable platform-specific unitary inversion and benefit quantum information processing.

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arXiv2026

Kirkwood-Dirac Nonpositivity is a Necessary Resource for Quantum Computing

We elucidate the boundary between classical and quantum computation by constructing qubit Clifford circuits with nonstabilizer inputs that can be efficiently simulated classically. We do so by casting the quantum circuits realizable by defect braiding in the surface code in terms of a Kirkwood-Dirac (KD) quasiprobability distribution, a generalization of a joint probability distribution. If this distribution remains a proper (positive) probability distribution throughout a circuit, then a classical algorithm can simulate the circuit efficiently. By leveraging recent results on the geometry of KD-positive states, we construct bound-magic states. Classical computers can efficiently simulate these bound-magic states' evolutions under the circuits, although other magic states enable universal quantum computation when inputted. Furthermore, we show that KD nonpositivity is a resource monotone in this model. Thus, we establish KD nonpositivity as a necessary resource for quantum-computational advantages.

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arXiv2026

Almost no experiments have classical Kirkwood-Dirac representations

A central problem in quantum information is determining quantum-classical boundaries. In the quasiprobability framework, a state is called classical if it is represented by a quasiprobability distribution that is positive, and thus a probability distribution. In recent years, the Kirkwood-Dirac (KD) distributions have gained much interest due to their numerous applications in modern quantum-information research. A particular advantage of the KD distributions is that they can be defined with respect to arbitrary observables. Here, we show that if two $d$-dimensional observables are picked at random, the set of classical (positive) states of the resulting KD distribution is a minimal polytope of dimension $2(d-1)$ with $2d$ explicitly known vertices. This implies minimality of the sets of KD-real observables, of KD-positive measurement elements and of KD-positivity-preserving unitaries. We show how these results have implications on robust observations of nonclassical phenomena, on classical simulations of quantum circuits, and on foundations of quantum theory.

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arXiv2026

Pulse-optimised circuit elements for scalable and noise-resilient quantum chemistry

Useful chemistry calculations on near-term quantum processors are hindered by current algorithmic runtimes. We develop a methodology to significantly reduce these runtimes. Typically, variational quantum eigensolver (VQE) algorithms are implemented as sequences of primitive gates. Our methodology instead relies on gradient-ascent pulse engineering to construct hardware-tailored pulses for the direct implementation of VQEs. As problem sizes increase, it quickly becomes intractable to optimise a pulse that implements an entire VQE ansatz circuit. However, leading VQEs are constructed in a modular fashion. A problem-tailored VQE is assembled from parameterised circuit elements that simulate hopping between two or four electronic spin orbitals. We show that these circuit elements can be implemented more efficiently using hardware-tailored pulses. We numerically demonstrate our methodology on a silicon spin-qubit quantum processor. We find that common circuit elements, known as single- and double-qubit excitations, can be implemented in less than 289 ns and 927 ns, respectively. Compared with conventional gate-based implementations, our pulse-accelerated qubit excitations provide a scalable approach for faster and therefore more noise-robust quantum chemistry simulations by reducing VQE runtimes by up to a factor of 15.3.

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arXiv2026

Hardware-Tailored Resource Estimation for Magic-State Distillation on Silicon Spin Qubits

We present a resource analysis for generating high-fidelity logical magic states on silicon spin-qubit platforms. We consider a range of architectures, including a shuttling-based SpinBus design, a dense nearest-neighbor layout, and a hybrid scheme with shuttling-connected patches. We compare surface, color, and biased error-correcting codes, and analyze the $5\to1$ and $15\to1$ magic-state distillation protocols. Our approach combines bottom-up and top-down methodologies. We construct a hardware-level noise model based on a silicon-processor Hamiltonian with realistic parameters and $1/f$ non-Markovian noise, enabling estimation of physical resources required to reach target logical error rates. These results are propagated to system-level overheads for applications including spin dynamics, integer factorization, and quantum chemistry. Conversely, we fix target logical fidelities and derive corresponding constraints on hardware performance. Our framework enables systematic evaluation of resource-reduction strategies. We find that optimized control pulses reduce magic-state distillation overhead by 42\% compared to standard gate implementations. In addition, silicon-tailored biased error-correcting codes achieve an approximately threefold reduction in physical footprint relative to the surface code, even without physical-bias-preserving operations.

