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David Wilkowski

Publications and source records attributed to David Wilkowski.

At least 19 recordsLinked to original sources

Collective dressed states for inelastic light scattering by atomic ensembles

We develop a general dressed-state framework for computing fluorescence spectra, probe absorption spectra, and photon-photon correlations of light scattered by ensembles of $N_\mathrm{at}$ two-level atoms with arbitrary $J_g \to J_e$ transitions driven by intense coherent fields. The approach employs a full vectorial treatment of the electromagnetic field, handles any atomic geometries, illumination directions, and polarizations, and yields optical observables as explicit sums of Lorentzian lines whose positions, widths, and weights are directly tied to the eigenvalues and eigenvectors of the Lindbladian. The framework is implemented in an open-source Python package and benchmarked against exact single- and two-atom calculations. We identify geometries in which the full vectorial description is essential, and the scalar approximation fails qualitatively. Applying the method to pairs of atoms with a $J_g=0\to J_e=1$ transition, we show that elastic and inelastic scattered intensities collapse onto universal master curves controlled by a single collective saturation parameter built from the dominant superradiant mode, across several orders of magnitude in drive strength and interatomic distance. We identify collective phenomena that require a description beyond this single-mode picture. Extending the analysis to atoms with ground-state degeneracy, we find that most collective features carry over, while two qualitatively new effects emerge: an incoherent spontaneous Raman channel that modifies the scaling of inelastic emission, and a slow timescale in the time-delayed correlations $g^{(2)}(\tau)$ governed by the competition between Raman scattering and subradiant decay, controlled by a single dimensionless parameter. These results provide both physical insight and practical computational tools for engineering collective optical responses in few-atom systems such as optical tweezer arrays.

physics.atom-ph

Magic-wavelength matter-wave interferometry with optical clock states

Optical clocks and atom interferometers provide complementary ways to measure time, motion and gravity. Combining these capabilities requires matter-wave beam splitters that manipulate different clock states in the same way, so that optical internal energy becomes a controlled degree of freedom rather than a source of systematic phase shifts. Here we realized a dual matter-wave interferometer operating simultaneously on the two states of the $^{88}$Sr optical clock transition, $^1S_0$ and $^3P_0$. The interferometer is driven by Bragg pulses at the 813 nm magic wavelength, for which the two clock states experience the same optical coupling strength. This realizes a common matter-wave beam splitter for atoms whose internal energies differ by an optical excitation. With a sensitivity of 30 mrad, our measurement is consistent with a zero differential phase shift between the two clock-state Mach-Zehnder interferometers, translating to an absence of state-dependent acceleration in free fall at the level of $10^{-5}$. We further used the same interferometer to measure state-dependent optical dipole forces and determine a tune-out wavelength of the metastable $^3P_0$ state to be 478.95(8) nm. These results establish magic-wavelength clock-state interferometry as a platform for differential force sensing, excited-state polarizability metrology and future quantum-clock tests of gravity.

physics.atom-ph

Toroidal Transitions in Hydrogenic and Alkali Atoms

In addition to electric and magnetic multipoles, the expansion of current density also yields toroidal terms, a lesser-known family of multipoles. A recent proposal, I. Kuprov $\textit{et al.}$, Science Adv. 8 abq6751 (2022), explores the possibility of a direct observation of optical toroidal transitions in hydrogen and alkali atoms in the presence of a large magnetic field that decouples the spin and the angular momentum of the electron. However, the difficulty of observing these transitions against the nearby electric dipole (E1) transitions were underestimated because of extra admixture coming from diamagnetic coupling. Here, we revisit the toroidal coupling in atoms, taking diamagnetic contribution into account, and discuss the technical challenges of observing toroidal coupling in atomic physics. We show that toroidal transition should be searched in transitions with low principal quantum numbers. The remaining strong electric-dipole contribution could be removed using an appropriate differential measurement.

physics.atom-ph

Magic wavelength at 477 nm for the strontium clock transition

We report the experimental measurement of a magic wavelength at 476.82362(8) nm for the 88Sr clock transition. The magic wavelength is determined through AC-Stark shift spectroscopy of atoms in an optical dipole trap. The value slightly deviates from the theoretical prediction by 0.061(54) nm. This magic wavelength, being shorter than the common one at 813 nm, will be important for applications such as Bragg pulses for matter-wave interferometry involving both clock states. This work also paves the way for quantum simulation with a shorter lattice.

physics.atom-ph

Topological optical skyrmion transfer to matter

The ability of structured light to mimic exotic topological skyrmion textures, encountered in high-energy physics, cosmology, magnetic materials, and superfluids has recently received considerable attention. Despite their promise as mechanisms for data encoding and storage, there has been a lack of studies addressing the transfer and storage of the topology of optical skyrmions to matter. Here, we demonstrate a high-fidelity mapping of skyrmion topology from a laser beam onto a gas of cold atoms, where it is detected in its new non-propagating form. Within the spatial overlap of the beam and atom cloud, the skyrmion topological charge is preserved, with a reduction from $Q \simeq 0.91$ to $Q \simeq 0.84$ mainly due to the beam width exceeding the sample size. Our work potentially opens novel avenues for topological photonics state storage and the analysis of more complex structured light topologies.

physics.optics

Super-resolution optical trapping of multiple cold atoms

Arrays of optical tweezers form the backbone of neutral atoms analog and digital quantum processors. However, the inter-trap distance remains generally much larger than the size of the tweezers to avoid interference-induced trap distortions, limiting the trap density. Here, we report single-atom trapping in four super-resolved tweezers, meaning with a separation below the Sparrow diffraction limit. The optical pattern is generated using superoscillatory phenomenon leading to subwavelength traps with full control of the trap relative phases. We investigate two sets of relative phases that impede or allow the hopping and the reshuffling of atoms. We envision that superoscillatory light structuring will bridge the gap between large-distance traps generated by tweezer arrays and short-distance traps formed with optical lattices.

physics.atom-ph

Experimental realization of a SU(3) color-orbit coupling in an ultracold gas

Spin-orbit interaction couples the spin of a particle to its motion and leads to spin-induced transport phenomena such as spin-Hall effects and Chern insulators. In this work, we extend the concept of internal-external state coupling to higher internal symmetry, exploring features beyond the established spin-orbit regime. We couple suitable resonant laser beams to a gas of ultracold atoms, thereby inducing artificial SU(3) non-Abelian gauge fields that act on a degenerate ground state manifold comprised of three dark states. We demonstrate the inherent all-state connectivity of SU(3) systems by performing targeted geometric transformations. Then, we investigate color-orbit coupling, an extension of SU(2) spin-orbit coupling to SU(3) systems. We reveal a rich dynamical interplay between three distinct oscillation frequencies, which possesses interesting analogies with neutrino oscillations and quark mixing mechanisms. In the future, the system should provide a testbed for exploring topological properties of SU(3) systems.

physics.atom-ph

Doppler-free selective reflection spectroscopy of electric-quadrupole transitions

Electric-dipole-forbidden transitions play an important role as in quantum sensing, quantum information, and fundamental test in physics. As such, the development of novel and sensitive spectroscopic methods is of major interest. Here, we present a Doppler-free selective reflection experiment on the 6S1/2 --> 5D5/2 electric-quadrupole transition of cesium vapor at the vicinity of a sapphire window. This is achieved by a precision experiment overcoming limitations due to the small signal amplitude of forbidden transitions. Narrow sub-Doppler lines allow for a collisional broadening measurement on the electric-quadrupole line. The interaction of cesium atoms with the sapphire surface of the cell is evidenced, but, due to its weak contribution, a quantitative analysis remains challenging. Nevertheless, our experiment paves the way for further studies of the Casimir-Polder interaction between exotic excited-state atoms and dielectric surfaces.

physics.atom-ph

Geometric Ramsey Interferometry with a Tripod Scheme

Ramsey interferometry is a key technique for precision spectroscopy and to probe the coherence of quantum systems. Typically, an interferometer is constructed using two quantum states and involves a time-dependent interaction with two short resonant electromagnetic pulses. Here, we explore a different type of Ramsey interferometer where we perform quantum state manipulations by geometrical means, eliminating the temporal dependence of the interaction. We use a resonant tripod scheme in ultracold strontium atoms where the interferometric operation is restricted to a two-dimensional dark-state subspace in the dressed-state picture. The observed interferometric phase accumulation is due to an effective geometric scalar term in the dark-state subspace, which remarkably does not vanish during the free evolution time when the light-matter interaction is turned off. This study opens the door for more robust interferometers operating on multiple input-output ports.