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arXiv2026

Quantum metrology enhanced by effective time reversal

Quantum metrology involves the application of quantum resources to enhance measurements. Several communities have developed quantum-metrology strategies that leverage effective time reversals. These strategies, we posit, form four classes. First, echo metrology begins with a preparatory unitary and ends with that unitary's time-reverse. The protocol amplifies the visibility of a small parameter to be sensed. Similarly, weak-value amplification enhances a weak coupling's detectability. The technique exhibits counterintuitive properties captured by a retrocausal model. Using the third strategy, one simulates closed timelike curves, worldlines that loop back on themselves in time. The fourth strategy involves indefinite causal order, which characterises channels applied in a superposition of orderings. We review these four strategies, which we unify under the heading of time-reverse metrology. We also outline opportunities for this toolkit in quantum metrology; quantum information science; quantum foundations; atomic, molecular, and optical physics; and solid-state physics.

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arXiv2026

Theory of direct measurement of the quantum pseudo-distribution via its characteristic function

We propose a method for directly measuring the quantum mechanical pseudo-distribution of observable properties via its characteristic function. Vandermonde matrices of the eigenvalues play a central role in the theory. This proposal directly finds the pseudo-distribution using weak measurements of the generator of position moments (momentum translations). While the pseudo-distribution can be extracted from the data in a theory-agnostic way, it is shown that under quantum-mechanical formalism, the predicted pseudo-distribution is identified with the Kirkwood-Dirac pseudo-distribution. We discuss the construction of both the joint pseudo-distribution and a conditional pseudo-distribution, which is closely connected to weak-value physics. By permuting position and momentum measurements, we give a prescription to directly probe the canonical commutation relation and verify it for any quantum state. This work establishes the theory of a characteristic function approach to pseudo-distributions, as well as providing a constructive approach to measuring them directly.

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arXiv2025

QuantGraph: A Receding-Horizon Quantum Graph Solver

Dynamic programming is a cornerstone of graph-based optimization. While effective, it scales unfavorably with problem size. In this work, we present QuantGraph, a two-stage quantum-enhanced framework that casts local and global graph-optimization problems as quantum searches over discrete trajectory spaces. The solver is designed to operate efficiently by first finding a sequence of locally optimal transitions in the graph (local stage), without considering full trajectories. The accumulated cost of these transitions acts as a threshold that prunes the search space (up to 60% reduction for certain examples). The subsequent global stage, based on this threshold, refines the solution. Both stages utilize variants of the Grover-adaptive-search algorithm. To achieve scalability and robustness, we draw on principles from control theory and embed QuantGraph's global stage within a receding-horizon model-predictive-control scheme. This classical layer stabilizes and guides the quantum search, improving precision and reducing computational burden. In practice, the resulting closed-loop system exhibits robust behavior and lower overall complexity. Notably, for a fixed query budget, QuantGraph attains a 2x increase in control-discretization precision while still benefiting from Grover-search's inherent quadratic speedup compared to classical methods.

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arXiv2025

Risk-minimizing states for the quantum-phase-estimation algorithm

The quantum-phase-estimation algorithm (QPEA) is widely used to find estimates of unknown phases. The original algorithm relied on an input state in a uniform superposition of all possible bit strings. However, it is known that other input states can reduce certain Bayesian risks of the final estimate. Here, we derive a method to find the risk-minimizing input state for any risk. These states are represented by an eigenvector of a Toeplitz matrix with elements given by the Fourier coefficients of the loss function of interest. We show that, while the true optimal state does not have a closed form for a general loss function, it is well approximated by a state with a cosine form. When the cosine frequency is chosen appropriately, these states outperform the original QPEA and achieve the optimal theoretical quantum-advantage scaling for three common risks. Furthermore, we prove that the uniform input state is suboptimal for any reasonable loss function. Finally, we design methods to mitigate the impact of depolarizing noise on the performance of QPEA.

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arXiv2025

Properties and Applications of the Kirkwood-Dirac Distribution

Recent years have seen the Kirkwood-Dirac (KD) distribution come to the forefront as a powerful quasi-probability distribution for analysing quantum mechanics. The KD distribution allows tools from statistics and probability theory to be applied to problems in quantum-information processing. A notable difference to the Wigner function is that the KD distribution can represent a quantum state in terms of arbitrary observables. This paper reviews the KD distribution, in three parts. First, we present definitions and basic properties of the KD distribution and its generalisations. Second, we summarise the KD distribution's extensive usage in the study or development of measurement disturbance; quantum metrology; weak values; direct measurements of quantum states; quantum thermodynamics; quantum scrambling and out-of-time-ordered correlators; and the foundations of quantum mechanics, including Leggett-Garg inequalities, the consistent-histories interpretation and contextuality. We emphasise connections between operational quantum advantages and negative or non-real KD quasi-probabilities. Third, we delve into the KD distribution's mathematical structure. We summarise the current knowledge regarding the geometry of KD-positive states (the states for which the KD distribution is a classical probability distribution), describe how to witness and quantify KD non-positivity, and outline relationships between KD non-positivity, coherence and observables' incompatibility.