quant-ph

Single atom in a superoscillatory optical trap

Optical tweezers have become essential tools to manipulate atoms or molecules at a single particle level. However, using standard diffracted-limited optical systems, the transverse size of the trap is lower bounded by the optical wavelength, limiting the application range of optical tweezers. Here we report trapping of single ultracold atom in an optical trap that can be continuously tuned from a standard Airy focus to a subwavelength hotspot smaller than the usual Abbe's diffraction limit. The hotspot was generated using the effect of superoscillations, by the precise interference of multiple free-space coherent waves. We argue that superoscillatory trapping and continuous potential tuning offer not only a way to generate compact and tenable ensembles of trapped atoms for quantum simulators but will also be useful in single molecule quantum chemistry and the study of cooperative atom-photon interaction within subwavelength arrays of quantum emitters.

physics.atom-ph

Evolution of an ultracold gas in a non-Abelian gauge fields: Finite temperature effect

We detail the cooling mechanisms of a Fermionic strontium-87 gas in order to study its evolution under a non-Abelian gauge field. In contrast to our previous work reported in Ref. [1], we emphasize here on the finite temperature effect of the gas. In addition, we provide the detail characterization for the efficiency of atoms loading in the cross-dipole trap, the quantitative performance of the evaporative cooling, and the characterization of a degenerate Fermi gas using a Thomas-Fermi distribution.

cond-mat.quant-gas

Bi-color atomic beam slower and magnetic field compensation for ultracold gases

Transversely loaded bidimensional-magneto-optical-traps (2D-MOT) have been recently developed as high flux sources for cold strontium atoms to realize a new generation of compact experimental setups. Here, we discuss on the implementation of a cross-polarized bi-color slower for a strontium atomic beam improving the 2D-MOT loading, and increasing the number of atoms in a final MOT by eleven times. Our slowing scheme addresses simultaneously two excited Zeeman substates of the 88Sr 1S0->1P1 transition at 461 nm. We also realized a 3-axis active feedback control of the magnetic field down to the microgauss regime. Such a compensation is performed thanks to a network of eight magnetic field probes arranged in a cuboid configuration around the atomic cold sample, and a pair of coils in Helmholtz configuration along each of three Cartesian directions. Our active feedback is capable of efficiently suppressing most of the magnetically-induced position fluctuations of the 689~nm intercombination-line MOT.

physics.atom-ph

Toroidal optical transitions in hydrogen-like atoms

It is commonly believed that electromagnetic spectra of atoms and molecules can be fully described by interactions of electric and magnetic multipoles. However, it has recently become clear that interactions between light and matter also involve toroidal multipoles - toroidal absorption lines have been observed in electromagnetic metamaterials. Here we show that a new type of spectroscopy of the hitherto largely neglected toroidal dipolar interaction becomes feasible if, apart from the classical r{\times}r{\times}p toroidal dipole density term responsible for the toroidal transitions in metamaterials, the spin-dependent r{\times}{\sigma} term (that only occurs in relativistic quantum mechanics) is taken into account. We show that toroidal transitions are odd under parity and time-reversal symmetries; they can therefore be observed and distinguished from electric multipole and magnetic dipole transitions.

physics.atom-ph

Datta-Das transistor for atomtronic circuits using artificial gauge fields

Spin-dependent electrical injection has found useful applications in storage devices, but fully operational spin-dependent semiconductor electronics remain a challenging task because of weak spin-orbit couplings and/or strong spin relaxations. These limitations are lifted considering atoms instead of electrons or holes as spin carriers. In this emerging field of atomtronics, we demonstrate the equivalent of a Datta-Das transistor using a degenerate Fermi gas of strontium atoms as spin carriers in interaction with a tripod laser-beams scheme. We explore the dependence of spin rotation, and we identify two key control parameters which we interpret as equivalent to the gate-source and drain-source voltages of a field effect transistor. Our finding broadens the spectrum of atomtronics devices for implementation of operational spin-sensitive circuits.