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arXiv2024

Contextuality Can be Verified with Noncontextual Experiments

We uncover new features of generalized contextuality by connecting it to the Kirkwood-Dirac (KD) quasiprobability distribution. Quantum states can be represented by KD distributions, which take values in the complex unit disc. Only for ``KD-positive'' states are the KD distributions joint probability distributions. A KD distribution can be measured by a series of weak and projective measurements. We design such an experiment and show that it is contextual iff the underlying state is not KD-positive. We analyze this connection with respect to mixed KD-positive states that cannot be decomposed as convex combinations of pure KD-positive states. Our result is the construction of a noncontextual experiment that enables an experimenter to verify contextuality.

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arXiv2024

Agnostic Phase Estimation

The goal of quantum metrology is to improve measurements' sensitivities by harnessing quantum resources. Metrologists often aim to maximize the quantum Fisher information, which bounds the measurement setup's sensitivity. In studies of fundamental limits on metrology, a paradigmatic setup features a qubit (spin-half system) subject to an unknown rotation. One obtains the maximal quantum Fisher information about the rotation if the spin begins in a state that maximizes the variance of the rotation-inducing operator. If the rotation axis is unknown, however, no optimal single-qubit sensor can be prepared. Inspired by simulations of closed timelike curves, we circumvent this limitation. We obtain the maximum quantum Fisher information about a rotation angle, regardless of the unknown rotation axis. To achieve this result, we initially entangle the probe qubit with an ancilla qubit. Then, we measure the pair in an entangled basis, obtaining more information about the rotation angle than any single-qubit sensor can achieve. We demonstrate this metrological advantage using a two-qubit superconducting quantum processor. Our measurement approach achieves a quantum advantage, outperforming every entanglement-free strategy.

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arXiv2024

Convex roofs witnessing Kirkwood-Dirac nonpositivity

Given two observables $A$ and $B$, one can associate to every quantum state a Kirkwood-Dirac (KD) quasiprobability distribution. KD distributions are like joint classical probabilities except that they can have negative or nonreal values, which are associated to nonclassical features of the state. In the last decade, KD distributions have come to the forefront as a versatile tool to investigate and construct quantum advantages and nonclassical phenomena. KD distributions are also used to determine quantum-classical boundaries. To do so, one must have witnesses for when a state is KD nonpositive. Previous works have established a relation between the uncertainty of a pure state with respect to the eigenbases of $A$ and $B$ and KD positivity. If this $\textit{support uncertainty}$ is large, the state cannot be KD positive. Here, we construct two witnesses for KD nonpositivity for general mixed states. Our first witness is the convex roof of the support uncertainty; it is not faithful, but it extends to the convex hull of pure KD-positive states the relation between KD positivity and small support uncertainty. Our other witness is the convex roof of the total KD nonpositivity, which provides a faithful witness for the convex hull of the pure KD-positive states. This implies that the convex roof of the total nonpositivity captures the nonpositive nature of the KD distribution at the underlying pure state level.

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arXiv2024

Minimal evolution times for fast, pulse-based state preparation in silicon spin qubits

Standing as one of the most significant barriers to reaching quantum advantage, state-preparation fidelities on noisy intermediate-scale quantum processors suffer from quantum-gate errors, which accumulate over time. A potential remedy is pulse-based state preparation. We numerically investigate the minimal evolution times (METs) attainable by optimizing (microwave and exchange) pulses on silicon hardware. We investigate two state preparation tasks. First, we consider the preparation of molecular ground states and find the METs for H$_2$, HeH$^+$, and LiH to be 2.4 ns, 4.4 ns, and 27.2 ns, respectively. Second, we consider transitions between arbitrary states and find the METs for transitions between arbitrary four-qubit states to be below 50 ns. For comparison, connecting arbitrary two-qubit states via one- and two-qubit gates on the same silicon processor requires approximately 200 ns. This comparison indicates that pulse-based state preparation is likely to utilize the coherence times of silicon hardware more efficiently than gate-based state preparation. Finally, we quantify the effect of silicon device parameters on the MET. We show that increasing the maximal exchange amplitude from 10 MHz to 1 GHz accelerates the METs, e.g., for H$_2$ from 84.3 ns to 2.4 ns. This demonstrates the importance of fast exchange. We also show that increasing the maximal amplitude of the microwave drive from 884 kHz to 56.6 MHz shortens state transitions, e.g., for two-qubit states from 1000 ns to 25 ns. Our results bound both the state-preparation times for general quantum algorithms and the execution times of variational quantum algorithms with silicon spin qubits.

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arXiv2024

Quantifying the effect of gate errors on variational quantum eigensolvers for quantum chemistry

Variational quantum eigensolvers (VQEs) are leading candidates to demonstrate near-term quantum advantage. Here, we conduct density-matrix simulations of leading gate-based VQEs for a range of molecules. We numerically quantify their level of tolerable depolarizing gate-errors. We find that: (i) The best-performing VQEs require gate-error probabilities between $10^{-6}$ and $10^{-4}$ ( $10^{-4}$ and $10^{-2}$ with error mitigation) to predict, within chemical accuracy, ground-state energies of small molecules with $4-14$ orbitals. (ii) ADAPT-VQEs that construct ansatz circuits iteratively outperform fixed-circuit VQEs. (iii) ADAPT-VQEs perform better with circuits constructed from gate-efficient rather than physically-motivated elements. (iv) The maximally-allowed gate-error probability, $p_c$, for any VQE to achieve chemical accuracy decreases with the number $\ncx$ of noisy two-qubit gates as $p_c\approxprop\ncx^{-1}$. Additionally, $p_c$ decreases with system size, even with error mitigation, implying that larger molecules require even lower gate-errors. Thus, quantum advantage via gate-based VQEs is unlikely unless gate-error probabilities are decreased by orders of magnitude.

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arXiv2023

Nonclassical advantage in metrology established via quantum simulations of hypothetical closed timelike curves

We construct a metrology experiment in which the metrologist can sometimes amend her input state by simulating a closed timelike curve, a worldline that travels backward in time. The existence of closed timelike curves is hypothetical. Nevertheless, they can be simulated probabilistically by quantum-teleportation circuits. We leverage such simulations to pinpoint a counterintuitive nonclassical advantage achievable with entanglement. Our experiment echoes a common information-processing task: A metrologist must prepare probes to input into an unknown quantum interaction. The goal is to infer as much information per probe as possible. If the input is optimal, the information gained per probe can exceed any value achievable classically. The problem is that, only after the interaction does the metrologist learn which input would have been optimal. The metrologist can attempt to change her input by effectively teleporting the optimal input back in time, via entanglement manipulation. The effective time travel sometimes fails but ensures that, summed over trials, the metrologist's winnings are positive. Our Gedankenexperiment demonstrates that entanglement can generate operational advantages forbidden in classical chronology-respecting theories.

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arXiv2023

Dynamic-ADAPT-QAOA: An algorithm with shallow and noise-resilient circuits

The quantum approximate optimization algorithm (QAOA) is an appealing proposal to solve NP problems on noisy intermediate-scale quantum (NISQ) hardware. Making NISQ implementations of the QAOA resilient to noise requires short ansatz circuits with as few CNOT gates as possible. Here, we present Dynamic-ADAPT-QAOA. Our algorithm significantly reduces the circuit depth and the CNOT count of standard ADAPT-QAOA, a leading proposal for near-term implementations of the QAOA. Throughout our algorithm, the decision to apply CNOT-intensive operations is made dynamically, based on algorithmic benefits. Using density-matrix simulations, we benchmark the noise resilience of ADAPT-QAOA and Dynamic-ADAPT-QAOA. We compute the gate-error probability $p_\text{gate}^\star$ below which these algorithms provide, on average, more accurate solutions than the classical, polynomial-time approximation algorithm by Goemans and Williamson. For small systems with $6-10$ qubits, we show that $p_{\text{gate}}^\star>10^{-3}$ for Dynamic-ADAPT-QAOA. Compared to standard ADAPT-QAOA, this constitutes an order-of-magnitude improvement in noise resilience. This improvement should make Dynamic-ADAPT-QAOA viable for implementations on superconducting NISQ hardware, even in the absence of error mitigation.

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arXiv2023

Layering and subpool exploration for adaptive Variational Quantum Eigensolvers: Reducing circuit depth, runtime, and susceptibility to noise

Adaptive variational quantum eigensolvers (ADAPT-VQEs) are promising candidates for simulations of strongly correlated systems on near-term quantum hardware. To further improve the noise resilience of these algorithms, recent efforts have been directed towards compactifying, or layering, their ansatz circuits. Here, we broaden the understanding of the algorithmic layering process in three ways. First, we investigate the non-commutation relations between the different elements that are used to build ADAPT-VQE ansätze. Doing so, we develop a framework for studying and developing layering algorithms, which produce shallower circuits. Second, based on this framework, we develop a new subroutine that can reduce the number of quantum-processor calls by optimizing the selection procedure with which a variational quantum algorithm appends ansatz elements. Third, we provide a thorough numerical investigation of the noise-resilience improvement available via layering the circuits of ADAPT-VQE algorithms. We find that layering leads to an improved noise resilience with respect to amplitude-damping and dephasing noise, which, in general, affect idling and non-idling qubits alike. With respect to depolarizing noise, which tends to affect only actively manipulated qubits, we observe no advantage of layering.

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