cond-mat.mes-hall

Wave-packet Dynamics in Synthetic Non-Abelian Gauge Fields

It is generally admitted that in quantum mechanics, the electromagnetic potentials have physical interpretations otherwise absent in classical physics as illustrated by the Aharonov-Bohm effect. In 1984, Berry interpreted this effect as a geometrical phase factor. The same year, Wilczek and Zee generalized the concept of Berry phases to degenerate levels and showed that a non-Abelian gauge field arises in these systems. In sharp contrast with the Abelian case, spatially uniform non-Abelian gauge fields can induce particle noninertial motion. We explore this intriguing phenomenon with a degenerated Fermionic atomic gas subject to a two-dimensional synthetic SU(2) non-Abelian gauge field. We reveal the spin Hall nature of the noninertial dynamic as well as its anisotropy in amplitude and frequency due to the spin texture of the system. We finally draw the similarities and differences of the observed wave packet dynamic and the celebrated Zitterbewegung effect of the relativistic Dirac equation.

cond-mat.quant-gas

Laser-induced thermal source for cold atoms

We demonstrate a simple and compact approach to laser cool and trap atoms based on laser-induced thermal ablation (LITA) of a pure solid granule. A rapid thermalisation of the granule leads to a fast recovery of the ultra-high vacuum condition required for a long trapping lifetime of the cold gas. We give a proof-of-concept of the technique, performing a magneto-optical trap on the 461 nm $^1S_0\rightarrow^1P_1$ transition of strontium. We get up to 3.5 million of cold strontium-88 atoms with a trapping lifetime of more than 4 s. The lifetime is limited by the pressure of the strontium-free residual background vapour. We also implement an original configuration of permanent magnets to create the quadruple magnetic field of the magneto-optical trap. The LITA technique can be generalized to other atomic elements such as transition metals and lanthanide atoms, and shows a strong potential for applications in quantum technologies ranging from quantum computing to precision measurements such as outdoor inertial sensing.

physics.atom-ph

Atom-surface physics: A review

An atom in front of a surface is one of the simplest and fundamental problem in physics. Yet, it allows testing quantum electrodynamics, while providing potential platforms and interfaces for quantum technologies. Despite, its simplicity, combined with strong scientific and technological interests, atom-surface physics, at its fundamental level, remains largely unexplored mainly because of challenges associated with precise control of the atom-surface distance. Nevertheless, substantial breakthroughs have been made over the last two decades. With the development of cold and quantum atomic gases, one has gained further control on atom-surface position, naturally leading to improved precision in the Casimir-Polder interaction measurement. Advances have also been reported in finding experimental knobs to tune and even reverse the Casimir-Polder interaction strength. So far, this has only been achieved for atoms in short-lived excited states, however, the rapid progresses in material sciences, e.g. metamaterials and topological materials have inspired new ideas for controlling the atom-surface interaction in long-lived states. In addition, combining nano-photonic and atom-surface physics is now envisioned for applications in quantum information processing. The first purpose of this review is to give a general overview on the latest experimental developments in atom-surface physics. The second main objective is to sketch a vision of the future of the field, mainly inspired by the abundant theoretical works and proposals available now in the literature.

physics.atom-ph

Homodyne detection of a two-photon resonance assisted by cooperative emission

Focusing on the transient regime, we explore atomic two-photon spectroscopy with self-aligned homodyne interferometry in a $\Lambda$-system with large optical depth. The two light sources at the origin of the interference are the single-photon transient transmission of the probe, and the slow light of the electromagnetically induced transparency. By switching off the probe laser abruptly (flash effect), the transient transmission signal is reinforced by cooperativity, showing enhanced sensitivity to the two-photon frequency detuning. If the probe laser is periodically switched on and off, the amplitude of the transmission signal varies and remains large even for high modulation frequency. This technique has potential applications in sensing, such as magnetometry and velocimetry, and in coherent population trapping clocks.

quant-ph